We perform multi-fluid simulations to study plasma dynamics and particle acceleration, and to investigate the formation of potential dips and peaks during an arc discharge in a plasma chamber. The initial condition of the simulation corresponds to a stable arc discharge that has already ionized the gas. We note that establishing an arc discharge requires a voltage of hundreds to thousands of volts to initiate the spark. A stable arc current can then be formed and maintained at a low voltage (e.g., 100 volts) with a current of a few to tens of amperes. The stable arc discharge is then used as the initial condition.
We set the cathode electric potential at zero volts and the anode electric potential of 100, 300, or 500 volts as the simulation boundary condition. The externally imposed potential is a time-independent boundary condition and is used for solving the one-dimensional electrostatic Poisson’s equation by using the tridiagonal matrix algorithm. It is similar to the formation of a conducting channel (return stroke) in gas-discharge lamps or in the air before the occurrence of lightning. It should be noted that the kink/sausage modes with their two-dimensional structure cannot occur in the one-dimensional approximation. In the proposed model, the emitted electrons at the cathode surface could further lead to the two-stream instability.
3.1. The Governing Equations
The discharge and current flow are mostly aligned along this thin, elongated conducting tube. Hence, we simplify the key physical process into a one-dimensional problem, similar to the approach for the conducting channel associated with lightning [
18]. Under this approximation, we developed a one-dimensional multi-fluid simulation code along the
x-axis to study the formation of the electrostatic potential in the arc discharge. The governing equations are Poisson’s equation in electrostatics:
the continuity equation:
the momentum equation:
and the ideal gas law:
where
e is the fundamental charge or
Coulomb,
is vacuum permittivity, and is
charge density. The subscript
indicates fluid species and can be electron (e) and proton (p), and the subscript “n” stands for “neutral”. The fluid quantities are number density
n, velocity
, pressure
p, the Boltzmann constant
J/K, charge
q, electric field
E, collision frequency for charge particles to neutral
and temperature
T. The real proton to electron mass ratio is used
. The diffusion of electron and ion velocities through viscosity will be included and discussed later.
In this paper, we use a three-fluid (electron, ion, and neutral) simulation. The electron and the ion are independent, with their own continuity equations and momentum equations. The quasi-neutrality is not assumed and not required.
In the simulation with the complete energy equation, we found that the arc plasma can be quickly heated to well above 1 eV. However, the plasma can be partially converted to other parts of the chamber, which lowers the plasma temperature in the conducting channel. The radiation loss also reduces the plasma temperature. The temperature of the plasma in the region where current flows through is estimated to be
6000 K [
19]. The simulation initial condition at
t = 0 corresponds to the time when the arc discharge is formed, and the plasma is heated to
We consider that the heating of the arc plasma from electricity and the heat loss through radiation and convection reach equilibrium during the simulation and that the temperature also reaches equilibrium in the conducting channel, which likely leads to constant temperature for all species
.
We have tried a different system length ranging from 2 to 50 mm, and the length can affect the stability of the simulation and the formation of electrostatic waves. In this paper, we present the results associated with the system length of 2 mm, 5 mm, 8 mm, 10 mm, 20 mm, 30 mm, 40 mm, and 50 mm. In the simulations, the length x is normalized by . The other normalization parameters are neutral number density for and , electric potential 1 volt, velocity m/s (velocity of 1 eV proton) and time . For , . The numerical time step and grid spacing are and . The neutrals in the conducting tube are assumed to be heated from 300 K to 6000 K. With a constant pressure across the chamber, the density in the conducting channel will be reduced as one-twentieth of .
The numerical time step was chosen to resolve the fastest physical time scale in the system. In the present simulations, the electron plasma frequency is on the order of Hz. In addition, the electron-neutral and proton-neutral collision frequencies are on the order of Hz and Hz, respectively. Therefore, the adopted time step, , is sufficiently small to resolve both the plasma oscillation time scale and the charge-neutral collision time scales. For example, when , s, and thus , which is much smaller than , and .
The grid spacing is selected based on our numerical experience with this model. To check the effect of grid resolution, we also repeat representative simulations using 1024 grid points. The main results, including the formation of the potential dip near the cathode and the subsequent potential peaks and dips caused by the electron-ion two-stream instability, do not change significantly. Therefore, 512 grid points are used in the simulations presented in the paper to reduce the computational cost while maintaining sufficient numerical resolution.
