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763 Results Found

  • Article
  • Open Access
22 Citations
6,479 Views
21 Pages

4 February 2017

This study assesses the quantitative effects of incorporating high-volume fly ash (HVFA) into tricalcium silicate (C3S) paste on the hydration, degree of silicate polymerization, and Al substitution for Si in calcium silicate hydrate (C–S–H). Thermog...

  • Article
  • Open Access
12 Citations
2,871 Views
10 Pages

Impacts of Space Restriction on the Microstructure of Calcium Silicate Hydrate

  • Yue Zhou,
  • Zhongping Wang,
  • Zheyu Zhu,
  • Yuting Chen,
  • Linglin Xu and
  • Kai Wu

30 June 2021

The effect of hydration space on cement hydration is essential. After a few days, space restriction affects the hydration kinetics which dominate the expansion, shrinkage and creep of cement materials. The influence of space restriction on the hydrat...

  • Article
  • Open Access
5 Citations
3,733 Views
17 Pages

The Properties of Magnesium Silicate Hydrate Prepared from the Magnesium Silicate Minerals in the Earth’s Crust

  • Qiang Song,
  • Qian He,
  • Jiao Nie,
  • Tiantian Song,
  • Hong Zhou,
  • Yaru Hu,
  • Yanxin Chen,
  • Yang Deng and
  • Fuan Cheng

23 April 2024

In order to explore a wider range and lower cost of raw materials for the preparation of magnesium silicate hydrate (M-S-H), an acid-leaching method was employed to extract and separate high-purity magnesium hydroxide (Mg(OH)2) with a purity higher t...

  • Article
  • Open Access
18 Citations
8,597 Views
17 Pages

Contact-Hardening Behavior of Calcium Silicate Hydrate Powders

  • Shuping Wang,
  • Xiaoqin Peng,
  • Luping Tang,
  • Chunpeng Cao and
  • Lu Zeng

25 November 2018

Calcium silicate hydrate (C-S-H) synthesized by a hydrothermal process from lime and siliceous materials was oven-dried and compressed into compacts. The microstructure and compaction properties of the resulting powders were characterized. The result...

  • Article
  • Open Access
3 Citations
2,406 Views
11 Pages

28 September 2022

Nanomaterials are promising candidates for refined performance optimization of cementitious materials. In recent years, numerous studies about the performance improvement of nanomaterials using polymers have been conducted, but the modification of ce...

  • Article
  • Open Access
52 Citations
3,838 Views
17 Pages

Immobilization of Radionuclide 133Cs by Magnesium Silicate Hydrate Cement

  • Tingting Zhang,
  • Tong Li,
  • Jing Zou,
  • Yimiao Li,
  • Shiwei Zhi,
  • Yuan Jia and
  • Christopher R. Cheeseman

30 December 2019

The radionuclide cesium (Cs) was solidified using magnesium silicate hydrate (M–S–H) cement. The influence of Cs+ on the reaction of the M–S–H gel system was evaluated by measuring the compressive strength and microscopic prop...

  • Article
  • Open Access
30 Citations
4,994 Views
11 Pages

Stabilization/Solidification of Strontium Using Magnesium Silicate Hydrate Cement

  • Tingting Zhang,
  • Jing Zou,
  • Yimiao Li,
  • Yuan Jia and
  • Christopher R. Cheeseman

1 February 2020

Magnesium silicate hydrate (M–S–H) cement, formed by reacting MgO, SiO2, and H2O, was used to encapsulate strontium (Sr) radionuclide. Samples were prepared using light-burned magnesium oxide and silica fume, with sodium hexametaphosphate...

  • Article
  • Open Access
414 Views
21 Pages

28 November 2025

Ion exchange resins are commonly utilized for treating liquid radioactive waste within nuclear power plants; however, the disposal of these waste resins presents a new challenge. In this study, magnesium silicate hydrate cement (MSHC) was used to imm...

