A Light-Driven Self-Spinning and Translation Disc Exploiting Photothermal Liquid Crystal Elastomers
Abstract
1. Introduction
2. Model and Theoretical Formulation
2.1. Temperature Distribution of a Steadily Rotating LCE-Based Disc
2.2. Light-Induced Driving Self-Spinning and Translational Torque by Gravity
3. LCE-Based Disc Exhibiting Steady Self-Spin and Translation
3.1. Mechanics Underlying Steady Self-Spinning and Translation
3.2. Limit Conditions of Self-Spinning and Translation
4. Steady Translational and Self-Rotational Velocities
4.1. The Influence Originating from Heat Flux
4.2. The Influence Originating from Gravitational Acceleration
4.3. The Influence Originating from Contraction Coefficient
4.4. The Influence Originating from Length of LCE
5. Conclusions
Author Contributions
Funding
Institutional Review Board Statement
Informed Consent Statement
Data Availability Statement
Conflicts of Interest
References
- Jenkins, A. Self-oscillation. Phys. Rep. 2013, 525, 167–222. [Google Scholar] [CrossRef]
- Chen, L.; Xia, Y.; Tang, Z.; Zhao, J.; Zhou, K. Self-sustaining chaotic characteristics of double pendulum based on self-shading effect. Chaos Solitons Fractals 2026, 208, 118031. [Google Scholar] [CrossRef]
- Yu, Y.; Zhou, L.; Du, C.; Zhu, F.; Dai, Y.; Ge, D.; Li, K. Self-galloping of a liquid crystal elastomer catenary cable under a steady temperature field. Thin-Walled Struct. 2024, 202, 112071. [Google Scholar] [CrossRef]
- Martella, D.; Nocentini, S.; Parmeggiani, C.; Wiersma, D.S. Self-regulating capabilities in photonic robotics. Adv. Mater. Technol. 2018, 4, 1800571. [Google Scholar] [CrossRef]
- Zhang, Z.; Duan, N.; Lin, C.; Hua, H. Coupled dynamic analysis of a heavily-loaded propulsion shafting system with continuous bearing-shaft friction. Int. J. Mech. Sci. 2020, 172, 105431. [Google Scholar] [CrossRef]
- Zhao, J.; Dai, C.; Dai, Y.; Wu, J.; Li, K. Self-oscillation of cantilevered silicone oil paper sheet system driven by steam. Thin-Walled Struct. 2024, 203, 112270. [Google Scholar] [CrossRef]
- Bai, C.; Kang, J.; Wang, Y.Q. Light-induced motion of three-dimensional pendulum with liquid crystal elastomeric fiber. Int. J. Mech. Sci. 2024, 266, 108911. [Google Scholar] [CrossRef]
- Wang, X.; Li, L.; Zhao, J.; Dai, Y. Scallop-inspired self-oscillating actuator via liquid crystal elastomer fibers. Chaos Solitons Fractals 2026, 202, 117620. [Google Scholar] [CrossRef]
- Kularatne, R.S.; Kim, H.; Boothby, J.M.; Ware, T.H. Liquid crystal elastomer actuators: Synthesis, alignment, and applications. J. Polym. Sci. Part B Polym. Phys. 2017, 55, 395–411. [Google Scholar] [CrossRef]
- Wang, Y.; Liu, J.; Yang, S. Multi-functional liquid crystal elastomer composites. Appl. Phys. Rev. 2022, 9, 011301. [Google Scholar] [CrossRef]
- Herbert, K.M.; Fowler, H.E.; McCracken, J.M.; Schlafmann, K.R.; Koch, J.A.; White, T.J. Synthesis and alignment of liquid crystalline elastomers. Nat. Rev. Mater. 2022, 7, 23–28. [Google Scholar] [CrossRef]