In the present simulation study, the effects of ionization and recombination are minor over the simulation time scale of tens of nanoseconds. The hot plasma only exists in the arc discharge region. The other initial parameters at
of our simulation are neutral density
charge densities
, boundary electric potential
, and velocities
The ionization ratio is determined by using Saha’s ionization equation [
20,
21]. The electron collisions are considered and lead to the high temperature at
. Saha’s equation [
20,
21] gives an ionized ratio of
for
. Since the ionization ratio is very small (
and the additional ionization and recombination effects are minor over the simulation time scale, the neutral density
and ion (electron) density
can be assumed as constant during the simulation.
The hydrogen gas is weakly ionized, with H
2 as the dominant neutral species. The proton-neutral collisional frequency [
22,
23,
24] is given by:
and the electron-neutral collisional frequency is given by:
Here, the proton-neutral collision cross-section is
and the electron-neutral collision cross-section
[
24]. Equation (6) gives that the electron-neutral collision frequency is on the order of
Hz. The term
in the momentum equation comes from the charge-neutral collision effect. Since the neutral fluid is affected mainly through the proton-neutral collisional effect, the proton-neutral collision frequency
is on the order of
Hz. Note here that the proton to neutral mass density ratio is
. The relation
gives that the neutral to proton collision frequency is
. As a result, the neutral-proton collision frequency is of the order of
Hz due to the high neutral density compared with the charged fluid. Hence, on the nanosecond time scale, the neutral fluid can be regarded as immobile during the simulation period, since the only momentum source for the neutral fluid is neutral-ion collisions. On the other hand, the collision effect exerts a “slowing-down” or drag force on the charged fluids.
The collision frequencies between protons and neutrons, as well as between electrons and neutrals, are described in Equations (5) and (6). The electron-neutral collision frequency
is on the order of
The proton-neutral collision frequency
is on the order of
The background geomagnetic field is assumed to be 0.5 G, and the gyro frequency of the electron can be obtained as follows:
The gyro frequency of a proton can be obtained as follows:
The results show that the collision frequencies of electrons and protons with neutrals are much higher than the gyro frequencies of electrons and protons. Moreover, the effects of the magnetic field generated by the current in the chamber on the electron dynamics are explained in
Supplementary Materials. An electron would suffer many collisions with neutrals before it could make a gyration. The gyration effect from the magnetic fields can be neglected.
In a weakly ionized gas, the electron and proton density diffusion coefficients due to thermal motion and collisions between charged and neutral fluids, to first order in the density, can be estimated as follows [
25]:
where
is the Boltzmann constant. We obtain
and
for
.
On the other hand, the coefficient associated with bulk viscosity without mass density for electron and proton fluids can be estimated as follows:
where
is a dimensionless factor in the range of 10–100 due to the fact that the bulk viscosity is usually 10–100 times higher than the shear viscosity with
. The bulk viscosity, used in the numerical simulation, is of the order of theoretical value.
At every time step, the density diffusion and velocity viscosity terms are applied to the charge density (
and
) and to the velocity (
and
) via a three-point smooth scheme based on the diffusion and viscosity coefficients, respectively. The smoothing scheme plays the role of dissipation and also reduces the steepening of the fluid, similar to the dissipation term in the Burger’s equation. The three-point smooth scheme is derived from the finite difference form of the diffusion equation:
where
and
for density or
for velocity.
In the continuity equations, a bounded (closed) boundary condition is used, i.e., the momentum and velocity are set to zero at the boundaries. However, the emission of electrons at the surface of the LaB
6 slab can lead to an increase in the electron density just outside the LaB
6 slab. The electron emission rate due to heating of LaB
6 slab is set to 10–15 amps [
26].
3.2. Two Simulation Cases Without and with Emission of Thermionic Electrons (
In order to examine the effect of the thermionic electron emission from LaB6, we simulate two cases without LaB6 and with LaB6.
Figure 3A shows a simulation without LaB
6 slab in the cathode and a 100 V electric potential is applied across the gas chamber
with
. For comparison,
Figure 3B shows the simulation results with the same parameters as in
Figure 3A, but a LaB
6 slab is applied in the cathode.
In
Figure 3A, an electric potential
is applied across the cathode (
. Some electrons in the plasma chamber are attracted by the applied positive potential at
to form a potential dip around point B. The lower potential at the cathode tends to attract ions to the left region between
and point A. The ion density near
is lower than the electron density near B. This may be due to a larger ion mass (lower electron mass) and hence a slower (faster) moving speed.