  • Article
  • Open Access
7 Citations
3,214 Views
18 Pages

18 October 2023

Magnesium silicate hydrate (MSH) cement has the advantages of low energy consumption, minimal environmental pollution, carbon negativity, and reduced alkalinity, but excessive drying shrinkage inhibits its application. This paper analyzed the influen...

  • Review
  • Open Access
96 Citations
10,461 Views
26 Pages

29 October 2020

With the continuous research efforts, sophisticated predictive molecular dynamics (MD) models for C-S-H have been developed, and the application of MD simulation has been expanded from fundamental understanding of C-S-H to nano-engineered cement comp...

  • Article
  • Open Access
3 Citations
1,795 Views
16 Pages

6 September 2024

Phosphogypsum is a by-product of the wet-process phosphoric acid production, and it is rich in Ca and S. Long-term storage of Phosphogypsum can cause serious pollution to the environment; therefore, promoting the sustainable utilization of Phosphogyp...

  • Article
  • Open Access
9 Citations
3,049 Views
16 Pages

Nanoindentation Study of Calcium-Silicate-Hydrate Gel via Molecular Dynamics Simulations

  • Hang Yin,
  • Xuefeng Wang,
  • Haifeng Qin,
  • Shijie Wang and
  • Kun Cai

18 September 2023

The mechanical properties of calcium-silicate-hydrate (C-S-H) gels in cementitious materials are mainly realized by nanoindentation experiments. There is limited research on the dynamic response of the molecular structure of C-S-H under nanoindentati...

  • Article
  • Open Access
11 Citations
2,431 Views
16 Pages

17 April 2023

Magnesium silicate hydrate (M-S-H) cement, a type of green building material, has poor volume stability (i.e., large shrinkage deformation), which limits its application. As a new type of admixture, the behavior of a shrinkage-reducing admixture (SRA...

  • Article
  • Open Access
73 Citations
7,633 Views
17 Pages

24 January 2022

Calcium silicate hydrate (CSH) gels, the main binding phases of hydrated cement, are the most widely utilized synthetic materials. To understand the influences of composition and polymers on the reaction kinetics and phase formation, CSH gels with va...

  • Article
  • Open Access
12 Citations
3,403 Views
16 Pages

Continuous Phosphate Removal and Recovery Using a Calcium Silicate Hydrate Composite Monolithic Cryogel Column

  • Chanadda Phawachalotorn,
  • Worawit Wongniramaikul,
  • Tarawee Taweekarn,
  • Bussakorn Kleangklao,
  • Wachiraporn Pisitaro,
  • Wadcharawadee Limsakul,
  • Wilasinee Sriprom,
  • Wanchitra Towanlong and
  • Aree Choodum

20 January 2023

Toward the development of a practical and green approach for removing phosphate from water, a monolithic cryogel based on starch and calcium silicate hydrate (Cry–CSH) was employed as a phosphate adsorbent in a continuous flow system for the fi...

  • Article
  • Open Access
33 Citations
4,261 Views
15 Pages

3 September 2019

To study the effect of water on the dynamic mechanical properties of calcium silicate hydrate (C–S–H) at the atomic scale, the molecular dynamics simulations were performed in uniaxial tension with different strain rates for C–S&nda...

  • Article
  • Open Access
5 Citations
2,662 Views
15 Pages

Recovering Phosphate from Complex Wastewater Using Macroporous Cryogel Composited Calcium Silicate Hydrate Nanoparticles

  • Tarawee Taweekarn,
  • Worawit Wongniramaikul,
  • Pariyaporn Roop-o,
  • Wanchitra Towanlong and
  • Aree Choodum

31 December 2023

Since currently used natural, nonrenewable phosphorus resources are estimated to be depleted in the next 30–200 years, phosphorus recovery from any phosphorus-rich residues has attracted great interest. In this study, phosphorus recovery from c...