- Xu, Z.; Chen, Y.; Zhu, L.; Ge, Q.; Wu, Z.L.; Qu, S.; Xiao, R. Tailored helix morphing of 3D-printed liquid crystal elastomer bilayers. Cell Rep. Phys. Sci. 2025, 6, 102835. [Google Scholar] [CrossRef]
- Bai, C.; Kang, J.; Wang, Y.Q. Kirigami-Inspired Light-Responsive conical spiral actuators with large contraction ratio using liquid crystal elastomer fiber. ACS Appl. Mater. Interfaces 2025, 17, 14488–14498. [Google Scholar] [CrossRef]
- Zhou, L.; Du, C.; Wang, W.; Li, K. A thermally-responsive fiber engine in a linear temperature field. Int. J. Mech. Sci. 2022, 225, 107391. [Google Scholar] [CrossRef]
- Chen, B.; Liu, C.; Xu, Z.; Wang, Z.; Xiao, R. Modeling the thermo-responsive behaviors of polydomain and monodomain nematic liquid crystal elastomers. Mech. Mater. 2024, 188, 104838. [Google Scholar] [CrossRef]
- White, T.J.; Bricker, R.L.; Natarajan, L.V.; Serak, S.V.; Tabiryan, N.V.; Bunning, T.J. Polymer stabilization of phototunable cholesteric liquid crystals. Soft Matter 2009, 5, 3623–3628. [Google Scholar] [CrossRef]
- Hrozhyk, U.; Serak, S.; Tabiryan, N.; White, T.J.; Bunning, T.J. Bidirectional photo response of surface pretreated azobenzene liquid crystal polymer networks. Opt. Express 2009, 17, 716–722. [Google Scholar] [CrossRef] [PubMed]
- Xu, P.; Zhu, H.; Zhou, K.; Ren, X.; Zhou, L. Self-sustained chaotic warning indicator system based on liquid crystal elastomer. Chaos Solitons Fractals 2026, 206, 117984. [Google Scholar] [CrossRef]
- Urayama, K.; Honda, S.; Takigawa, T. Deformation coupled to director rotation in swollen nematic elastomers under electric fields. Macromolecules 2006, 39, 1943–1949. [Google Scholar] [CrossRef]
- Kotikian, A.; Truby, R.L.; Boley, J.W.; White, T.J.; Lewis, J.A. 3d printing of liquid crystal elastomeric actuators with spatially programed nematic order. Adv. Mater. 2018, 30, 1870063. [Google Scholar] [CrossRef]
- Cedric, P.; Ambulo Julia, J.; Burroughs Jennifer, M.B.; Hyun, K.; Ravi Shankar, M.; Taylor, H.W. Four-dimensional printing of liquid crystal elastomers. ACS Appl. Mater. Interfaces 2017, 9, 37332–37339. [Google Scholar] [CrossRef]
- Chen, J.; Ye, Q.; Hu, Z.; Wang, X.; Zhou, X. Jellyfish-inspired non-reciprocal light-fueled self-propelling liquid crystal elastomer-based fluidic saucer. Chaos Solitons Fractals 2026, 206, 117889. [Google Scholar] [CrossRef]
- Bai, C.; Kang, J.; Wang, Y.Q. Light-induced wrinkling in annulus anisotropic liquid crystal elastomer films. Phys. Rev. E 2025, 111, 015421. [Google Scholar] [CrossRef]
- Xu, T.; Pei, D.; Yu, S.; Zhang, X.; Yi, M.; Li, C. Design of mxene composites with biomimetic rapid and self-oscillating actuation under ambient circumstances. ACS Appl. Mater. Interfaces 2021, 13, 31978–31985. [Google Scholar] [CrossRef]
- Ohzono, T.; Saed, M.O.; Yue, Y.; Norikane, Y.; Terentjev, E.M. Dynamic manipulation of friction in smart textile composites of liquid-crystal elastomers. Adv. Mater. Interfaces 2019, 1, 1901996. [Google Scholar] [CrossRef]
- Jung, W.; Oh, S.; Bang, S.; Lee, Y.; Foo, Z.; Kim, G.; Zhang, Y.; Sylvester, D.; Blaauw, D. An ultra-low power fully integrated energy harvester based on self-oscillating switched-capacitor voltage doubler. IEEE J. Solid-State Circuits 2014, 49, 2800–2811. [Google Scholar] [CrossRef]
