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Next-Generation Low-Dimensional Semiconductor Materials: Synthesis and Applications for Photocatalysis and Photodetection

A special issue of Materials (ISSN 1996-1944). This special issue belongs to the section "Electronic Materials".

Deadline for manuscript submissions: 1 January 2026 | Viewed by 502

Special Issue Editors


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Guest Editor
Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Optoelectronic Science and Engineering, South China Normal University, Guangzhou 510006, China
Interests: nanophotonics; optoelectronics; laser fabrication; biosensor; photodetector
Special Issues, Collections and Topics in MDPI journals

E-Mail Website
Guest Editor
Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Optoelectronic Science and Engineering, South China Normal University, Guangzhou 510006, China
Interests: sensor; functional 2D materials; optoelectronics; synthetic chemistry; photocatalysis; photodetector
Special Issues, Collections and Topics in MDPI journals

E-Mail Website
Guest Editor
Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin 150040, China
Interests: photoelectrochemical; catalysis; biosensor; materials chemistry

Special Issue Information

Dear Colleagues,

Low-dimensional semiconductors (0D, 1D, 2D) exhibit quantum confinement effects and tunable optoelectronic properties, enabling breakthroughs in energy conversion, environmental remediation, and high-sensitivity photodetection. This Special Issue seeks to advance the synthesis, characterization, and application of low-dimensional semiconductors, emphasizing scalable fabrication, stability enhancement, and device integration for sustainable energy and sensing technologies.

Research History

  • Post-2020: Integration of 2D materials (MoS2, MXenes) and stimuli-responsive systems for adaptive optoelectronics.
  • 2010s–2020s: Emergence of hybrid materials (e.g., plasmonic–semiconductor nanostructures) and organic–inorganic perovskites, improving responsivity and catalytic efficiency.
  • 2000s–2010s: Focus on inorganic nanowires (e.g., ZnO, CdS) and graphene for UV photodetectors and photocatalytic water splitting.

Latest Research Progress

  • Plasmonic Hybrids: Enhanced light–matter interaction in Au/ZnO and graphene/MoS2 heterostructures for ultrasensitive photodetection and SERS-based biosensing.
  • Perovskite Nanocrystals: CsCu2I3 and Cs3Cu2I5 demonstrate high photoluminescence quantum yield (PLQY >80%) for photocatalytic CO2 reduction.
  • Flexible Organic Crystals: Low-dimensional organic semiconductors (e.g., S-BF2 nanowires) enable wearable UV photodetectors and optically pumped lasers 1013.
  • 2D Ferroelectrics: Materials like 1T′-MoS2 show room-temperature ferroelectricity, which is promising for non-volatile memory and energy-efficient photodetectors.

We invite contributions addressing, but not limited to, the following:

  • Synthesis: Novel methods (CVD, solution-phase epitaxy) for low-dimensional materials (quantum dots, nanowires, 2D perovskites).
  • Characterization: Advanced techniques (in situ TEM, low-wave Raman spectroscopy) to probe atomic-scale structure–property relationships.
  • Applications: Photocatalysis (H2 generation, pollutant degradation), photodetectors (UV-IR range), and integrated systems (e.g., perovskite/organic tandems).

We welcome the following:

  • Original Research: Innovations in material design (e.g., defect engineering, phase-selective synthesis).
  • Reviews: Critical analyses of challenges in scalability, stability, and interfacial charge transfer.
  • Device Studies: Photodetectors with ultrahigh responsivity (>10⁴ A/W) or photocatalysts with >90% quantum efficiency.
  • Theoretical Work: Computational modeling of exciton dynamics, carrier mobility, and heterostructure interfaces.

Prof. Dr. Lijun Wu
Dr. Jagadeesh Suriyaprakash
Dr. Lianwei Shan
Guest Editors

Manuscript Submission Information

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Keywords

  • low-dimensional semiconductors
  • quantum-confined nanomaterials
  • plasmonic–semiconductor hybrids
  • photocatalytic CO2 reduction
  • ultrahigh-responsivity photodetectors
  • 2D perovskites
  • solution-phase epitaxy
  • exciton dynamics
  • flexible optoelectronics
  • defect engineering in nanostructures

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Published Papers (1 paper)

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Review

28 pages, 6012 KiB  
Review
Semiconductor-Based Photoelectrocatalysts in Water Splitting: From the Basics to Mechanistic Insights—A Brief Review
by W. J. Pech-Rodríguez, Nihat Ege Şahin, G. G. Suarez-Velázquez and P. C. Meléndez-González
Materials 2025, 18(9), 1952; https://doi.org/10.3390/ma18091952 - 25 Apr 2025
Viewed by 370
Abstract
Hydrogen and oxygen serve as energy carriers that can ease the transition of energy due to their high energy densities. Nonetheless, their production processes entail the development of efficient and low-cost storage and conversion technologies. In this regard, photoelectrocatalysts are materials based on [...] Read more.
Hydrogen and oxygen serve as energy carriers that can ease the transition of energy due to their high energy densities. Nonetheless, their production processes entail the development of efficient and low-cost storage and conversion technologies. In this regard, photoelectrocatalysts are materials based on the photoelectronic effect where electrons and holes interact with H2O, producing H2 and O2, and in some cases, this is achieved with acceptable efficiency. Although there are several reviews on this topic, most of them focus on traditional semiconductors, such as TiO2 and ZnO, neglecting others, such as those based on non-noble metals and organic ones. Herein, semiconductors like CdSe, NiWO4, Fe2O3, and others have been investigated and compared in terms of photocurrent density, band gap, and charge transfer resistance. In addition, this brief review aims to discuss the mechanisms of overall water-splitting reactions from a photonic point of view and subsequently discusses the engineering of material synthesis. Advanced composites are also addressed, such as WO3/BiVO4/Cu2O and CN-FeNiOOH-CoOOH, which demonstrate high efficiency by delivering photocurrent densities of 5 mAcm−2 and 3.5 mA cm−2 at 1.23 vs. RHE, respectively. Finally, the authors offer their perspectives and list the main challenges based on their experience in developing semiconductor-based materials applied in several fields. In this manner, this brief review provides the main advances in these topics, used as references for new directions in designing active materials for photoelectrocatalytic water splitting. Full article
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