Feature Papers in Atmospheric Techniques, Instruments, and Modeling

A special issue of Atmosphere (ISSN 2073-4433). This special issue belongs to the section "Atmospheric Techniques, Instruments, and Modeling".

Deadline for manuscript submissions: 31 May 2025 | Viewed by 9586

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Guest Editor
Met Office, Foundation and Weather Science, Exeter EX1 3PB, UK
Interests: atmospheric radiative transfer; satellite; airborne and ground-based remote sensing; retrieval of atmospheric and surface properties; electromagnetic scattering theory; cirrus; operational satellite data assimilation; numerical methods; big data; machine learning techniques
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Dear Colleagues,

We are pleased to announce that the section Atmospheric Techniques, Instruments, and Modeling is now compiling a collection of papers submitted by the Editorial Board Members (EBMs) of our journal and outstanding scholars in this research field. We welcome contributions and recommendations from the EBMs.

The purpose of this Special Issue is to publish a set of papers that typify the most exceptional, insightful, influential, and original research articles or reviews. We expect these papers to be widely read and highly influential within the field. All the papers in this Special Issue will be collated into a printed edition book after the deadline and will be well promoted.

We would also like to take this opportunity to call on more scholars to join the journal section Atmospheric Techniques, Instruments, and Modeling so that we can work together to further develop this exciting field of research.

Dr. Stephan Havemann
Guest Editor

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Keywords

  • remote sensing
  • instruments
  • laboratory measurement techniques
  • artificial intelligence
  • machine learning
  • data science
  • model development
  • algorithm
  • satellite
  • carbon balance/carbon cycle
  • infrared spectroscopy
  • lidar
  • radar
  • unmanned aerial vehicles/drone
  • point cloud
  • GNSS
  • microwave radiometry

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Published Papers (13 papers)

