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15 Results Found

  • Article
  • Open Access
2 Citations
2,562 Views
16 Pages

12 April 2022

Soft nanomaterials like aerogels are subject to thermal fluctuations, so that their structure randomly fluctuates with time. Neutron elastic and inelastic scattering experiments provide unique structural and dynamic information on such systems with n...

  • Review
  • Open Access
5 Citations
4,630 Views
27 Pages

Water and Ion Dynamics in Confined Media: A Multi-Scale Study of the Clay/Water Interface

  • Patrice Porion,
  • Ali Asaad,
  • Thomas Dabat,
  • Baptiste Dazas,
  • Alfred Delville,
  • Eric Ferrage,
  • Fabien Hubert,
  • Mónica Jiménez-Ruiz,
  • Laurent J. Michot and
  • Sébastien Savoye
  • + 1 author

This review details a large panel of experimental studies (Inelastic Neutron Scattering, Quasi-Elastic Neutron Scattering, Nuclear Magnetic Resonance relaxometry, Pulsed-Gradient Spin-Echo attenuation, Nuclear Magnetic Resonance Imaging, macroscopic...

  • Article
  • Open Access
5 Citations
2,270 Views
19 Pages

Variation of Structural and Dynamical Flexibility of Myelin Basic Protein in Response to Guanidinium Chloride

  • Luman Haris,
  • Ralf Biehl,
  • Martin Dulle,
  • Aurel Radulescu,
  • Olaf Holderer,
  • Ingo Hoffmann and
  • Andreas M. Stadler

Myelin basic protein (MBP) is intrinsically disordered in solution and is considered as a conformationally flexible biomacromolecule. Here, we present a study on perturbation of MBP structure and dynamics by the denaturant guanidinium chloride (GndCl...

  • Review
  • Open Access
21 Citations
5,081 Views
32 Pages

21 August 2020

The physical properties of polymers depend on a range of both structural and chemical parameters, and in particular, on molecular topology. Apparently simple changes such as joining chains at a point to form stars or simply joining the two ends to fo...

  • Article
  • Open Access
5 Citations
3,911 Views
12 Pages

Influence of Concentration Fluctuations on Relaxation Processes in Spin Glasses

  • Julia N. Wagner,
  • Wolfgang Häußler,
  • Olaf Holderer,
  • Andreas Bauer,
  • Stephen M. Shapiro and
  • Peter Böni

Using the unique combination of atomically resolved atom probe tomography (APT) and volume averaged neutron (resonance) spin echo (NRSE and NSE) experiments, the influence of nano-scaled clusters on the spin relaxation in spin glasses was studied. Fo...

  • Article
  • Open Access
3 Citations
3,222 Views
18 Pages

28 February 2023

The interaction of many peptides with lipid bilayer membranes strongly depends on the lipid composition. Here, a study of the impact of unsaturated lipid acyl chains on the interaction of a derivative of the HIV-1 fusion peptide with lipid bilayer ve...

  • Feature Paper
  • Article
  • Open Access
7 Citations
4,115 Views
12 Pages

Nanoscale Bending Dynamics in Mixed-Chain Lipid Membranes

  • Elizabeth G. Kelley,
  • Moritz P. K. Frewein,
  • Orsolya Czakkel and
  • Michihiro Nagao

9 January 2023

Lipids that have two tails of different lengths are found throughout biomembranes in nature, yet the effects of this asymmetry on the membrane properties are not well understood, especially when it comes to the membrane dynamics. Here we study the na...

  • Article
  • Open Access
2 Citations
3,302 Views
11 Pages

Transmission Bender as an Analyzer Device for MIEZE

  • Johanna K. Jochum,
  • Jos F. K. Cooper,
  • Lukas M. Vogl,
  • Peter Link,
  • Olaf Soltwedel,
  • Peter Böni,
  • Christian Pfleiderer and
  • Christian Franz

MIEZE (Modulation of IntEnsity with Zero Effort) spectroscopy is a high-resolution spin echo technique optimized for the study of magnetic samples and samples under depolarizing conditions. It requires a polarization analyzer in between spin flippers...

  • Article
  • Open Access
7 Citations
4,171 Views
17 Pages

Alkanes as Membrane Regulators of the Response of Early Membranes to Extreme Temperatures

  • Loreto Misuraca,
  • Antonino Caliò,
  • Josephine G. LoRicco,
  • Ingo Hoffmann,
  • Roland Winter,
  • Bruno Demé,
  • Judith Peters and
  • Philippe M. Oger

17 March 2022

One of the first steps in the origin of life was the formation of a membrane, a physical boundary that allowed the retention of molecules in concentrated solutions. The proto-membrane was likely formed by self-assembly of simple readily available amp...

  • Article
  • Open Access
6 Citations
2,925 Views
10 Pages

9 December 2020

The translational motion of polymers is a complex process and has a big impact on polymer structure and chemical reactivity. The process can be described by the segment velocity autocorrelation function or its diffusion spectrum, which exhibit severa...

  • Article
  • Open Access
3 Citations
3,775 Views
6 Pages

Measurements of Dynamic Contributions to Coherent Neutron Scattering

  • Sebastian Jaksch,
  • Alexandros Koutsioubas,
  • Stefan Mattauch,
  • Olaf Holderer and
  • Henrich Frielinghaus

In this manuscript, we are investigating the contribution of dynamic membrane properties of phospholipid membranes to coherent scattering signals under grazing incidence. Spectroscopic measurements under grazing incidence can provide useful insight i...

  • Review
  • Open Access
9 Citations
3,961 Views
38 Pages

Disordered molecular solids present a rather broad class of substances of different origin—amorphous polymers, materials for photonics and optoelectronics, amorphous pharmaceutics, simple molecular glass formers, and others. Frozen biological m...

  • Article
  • Open Access
8 Citations
3,312 Views
14 Pages

Collective Motions and Mechanical Response of a Bulk of Single-Chain Nano-Particles Synthesized by Click-Chemistry

  • Jon Maiz,
  • Ester Verde-Sesto,
  • Isabel Asenjo-Sanz,
  • Peter Fouquet,
  • Lionel Porcar,
  • José A. Pomposo,
  • Paula Malo de Molina,
  • Arantxa Arbe and
  • Juan Colmenero

25 December 2020

We investigate the effect of intra-molecular cross-links on the properties of polymer bulks. To do this, we apply a combination of thermal, rheological, diffraction, and neutron spin echo experiments covering the inter-molecular as well as the interm...

  • Article
  • Open Access
4 Citations
4,071 Views
11 Pages

Determining the Bending Rigidity of Free-Standing Planar Phospholipid Bilayers

  • Oscar Zabala-Ferrera,
  • Paige Liu and
  • Peter J. Beltramo

19 January 2023

We describe a method to determine membrane bending rigidity from capacitance measurements on large area, free-standing, planar, biomembranes. The bending rigidity of lipid membranes is an important biological mechanical property that is commonly opti...

  • Article
  • Open Access
35 Citations
8,782 Views
21 Pages

4 August 2016

We have performed molecular dynamics (MD) simulations of melt systems consisting of a small number of long ring poly(ethylene oxide) (PEO) probes immersed in a host matrix of linear PEO chains and have studied their microscopic dynamics and topology...