  • Article
  • Open Access
12 Citations
2,968 Views
29 Pages

Cd(II) and Cu(II) ions cause many diseases in humans. Therefore, they should be removed from water sources using simple and cost-effective adsorbents. Consequently, sodium magnesium silicate hydroxide/sodium magnesium silicate hydrate nanostructures...

  • Article
  • Open Access
4 Citations
1,903 Views
20 Pages

The discharge of lead and cadmium wastewater, along with the pollution caused by phosphogypsum, represents a particularly urgent environmental issue. This study employed a straightforward hydrothermal method to convert phosphogypsum into porous calci...

  • Article
  • Open Access
8 Citations
2,779 Views
14 Pages

30 November 2022

Calcium silicate hydrate (C-S-H) is the main product of cement hydration and has also been shown to be the main sorbing phase of actinide ions interacting with cement. U(IV) has been chosen as an exemplary actinide ion to study actinide sorption at C...

  • Article
  • Open Access
52 Citations
8,360 Views
16 Pages

15 July 2013

The primary objective of this paper was to synthesize a porous calcium silicate hydrate (CSH) with enhanced phosphate recovery property using polyethyleneglycol (PEG) as pore-generation agent. The formation mechanism of porous CSH was proposed. PEG m...

  • Review
  • Open Access
46 Citations
5,960 Views
16 Pages

Hydration Activity and Carbonation Characteristics of Dicalcium Silicate in Steel Slag: A Review

  • Hao Na,
  • Yajun Wang,
  • Xi Zhang,
  • Junguo Li,
  • Yanan Zeng and
  • Pengyao Liu

4 October 2021

Dicalcium silicate is one of the main mineral phases of steel slag. Ascribed to the characteristics of hydration and carbonation, the application of slag in cement production and carbon dioxide sequestration has been confirmed as feasible. In the cur...

  • Article
  • Open Access
20 Citations
5,900 Views
16 Pages

In Situ Soft X-ray Spectromicroscopy of Early Tricalcium Silicate Hydration

  • Sungchul Bae,
  • Manabu Kanematsu,
  • Daniel Hernández-Cruz,
  • Juhyuk Moon,
  • David Kilcoyne and
  • Paulo J. M. Monteiro

1 December 2016

The understanding and control of early hydration of tricalcium silicate (C3S) is of great importance to cement science and concrete technology. However, traditional characterization methods are incapable of providing morphological and spectroscopic i...

  • Article
  • Open Access
1,396 Views
23 Pages

Superabsorbent polymers (SAPs) are widely employed as an internal curing agent to enhance the durability and shrinkage–cracking resistance of concrete. However, while its macroscopic effects on concrete properties (e.g., strength reduction) hav...

  • Review
  • Open Access
170 Citations
14,729 Views
34 Pages

Structure, Fractality, Mechanics and Durability of Calcium Silicate Hydrates

  • Shengwen Tang,
  • Yang Wang,
  • Zhicheng Geng,
  • Xiaofei Xu,
  • Wenzhi Yu,
  • Hubao A and
  • Jingtao Chen

Cement-based materials are widely utilized in infrastructure. The main product of hydrated products of cement-based materials is calcium silicate hydrate (C-S-H) gels that are considered as the binding phase of cement paste. C-S-H gels in Portland ce...

  • Article
  • Open Access
3 Citations
2,825 Views
14 Pages

Effect of Sodium Silicate on the Hydration of Alkali-Activated Copper-Nickel Slag Materials

  • Jie Yang,
  • Tingting Zhang,
  • Lijie Guo,
  • Shiwei Zhi and
  • Junnan Han

15 March 2023

This paper studied the influence of the modulus and dosage of sodium silicate on the hydration of alkali-activated copper-nickel slag (CNS) materials. CNS was used as the main raw material, and ground granulated blast furnace slag (GBFS) powder was s...