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Research

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18 pages, 12576 KiB  
Article
Global Methane Retrieval, Monitoring, and Quantification in Hotspot Regions Based on AHSI/ZY-1 Satellite
by Tong Lu, Zhengqiang Li, Cheng Fan, Zhuo He, Xinran Jiang, Ying Zhang, Yuanyuan Gao, Yundong Xuan and Gerrit de Leeuw
Atmosphere 2025, 16(5), 510; https://doi.org/10.3390/atmos16050510 - 28 Apr 2025
Viewed by 83
Abstract
Methane is the second largest greenhouse gas. The detection of methane super-emitters and the quantification of their emission rates are necessary for the implementation of methane emission reduction policies to mitigate global warming. High-spectral-resolution satellites such as Gaofen-5 (GF-5), EMIT, GHGSat, and MethaneSAT [...] Read more.
Methane is the second largest greenhouse gas. The detection of methane super-emitters and the quantification of their emission rates are necessary for the implementation of methane emission reduction policies to mitigate global warming. High-spectral-resolution satellites such as Gaofen-5 (GF-5), EMIT, GHGSat, and MethaneSAT have been successfully employed to detect and quantify methane point source leaks. In this study, a matched filter (MF) algorithm is improved using data from the EMIT instrument and applied to data from the Advanced Hyperspectral Imager (AHSI) onboard the Ziyuan-1 (ZY-1) satellite. Validation by comparison with EMIT′s L2 XCH4 products shows the good performance of the improved MF algorithm, in spite of the lower spectral resolution of AHSI/ZY-1 in comparison with other point source imagers. The improved MF algorithm applied to AHSI/ZY-1 data was used to detect and quantify methane super-emitters in global methane hotspot regions. The results show that the improved MF algorithm effectively suppresses noise in retrieval results over both land and ocean surfaces, enhancing algorithm robustness. Sixteen methane plumes were detected in global hotspot regions, originating from coal mines, oil and gas fields, and landfills, with emission rates ranging from 0.57 to 78.85 t/h. The largest plume was located at an offshore oil and gas field in the Gulf of Mexico, with instantaneous emissions nearly equal to the combined total of the other 15 plumes. The findings demonstrate that AHSI, despite its lower spectral resolution, can detect sources with emission rates as small as 571 kg/h and achieve faster retrieval speeds, showing significant potential for global methane monitoring. Additionally, this study highlights the need to focus on methane emissions from marine sources, alongside terrestrial sources, to efficiently implement reduction strategies. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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15 pages, 6167 KiB  
Article
Comparison of Sensors for Air Quality Monitoring with Reference Methods in Zagreb, Croatia
by Silvije Davila, Marija Jelena Lovrić Štefiček, Ivan Bešlić, Gordana Pehnec, Marko Marić and Ivana Hrga
Atmosphere 2025, 16(4), 472; https://doi.org/10.3390/atmos16040472 - 18 Apr 2025
Viewed by 166
Abstract
Within the scope of “Eco Map of Zagreb” project, eight sensor sets (type AQMeshPod) were set up at an automatic measuring station at the Institute for Medical Research and Occupational Health (IMROH) for comparison with reference methods for air quality measurement during 2018. [...] Read more.
Within the scope of “Eco Map of Zagreb” project, eight sensor sets (type AQMeshPod) were set up at an automatic measuring station at the Institute for Medical Research and Occupational Health (IMROH) for comparison with reference methods for air quality measurement during 2018. This station is a city background station within the Zagreb network for air quality monitoring, where measurements of SO2, CO, NO2, O3, PM10 and PM2.5, are performed using standardized methods accredited according to EN ISO/IEC 17025. This paper presents a comparison of pollutant mass concentrations determined by sensors with reference methods. The data were compared and filtered to remove outliers and handle deviations between the results obtained by sensors and reference methods, considering the different approaches to gas and PM data. A comparison of sensor results with the reference methods showed a large scattering of all gaseous pollutants while the comparison for PM10 and PM2.5 indicated a satisfactory low dispersion. The results of a regression analysis showed a significant seasonal dependence for all pollutants. Significant statistical differences between the reference methods and sensors for the whole year and in all seasons for all gas pollutants, as well as for PM10, were observed, while for PM2.5 statistical significance showed varying results. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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12 pages, 4073 KiB  
Article
Characteristics of Observed Electromagnetic Wave Ducts in Tropical, Subtropical, and Middle Latitude Locations
by Sandra E. Yuter, McKenzie M. Sevier, Kevin D. Burris and Matthew A. Miller
Atmosphere 2025, 16(3), 336; https://doi.org/10.3390/atmos16030336 - 17 Mar 2025
Viewed by 189
Abstract
Where and at what altitudes electromagnetic wave ducts within the atmosphere are likely to occur is important for a variety of communication and military applications. We examined the modified refractivity profiles and wave duct characteristics derived from nearly 50,000 observed upper air soundings [...] Read more.
