Journal Description
Pollutants
Pollutants
is an international, peer-reviewed, open access journal on all aspects of environmental pollution published quarterly online by MDPI.
- Open Access— free to download, share, and reuse content. Authors receive recognition for their contribution when the paper is reused.
- High Visibility: indexed within AGRIS, and many other databases.
- Rapid Publication: first decisions in 15 days; acceptance to publication in 3 days (median values for MDPI journals in the second half of 2021).
- Recognition of Reviewers: APC discount vouchers, optional signed peer review, and reviewer names published annually in the journal.
Latest Articles
Reduction of Heavy Hydrocarbons from Oilfield Produced Water
Pollutants 2022, 2(2), 234-251; https://doi.org/10.3390/pollutants2020016 - 07 May 2022
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This paper presents attempts to reduce the concentration of organic pollutants in oilfield produced wastewater before its discharge into natural water bodies or reinjection into the wells. The contaminant content was significantly decreased by wastewater treatment, based on solid phase adsorption, photocatalytic degradation
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This paper presents attempts to reduce the concentration of organic pollutants in oilfield produced wastewater before its discharge into natural water bodies or reinjection into the wells. The contaminant content was significantly decreased by wastewater treatment, based on solid phase adsorption, photocatalytic degradation of organic molecules and chemical oxidation of oily compounds. The study was conducted with real wastewater, which is in practice released in the environment. The produced water samples, taken from four sampling points in the oilfield site, were analyzed for physicochemical (temperature, redox potential (Eh), conductivity, pH, dissolved oxygen) and specific (chemical oxygen demand (COD), total oily hydrocarbons (TOH), phenols) parameters, cations (Ca2+, Mg2+, Na+, K+) and anions (Cl−, HCO3−, SO42−, S2−), in order to determine the initial water status. The organic contaminants in oilfield produced water showed COD of 39–58 mg/L, TOH of 152–363 mg/L and phenols of 0.07–0.21 mg/L. The TOH was chosen as a suitable parameter for the evaluation of the treatment method efficiency. The adsorption on activated charcoal decreased the TOH levels up to 52 mg/L, which corresponds to 85% removal of oily compounds. Chemical oxidation, carried out with Ca(ClO)2 in a concentration of 400 mg/L for 1 h at room temperature, showed TOH removal in the range of 80–94% for different wastewater samples. The use of 300 mg/L TiO2 or ZnO under UV irradiation for 12 h led to TOH removal of 25–78% and 82–92%, respectively. Both photocatalysts were characterized by using X-ray diffraction, reflectance UV-vis spectroscopy and scanning electron microscopy. The crystal forms anatase and wurtzite for TiO2 and ZnO, respectively, were found. The estimated band gap of 3.48 eV for direct transition in TiO2 and 3.25 eV for ZnO agrees well with that reported in the literature. Higher photodegradation of organic compounds was observed for ZnO, indicating that it absorbed more light photons than TiO2 did. A mechanism for photocatalytic degradation over a more efficient photocatalyst, ZnO, was proposed based on the GC-MS analysis of raw water and treated effluents produced for 6 and 12 h.
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Open AccessArticle
A Trans-Disciplinary and Integral Model of Participatory Planning for a More Sustainable and Resilient Basilicata
Pollutants 2022, 2(2), 205-233; https://doi.org/10.3390/pollutants2020015 - 07 May 2022
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This article focuses on the importance of a trans-disciplinary and participatory planning approach aiming at promoting a more resilient community. The COVID-19 outbreak is not just a health pandemic, but also a compound crisis in a globalized world, which emphasizes the need for,
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This article focuses on the importance of a trans-disciplinary and participatory planning approach aiming at promoting a more resilient community. The COVID-19 outbreak is not just a health pandemic, but also a compound crisis in a globalized world, which emphasizes the need for, and urgency of, an ecological transition towards a new development model. This paper presents the outcomes of a research experience aimed at implementing a new development model inspired by integral sustainability for a transformative resilience of Basilicata region (Southern Italy). The research approach was implemented according to a participatory planning methodology to overcome the significant impacts of the pandemic and guide the transition towards real, sustainable development in all its dimensions (economic, social, environmental, and institutional). Community engagement in a research partnership allowed stakeholders to benefit from collective wisdom, creating more meaningful findings in preparing the regional community to face the challenges of the ecological transition. Scientific support of the research was fundamental in supporting political decision making in identifying strategic actions for a more sustainable and resilient Basilicata in this delicate historical moment of awareness, where the future will depend on today’s choices.
