Abstract
In this work, the existence and nonexistence of stationary radial solutions to the elliptic partial differential equation arising in the molecular beam epitaxy are studied. Since we are interested in radial solutions, we focus on the fourth-order singular ordinary differential equation. It is non-self adjoint, it does not have exact solutions, and it admits multiple solutions. Here, measures the intensity of the flux and G is stationary flux. The solution depends on the size of the parameter . We use a monotone iterative technique and integral equations along with upper and lower solutions to prove that solutions exist. We establish the qualitative properties of the solutions and provide bounds for the values of the parameter , which help us to separate existence from nonexistence. These results complement some existing results in the literature. To verify the analytical results, we also propose a new computational iterative technique and use it to verify the bounds on and the dependence of solutions for these computed bounds on .
1. Introduction
Epitaxy means the growth of a single thin film on top of a crystalline substrate. It is crucial for semiconductor thin film technology, hard and soft coatings, protective coatings, optical coatings, etc. The epitaxial growth technique is used to produce the growth of semiconductor films and multilayer structures under high vacuum conditions [1]. The major advantages of epitaxial growth are reducing the growth time, better structural and superior electrical properties, eliminating waste caused during growth, wafering cost, cutting, polishing, etc. Several types of epitaxial growth techniques, such as hybrid vapor phase epitaxy [2], chemical beam epitaxy [3], and molecular beam epitaxy (MBE), have been used for the growth of compound semiconductors and other materials. In this work, we strictly focus on MBE, and we restrict our attention to the differential equation model, which was proposed by Escudero et al. [4,5,6,7]. The mathematical description of epitaxial growth is carried out by means of a function defined as
which describes the height of the growing interface in the spatial point at time . The authors in [4,5,6,7] show that the function obeys the fourth-order partial differential equation
where models the incoming mass entering the system through epitaxial deposition, measures the intensity of this flux, and the determinant of Hessian matrix is
The stationary counterpart of the partial differential Equation (1) subject to the homogeneous Dirichlet boundary condition (4) and homogeneous Navier boundary condition (5) is defined as (see [6])
where is a stationary flux, and n is the unit out drawn normal to .
Using the transformation and , as a result of symmetry, the above set of equations are transformed into the following set of equations:
where .
In this paper, we also impose the following boundary conditions which complements the work in [6]:
For simplicity, we take , which physically means that the new material is being deposited uniformly on the unit disc.
Now, using , and integrating parts from Equation (6), we have
Using the transformation and , it is possible to reduce Equation (10) into the following equation:
The BVPs (12), (13) and (14) can be equivalently described as the following integral equations (IE):
- IE corresponding to Problem 1:
- IE corresponding to Problem 2:
- IE corresponding to Problem 3:
We assume that , where is defined as
In [6], Escudero et al. proved the existence and nonexistence of solutions of Problems 1 and 3 using upper and lower solution techniques. Corresponding to Problems 1 and 3, they have also provided the rigorous bounds of the values of the parameter , which helps us to separate existence from nonexistence. In [8], Verma et al. provide numerical illustrations via VIM to verify the results of Escudero et al. [6]. To verify their numerical results, they provided other iterative schemes based on homotopy [9] and the Adomian decomposition method [10].
Equation (13) has not been investigated theoretically in the existing literature to the best of our knowledge. Moreover, many investigations are still pending relating to BVPs (12), (13), and (14). Here, we focus on both theoretical and numerical work. We derive the sign of the solution and prove its existence in continuous space. We also compute the bounds of the parameter . The results of this paper complements existing theoretical results. We also provide an iterative scheme based on Green’s function to compute the bounds and solutions to demonstrate the existence and nonexistence, which is dependent on .
