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Recent Advances in Magnetic and Electronic Materials and Their Applications

A special issue of Materials (ISSN 1996-1944). This special issue belongs to the section "Electronic Materials".

Deadline for manuscript submissions: 20 April 2026 | Viewed by 7000

Special Issue Editors


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Guest Editor
Key Laboratory for Anisotropy and Texture of Materials (Ministry of Education), School of Material Science and Engineering, Northeastern University, Shenyang 110819, China
Interests: magnetic materials; spintronics; first-principle calculation; memristor; 2D magnetic materials; topological materials; spin transport; spin valves; single-molecule magnets

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Guest Editor
Department of Physics, Freie Universität Berlin, 14195 Berlin, Germany
Interests: spintronics; first-principle calculation; terahertz spintronics

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Guest Editor
Zhejiang Laboratory, Hangzhou 311100, China
Interests: magnetic materials; single-molecule magnets; haptic devices; sensors; actuators

Special Issue Information

Dear Colleagues,

Magnetic and electronic materials can respond to external magnetic and electronic fields, exhibiting unique physical properties. They have broad applications in various technological fields, including data storage, sensors, medical imaging, and energy conversion. The development of magnetic and electronic functional materials has recently gained significant attention in the fields of solid-state physics, materials science, and engineering. To obtain high-performance materials, scientists have implemented various strategies such as predicting and synthesizing new magnetic and electronic materials through alloying, energy band engineering, element doping, etc. These strategies have greatly promoted the application of functional materials. By continuously optimizing the magnetic and electronic properties, innovative strategies provide new possibilities for future industrial applications in magnetic and electronic technological fields.

We are pleased to invite you to submit your research to this Special Issue, entitled "Recent Advances in Magnetic and Electronic Materials and Their Applications".

This Special Issue, entitled “Recent Advances in Magnetic and Electronic Materials and Their Applications”, aims to provide a unique international forum for researchers working in magnetic and electronic functional materials to report on their latest endeavors in advancing this field. Topics of interest include the following: new pristine magnetic and electronic materials, strategies to improve the performance, theoretical understanding, physical insights into engineering high-performance magnetic and electronic materials, computational discovery of new materials, and more. This Special Issue seeks to collate cutting-edge research and developments in the field, fostering collaboration and innovation among scientists and engineers dedicated to exploring and enhancing the capabilities of magnetic and electronic functional materials.

In this Special Issue, original research articles and reviews are welcome to be submitted. Research areas may include, but are not limited to, the following: magnetic materials; electronic materials; electronic transition; 2D magnetic materials; antiferromagnetic materials; half-metal; topological materials; spin transport; spinterface; single-molecule magnets; spin–orbit torque; spin Hall effect; multiferroic materials; and magnetoresistance.

We look forward to receiving your contributions.

Prof. Dr. Xianmin Zhang
Dr. Junwei Tong
Dr. Liuxia Ruan
Guest Editors

Manuscript Submission Information

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Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Materials is an international peer-reviewed open access semimonthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2600 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • magnetic materials
  • electronic materials
  • 2D materials
  • antiferromagnetic
  • spintronics
  • topological materials
  • Curie temperature
  • magnetoresistance
  • phase transition
  • electronic transition

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Published Papers (6 papers)