  • Article
  • Open Access
22 Citations
3,152 Views
12 Pages

Adsorption of Lead Ion from Wastewater Using Non-Crystal Hydrated Calcium Silicate Gel

  • Shijie Liu,
  • Suping Cui,
  • Hongxia Guo,
  • Yali Wang and
  • Yan Zheng

10 February 2021

In order to obtain low-cost and excellent adsorption materials, this paper used calcium acetate and water glass as raw materials to synthesis hydrated calcium silicate gel by precipitation method. The performance and structure of hydrated calcium sil...

  • Article
  • Open Access
1 Citations
911 Views
16 Pages

11 April 2025

Coal gangue, a prevalent solid waste in the coal industry, has long been a significant concern due to its substantial production volume and potential environmental hazards. However, it contains valuable components such as silica and alumina, making i...

  • Article
  • Open Access
14 Citations
3,636 Views
21 Pages

Increase the Performances of Lime Finishing Mixes Due to Modification with Calcium Silicate Hydrates

  • Valentina Loganina,
  • Kristina Sergeeva,
  • Roman Fediuk,
  • Valery Uvarov,
  • Nikolai Vatin,
  • Yuriy Vasilev,
  • Mugahed Amran and
  • Maciej Szelag

9 April 2021

Lime plaster mixes are becoming more and more popular in the world’s building materials market every year. Therefore, the issue of increasing the efficiency of lime finishing coatings is relevant. The paper aim is the modification of lime binders wit...

  • Article
  • Open Access
3 Citations
1,339 Views
17 Pages

Kinetic Study and Catalytic Activity of Cr3+ Catalyst Supported on Calcium Silicate Hydrates for VOC Oxidation

  • Ramune Sidaraite,
  • Kestutis Baltakys,
  • Andrius Jaskunas,
  • Nedas Naslenas,
  • Darius Slavinskas,
  • Edvinas Slavinskas and
  • Tadas Dambrauskas

14 July 2024

Volatile organic compounds (VOCs) are pollutants that pose significant health and environmental risks, necessitating effective mitigation strategies. Catalytic oxidation emerges as a viable method for converting VOCs into non-toxic end products. This...

  • Article
  • Open Access
11 Citations
4,717 Views
13 Pages

20 November 2022

This paper presents the results of calorimetric and strength tests of mortars with ordinary Portland cement and two substitution rates (10 and 20%) of cement by siliceous fly ash. The prepared samples were cured under isothermal conditions at four di...

  • Article
  • Open Access
8 Citations
1,946 Views
22 Pages

Increasing the Hydration Activity of Tricalcium Silicate by Adding Microdispersed Ettringite as a Nucleating Agent

  • Yurii R. Krivoborodov,
  • Svetlana V. Samchenko,
  • Andrey V. Korshunov,
  • Irina V. Kozlova and
  • Dmitrii G. Alpacky

8 November 2023

Tricalcium silicate (C3S) as a binder material has a decisive influence on the processes of hardening and strength gain of cements and concretes. One of the promising directions is the introduction of dispersed additives into cement mixtures, which a...

  • Article
  • Open Access
4 Citations
2,831 Views
17 Pages

Effect of Iron-Doped TiO2 Nanotubes on the Hydration of Tricalcium Silicate

  • S. Mohd. Yonos Qattali,
  • Christian Pritzel,
  • Torsten Kowald,
  • S. M. Fuad Kabir Moni,
  • Manuela S. Killian and
  • Reinhard Trettin

Environmental pollution is one of the most serious and global problems for humans. Photocatalysis is a promising technology to control environmental pollution via the utilization of semiconductor materials as a photocatalyst. In this study, iron-dope...

  • Article
  • Open Access
4 Citations
1,964 Views
15 Pages

17 May 2024

The production of municipal solid waste incineration bottom ash (MSWIBA) is substantial and has the potential to replace cement, despite challenges such as complex composition, uneven particle size distribution, and low reactivity. This paper employs...