To prove the existence of the solutions, we use the monotone iterative technique [11,12,13,14,15,16,17]. Recently, many researchers applied this technique on the initial value problem (IVP) for the nonlinear noninstantaneous impulsive differential equation (NIDE) [18], p-Laplacian boundary value problems with the right-handed Riemann–Liouville fractional derivative [19], etc. to prove the existence of the solution. Here, we also present numerical results to verify the theoretical results. To develop the iterative scheme based on Green’s function, we consider Equations (12)–(14). Recently, many authors have used numerical approximate methods like the VIM [8], the Adomian decomposition method (ADM), the homotopy perturbation method (HPM) etc. to find approximate solutions for different models involving differential equations [20,21], integral equations [22,23,24], fractional differential equations [25,26], the Stefan problem [27,28,29,30], system of integral equations [31], etc. Thereafter, Waleed Al Hayani [32] and Singh et al. [33] applied ADM with Green’s function to compute the approximate solution. Recently, Noeiaghdam et al. [34] proposed a technique based on ADM for solving Volterra integral equation with discontinuous kernels using the CESTAC method. To find out more about this method, please see [35,36]. They focused on the BVPs which have a unique solution. The major advantage of our proposed technique is its ability to capture multiple solutions together with a desired accuracy.
The remainder of the paper is focused on both theoretical and numerical results. We prove some of the basic properties of the BVPs in Section 2. The monotone iterative technique is presented in Section 3 to prove the existence of a solution. A wide range of for Equation (6), corresponding to different types of boundary conditions, is shown in Section 4. In Section 5, we apply our proposed technique to the integral equations and show a wide range of numerical results. Finally, in Section 6, we draw our main conclusions.
2. Preliminary Work
Corresponding to , we prove some basic qualitative properties of the solution , which satisfies the following inequality:
Here, we omit the proof of Lemmas 1–3, Corollary 1, and Lemma 4, which were done by Escudero et al. in [6].
Lemma 1.
Let satisfy and Equation (18), then .
Lemma 2.
Let satisfy , and Equation (18), then for all .
Lemma 3.
Let satisfy , and Equation (18), then for all .
Corollary 1.
Let satisfy , and Equation (18), then if and only if .
Lemma 4.
Let satisfy . Then, for every , we have
Lemma 5.
Let satisfy , and Equation (18), then for all .
Proof.
First, we show that . Assume . Since , there exist a such that . Now, from (18), is an increasing function on . Again, by mean value theorem, we have
Since , we have Hence, we get , which is a contradiction. Therefore, we have Furthermore, is a convex function along with . Moreover, is increasing, which implies . Again, is a decreasing function on . Therefore, and lead to on . □
Lemma 6.
Let be the solution of Problem 3, then satisfies the following integral equation:
and
Proof.
The Green’s function of Problem 3 can be written as
Therefore, from Equation (23) and Problem 3, we can easily deduce the integral Equation (21). Now, using the result of Lemma 1, we have
Now, put
Therefore, we get provided . Consequently, we have
Lemma 7.
Let be the solution of Problem 2, then can be written in the following form:
and also satisfies
Proof.
Using the boundary condition and properties of Green’s function, we have
Lemma 8.
Let be the solution of Problem 1, then can be written in the following form:
and satisfies
3. Existence of Solutions
In this section, we apply the monotone iterative technique coupled with lower and upper solutions to prove the existence of at least one solution for Problems 1–3. For this purpose, we need to prove some lemmas, which help us to prove the main results of this paper.
3.1. Construction of Green’s Function
To investigate the Problems 1–3, we consider the corresponding nonlinear singular boundary value problems, which are given by
where , , , and . Throughout the paper, we assume the following conditions:
- ;
- ;
- ;
- ;
- .
Lemma 9.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
and for all and .
Proof.
Using the boundary condition of Problem and the properties of Green’s function, we can easily prove Equation (39). Furthermore, we have for all and . □
Lemma 10.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
and for all and .
Proof.
In a similar manner to that in Lemma 9, we can easily obtain Equation (41) and prove for all and . □
Lemma 11.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
where Moreover, for all and .
Proof.
Again, using a similar analysis, we can easily derive the Green’s function. Now,
Hence, from (43), we have for all and . □
Lemma 12.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
and for all and .
Proof.
The proof is similar to that shown in Lemma 9. □
Lemma 13.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
and for all and .
Proof.
The proof is similar to that shown in Lemma 10. □
Lemma 14.
Let k satisfy and be the solution of Problem , then
where Green’s function is given by
where Moreover, for all and .