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Research

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14 pages, 7130 KB  
Article
The Ta Seed-Buffer Layer Microstructure and Its Influence on the Magnetic and Structural Parameters of CoFeB/MgO Layers
by Jarosław Kanak, Monika Cecot, Witold Skowroński, Antoni Żywczak, Marta Gajewska, Jerzy Wrona, Wiesław Powroźnik and Maciej Czapkiewicz
Materials 2025, 18(24), 5558; https://doi.org/10.3390/ma18245558 - 11 Dec 2025
Viewed by 414
Abstract
In this paper, we discuss the structural and magnetic properties of Ta(d)/Co40Fe40B20/MgO/Ta multilayers. The CoFeB wedge layer was deposited on three buffers differing in Ta layer thickness: d = 5, 10, and 15 nm. A [...] Read more.
In this paper, we discuss the structural and magnetic properties of Ta(d)/Co40Fe40B20/MgO/Ta multilayers. The CoFeB wedge layer was deposited on three buffers differing in Ta layer thickness: d = 5, 10, and 15 nm. A structural analysis showed that the Ta seed-buffer of 5 nm was amorphous, whereas thicker Ta grew in a β-tetragonal disordered structure. X-ray reflectivity measurements revealed that the Ta/CoFeB interface roughness for annealed samples ranged from 0.55 to 0.67 nm for a sample with a 0.85 nm CoFeB layer and decreased to approximately 0.47 nm for thicker CoFeB layers, while the average interface CoFeB/MgO thickness was about 0.2–0.3 nm. The morphological roughness of the amorphous single 5 nm Ta layer was the lowest, whereas crystalline grains in thicker Ta buffers induced higher roughness. The 5 nm thick MgO layer exhibited a strong (001)-oriented texture, which was the highest for the smoothest 5 nm Ta buffer. The magnetic dead layer thickness for the annealed sample with a 15 nm Ta buffer was 0.39 nm and increased with the decrease in the Ta buffer thickness. Temperature-dependent measurements offered further insight into the diffusion processes and the formation of the magnetic dead layer (MDL) at the Ta/CoFeB interface. Full article
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19 pages, 4484 KB  
Article
Near-Compensated Ferrimagnetism in Disordered Co0.5Mn1.5Al Half-Heusler Alloy: Experimental and Theoretical Studies
by Emese Bender, Răzvan Hirian, Cristian Leoştean, Roman Atanasov, Radu George Haţegan, Lucian Barbu-Tudoran and Diana Benea
Materials 2025, 18(19), 4449; https://doi.org/10.3390/ma18194449 - 23 Sep 2025
Viewed by 898
Abstract
This study investigates the electronic, magnetic, and transport properties of the Co0.5Mn1.5Al half-Heusler alloy, a promising candidate for spintronic applications due to its potential half-metallic and ferrimagnetic characteristics. Experimental efforts focus on structural characterization using X-ray diffraction to examine [...] Read more.
This study investigates the electronic, magnetic, and transport properties of the Co0.5Mn1.5Al half-Heusler alloy, a promising candidate for spintronic applications due to its potential half-metallic and ferrimagnetic characteristics. Experimental efforts focus on structural characterization using X-ray diffraction to examine substitutional disorder, such as Co/Mn site migration and Mn/Al site mixing, and their impacts on magnetic and transport properties. Magnetic characterization, including magnetization and susceptibility, reveals an N-type ferrimagnetic behaviour with a Curie temperature of 670 K. Transport experiments probe resistance and magnetoresistance across various temperatures and magnetic fields to uncover conduction mechanisms and spin-dependent effects. Theoretical band structure calculations, utilizing the Korringa–Kohn–Rostoker Green’s function method, investigate the electronic structure and the role of disorder in shaping magnetic and transport properties. This integrated experimental and theoretical approach aims to clarify the alloy’s suitability for applications in exchange bias or antiferromagnetic spintronics. Full article
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17 pages, 2892 KB  
Article
Stoichiometry of Bulk Nb1−βSnβ Superconductors Synthesised by Arc Melting
by Mahboobeh Shahbazi, Henrietta E. Cathey, Ali Dehghan Manshadi, Jose Alarco and Ian D. R. Mackinnon
Materials 2025, 18(13), 3050; https://doi.org/10.3390/ma18133050 - 27 Jun 2025
Viewed by 861
Abstract
We present an alternative process for production of binary Nb1−βSnβ superconducting phases using pre- and post-treatment of arc-melted Nb + Sn ingots. This process combines sequential sintering, arc melting, and annealing procedures that provide dense, bulk samples of Nb1−β [...] Read more.
We present an alternative process for production of binary Nb1−βSnβ superconducting phases using pre- and post-treatment of arc-melted Nb + Sn ingots. This process combines sequential sintering, arc melting, and annealing procedures that provide dense, bulk samples of Nb1−βSnβ with varying stoichiometry between 0.18 < β < 0.25 depending on annealing time and temperature. We show, through magnetization measurements of these Nb1−βSnβ bulks, that annealing of arc-melted samples at 900 °C for 3 h significantly enhances Jc values compared with arc-melted Nb1−βSnβ samples without annealing. Microstructural analyses show that optimum grain size and orientation are achieved by sintering and annealing at lower temperatures (i.e., 720 °C and 900 °C, respectively) with short annealing times (i.e., <10 h). Processing at higher temperatures and for longer times enhances grain growth and results in fewer pinning centres. The optimum process creates effective pinning centres that deliver a Jc = 6.16 × 104 A/cm2 at 10 K (and ~0.2 T), compared with Jc = 3.4 × 104 A/cm2 for Nb1−βSnβ subjected to a longer annealing time at a higher temperature and Jc = 775 A/cm2 for an arc-melted sample without post-annealing. We suggest that further work addressing post-treatment annealing times between 3 h < tpost < 60 h at temperatures between 900 °C and 1000 °C will provide the opportunity to control stoichiometric and microstructural imperfections in bulk Nb1−βSnβ materials. Full article
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14 pages, 3776 KB  
Article
Magnetocaloric Properties and Microstructures of HoB2 and Nb-Substituted HoB2
by Mahboobeh Shahbazi, Ali Dehghan Manshadi, Kiran Shinde and Ian D. R. Mackinnon
Materials 2025, 18(4), 866; https://doi.org/10.3390/ma18040866 - 17 Feb 2025
Cited by 1 | Viewed by 1222
Abstract
We report on the arc melt syntheses of HoB2 and Nb-substituted HoB2 polycrystalline ingots and their magnetocaloric and microstructural properties. XRD data and microstructural analysis reveal that a nominal 10% Nb addition during synthesis results in changes to unit cell parameters [...] Read more.
We report on the arc melt syntheses of HoB2 and Nb-substituted HoB2 polycrystalline ingots and their magnetocaloric and microstructural properties. XRD data and microstructural analysis reveal that a nominal 10% Nb addition during synthesis results in changes to unit cell parameters and grain morphology. Interpretation of the refined cell parameters using Vegard’s law shows that Nb substitutes into HoB2 with stoichiometry Ho0.93Nb0.07B2. Arc-melted products are polycrystalline bulk samples containing minor phases such as Ho2O3, Ho, and HoB4. Nb substitution results in a smaller grain size (~sub-micron) and a higher Curie temperature, TC, compared to HoB2. With a 10 T applied field, the maximum magnetic entropy, ΔSM, for HoB2 and for Ho0.93Nb0.07B2, is 46.8 Jkg−1K−1 and 38.2 Jkg−1K−1 at 18 K and 21 K, respectively. Both samples show second-order phase transitions. Despite high totals of minor phases (e.g., ~10 wt.% and ~25 wt.%), the calculated relative cooling powers are greater than 1300 Jkg−1 and 600 Jkg−1 at 10 T and 5 T, respectively. The magnetocaloric properties of both samples are consistent with Holmium boride compounds prepared via alternative methods. Full article
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14 pages, 4706 KB  
Article
Valley-Related Multipiezo Effect in Altermagnet Monolayer V2STeO
by Yufang Chang, Yanzhao Wu, Li Deng, Xiang Yin and Xianmin Zhang
Materials 2025, 18(3), 527; https://doi.org/10.3390/ma18030527 - 24 Jan 2025
Cited by 7 | Viewed by 1766
Abstract
The multipiezo effect realizes the coupling of strain with magnetism and electricity, which provides a new way of designing multifunctional devices. In this study, monolayer V2STeO is demonstrated to be an altermagnet semiconductor with a direct band gap of 0.41 eV. [...] Read more.
The multipiezo effect realizes the coupling of strain with magnetism and electricity, which provides a new way of designing multifunctional devices. In this study, monolayer V2STeO is demonstrated to be an altermagnet semiconductor with a direct band gap of 0.41 eV. The spin splittings of monolayer V2STeO are as high as 1114 and 1257 meV at the valence and conduction bands, respectively. Moreover, a pair of energy degeneracy valleys appears at X and Y points in the first Brillouin zone. The valley polarization and reversion can be achieved by applying uniaxial strains along different directions, indicating a piezovalley effect. In addition, a net magnetization coupled with uniaxial strain and hole doping can be induced in monolayer V2STeO, presenting the piezomagnetic feature. Furthermore, due to the Janus structure, the inversion symmetry of monolayer V2STeO is naturally broken, resulting in the piezoelectric property. The integration of the altermagnet, piezovalley, piezomagnetic, and piezoelectric properties make monolayer V2STeO a promising candidate for multifunctional spintronic and valleytronic devices. Full article
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Review