  • Article
  • Open Access
2 Citations
1,174 Views
11 Pages

The Effect of Ethylene Diamine Tetra(Methylene Phosphonic Acid) Sodium on the Hydration of Tricalcium Silicate at 80 °C

  • Yiwei Zou,
  • Weikai Song,
  • Chao Sun,
  • Tianshuai Yu,
  • Sijia Zhu,
  • Chunyu Wang and
  • Xiao Yao

1 November 2024

In the field of oil well cementing, controlling the hydration process of cement slurries is essential to ensure successful placement and long-term well integrity, especially under challenging high-temperature and high-pressure conditions. Organic pho...

  • Article
  • Open Access
36 Citations
4,414 Views
14 Pages

31 August 2021

Graphene is a two-dimensional material, with exceptional mechanical, electrical, and thermal properties. Graphene-based materials are, therefore, excellent candidates for use in nanocomposites. We investigated reduced graphene oxide (rGO), which is p...

  • Article
  • Open Access
705 Views
19 Pages

8 August 2025

Currently, the partial substitution of mineral aggregates with rubber particles in the preparation of rubber concrete (RC) is an effective method for recycling waste rubber materials. However, the mechanism of interfacial interactions in RC at high t...

  • Article
  • Open Access
9 Citations
3,130 Views
11 Pages

Three-Dimensional Characterization of Hardened Paste of Hydrated Tricalcium Silicate by Serial Block-Face Scanning Electron Microscopy

  • Yongjuan Zhao,
  • Xianping Liu,
  • Bo Chen,
  • Fei Yang,
  • Yongming Zhang,
  • Peiming Wang and
  • Ian Robinson

12 June 2019

With the application of a three-dimensional (3D) characterization technique, serial block-face scanning electron microscopy (SBFSEM), the 3D microstructure of a hydrated cement monomineral, tricalcium silicate (C3S), was measured with nanoscale resol...

  • Article
  • Open Access
8 Citations
4,852 Views
24 Pages

Formation of Natural Silicate Hydrates by the Interaction of Alkaline Seepage and Sediments Derived from Serpentinized Ultramafic Rocks at Narra, Palawan, the Philippines

  • Misato Shimbashi,
  • Shingo Yokoyama,
  • Yasutaka Watanabe,
  • Tsutomu Sato,
  • Tsubasa Otake,
  • Ryosuke Kikuchi,
  • Minoru Yamakawa and
  • Naoki Fujii

17 August 2020

In radioactive waste disposal facilities, low-permeability engineered barrier materials are important for inhibiting radionuclide migration. However, dissolution–precipitation reactions under alkaline conditions change the permeability of engin...

  • Article
  • Open Access
32 Citations
6,239 Views
11 Pages

Fabrication and Adsorption Behavior of Magnesium Silicate Hydrate Nanoparticles towards Methylene Blue

  • Renyao Huang,
  • Li He,
  • Tao Zhang,
  • Dianqing Li,
  • Pinggui Tang,
  • Yingying Zhao and
  • Yongjun Feng

24 April 2018

Magnesium silicate as a high-performance adsorption material has attracted increasing attention for the removal of organic dye pollution. Here, we prepared a series of magnesium silicate hydrates (MSH) in a hydrothermal route, and carefully investiga...

  • Article
  • Open Access
4 Citations
1,786 Views
16 Pages

Hydrated Calcium Silicate Erosion in Sulfate Environments a Molecular Dynamics Simulation Study

  • Mengjie You,
  • Xiaosan Yin,
  • Yuzhou Sun,
  • Hairong Wu,
  • Jimin Li and
  • Xiangming Zhou

7 December 2024

To investigate the micro-mechanism of the erosion of hydrated calcium silicate (C-S-H gel) in a sulfate environment, a solid–liquid molecular dynamics model of C-S-H gel/sodium sulfate was developed. This model employs molecular dynamics method...