- Grédiac, M.; Pierron, F.; Surrel, Y. Novel procedure for complete in-plane composite characterization using a single t-shaped specimen. Exp. Mech. 1999, 39, 142–149. [Google Scholar] [CrossRef]
- Tang, R.; Liu, Z.; Xu, D.; Liu, J.; Yu, L.; Yu, H. Optical pendulum generator based on photomechanical liquid-crystalline actuators. ACS Appl. Mater. Interfaces 2015, 7, 8393–8397. [Google Scholar] [CrossRef]
- He, Q.; Yin, R.; Hua, Y.; Jiao, W.; Mo, C.; Shu, H.; Raney, J.R. A modular strategy for distributed, embodied control of electronics-free soft robots. Sci. Adv. 2023, 9, eade9247. [Google Scholar] [CrossRef]
- Yang, H.; Yin, X.; Zhang, C.; Chen, B.; Sun, P.; Xu, Y. Weaving liquid crystal elastomer fiber actuators for multifunctional soft robotics. Sci. Adv. 2025, 11, eade3058. [Google Scholar] [CrossRef] [PubMed]
- Hu, Y.; Ji, Q.; Huang, M.; Chang, L.; Zhang, C.; Wu, G.; Zi, B.; Bao, N.; Chen, W.; Wu, Y. Light-Driven self-scillating actuators with phototactic locomotion based on black phosphorus heterostructure. Angew. Chem. 2021, 60, 20511–20517. [Google Scholar] [CrossRef] [PubMed]
- Ge, D.; Yang, Q. Light-powered self-sustained jumper via splay-aligned liquid crystal elastomer. Chaos Solitons Fractals 2026, 206, 117918. [Google Scholar] [CrossRef]
- Akbar, F.; Rivkin, B.; Aziz, A.; Becker, C.; Karnaushenko, D.D.; Medina-Sánchez, M.; Karnaushenko, D.; Schmidt, O.G. Self-sufficient self-oscillating microsystem driven by low power at low Reynolds number. Sci. Adv. 2021, 7, eabj0767. [Google Scholar] [CrossRef]
- Liang, X.; Hu, Y. A Light-Spurred self-oscillator of liquid crystal elastomer with tunable shielding area under constant irradiation. Mech. Solids 2024, 59, 3584–3600. [Google Scholar] [CrossRef]
- Feng, X.L.; White, C.J.; Hajimiri, A.; Roukes, M.L. A self-sustaining ultrahigh-frequency nanoelectromechanical oscillator. Nat. Nanotechnol. 2008, 3, 342–346. [Google Scholar] [CrossRef]
- Yu, H.; Tang, W.; Mu, G.; Wang, H.; Chang, X.; Dong, H.; Qi, L.; Zhang, G.; Li, T. Micro-nanorobots propelled by oscillating magnetic fields. Micromachines 2018, 9, 540. [Google Scholar] [CrossRef]
- Kotikian, A.; Mcmahan, C.; Davidson, E.C.; Muhammad, J.M.; Weeks, R.D.; Daraio, C.; Lewis, J.A. Untethered soft robotic matter with passive control of shape morphing and propulsion. Sci. Robot. 2019, 4, eaax7044. [Google Scholar] [CrossRef]
- Manna, R.K.; Shklyaev, O.E.; Balazs, A.C. Chemical pumps and flexible sheets spontaneously form self-regulating oscillators in solution. Proc. Natl. Acad. Sci. USA 2021, 118, e2022987118. [Google Scholar] [CrossRef]
- Shin, B.; Ha, J.; Lee, M.; Park, K.; Park, G.H.; Choi, T.H.; Cho, K.-J.; Kim, H.Y. Hygrobot: A self-locomotive ratcheted actuator powered by environmental humidity. Sci. Robot. 2018, 3, aar2629. [Google Scholar] [CrossRef] [PubMed]
- Zhu, L.; He, M.; Chen, B.; Qian, J.; Xiao, R. Inflation of a polydomain nematic elastomeric membrane. J. Mech. Phys. Solids 2025, 198, 106075. [Google Scholar] [CrossRef]