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(This article belongs to the Special Issue A New Development Model for a More Sustainable, Resilient and Fairer world)
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Indoor CO2 and Thermal Conditions in Twenty Scottish Primary School Classrooms with Different Ventilation Systems during the COVID-19 Pandemic
Pollutants 2022, 2(2), 180-204; https://doi.org/10.3390/pollutants2020014 - 03 May 2022
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Healthy indoor environments influence the comfort, health and wellbeing of the occupants. Monitoring the indoor temperature, relative humidity and CO2 levels in primary schools during the COVID-19 pandemic was mandated by a local authority in Scotland. The aim was to investigate the
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Healthy indoor environments influence the comfort, health and wellbeing of the occupants. Monitoring the indoor temperature, relative humidity and CO2 levels in primary schools during the COVID-19 pandemic was mandated by a local authority in Scotland. The aim was to investigate the comfort and safety of the teachers and their pupils. This paper presents the measurements of indoor climate in 20 classrooms in four different primary schools in Scotland. The schools were of different architypes. The classrooms were of different sizes, orientations and occupancy, and had different ventilation systems. Ventilation was achieved either by manually opening the windows, or by a mechanical ventilation system. Indoor air temperature, relative humidity and carbon dioxide (CO2) concentrations were continuously monitored for one week during the heating season 2020/21. Occupancy and opening of the windows were logged in by the teachers. The ventilation rates in the classrooms were estimated by measuring the CO2 concentrations. On the 20 classrooms of the study, data of 19 were analysed. The results show that four of the five mechanically ventilated classrooms performed better than natural ventilation, which indicates that opening the windows depended on the customs and habits. Classrooms in naturally ventilated Victorian buildings have the worst average ventilation rate (4.38 L/s per person) compared to the other classrooms (5.8 L/s per person for the more recent naturally ventilated ones, and 6.08 L/s per person for the mechanically ventilated ones). The results of this preliminary study will be used as the basis to find ways to ensure adequate ventilation in natural ventilated classrooms.
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(This article belongs to the Special Issue Pollutants in Indoor Air)
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Active and Passive Sustainability: Measuring the Anti-Fragility of Territories
Pollutants 2022, 2(2), 172-179; https://doi.org/10.3390/pollutants2020013 - 01 May 2022
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Sustainability is a paradigm of generative action if combined with the principle of antifragility. This contribution, adhering to a transdisciplinary approach, proposes a reinterpretation of the principles of the 2030 Agenda, orienting them towards a community-building model. Sustainability can be seen as passive
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Sustainability is a paradigm of generative action if combined with the principle of antifragility. This contribution, adhering to a transdisciplinary approach, proposes a reinterpretation of the principles of the 2030 Agenda, orienting them towards a community-building model. Sustainability can be seen as passive (care) and active (custody), determining paths to be activated at the territorial level. Sustainability is a communitarian learning path measured by one’s antifragility capacity. The effectiveness of the Agenda is linked to the dissemination and accountability of the challenges contained in the 17 objectives. The local scale is perhaps the most suitable for activating this process. However, this requires a strengthening of the anti-fragility of communities and organizations, which must be more capable of recognizing and reducing vulnerabilities and weaknesses. A promising field of application is that of impact assessment, to be reworked in the light of the antifragility approach.