Where and at what altitudes electromagnetic wave ducts within the atmosphere are likely to occur is important for a variety of communication and military applications. We examined the modified refractivity profiles and wave duct characteristics derived from nearly 50,000 observed upper air soundings obtained over four years from seven tropical and subtropical islands, as well as middle latitude sites at four US coastal locations, three sites near the Great Lakes, and four US inland sites. Across all location types, elevated ducts were found to be more common than surface-based ducts, and the median duct thicknesses were ~100 m. There was a weak correlation between duct thickness and strength and, essentially, no correlation between the duct strength and duct base height. EM ducts more frequently occurred at the tropical and subtropical island locations (~60%) and middle latitude coastal locations (70%) as compared to the less than 30% of the time that occurred at the Great Lake and US inland sites. The tropical and subtropical island sites were more likely than the other location types to have ducts at altitudes higher than 2 km, which is above the boundary layer height. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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26 pages, 13054 KiB  
Article
Retrieval of Atmospheric XCH4 via XGBoost Method Based on TROPOMI Satellite Data
by Wenhao Zhang, Yao Li, Bo Li, Tong Li, Zhengyong Wang, Xiufeng Yang, Yongtao Jin and Lili Zhang
Atmosphere 2025, 16(3), 279; https://doi.org/10.3390/atmos16030279 - 26 Feb 2025
Viewed by 314
Abstract
Accurate retrieval of column-averaged dry-air mole fraction of methane (XCH4) in the atmosphere is important for greenhouse gas emission management. Traditional XCH4 retrieval methods are complex, while machine learning can be used to model nonlinear relationships by analyzing large datasets, [...] Read more.
Accurate retrieval of column-averaged dry-air mole fraction of methane (XCH4) in the atmosphere is important for greenhouse gas emission management. Traditional XCH4 retrieval methods are complex, while machine learning can be used to model nonlinear relationships by analyzing large datasets, providing an efficient alternative. This study proposes an XGBoost algorithm-based retrieval method to improve the efficiency of atmospheric XCH4 retrieval. First, the key wavelengths affecting XCH4 retrieval were determined using a radiative transfer model. The TROPOspheric Monitoring Instrument (TROPOMI) L1B satellite data, L2 XCH4 products, and auxiliary data were matched to construct the dataset. The dataset constructed was used to train the XGBoost model and obtain the TRO_XGB_XCH4 model. Finally, the accuracy of the proposed model was evaluated using various parameter values and validated against XCH4 products and Total Carbon Column Observing Network (TCCON) ground-based observations. The results showed that the proposed TRO_XGB_XCH4 model had a tenfold cross-validation accuracy R of 0.978, a ground-based validation R of 0.749, and a temporal extension accuracy R of 0.863. Therefore, the accuracy of the TRO_XGB_XCH4 retrieval model is comparable to that of the official TROPOMI L2 product. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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30 pages, 6396 KiB  
Article
A Modified Kalman Filter Based on Radial Basis Function Neural Networks for the Improvement of Numerical Weather Prediction Models
by Athanasios Donas, George Galanis, Ioannis Pytharoulis and Ioannis Th. Famelis
Atmosphere 2025, 16(3), 248; https://doi.org/10.3390/atmos16030248 - 22 Feb 2025
Viewed by 577
Abstract
This study introduces a novel enhancement to the Kalman filter algorithm by integrating it with Radial Basis Function neural networks to improve numerical weather prediction models. Traditional Kalman filters frequently underperform when used by dynamical systems due to their reliance on fixed covariance [...] Read more.
This study introduces a novel enhancement to the Kalman filter algorithm by integrating it with Radial Basis Function neural networks to improve numerical weather prediction models. Traditional Kalman filters frequently underperform when used by dynamical systems due to their reliance on fixed covariance matrices, resulting in inaccuracies and forecast uncertainty. The proposed modified Kalman filter utilizes Radial Basis Function neural networks to estimate covariance matrices adaptively during the filtering process. This self-adaptive computational system enables the simultaneous targeting of the systematic and the remaining non-systematic parts of the forecast error, producing an innovative and efficient post-process strategy. The suggested methodology is evaluated on predictions of 10-meter wind speed and 2-meter air temperature obtained from the Weather Research and Forecasting model for observation stations in northern Greece. The derived results demonstrate a significant reduction in systematic error, as the bias decreased by up to 88% for 10-meter wind speed and 58% for 2-meter air temperature. Additionally, the forecast variability was successfully mitigated, with the RMSE reduced by 39% and 40%, respectively. Compared to the traditional Kalman filter, which exhibited increased RMSE in several cases and failed to control forecast uncertainty, the proposed approach consistently outperformed by providing stable and reliable predictions across all examined scenarios. These improvements validate the robustness of the method in comparison to conventional techniques, highlighting its potential to produce reliable and stable predictions for environmental applications. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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17 pages, 4857 KiB  
Article
Biomonitoring of Potentially Toxic Elements in the Urban Atmosphere of Tehran Metropolis Using the Lichen Anaptychia setifera (Mereschk.) Räsänen