Proof.
The proof is similar to that shown in Lemma 11. □
Proposition 1.
Let k satisfy or (respectively, or and or ) and is such that , then the solution of Problem (respectively, Problem and Problem ) is nonpositive.
3.2. Monotone Iterative Technique
Here, we define lower and upper solutions corresponding to Problems 1–3.
Definition 1
([37]). A function is the upper solution of Problem 1 (respectively, Problem 2 and Problem 3) if
with and (respectively, and ).
Definition 2
([37]). A function is the lower solution of Problem 1 (respectively, Problem 2 and Problem 3) if
with and (respectively, and ).
Now, we construct two sequences and corresponding to Problem (respectively, Problem and Problem ), which are defined by
and
. We assume the following properties:
- : and satisfiesand
- : is continuous on where
Now, we state our main existence theorems.
Theorem 1.
Assume (respectively, and ) is true, there exist , and are upper and lower solutions of Problem 1 (respectively, Problem 2 and Problem 3), which satisfy the properties and such that , then the Problem 1 (respectively, Problem 2 and Problem 3) has at least one solution in the region and the sequences , defined by (52)–(55) converge to solutions u, v uniformly and monotonically, respectively, such that
Proof.
We divide the proof into three parts. In the first part, we prove that
We apply mathematical induction on n. For , from (54) and (55), we have
Now, from Equation (51), we have
Therefore, by Proposition 1, we have . Again from (50) and (60), we have
Since , we have
Hence, by Proposition 1, we have . Therefore, our assumptions are true for . Let our assumptions be true up to . Then, we find that
Now, we want to show that our assumptions are true for . Therefore, from Equation (54), we have
Again, by using conditions (68), we have
Hence, is a lower solution of Problem 1. Now, from Equation (54) and (71), we have
Therefore, by Proposition 1, we have . Again, from (50) and (54), we have
Using a similar analysis, we have . Hence, by mathematical induction, we find that
In the second part of the proof, we have to show that
Now, from (52) and (53), we have
Therefore, by using (50), we have
Again,
Hence, by Proposition 1, we have . Therefore, our assumptions are true for . Let our assumptions be true up to Then, we find that
Now, for , we have
Therefore,
and
Hence, is an upper solution of Problem 1. Therefore, by using (86), (52), and (53), we have
and
Therefore, by Proposition 1, . Hence, by mathematical induction, we conclude that
In the last part of the proof, we want to show for all . Again, from (71) and (86), we have
Since , we have
and
Hence, by Proposition 1, . Finally, we have
Let for such that
Therefore, for every , there exists a solution and to Equations (52) and (53), while (54) and (55) satisfy the inequality (95) on the interval . Since and are monotone and bounded, they converge to function and , respectively. Therefore, by Dini’s theorem, there exists and such that
of . Hence, from (52)–(55) and (38), there exists solutions and to Problem 1, satisfying
Hence, the proof is complete. □
Now, we assume the following conditions:
- ,
- ,
- ,.
Theorem 2.
Let , be the upper and lower solutions of Problem 1 (respectively, Problem 2 and Problem 3), which satisfy the properties and such that . Assume (respectively, and ) is true and . Then, Problem 1 (respectively, Problem 2 and Problem 3) has at least one solution in the region and the sequences , defined by (52)–(55) converge to solutions u, v uniformly and monotonically, respectively, such that
Proof.
The proof is same as that shown in Theorem 1. □
4. Estimations of
The objective of this section is to derive some qualitative bounds of the parameter , from which we can conclude about the nonexistence of solutions. Equation (11) can be written in the following form:
Put and integrating from 0 to t, Equation (100) becomes
Therefore, we have
In view of the transformation, the boundary condition at becomes
Escudero et al. in [6] prove the following two lemmas:
Lemma 15.
The set of numbers , for which there exists a solution of Equation (11) satisfying and , is nonempty and bounded from above.
Lemma 16.
If Problem 1, Problem 2, and Problem 3 are solvable for some , then these are solvable for every .
We present the following results which complement the results proved by Escudero et al. [6].
Proof.