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(This article belongs to the Special Issue A New Development Model for a More Sustainable, Resilient and Fairer world)
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Trends of CO and NO2 Pollutants in Iran during COVID-19 Pandemic Using Timeseries Sentinel-5 Images in Google Earth Engine
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, , , , , and
Pollutants 2022, 2(2), 156-171; https://doi.org/10.3390/pollutants2020012 - 21 Apr 2022
Abstract
The first case of COVID-19 in Iran was reported on 19 February 2020, 1 month before the Nowruz holidays coincided with the global pandemic, leading to quarantine and lockdown. Many studies have shown that environmental pollutants were drastically reduced with the spread of
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The first case of COVID-19 in Iran was reported on 19 February 2020, 1 month before the Nowruz holidays coincided with the global pandemic, leading to quarantine and lockdown. Many studies have shown that environmental pollutants were drastically reduced with the spread of this disease and the decline in industrial activities. Among these pollutants, nitrogen dioxide (NO2) and carbon monoxide (CO) are widely caused by anthropogenic and industrial activities. In this study, the changes in these pollutants in Iran and its four metropolises (i.e., Tehran, Mashhad, Isfahan, and Tabriz) in three periods from 11 March to 8 April 2019, 2020, and 2021 were investigated. To this end, timeseries of the Sentinel-5P TROPOMI and in situ data within the Google Earth Engine (GEE) cloud-based platform were employed. It was observed that the results of the NO2 derived from Sentinel-5P were in agreement with the in situ data acquired from ground-based stations (average correlation coefficient = 0.7). Moreover, the results showed that the concentration of NO2 and CO pollutants in 2020 (the first year of the COVID-19 pandemic) was 5% lower than in 2019, indicating the observance of quarantine rules, as well as people’s initial fear of the coronavirus. Contrarily, these pollutants in 2021 (the second year of the COVID-19 pandemic) were higher than those in 2020 by 5%, which could have been due to high vehicle traffic and a lack of serious policy- and law-making by the government to ban urban and interurban traffic. These findings are essential criteria that might be used to guide future manufacturing logistics, traffic planning and management, and environmental sustainability policies and plans. Furthermore, using the COVID-19 scenario and free satellite-derived data, it is now possible to investigate how harmful gas emissions influence air quality. These findings may also be helpful in making future strategic decisions on how to cope with the virus spread and lessen its negative social and economic consequences.
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(This article belongs to the Special Issue The Impact of COVID Lockdowns on Reducing Air Pollution)
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Characterization of Annual Air Emissions Reported by Pulp and Paper Mills in Atlantic Canada
Pollutants 2022, 2(2), 135-155; https://doi.org/10.3390/pollutants2020011 - 08 Apr 2022
Abstract
The pulp and paper industry is a major contributor to water and air pollution globally. Pulp and paper processing is an intensive energy consuming process that produces multiple contaminants that pollute water, air, and affect ecological and human health. In Canada, the National
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The pulp and paper industry is a major contributor to water and air pollution globally. Pulp and paper processing is an intensive energy consuming process that produces multiple contaminants that pollute water, air, and affect ecological and human health. In Canada, the National Pollutant Release Inventory (NPRI) is used to assess the release of air pollutants into the atmosphere from industrial facilities (including pulp and paper mills) and provides a repository of annual emissions reported by individual facilities. This study compared annual air emissions of carbon monoxide, nitrogen oxides, total particulate matter (TPM), PM2.5, PM10, sulphur dioxide, and volatile organic compounds from nine different pulp and/or paper mills in Atlantic Canada from three provinces (Nova Scotia, New Brunswick, and Newfoundland and Labrador) between 2002 and 2019. Results revealed that annual releases were several orders of magnitude higher than federal reporting thresholds suggested by Environment and Climate Change Canada. Pulp mills emit higher pollutant loads than those producing paper. The highest exceedance of a reporting threshold was for particulate matter (PM2.5) at Northern Pulp in Nova Scotia. The emissions of PM2.5 were on average (over a 17-year period) about 100,000% above the reporting threshold of 0.3 tonnes per year.
