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Sustainable Functional Coatings and Surface Engineering: Materials, Processes, and Applications

A special issue of Molecules (ISSN 1420-3049). This special issue belongs to the section "Applied Chemistry".

Deadline for manuscript submissions: 31 October 2026 | Viewed by 1701

Editor

Department of Chemistry, Kyungpook National University, Daegu 41566, Republic of Korea
Interests: bioinspired materials; polyphenol chemistry; surface and interface engineering; sustainable polymers; functional coatings; biomaterials; adhesive hydrogels; polymer informatics; green chemistry

Special Issue Information

Dear Colleagues,

This Special Issue highlights the sustainable functional coatings and surface engineering strategies that improve performance, durability, and environmental compatibility across diverse substrates and use conditions. We particularly welcome papers on the advances in eco-friendly and bioinspired coating chemistries that deliver high-value surface functions—such as anti-fouling, corrosion resistance, adhesion control, barrier properties, antimicrobial activity, wettability tuning, and flame retardancy—while minimizing hazardous reagents, high-energy processing, and persistent fluorinated components. Submissions may address coating design principles, interfacial mechanisms, and scalable processing routes including solution/sol–gel methods, layer-by-layer assembly, spray/spin/dip coating, electrochemical approaches, and plasma/laser surface structuring. For flame-retardant coatings, contributions that elucidate char formation, heat/smoke suppression, self-extinguishing behavior, durability under abrasion/washing, and performance on textiles, polymers, wood, and metals are especially encouraged. Studies that establish clear structure–property relationships through rigorous characterization (e.g., wettability, adhesion, mechanical robustness, thermal stability, LOI/UL-94, cone calorimetry, smoke toxicity) are of high interest. Application-driven demonstrations for infrastructure, transportation, electronics, packaging, and protective materials are welcome, as are works that quantify sustainability metrics such as renewability, water-based formulations, low-VOC processing, and life-cycle considerations. Both original articles and comprehensive reviews synthesizing emerging directions and translational opportunities are encouraged.

Dr. Kyueui Lee
Guest Editor

Manuscript Submission Information

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Keywords

  • sustainable coatings
  • surface engineering
  • flame-retardant coatings
  • green chemistry
  • bioinspired materials
  • barrier coatings
  • anti-fouling
  • corrosion protection
  • multifunctional interfaces
  • scalable coating processes

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Published Papers (2 papers)

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Research

17 pages, 8387 KB  
Article
Simultaneous Enhancement of Mildew Resistance and Dimensional Stability of Bamboo with a Facile One-Step In Situ Growth of ZnO/TA/Ag Composites
by Juan Xu, Jinju Ma, Lanxiang Liu, Baoshan Tang, Hong Zhang, Wenwen Zhang and Zhengjun Shi
Molecules 2026, 31(10), 1737; https://doi.org/10.3390/molecules31101737 - 19 May 2026
Viewed by 322
Abstract
Bamboo is a renewable and fast-growing biomass resource with limited utilization and service life owing to its susceptibility to mold. Conventional nano-modification methods, particularly two-step approaches, are limited by weak interfacial bonding between nanoparticles and the bamboo substrate, complex processing, and an inability [...] Read more.
Bamboo is a renewable and fast-growing biomass resource with limited utilization and service life owing to its susceptibility to mold. Conventional nano-modification methods, particularly two-step approaches, are limited by weak interfacial bonding between nanoparticles and the bamboo substrate, complex processing, and an inability to simultaneously enhance antimildew performance and dimensional stability. To address these limitations, we developed a one-step hydrothermal method involving the use of tannic acid (TA) for in situ fabrication of ZnO/TA/Ag composite particles on bamboo surfaces. Process parameters were optimized to 100 °C, 10 h, and a zinc acetate-to-tannic acid molar ratio of 20:1. The modified bamboo was characterized using Fourier-transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, scanning electron microscopy coupled with energy-dispersive spectroscopy, and thermogravimetric analysis. We demonstrated that ZnO/TA/Ag composite particles were successfully loaded onto the bamboo surface, thus improving the all-around performance of the bamboo simultaneously. Antimildew activity against Aspergillus niger and Penicillium citrinum increased from grade 4 in untreated bamboo to grades 1 and 0, respectively; water absorption decreased by 52.85%, and anti-swelling efficiency reached 30.41%, indicating improved mold resistance and dimensional stability. Thus, our technique could serve as a green and efficient one-step in situ modification strategy for high-performance functionalization of bamboo, making it suitable for applications in humid outdoor and indoor environments. Full article
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14 pages, 4346 KB  
Article
Polarization-Controlled Femtosecond Laser Texturing Enables Robust Antifouling Stainless Steel Surfaces
by Eunyeop Ji, Daesik Ko, Chan Hyeon Yang, Vassilia Zorba, Jung Hwan Park, Kyueui Lee and Minok Park
Molecules 2026, 31(3), 480; https://doi.org/10.3390/molecules31030480 - 29 Jan 2026
Cited by 1 | Viewed by 1121
Abstract
In this work, we demonstrate precise control over laser-induced periodic surface structures (LIPSS) on stainless steel (SS) using femtosecond (fs) laser processing to suppress bacterial adhesion. We systematically compare the antifouling behavior of laser-textured surfaces with distinct pattern directionalities—linear and circular. Fs laser [...] Read more.
In this work, we demonstrate precise control over laser-induced periodic surface structures (LIPSS) on stainless steel (SS) using femtosecond (fs) laser processing to suppress bacterial adhesion. We systematically compare the antifouling behavior of laser-textured surfaces with distinct pattern directionalities—linear and circular. Fs laser irradiation with linear polarization produces directional and anisotropic LIPSS, which progressively evolve into more complex hierarchical surface textures as processing conditions vary. In contrast, fs laser irradiation with circular polarization yields isotropic surface morphologies. Despite these morphological differences, the surface wettability remains nearly constant, with contact angles confined to a narrow range of 32.6–36.9°. Bacterial adhesion tests using Escherichia coli reveal that surfaces patterned with anisotropic features generated by linear polarization—particularly at an incident power of 30 mW—exhibit enhanced antifouling performance compared to isotropic counterparts. These results indicate that antifouling efficacy is governed not only by surface wettability but also by the spatial organization and anisotropy of the LIPSS. This study highlights the critical role of polarization-controlled fs laser processing in tailoring surface architectures and provides a rational strategy for designing bio-resistant metallic surfaces. Full article
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