by Sara Abdollahi, Nasrin Hassanzadeh, Mohammad Sohrabi and Stefano Loppi
Atmosphere 2025, 16(2), 206; https://doi.org/10.3390/atmos16020206 - 11 Feb 2025
Cited by 1 | Viewed by 732
Abstract
This study investigated the bioaccumulation of PTEs in the 22 districts of the Tehran metropolis using the lichen Anaptychia setifera collected from Kalpoosh unpolluted area in Semnan province and exposed for 4 months in the study area using the lichen transplant technique. The [...] Read more.
This study investigated the bioaccumulation of PTEs in the 22 districts of the Tehran metropolis using the lichen Anaptychia setifera collected from Kalpoosh unpolluted area in Semnan province and exposed for 4 months in the study area using the lichen transplant technique. The concentrations of eight potentially toxic elements in the lichen were quantified using ICP-OES analysis. PCA was used to detect common sources of PTEs, and distribution maps were produced using QGIS. A statistically significant difference in the toxic elements was observed among the different stations in the Tehran metropolis. The CF index results indicate severe pollution (CF ≥ 3) for all eight studied toxic elements in the atmosphere of the Tehran metropolis. The values of the PLI index in the monitoring stations were calculated in the range of 14–31, confirming very high pollution (PLI ≥ 2.5) in the study area. The results showed a significant accumulation of all investigated toxic elements. Toxic elements such as Fe, Al, and Cr were primarily derived from natural geogenic sources, whereas Co, Cu, Ni, Pb, and Zn originated from anthropogenic sources, predominantly vehicular traffic, as depicted by the distribution patterns of these toxic elements, with peaks near sites with heavy traffic. Overall, the entire study area exhibited severe pollution levels. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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20 pages, 11520 KiB  
Article
Detection of High Radar Reflectivity Volumes at High Tropospheric Levels in Large Hail Events
by Tomeu Rigo and Carme Farnell
Atmosphere 2025, 16(1), 33; https://doi.org/10.3390/atmos16010033 - 31 Dec 2024
Viewed by 709
Abstract
Different giant and very large hail events have occurred in Catalonia (NE of the Iberian Peninsula) in the last three years, with stones ranging between 8 and more than 10 cm in diameter. These sizes have not occurred in this area in at [...] Read more.
Different giant and very large hail events have occurred in Catalonia (NE of the Iberian Peninsula) in the last three years, with stones ranging between 8 and more than 10 cm in diameter. These sizes have not occurred in this area in at least thirty years. This research analyzed all those events with at least one severe hail register (more than 2 cm diameter) in the region for 2013–2023. The present study considered large volumes of high reflectivity in weather radar 3D fields at high tropospheric levels (more than 10 km). The goal was to determine if high reflectivity cores (over 55 dBZ) occurred at those levels before or during the hail-fall. The main question was whether this radar signature could reveal the occurrence of very large or giant hail. The 55 dBZ volumes occurred and were maintained over 10 km between six and sixty minutes in a high percentage of large-hail cases. However, giant hail cases did not present the maximum duration of high reflectivity at high levels as was initially expected. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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23 pages, 10950 KiB  
Article
Zenith Tropospheric Delay Forecasting in the European Region Using the Informer–Long Short-Term Memory Networks Hybrid Prediction Model
by Zhengdao Yuan, Xu Lin, Yashi Xu, Jie Zhao, Nage Du, Xiaolong Cai and Mengkui Li
Atmosphere 2025, 16(1), 31; https://doi.org/10.3390/atmos16010031 - 29 Dec 2024
Cited by 1 | Viewed by 783
Abstract
Zenith tropospheric delay (ZTD) is a significant atmospheric error that impacts the Global Navigation Satellite System (GNSS). Developing a high-precision, long-term forecasting model for ZTD can provide valuable insights into the overall trends of predicted ZTD, which is essential for improving GNSS positioning [...] Read more.
Zenith tropospheric delay (ZTD) is a significant atmospheric error that impacts the Global Navigation Satellite System (GNSS). Developing a high-precision, long-term forecasting model for ZTD can provide valuable insights into the overall trends of predicted ZTD, which is essential for improving GNSS positioning and analyzing changes in regional climate and water vapor. To address the challenges of incomplete information extraction and gradient explosion in a single neural network when forecasting ZTD long-term, this study introduces an Informer–LSTM Hybrid Prediction Model. This model employs a parallel ensemble learning strategy that combines the strengths of both the Informer and LSTM networks to extract features from ZTD data. The Informer model is effective at capturing the periodicity and long-term trends within the ZTD data, while the LSTM model excels at understanding short-term dependencies and dynamic changes. By merging the features extracted by both models, the prediction capabilities of each can complement one another, allowing for a more comprehensive analysis of the characteristics present in ZTD data. In our research, we utilized ERA5-derived ZTD data from 11 International GNSS Service (IGS) stations in Europe to interpolate the missing portions of GNSS-derived ZTD. We then employed this interpolated data from 2016 to 2020, along with an Informer–LSTM Hybrid Prediction Model, to develop a long-term prediction model for ZTD with a prediction duration of