It is interesting to point out that the electric potential profile is similar to the potential distribution between the cathode and anode in
Figure 4 of the review paper by Anders [
14]. The potential drop between points B and C is the positive anode fall, while the potential drop between the origin and point A is the negative cathode fall.
In
Figure 3B, a simulation with a LaB
6 slab installed in the cathode and 100 V potential is applied in the 20 mm chamber (
) between the cathode and the anode. The neutral H
2 is filled with
, which is equivalent to the density of
. The thermionic electrons are emitted from the LaB
6 surface and carry a 10 A current. In this case, a potential dip near the LaB
6 surface can exceed 1000 volts. In the arc discharge, the two-stream instability occurs and leads to potential peaks of a few hundred volts. The theory of two-stream instability will be developed in the following simulation case.
In the simulation case shown in
Figure 4, the density and velocity distributions in the x–t plane show clearly the presence and growth of wavy patterns, which are caused by the electron-ion two-stream instability. This case shows a clear pattern of the electrostatic waves. The potential peak can reach nearly 11.4 kV at
, and the dip can reach about −0.6 kV (listed in Case 9 of
Table S1). The wavy potential structure may last for a few nanoseconds and quickly fades away. The number of peaks and dips depends on the plasma density and electron velocity. These waves are nearly stationary oscillations in the plasma (electron) frame and can move in the laboratory frame.
The electron-ion two-stream instability can be solved by the linear plasma dispersion relation:
where
is the electron plasma frequency,
is the proton plasma frequency, and
is the wave number [
3,
27,
28,
29]. The electron plasma frequency and the proton plasma frequency
and
) can be obtained from:
Here,
is the wave frequency. The linear dispersion relation is solved based on the electrostatic two-fluid equations for cold and homogeneous plasmas [
28]. Note that the plasma frequency is on the order of
Hz, about one order of magnitude higher than the electron-neutral collision frequency. Hence, the collision effect can be ignored when solving this dispersion relation.
The electron plasma frequency is estimated from the electron density used in the simulation. For approximately , the electron plasma frequency is approximately rad/s. The electron-neutral collision frequency is estimated from the neutral density, temperature, and electron-neutral collision cross section, as described in Equation (6). With the parameters used in the simulation, is on the order of Hz. Therefore, the statement that the plasma frequency is about one order of magnitude higher than the electron-neutral collision frequency is based on these calculated characteristic frequencies.
As illustrated in Lyu [
28], Equation (11) can be replaced as follows:
where
There are four roots in Equation (14). Only the roots with positive growth rate (
are plotted in
Figure 5. As shown in
Figure 5, there is a long channel tube, in which the wave structure can be analyzed by the Fourier analysis of
and
k. The solution of
with non-zero wave growth rate
gives (a) the wave frequency
and (b) the wave number
The maximum wave growth rate
occurs at
and
as shown in
Figure 5. The corresponding wavelength can be expressed as follows:
Based on the plasma parameters (
m/s,
, and obtain
from Equation (12)) and the linear theory, we obtain
and the maximum growth rate
from (15). For the simulation in
Figure 4, there are four potential peaks, and the corresponding wavelength is
, close to the theoretical value
In
Figure 6a, we plot the electric potential as a function of
x at different simulation times,
t = 0.9, 1.0, …, 1.2 ns. It can be seen that the magnitude of the electric potential peak and dip grows with time t for all four wave peaks and dips.
The growth rate of the electric potential Peak 2 can be calculated from electron density peak values at different times. The growth rate of peaks is plotted as a function of time in
Figure 6b. The growth rate of wave Peak 2 ranges from
to
, which is smaller than the maximum theoretical growth rate. This difference may be caused by the non-uniform profile of
and difference between the simulated wavelength
and theoretical peak wavelength
.
In
Figure 7, we show the simulation (Case B in
Figure 3B) results at time
0.9, 1.0, 1.1, and 1.2 ns. In this case, an electric potential dip is formed due to the high-density electron layer and the magnitude can reach one kilovolt as shown in the electric potential profiles.
