Materials, Volume 18, Issue 10
2025 May-2 - 248 articles
Cover Story: The oxidative dehydrogenation (ODH) of ethanol to acetaldehyde is an important production process. However, it tends to suffer from low activity, selectivity, and high costs. Herein, we have developed a new strategy for preparing mesoporous nitrogen-doped carbon catalysts. The C=O functional group on the catalyst surface is found to be the active center, with the introduction of nitrogen atoms reducing the adsorption capacity of acetaldehyde molecules on the active site, improving selectivity to acetaldehyde. This work reveals the structure–activity relationship of nitrogen-doped carbon-based catalysts in ethanol ODH, providing a theoretical basis for the development of efficient non-metallic carbon-based catalysts for this reaction. View this paper - Issues are regarded as officially published after their release is announced to the table of contents alert mailing list .
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