one year. Our numerical results demonstrate that the proposed model outperforms several comparative models, including the LSTM–Informer based on a serial ensemble learning model, as well as the Informer, Transformer, LSTM, and GPT3 empirical ZTD models. The performance metrics indicate a root mean square error (RMSE) of 1.91 cm, a mean absolute error (MAE) of 1.45 cm, a mean absolute percentage error (MAPE) of 0.60, and a correlation coefficient (R) of 0.916. Spatial distribution analysis of the accuracy metrics showed that predictive accuracy was higher in high-latitude regions compared to low-latitude areas, with inland regions demonstrating better performance than those near the ocean. This study introduced a novel methodology for high-precision ZTD modeling, which is significant for improving accurate GNSS positioning and detecting water vapor content. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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15 pages, 3080 KiB  
Article
Assessment of Doppler Wind Lidar Detection Efficiency and Influencing Factors at Plateau Airport: A Case Study of Lhasa Gonggar Airport
by Junjie Wu, Hongyu Du, Chunjiong Xia and Xiaoyuan Huang
Atmosphere 2024, 15(12), 1530; https://doi.org/10.3390/atmos15121530 - 20 Dec 2024
Viewed by 777
Abstract
Doppler wind lidar (DWL) demonstrates significant advantages in wind field detection under clear weather conditions and has been widely applied in airports with complex wind environments. However, its detection performance is highly susceptible to weather conditions and meteorological factors. To address this issue, [...] Read more.
Doppler wind lidar (DWL) demonstrates significant advantages in wind field detection under clear weather conditions and has been widely applied in airports with complex wind environments. However, its detection performance is highly susceptible to weather conditions and meteorological factors. To address this issue, this study analyzes the detection efficiency of DWL based on data collected at Lhasa Gonggar Airport from August 2023 to April 2024, along with ground-based meteorological observations. The results indicate that when the detection efficiency dropped to 40%, the average detection range for the plan position indicator (PPI) mode and Doppler beam swinging (DBS) mode were 5.3 km and 2.7 km, respectively. The influence of different underlying surface types on detection efficiency was minimal, with detection efficiency at a 270° azimuth slightly better than at a 90° azimuth. A 4° elevation angle performed better than a 6° elevation angle. During the study period, the detection efficiency generally improved, with the lowest detection efficiency being observed in August, suggesting that precipitation significantly impacts performance. In August, the detection efficiency of the PPI mode dropped below 50% at 4 km, while the highest detection efficiency occurred in April, where performance remained above 50% at 7 km. This is associated with enhanced thermal and dynamic activity in the lower atmosphere. Low-cloud activity also affected the detection performance of the DBS mode. The daily variation in the detection range in April was more pronounced than in January, with the detection range generally being larger. The increase in detection range was related to the more active vertical atmospheric mixing. The PPI mode was more sensitive to changes in meteorological factors, with its median detection range being 0.2–0.6 km shorter than that of the DBS mode when the meteorological optical range (MOR) was less than 4 km. Additionally, the PPI mode showed weaker stability than the DBS mode when relative humidity was below 75%. When relative humidity exceeded 80%, both modes showed a linear decrease in detection efficiency. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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26 pages, 13796 KiB  
Article
The BIRDIES Experiment: Measuring Beryllium Isotopes to Resolve Dynamics in the Stratosphere
by Sonia Wharton, Alan J. Hidy, Thomas S. Ehrmann, Wenbo Zhu, Shaun N. Skinner, Hassan Beydoun, Philip J. Cameron-Smith, Marisa Repasch, Nipun Gunawardena, Jungmin M. Lee, Ate Visser, Matthew Griffin, Samuel Maddren and Erik Oerter
Atmosphere 2024, 15(12), 1502; https://doi.org/10.3390/atmos15121502 - 17 Dec 2024
Viewed by 1084
Abstract
Cosmogenic beryllium-10 and beryllium-7, and the ratio of the two (10Be/7Be), are powerful atmospheric tracers of stratosphere–troposphere exchange (STE) processes; however, measurements are sparse for altitudes well above the tropopause. We present a novel high-altitude balloon campaign aimed to measure these isotopes in [...] Read more.
Cosmogenic beryllium-10 and beryllium-7, and the ratio of the two (10Be/7Be), are powerful atmospheric tracers of stratosphere–troposphere exchange (STE) processes; however, measurements are sparse for altitudes well above the tropopause. We present a novel high-altitude balloon campaign aimed to measure these isotopes in the mid-stratosphere called Beryllium Isotopes for Resolving Dynamics in the Stratosphere (BIRDIES). BIRDIES targeted gravity waves produced by tropopause-overshooting convection to study their propagation and impact on STE dynamics, including the production of turbulence in the stratosphere. Two custom-designed payloads called FiSH and GASP were flown at altitudes approaching 30 km to measure in situ turbulence and beryllium isotopes (on aerosols), respectively. These were flown on nine high-altitude balloon flights over Kansas, USA, in summer 2022. The atmospheric samples were augmented with a ground-based rainfall collection targeting isotopic signatures of deep convection overshooting. Our GASP samples yielded mostly negligible