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(This article belongs to the Topic Air Pollution – An Interdisciplinary Approach to the Problem of Air Pollution and Improvement of Air Quality)
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Experimental Evaluations of the Impact of an Additive Oxidizing Electronic Air Cleaner on Particles and Gases
Pollutants 2022, 2(2), 98-134; https://doi.org/10.3390/pollutants2020010 - 06 Apr 2022
Abstract
Electronic air cleaning (EAC) technologies have garnered significant attention for use in buildings. Many EAC technologies rely on the addition of reactive constituents to indoor air to react with gas-phase compounds, enhance particle deposition, and/or inactivate microorganisms. However, limited data are available on
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Electronic air cleaning (EAC) technologies have garnered significant attention for use in buildings. Many EAC technologies rely on the addition of reactive constituents to indoor air to react with gas-phase compounds, enhance particle deposition, and/or inactivate microorganisms. However, limited data are available on the efficacy of many EAC technologies and their potential to form chemical byproducts during operation. Here we experimentally evaluate the indoor air quality impacts, specifically targeting particles and gases but not microbial constituents, of a commercially available additive oxidizing EAC that generates positive and negative ions and hydrogen peroxide (H2O2). Tests were conducted in a large unoccupied test chamber in Chicago, IL and an unoccupied laboratory in Portland, OR under a combination of natural conditions (i.e., without pollutant injection) and perturbation conditions (i.e., with pollutant injection and decay). A combination of integrated and time-resolved measurements was used across both test locations. Chamber tests at lower airflow rates demonstrated that operation of the EAC: (i) had no discernible impact on particle concentrations or particle loss rates, with estimated clean air delivery rates (CADRs) for various particle measures less than ±10 m3/h, (ii) was associated with apparent decreases in some volatile organic compounds (VOCs) and increases in other VOCs and aldehydes, especially acetaldehyde, although a combination of high propagated uncertainty, limitations in test methods (e.g., lack of replicates), and variability between repeated tests limit what quantitative conclusions can be drawn regarding gas-phase organics; (iii) did generate H2O2, assessed using a crude measure, and (iv) did not generate ozone (O3). Laboratory tests at higher airflow rates, which involved injection and decay of particles and a single VOC (limonene), both simultaneously and separately, demonstrated that: (i) pollutant loss rates for both particles and limonene were slightly lower with the EAC on compared to off, yielding slightly negative pollutant removal efficiencies (albeit largely within propagated uncertainty) and (ii) there was a change in observed concentrations of one potential limonene degradation product, m/z 59 (putatively identified as acetone), with steady-state levels increasing from 10 ppb (air cleaner off) to 15 ppb (air cleaner on). No increases or decreases beyond measurement uncertainty were observed for other analyzed gaseous limonene degradation products. Overall, both chamber and laboratory tests demonstrated negligible effectiveness of this device at the test conditions described herein for removing particles and mixed results for VOCs, including decreases in some VOCs, no discernible differences in other VOCs, and apparent increases in other compounds, especially lower molecular weight aldehydes including acetaldehyde.
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(This article belongs to the Special Issue Pollutants in Indoor Air)
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Investigation of Indoor and Outdoor Fine Particulate Matter Concentrations in Schools in Salt Lake City, Utah
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, , , , , , and
Pollutants 2022, 2(1), 82-97; https://doi.org/10.3390/pollutants2010009 - 04 Mar 2022
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Although there is mounting evidence that suggests that air pollution is impactful to human health and educational outcomes, this is especially problematic in schools with higher air pollution levels. To understand whether all schools in an urban area are exposed to similar outdoor
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Although there is mounting evidence that suggests that air pollution is impactful to human health and educational outcomes, this is especially problematic in schools with higher air pollution levels. To understand whether all schools in an urban area are exposed to similar outdoor air quality and whether school infrastructure protects children equally indoors, we installed research-grade sensors to observe PM2.5 concentrations in indoor and outdoor settings to understand how unequal exposure to indoor and outdoor air pollution impacts indoor air quality among high- and low-income schools in Salt Lake City, Utah. These data and resulting analysis show that poor air quality may impact school settings and the potential implications with respect to environmental inequality. Based on this approach, we found that during atmospheric inversions and dust events, there was a lag ranging between 35 and 73 min for the outdoor PM2.5 concentrations to follow a similar temporal pattern as the indoor PM2.5. This lag has policy and health implications and may help to explain rising concerns regarding reduced educational outcomes related to air pollution in urban areas.
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A Longitudinal Study of Bacteriophages as Indicators of Norovirus Contamination of Mussels (Mytilus edulis) and Their Overlying Waters
Pollutants 2022, 2(1), 66-81; https://doi.org/10.3390/pollutants2010008 - 01 Mar 2022
Abstract
Sewage pollution leads to the contamination of bivalve shellfish by pathogenic microorganisms. Bacterial indicators support the management of risks associated with the consumption of shellfish; however, they often fail to indicate adequately the potential hazard to human health posed by certain human enteric
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Sewage pollution leads to the contamination of bivalve shellfish by pathogenic microorganisms. Bacterial indicators support the management of risks associated with the consumption of shellfish; however, they often fail to indicate adequately the potential hazard to human health posed by certain human enteric viruses. Bacteriophages have been proposed as alternative indicators that may more effectively predict the presence of enteric viral pathogens. This study explored the relationships between bacterial indicators (Escherichia coli (E. coli), faecal coliforms (FC) and intestinal enterococci (IE)), phages (somatic (SOMPH), F-specific RNA (F + PH) and human-specific Bacteroides GB-124 phages (GB124PH)) and Norovirus (NoV) (GI/GII) in mussels (Mytilus edulis) and their overlying waters. The bioaccumulation of these indicators and Norovirus in shellfish matrices (e.g., flesh, digestive gland) was investigated bimonthly over a 12-month period in an English estuary. The findings revealed a marked seasonality in the distribution of all organisms, with the highest levels occurring during the autumn/winter months. The levels of all phages in shellfish and their overlying waters correlated better with the levels of Norovirus than with those of bacterial indicators. Somatic coliphages were the indicator that exhibited the strongest correlations with NoV (rho = 0.929). This study suggests that relatively low-cost culture-based phage enumeration appears to offer a more accurate indication of the likely presence of Norovirus in mussels than traditional bacterial indicators.