Thermionic emitted electrons lead to the formation of an electron layer near the left boundary (). As a result of this electron layer, the electric potential has a sharp decrease from to . The electric potential then increases gradually to volts at the right boundary (anode). The potential difference between and at is large. The average electric field in the chamber is negative (). The negative electric field in the chamber will accelerate electrons to high speed m/s, while ions are accelerated in the left direction with small velocity due to their large mass. The electrons and ions are accelerated in the opposite directions, which can lead to the electron-ion two-stream instability. In the electric potential profile, large amplitude electrostatic waves are formed due to this instability, and the wave amplitude may reach tens of kilovolts. The electron and ion number density and velocity profiles also show similar patterns. The wavy potential structure may last for a few ns.
In
Figure 7, the peak electric potential can reach about 2000 V, the electric potential dip can reach −6.0 kV. Note that, in a weakly ionized plasma with temperature
0.5–0.75 eV, an electron can attach to a hydrogen atom H to form a negative hydrogen particle
. The density of negative hydrogen (
) is expected to be small compared with
density due to its low production rate [
30]. We ignore the contribution from
ions in the multi-fluid simulation. The formation of negative electric potential dips (positive electric potential peaks) can accelerate negative hydrogen ions (positive protons) toward the LaB
6 slab.
In the multi-fluid theory, unstable normal modes can arise whenever the electron and ion flowing velocities are different [
28,
29,
31]. The total electron flow energy, integrated over the entire tube, decreases during the growth of streaming instability. The growth wave energy arises mainly from the decrease in the electron flow energy within the simulation domain. In this study, we found that the two-fluid plasma electron-ion two-stream instability can be excited. It is the relative velocity between ion flow and electron flow that provides the free energy for the electron-ion two-stream instability.
We estimate the diameter of the arc discharge by comparing a power input of 200 watts for the arc charge with the total kinetic and electric energy in the simulation domain. We calculate the total kinetic energy (electric energy) per area at
1.8 ns of the entire simulation domain and obtain 150
(164
). The energy provided by the power input at 200 watts over the period of 1.8 ns is
. We obtain an upper bound for the diameter
of the arc discharge:
Note that the length of the arc discharge is 2 mm, which is 10 times of . Moreover, we also simulate cases of emitted thermionic current as 15 A for three different sets of hydrogen pressure, three sets of applied voltage, and three sets of distances in the next section.
3.3. Comparisons for Simulation Results with Different Parameters
Table S1 lists 48 cases simulated with different sets of parameters, which include the neutral H
2 pressure p, the neutral density
, the electric potential
at the anode, and the system (tube) length
. The resulting potential peak
and potential dip
are also listed in
Table S1.
Figure 8 shows the resulting
and
as a function of
(distance between cathode and anode) under applied voltages of 100 V, 300 V, and 500 V from left to right columns. The top (bottom) panels in
Figure 8 show the resulting
. The red hollow circles are for the cases with 1 torr of neutral hydrogen pressure in the chamber. The black (blue) hollow circles denote the cases with 5 torr (10 torr) of neutral hydrogen (H
2) in the chamber. The resulting
ranges from 0.1 kV to 45.0 kV, while the resulting
ranges from 0.6 kV to 38.0 kV.
Table S1 and
Figure 8 show that Case 47 has the largest potential peak
. The largest potential dip is
in Case 47. In Case 47,
.
Figure 8 shows that the twenty-four cases with 1 torr have quasi-proportional value of
and of
with applied voltage
.
Regarding the dependence on (distance between cathode and anode), a larger has a larger with the same filling H2 pressure, while the dependence of is mixing. For the cases (blue line) with and long chambers (), the plasma density is high and can lead to electron density pile up and interrupting the simulation.
Figure 9 shows the simulation results of Case 47 at
2.0 ns, 2.2 ns, 2.4 ns, and 2.6 ns. In this case, an electric potential dip is formed due to the high-density electron layer and the magnitude can reach −15.0 kV as shown in the electric potential profiles.
Thermionic emitted electrons lead to the formation of an electron layer near the left boundary (). As a result of this electron layer, the electric potential has a sharp decrease from to . The electric potential then increases gradually to volts at the right boundary (anode). The average electric field in the chamber is negative (). This negative average electric field in the chamber will accelerate electrons to high speed m/s, while ions are accelerated in the left direction with small velocity due to their large mass. The electrons and ions are accelerated in the opposite directions, which can lead to the electron-ion two-stream instability as discussed earlier. In the electric potential profile, large amplitude electrostatic waves are formed due to this instability, and the wave amplitude may reach tens of kilovolts. The electron and ion number density and velocity profiles also show similar patterns. The wavy potential structure may last for a few ns.