amounts of both 10Be and 7Be collected in the mid-stratosphere but led to design improvements to increase aerosol capture in low-pressure environments. Observations from FiSH and the precipitation collection were more fruitful. FiSH showed the presence of turbulent velocity, temperature, and acoustic fluctuations in the stratosphere, including length scales in the infra-sonic range and inertial subrange that indicated times of elevated turbulence. The precipitation collection, and subsequent statistical analysis, showed that large spatial datasets of 10Be/7Be can be measured in individual rainfall events with minimum terrestrial contamination. While the spatial patterns in rainfall suggested some evidence for overshooting convection, inter-event temporal variability was clearly observed and predicted with good agreement using the 3D chemical transport model GEOS-CHEM. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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13 pages, 4497 KiB  
Article
A Comparison of the Effects of Climate and Human Variability on the Thermal Resistance of Clothing
by Ferenc Ács, Zsófia Szalkai, Erzsébet Kristóf and Annamária Zsákai
Atmosphere 2024, 15(12), 1474; https://doi.org/10.3390/atmos15121474 - 10 Dec 2024
Viewed by 597
Abstract
We used a clothing thermal resistance model to investigate and compare the effects of climate and human variability on human thermal load. To investigate the effect of climate variability, we introduced the mean clothing thermal resistance rcl¯. For characterizing [...] Read more.
We used a clothing thermal resistance model to investigate and compare the effects of climate and human variability on human thermal load. To investigate the effect of climate variability, we introduced the mean clothing thermal resistance rcl¯. For characterizing the effect of human variability, we used the standard deviation of clothing thermal resistance rcl. We distinguished people based on their body type. We also defined the average human, a man and a woman, with thermal resistances of rcl,m and rcl,f. The investigation was carried out for the European region in the cold season for the period of 1981–2010. The climate variables were taken from the ERA5 reanalysis database. Our most important results are the following. (1) The macroscale pattern of the rcl¯ and rcl fields are very similar, based on which it can be stated that human variability does not modify the spatial distribution of rcl¯. (2) The rcl values are roughly a quarter of the rcl¯ values. The highest rcl¯ values (3.2–3.4 clo) are in Lapland, and the smallest (1–1.2 clo) in Andalusia. (3) The macroscale pattern of the rcl,m and rcl,f fields is similar to the macroscale pattern of the rcl values of the mesomorphic person rcl,2. The field of rcl,2 can be used for climate classification purposes. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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31 pages, 7104 KiB  
Article
Assessing Nitrogen Dioxide in the Highveld Troposphere: Pandora Insights and TROPOMI Sentinel-5P Evaluation
by Refilwe F. Kai-Sikhakhane, Mary C. Scholes, Stuart J. Piketh, Jos van Geffen, Rebecca M. Garland, Henno Havenga and Robert J. Scholes
Atmosphere 2024, 15(10), 1187; https://doi.org/10.3390/atmos15101187 - 3 Oct 2024
Cited by 1 | Viewed by 986
Abstract
Nitrogen oxides, particularly NO2, are emitted through a variety of industrial and transport processes globally. The world’s continuous economic development, including in developing countries, results in an increasing concentration of those gases in the atmosphere. Yet, there is scant information on [...] Read more.
Nitrogen oxides, particularly NO2, are emitted through a variety of industrial and transport processes globally. The world’s continuous economic development, including in developing countries, results in an increasing concentration of those gases in the atmosphere. Yet, there is scant information on the current state and recent evolution of these atmospheric pollutants over a range of spatial and temporal scales, especially in Africa. This, in turn, hinders the assessment of the emissions and the evaluation of potential risks or impacts on societies and their economies, as well as on the environment. This study attempts to fill the gap by leveraging data from a Pandora-2S ground-based, column-integrating instrument located in Wakkerstroom in the Mpumalanga Province of South Africa and space-based remote sensing data obtained from the TROPOMI instrument onboard the ESA Sentinel-5P satellite. We compare these two spatially (horizontal) representative data sets using statistical tools to investigate the concentrations of emitted and transported NO2 at this particular location, expecting that a significant positive correlation between the NO2 tropospheric vertical column (TVC) data might justify using the TROPOMI data, available globally, as a proxy for tropospheric and boundary layer NO2 concentrations over the Highveld of South Africa more generally. The data from the two instruments showed no significant difference between the interannual mean TVC-NO2 in 2020 and 2021. The seasonal patterns for both instruments were different in 2020, but in 2021, both measured peak TVC-NO2 concentrations in late winter (week 34). The instruments both detected higher TVC-NO2 concentrations during transitions between seasons, particularly from winter to spring. The TVC-NO2 concentrations measured in Wakkerstroom Mpumalanga are mostly contributed to by the emission sources in the low troposphere, such as biomass burning and emissions from local power stations. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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Review