  • Article
  • Open Access
16 Citations
3,871 Views
14 Pages

12 September 2020

Microcapsule based self-healing concrete can automatically repair damage and improve the durability of concrete structures, the performance of which depends on the binding behavior between the microcapsule wall and cement matrix. However, conventiona...

  • Article
  • Open Access
97 Citations
9,154 Views
15 Pages

Characterization of Magnesium Silicate Hydrate (MSH) Gel Formed by Reacting MgO and Silica Fume

  • Tingting Zhang,
  • Jing Zou,
  • Baomin Wang,
  • Zhenlin Wu,
  • Yuan Jia and
  • Christopher R. Cheeseman

28 May 2018

Magnesium silicate hydrate (MSH) gel was formed by reacting magnesium oxide (MgO) with silica fume (SF) in distilled water. The MSH was prepared using a MgO/SF molar ratio of 1.0 (40:60 weight ratio). Samples were analyzed during hydration process up...

  • Article
  • Open Access
27 Citations
4,917 Views
14 Pages

25 May 2020

The objective of this study was to investigate the effects of hydrated calcium silicate filler (hCS) on resin-based pit and fissure sealants’ acid neutralization, calcium ion release, and mechanical and physical properties. To produce the hCS f...

  • Article
  • Open Access
92 Citations
7,748 Views
14 Pages

18 April 2019

The effects of Ca/Si ratio, aluminum and magnesium on the carbonation behavior of calcium silicate hydrate (C-S-H) were investigated by using X-ray powder diffraction (XRD), nuclear magnetic resonance (NMR) and thermogravimetric analyzer (TGA). The r...

  • Article
  • Open Access
25 Citations
6,335 Views
18 Pages

30 March 2018

Calcium-silicate-hydrate (CSH)/polymer nanocomposites were synthesized with the layer-by-layer (LBL) method, and their morphology and mechanical properties were investigated using atomic force microscopy (AFM) imaging and AFM nanoindentation. Differe...

  • Article
  • Open Access
10 Citations
4,516 Views
20 Pages

Quantitative Evaluation of Carbon Fiber Dispersion in Amorphous Calcium Silicate Hydrate-Based Contact-Hardening Composites

  • Guangxiang Ji,
  • Guangqi Xiong,
  • Xiaoqin Peng,
  • Shuping Wang,
  • Chong Wang,
  • Keke Sun and
  • Lu Zeng

30 January 2021

Carbon fiber dispersion has a substantial influence on the properties of amorphous calcium silicate hydrate-based contact-hardening composites. In this study, a mixture of carbon fiber and calcium silicate hydrate powder was compressed into solid com...

  • Article
  • Open Access
9 Citations
4,231 Views
10 Pages

28 August 2021

The interaction of EDTA with calcium silicate hydrate (C-S-H) and its impact on the sorption of U(VI) by C-S-H in the presence of EDTA at varying concentrations has been investigated under N2 and ambient atmosphere. The solid phase characterization w...

  • Article
  • Open Access
6 Citations
2,213 Views
17 Pages

30 November 2023

The failure of the interfacial transition zone has been identified as the primary cause of damage and deterioration in cement-based materials. To further understand the interfacial failure mechanism, interfacial composite structures between the main...

  • Article
  • Open Access
12 Citations
4,021 Views
16 Pages

Microstructure, Thermal Stability, and Catalytic Activity of Compounds Formed in CaO-SiO2-Cr(NO3)3-H2O System

  • Domante Niuniavaite,
  • Kestutis Baltakys,
  • Tadas Dambrauskas,
  • Anatolijus Eisinas,
  • Dovile Rubinaite and
  • Andrius Jaskunas

In this work, the thermal stability, microstructure, and catalytic activity in oxidation reactions of calcium silicate hydrates formed in the CaO-SiO2-Cr(NO3)3-H2O system under hydrothermal conditions were examined in detail. Dry primary mixture with...

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