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Inorganics, Volume 7, Issue 11 (November 2019)
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Cover Story (view full-size image) A discrete Zn-based metallocycle can be exploited as a platform to self-assemble intertwined [...] Read more. A discrete Zn-based metallocycle can be exploited as a platform to self-assemble intertwined polyrotaxane-like architectures by using an ancillary ligand that coordinates the metallocycle. The proposed approach builds up entangled structures, starting from metallocycles with two main features: (i) host–guest properties and (ii) metal centers capable of expanding their coordination sphere. When pyridine is used as an ancillary ligand, a polyrotaxane with a rare 1D + 1D -> 1D topology is self-assembled. The entangled architectures are driven and supported by π···π stacking. View this paper.