Now from Equation (101), we have
Again, from Equation (101), we get
Therefore, by using (107) and (102), from (108), we have
Therefore, is increasing in Now,
Therefore, we have
where
Now, integrating Equation (111) from 0 to t and by using Equation (104), we have
Therefore, from Equations (112) and (113), we get
which implies Equation (106). □
Lemma 18.
Proof.
We put
Obviously, satisfies assumption . Now, implies . Therefore, is also fulfilled. Now, we have
Hence, the inequality (51) is satisfied. □
Lemma 19.
Proof.
We put
Again, satisfies the assumption . Now, implies . Hence, is also fulfilled. Now, we have
This completes the proof. □
Lemma 20.
Proof.
We put
Now, also satisfies assumption . Similarly, implies . Therefore, is also fulfilled. Then, we have
Hence, the proof is complete. □
Theorem 3.
Let . If , then Equation (10) corresponding to different types of boundary conditions are solvable. Moreover, there is no solution to these problems if . Furthermore, every solution of a governing equation corresponding to these three types of boundary condition satisfy
Proof.
The proof of this can be deduced from Lemma 15, Lemma 16, Lemma 1, Lemma 2, Lemma 3, and Lemma 5. □
Proposition 2.
Corresponding to Equations (6) and (7), the value of admits the estimates
Proof.
From Lemma in [6] and Lemma 19, we get Equation (140). □
Proof.
From Lemmas 17 and 18, we have Equation (141). □
Proposition 4.
Corresponding to Equations (6) and (8), the value of admits the estimates
Proof.
By using Lemma in [6] and Lemma 20, we have Equation (142). □
5. Numerical Results and Discussion
Here, we present the numerical data to validate our derived theoretical results. In Section 5.1, we derive the numerical estimation of the bounds computed by ADM. In Section 5.3, we numerically show the existence of at least one solution.
5.1. ADM
To find the approximate solutions, we develop the iterative numerical schemes with the help of the Fredholm integral Equations (15), (16), and (17), respectively. Now, we decompose the solution of the form , and approximate the nonlinear term in terms of Adomian’s polynomials [38], which is given by
where
Therefore, from integral Equation (15), we define
We compute the arbitary constant c using the Mathematica program. For better understanding, we present the algorithm of our proposed technique corresponding to Equation (15) below.
Residue Error:
Here, we define the residue error [39] corresponding to Equation (15) for error analysis, which is given by
where is the parameter. Therefore, the maximum absolute residue error can be defined as
5.2. Algorithm
Step Convert Fredholm integral Equation (15) into the Voltera integral equation.
Step Identify the constant term, and approximate the nonlinear term by Equation (143).
Step Consider as in (145), and obtain for .
Step Approximate the term by in the equation .
Step Compute the values of the constant and the approximate solutions .
Step Determine the residue error and set the stopping criteria where is the tolerance.
Again, we apply the algorithm Section 5.2 to Equations (16) and (17), and we define the following iterative schemes:
Approximate solutions for Equations (16) and (17) can be written as , provided the series is convergent for . Recently, the convergence of ADM was established by Verma et al. in [9]. Now, by using the transformation , , , and , we get the solutions of Equation (6). We arrive at two cases:
Case (a):
For , we get one trivial and one nontrivial solution. For , we always find two nontrivial solutions. We may refer to them as upper and lower solutions, respectively. Corresponding to Equations (9), (8), and (7), we find the critical values of , i.e., , are , , and , respectively. For , we do not find any numerical solutions, as the value of c become imaginary. In Section 5.2.1, we tabulate residual errors of the approximate solutions corresponding to some .
Case (b):
In this case, we always have two nontrivial numerical solutions corresponding to three types of boundary conditions. One solution is negative (namely, the negative solution) and the other solution is positive (namely, the positive solution). We do not find any negative critical . Please refer to Section 5.2.1 as regards residue errors.
5.2.1. Tables
Here, we have placed some numerical data of approximate solutions of corresponding to different types of boundary conditions below. If we are increasing the value of , we see that the residue error of the lower solution is increasing and the residue error of the upper solution is decreasing (see: Table 1). Similarly, if we are decreasing the value of negative , we see that the residue error of both positive and negative solutions are decreasing (see: Table 2). The same can be seen in Table 3, Table 4, Table 5 and Table 6.