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14 pages, 2057 KiB  
Review
Methods, Progress and Challenges in Global Monitoring of Carbon Emissions from Biomass Combustion
by Ge Qu, Yusheng Shi, Yongliang Yang, Wen Wu and Zhitao Zhou
Atmosphere 2024, 15(10), 1247; https://doi.org/10.3390/atmos15101247 - 18 Oct 2024
Cited by 1 | Viewed by 1755
Abstract
Global biomass burning represents a significant source of carbon emissions, exerting a substantial influence on the global carbon cycle and climate change. As global carbon emissions become increasingly concerning, accurately quantifying the carbon emissions from biomass burning has emerged as a pivotal and [...] Read more.
Global biomass burning represents a significant source of carbon emissions, exerting a substantial influence on the global carbon cycle and climate change. As global carbon emissions become increasingly concerning, accurately quantifying the carbon emissions from biomass burning has emerged as a pivotal and challenging area of scientific research. This paper presents a comprehensive review of the primary monitoring techniques for carbon emissions from biomass burning, encompassing both bottom-up and top-down approaches. It examines the current status and limitations of these techniques in practice. The bottom-up method primarily employs terrestrial ecosystem models, emission inventory methods, and fire radiation power (FRP) techniques, which rely on the integration of fire activity data and emission factors to estimate carbon emissions. The top-down method employs atmospheric observation data and atmospheric chemical transport models to invert carbon emission fluxes. Both methods continue to face significant challenges, such as limited satellite resolution affecting data accuracy, uncertainties in emission factors in regions lacking ground validation, and difficulties in model optimization due to the complexity of atmospheric processes. In light of these considerations, this paper explores the prospective evolution of carbon emission monitoring technology for biomass burning, with a particular emphasis on the significance of high-precision estimation methodologies, technological advancements in satellite remote sensing, and the optimization of global emission inventories. This study aims to provide a forward-looking perspective on the evolution of carbon emission monitoring from biomass burning, offering a valuable reference point for related scientific research and policy formulation. Full article
(This article belongs to the Special Issue Feature Papers in Atmospheric Techniques, Instruments, and Modeling)
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