- Fang, X.; Lou, J.; Wang, J.; Chuang, K.C.; Wu, H.M.; Huang, Z.L. A self-excited bistable oscillator with a light-powered liquid crystal elastomer. Int. J. Mech. Sci. 2024, 271, 109124. [Google Scholar] [CrossRef]
- Cunha, M.P.D.; Peeketi, A.R.; Ramgopal, A.; Annabattula, R.K.; Schenning, A.P.H.J. Light-driven continual oscillatory rocking of a polymer film. Chem. Open 2020, 9, 1149–1152. [Google Scholar]
- Hu, J.; Nie, Z.; Wang, M.; Liu, Z.; Huang, S.; Yang, H. Springtail-inspired light-driven soft jumping robots based on liquid crystal elastomers with monolithic three-leaf panel fold structure. Angew. Chem. 2023, 62, e202218227. [Google Scholar] [CrossRef]
- Kim, Y.; Berg, J.V.D.; Crosby, A.J. Autonomous snapping and jumping polymer gels. Nat. Mater. 2021, 20, 1695–1701. [Google Scholar] [CrossRef]
- Zhou, L.; Chen, H.; Li, Z.; Chen, X.; Gao, T.; Ge, D. Self-oscillation of a photo-actuated dual-beam system under linear optical excitation. Chaos Solitons Fractals 2026, 204, 117740. [Google Scholar] [CrossRef]
- Wei, L.; Jiang, X.; Hu, X.; Ge, D.; Li, K. Gravity-independent self-rolling of a photothermal liquid crystal elastomer rod for microgravity actuation. Commun. Nonlinear Sci. Numer. Simul. 2026, 157, 109764. [Google Scholar] [CrossRef]
- Xu, P.; Ren, X.; Zhu, H.; Yu, Y. Development of a self-sustained chaotic stirrer with electrothermal response liquid crystal elastomers. Chaos Solitons Fractals 2026, 203, 117656. [Google Scholar] [CrossRef]
- Chen, J.; Qiu, Y.; Zhou, X.; Ge, D.; Li, K. Impatiens-inspired self-sustained photo-ejector with liquid crystal elastomer shell. Thin-Walled Struct. 2026, 219, 114312. [Google Scholar] [CrossRef]
- Wei, L.; Jiang, X.; Li, S.; Ge, D.; Li, K. Gravity-independent self-rolling of liquid crystal elastomer rods via magnetically assisted photothermal actuation. Chaos Solitons Fractals 2026, 203, 117617. [Google Scholar] [CrossRef]
- Ge, D.; Wei, S.; Liang, Y.; Li, K. Snap-through self-peeling of liquid crystal elastomer bilayers under constant light. Thin-Walled Struct. 2026, 219, 114260. [Google Scholar] [CrossRef]
- Boissonade, J.; Kepper, P.D. Multiple types of spatio-temporal oscillations induced by differential diffusion in the landolt reaction. Phys. Chem. Chem. Phys. 2011, 13, 4132–4137. [Google Scholar] [CrossRef]
- Wang, X.; Dai, Y.; Zhao, J. Light-driven self-swing of a liquid crystal elastomer fiber-based composite pendulum in magnetic field. Chaos Solitons Fractals 2026, 202, 117570. [Google Scholar] [CrossRef]
- Yu, Y.; Quan, Y.; Li, T.; Huang, C.; Ma, H.; Li, K. Self-synchronization of a two-span liquid crystal elastomer continuous beam above a hot platform. Chaos Solitons Fractals 2026, 202, 117528. [Google Scholar] [CrossRef]
- Norouzikudiani, R.; Teresi, L.; Desimone, A. Self-Oscillations of submerged liquid crystal elastomer beams driven by light and self-shadowing. J. Elast. 2024, 156, 1243–1260. [Google Scholar] [CrossRef]
- Liu, C.-Y.; Wang, Z.-X.; Li, T.-Y.; Yang, J.-P.; Wang, Z.-J. Active pillar array structure by solvent-free liquid crystal elastomer resin. Chin. J. Polym. Sci. 2025, 43, 1012–1021. [Google Scholar] [CrossRef]