Table 1.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (8).
Table 2.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (8).
Table 3.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (9).
Table 4.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (9).
Table 5.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (7).
Table 6.
Maximum absolute residue error of approximate solutions corresponding to boundary conditions (7).
5.3. Monotone Iterative Method
Here, we compute the monotone iterations using Equations (52)–(55) corresponding to three types of boundary condition.
Corresponding to problem (12): By using Lemma 19, we chose the lower and upper iterations
Therefore, it is easy to show that and both satisfy the inequalities (50), (51), (56), and (57), such that . We consider that . Hence, by using Theorem 1, we have a monotonically and uniformly convergent sequence and , which are converging to the solution v and u of the problem (12). We denote as the approximation of the solution of (12) computed by ADM. By using the transformation , , and , we have the fourth-order iterations corresponding to the monotone iteration and . and are the fourth-order solutions corresponding to the monotone iteration and for , respectively.
In Figure 1a, we plotted , , , , and corresponding to problem (12) for . We have seen that the lower sequence and upper sequence always satisfies the inequality . In Figure 1b, we have placed the monotone iterations of fourth-order SBVP corresponding to problem (12) for . Here, we also observed the existence of at least one solution for a fourth-order SBVP corresponding to the Dirichlet boundary condition.
Figure 1.
Approximate monotone iterations of Equations (52)–(55) corresponding to problem (12) for k = −1 and .
Corresponding to problem (13): From Lemma 18, we chose the initial monotone iterations as follows:
The same remarks follow as discussed above.
In Figure 2a,b, we present the numerical results for and . We noticed that the approximate solution and always lies between the lower sequence and upper sequence .
Figure 2.
Approximate monotone iterations of Equations (52)–(55) corresponding to problem (13) for k = −1 and .
Corresponding to problem (14): Here, we consider the initial monotone iterations
We also included the same remarks as those stated above.
Monotone lower and upper iterations corresponding to the second-order and the fourth-order differential equation are plotted in Figure 3.
Figure 3.
Approximate monotone iterations of Equations (52)–(55) corresponding to problem (14) for k = −1 and .
6. Conclusions
In this work, we derived some qualitative properties of the singular boundary value problems that arise in the theory of epitaxial growth. Moreover, we proved the existence of a solution and discovered a range of parameter k, for which the nonlinear problem has multiple solutions in the region . We established the bounds of the parameter , from which we confirmed the nonexistence of solutions. Furthermore, the boundary value problems have multiple solutions, therefore it is challenging for researchers to obtain a suitable scheme to capture both solutions with the desired accuracy. However, we successfully developed iterative schemes and captured both solutions with a high accuracy. From Table 1, Table 2, Table 3 and Table 4, we can see that the approximate solutions computed by our proposed method converge to the exact solutions very quickly. Corresponding to the boundary conditions (7), we notice that the positive approximate solution converges to the exact positive solution very slowly (See Table 6). We verified that our numerical results matched well with our theoretical results as well as the existing numerical results [9]. We conclude that our proposed technique is relatively powerful and efficient. Furthermore, this technique is an effective tool to solve BVPs, which have multiple solutions.
Author Contributions
Conceptualization, A.K.V. and B.P.; validation, R.P.A. and B.P.; writing—original draft preparation, A.K.V. and B.P.; writing—review and editing, A.K.V., B.P. and R.P.A.; visualization, A.K.V., B.P. and R.P.A.; supervision, R.P.A.; project administration, A.K.V. All authors have read and agreed to the published version of the manuscript.
Funding
This work is supported by grant provided by DST project, file name: SB/S4/MS/805/12 and INSPIRE Program Division, Department of Science & Technology, file no: IF160984 New Delhi, India-110016.
Institutional Review Board Statement
Not applicable.
Informed Consent Statement
Not applicable.
Data Availability Statement
Not applicable.
Conflicts of Interest
The authors declare no conflict of interest.
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