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28 pages, 597 KB  
Review
Ab Initio Calculations of Spin Waves: A Review of Theoretical Approaches and Applications
by Michael Neugum and Arno Schindlmayr
Materials 2025, 18(18), 4431; https://doi.org/10.3390/ma18184431 - 22 Sep 2025
Viewed by 1046
Abstract
Spin waves represent an important class of low-energy excitations in magnetic solids, which influence the thermodynamic properties and play a major role in technical applications, such as spintronics or magnetic data storage. Despite the enormous advances of ab initio simulations in materials science, [...] Read more.
Spin waves represent an important class of low-energy excitations in magnetic solids, which influence the thermodynamic properties and play a major role in technical applications, such as spintronics or magnetic data storage. Despite the enormous advances of ab initio simulations in materials science, quantitative calculations of spin-wave spectra still pose a significant challenge, because the collective nature of the spin dynamics requires an accurate treatment of the Coulomb interaction between the electrons. As a consequence, simple lattice models like the Heisenberg Hamiltonian are still widespread in practical investigations, but modern techniques like time-dependent density-functional theory or many-body perturbation theory also open a route to material-specific spin-wave calculations from first principles. Although both are in principle exact, actual implementations necessarily employ approximations for electronic exchange and correlation as well as additional numerical simplifications. In this review, we recapitulate the theoretical foundations of ab initio spin-wave calculations and analyze the common approximations that underlie present implementations. In addition, we survey the available results for spin-wave dispersions of various magnetic materials and compare the performance of different computational approaches. In this way, we provide an overview of the present state of the art and identify directions for further developments. Full article
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