- Yu, Y.; Liu, F.; Huang, C.; Li, K. Self-swing of a thermo-responsive L-shaped rod partially resting on a hot plate. Thin-Walled Struct. 2026, 22, 114464. [Google Scholar] [CrossRef]
- Wu, H.; Hou, H.; Qiu, Y.; Ge, D.; Li, K. Light-powered self-rolling liquid crystal elastomer rovers between two hollows. Commun. Nonlinear Sci. Numer. Simul. 2026, 156, 109723. [Google Scholar] [CrossRef]
- Sun, J.; Wang, Y.; Liao, W.; Yang, Z. Ultrafast, high-contractile electrothermal-driven liquid crystal elastomer fibers towards artificial muscles. Small 2021, 17, 2103700. [Google Scholar] [CrossRef]
- Wei, L.; Yang, Z. The integration of sensing and actuating based on a simple design fiber actuator towards intelligent soft robots. Adv. Mater. Technol. 2022, 7, 2101260. [Google Scholar]
- Sun, X.; Zhao, J. Photomechanical self-oscillation of a bifilar pendulum with liquid crystal elastomeric fiber. Chaos Solitons Fractals 2026, 205, 117838. [Google Scholar] [CrossRef]
- Kang, W.; Cheng, Q.; Liu, C.; Wang, Z.; Li, D.; Liang, X. A constitutive model of monodomain liquid crystal elastomers with the thermal-mechanical-nematic order coupling. J. Mech. Phys. Solids 2025, 196, 105995. [Google Scholar] [CrossRef]
- Xu, P.; Zhang, J.; Zhou, K.; Wang, M.; Hu, W. Self-sustaining chaotic characteristics of liquid crystal elastomer pendulum under different linear temperature fields. Chaos Solitons Fractals 2026, 205, 117812. [Google Scholar] [CrossRef]
- Xu, S.; Hao, Z.; Chen, X.; Wan, C.; Yu, L.; Feng, X.-Q. Viscoelastic dynamics of photothermal-responsive liquid crystal elastomer fibers. Adv. Funct. Mater. 2024, 34, 2311425. [Google Scholar] [CrossRef]
- Wang, Y.; Dang, A.; Zhang, Z.; Yin, R.; Gao, Y.; Feng, L.; Yang, S. Repeatable and reprogrammable shape morphing from photoresponsive gold nanorod/liquid crystal elastomers. Adv. Mater. 2020, 32, 2004270. [Google Scholar] [CrossRef]
- Wang, Y.; Yin, R.; Jin, L.; Liu, M.; Gao, Y.; Raney, J.; Yang, S. 3D-Printed Photoresponsive Liquid Crystal Elastomer Composites for Free-Form Actuation. Adv. Funct. Mater. 2023, 33, 2210614. [Google Scholar] [CrossRef]
- Dai, L.; Wang, L.; Chen, B.; Xu, Z.; Wang, Z.; Xiao, R. Shape memory behaviors of 3D printed liquid crystal elastomers. Soft Sci. 2023, 3, 5. [Google Scholar] [CrossRef]
- Liu, J.; Xu, L.; Ji, Q.; Chang, L.; Hu, Y.; Peng, Q.; He, X. A MXene-Based Light-Driven Actuator and Motor with Self-Sustained Oscillation for Versatile Applications. Adv. Funct. Mater. 2024, 34, 2310955. [Google Scholar] [CrossRef]
- Zhou, X.; Peng, H.; Qiu, Y.; Li, K. Delayed oscillation of light-responsive hydrogel layers bonded to arigid substrate under periodic illumination. Chaos Solitons Fractals 2026, 202, 117445. [Google Scholar] [CrossRef]
- Xu, P.; Zhou, K.; Sun, X.; Li, K. Self-sustainable chaotic dynamics of a liquid crystal elastomer pendulum in radial linear temperature fields. Commun. Nonlinear Sci. Numer. Simul. 2026, 152, 109338. [Google Scholar] [CrossRef]
- Li, K.; Chen, Z.; Xu, P. Light-propelled self-sustained swimming of a liquid crystal elastomer torus at low Reynolds number. Int. J. Mech. Sci. 2022, 219, 107128. [Google Scholar] [CrossRef]
- Saeed, M.H.; Herman, J.A.; Das, A.; Kennedy, D.T.; White, T.J. Inverse Elastocaloric Output in Supramolecular Liquid Crystalline Elastomers. ACS Mater. Lett. 2025, 7, 2688–2694. [Google Scholar] [CrossRef]
- Zha, J.; Li, K.; Liu, J. The Light-Fueled Stable Self-Rolling of a Liquid Crystal Elastomer-Based Wheel. Polymers 2025, 17, 436. [Google Scholar] [CrossRef] [PubMed]
- Braun, L.B.; Hessberger, T.; Pütz, E.; Müller, C.; Giesselmann, F.; Serra, C.A.; Zentel, R. Actuating thermo-and photo-responsive tubes from liquid crystalline elastomers. J. Mater. Chem. C 2018, 6, 9093–9101. [Google Scholar] [CrossRef]
- Ge, D.; Li, K. Self-oscillating buckling and postbuckling of a liquid crystal elastomer disk under steady illumination. Int. J. Mech. Sci. 2022, 221, 107233. [Google Scholar] [CrossRef]
- Hessberger, T.; Braun, L.B.; Serra, C.A.; Zentel, R. Microfluidic preparation of liquid crystalline elastomer actuators. J. Vis. Exp. 2018, 20, 57715. [Google Scholar]
- Braun, L.B.; Linder, T.G.; Hessberger, T.; Zentel, R. Influence of a crosslinker containing an azo group on the actuation properties of a photoactuating LCE system. Polymers 2018, 10, 435. [Google Scholar] [CrossRef]
- Wang, Y.; Sun, J.; Liao, W.; Yang, Z. Liquid crystal elastomer twist fibers toward rotating microengines. Adv. Mater. 2022, 34, 2107840. [Google Scholar]
- Hogan, P.M.; Tajbakhsh, A.R.; Terentjev, E.M. UV manipulation of order and macroscopic shape in nematic elastomers. Phys. Rev. E 2002, 65, 041720. [Google Scholar] [CrossRef]
- Chaikin, P.M.; Lubensky, T.C. Principles of Condensed Matter Physics; Cambridge University Press: New York, NY, USA, 2000. [Google Scholar]










| Parameter | Value | Unit |
|---|---|---|
| A | 0~0.001 | cm/K |
| R | 5 | cm |
| L | 0.5~10 | cm |
| 0~2π | rad | |
| 0~2π | rad | |
| 0~0.001 | ||
| 0.001~0.1 | s | |
| 0~2 × 103 | W | |
| K | 0~8 | W/K |
| 0.1 | J/K | |
| 300 | K | |
| g | 0~50 | |
| m | 0~0.01 | kg |
| k | 10~1000 | / |
| 0~0.8 | / | |
| 0~10 | / | |
| 0~1.5 | / | |
| 0.1~2 | / | |
| 0~2π | / | |
| 0~0.1 | / |
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Li, C.; Xu, L.; Dai, Y.; Dai, Y. A Light-Driven Self-Spinning and Translation Disc Exploiting Photothermal Liquid Crystal Elastomers. Micromachines 2026, 17, 284. https://doi.org/10.3390/mi17030284
Li C, Xu L, Dai Y, Dai Y. A Light-Driven Self-Spinning and Translation Disc Exploiting Photothermal Liquid Crystal Elastomers. Micromachines. 2026; 17(3):284. https://doi.org/10.3390/mi17030284
Chicago/Turabian StyleLi, Cong, Leyi Xu, Yuntong Dai, and Yu Dai. 2026. "A Light-Driven Self-Spinning and Translation Disc Exploiting Photothermal Liquid Crystal Elastomers" Micromachines 17, no. 3: 284. https://doi.org/10.3390/mi17030284
APA StyleLi, C., Xu, L., Dai, Y., & Dai, Y. (2026). A Light-Driven Self-Spinning and Translation Disc Exploiting Photothermal Liquid Crystal Elastomers. Micromachines, 17(3), 284. https://doi.org/10.3390/mi17030284