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(This article belongs to the Section Water Pollution)
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Phytoremediation Capability and Copper Uptake of Maize (Zea mays L.) in Copper Contaminated Soils
Pollutants 2022, 2(1), 53-65; https://doi.org/10.3390/pollutants2010007 - 01 Mar 2022
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Copper is a frequently used heavy metal worldwide and known to be an essential micronutrient for most living organisms including plants. However, excessive levels of copper in soil may adversely affect plant growth and survival. The continuing introduction of copper to soil, e.g.,
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Copper is a frequently used heavy metal worldwide and known to be an essential micronutrient for most living organisms including plants. However, excessive levels of copper in soil may adversely affect plant growth and survival. The continuing introduction of copper to soil, e.g., through excessive utilization of agrochemicals has raised serious environmental concerns throughout the world. A variety of plants have the capability to eliminate pollutants from soil through different mechanisms; however, limited information is reported on phytoremediation potential of maize (Zea mays L.) and its uptake and the accumulation potential in copper-containing soils. The effects of additions of 0, 50, 100, 200 and 300 mg kg−1 of copper to soil on growth parameters of Z. mays, copper uptake from soil and accumulation in roots and shoots, and phytoremediation potential of Z. mays were investigated in this research. Copper content in soil and plant samples were determined using atomic absorption spectrophotometry. The addition of 50 mg kg−1 Cu stimulated Z. mays growth parameters, while higher content of Cu exhibited inhibitory effects of plant growth. Results indicated that roots accumulated significantly higher levels of Cu than shoots in all treatments, suggesting dominancy of phytostabilization mechanism in remediation of Cu-polluted soil by Z. mays. However, translocation of Cu from the roots to the aerial parts enhanced to some extent with copper level in soil. The greatest Cu accumulation capacity of 5210 µg per pot was gained in Z. mays cultivated in soil treated with 200 mg kg−1 copper. Results demonstrated that Z. mays can promisingly remediate low to moderately copper-contaminated soils.
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Open AccessArticle
Pharmaceuticals Influence on Phragmites australis Phytoremediation Potential in Cu Contaminated Estuarine Media
Pollutants 2022, 2(1), 42-52; https://doi.org/10.3390/pollutants2010006 - 11 Feb 2022
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The aim of the present work was to evaluate the influence of two different pharmaceutical compounds (bezafibrate and paroxetine) on the phytoremediation potential of Phragmites australis in an estuarine medium contaminated by copper. Plants were exposed for seven days to a simplified estuarine
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The aim of the present work was to evaluate the influence of two different pharmaceutical compounds (bezafibrate and paroxetine) on the phytoremediation potential of Phragmites australis in an estuarine medium contaminated by copper. Plants were exposed for seven days to a simplified estuarine medium, elutriate solution, with or without sediment. The medium was doped with copper and bezafibrate or paroxetine. P. australis plants were able to accumulate a significant amount of Cu, particularly in their roots (600 and 250 times increase in copper levels in the absence and presence of sediment, respectively), corroborating the phytostabilization potential of salt marsh plants. Metal uptake and translocation was significantly lower in the presence of sediment (Cu in leaves increased 20 times in the absence and only 4 times in the presence of sediment). An effect of either pharmaceutical compound on metal accumulation was not observed (levels of Cu in plants tissues were in general identical) but, in the presence of sediment, both bezafibrate and paroxetine changed Cu solubility in elutriate solution, either decreasing or increasing it. The current study highlights the possible influence the presence of contaminants of different characteristics (inorganic and organic contaminants) can have on salt marsh phytoremediation potential in the long run, and the effects pollutants might have in the environment.
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Open AccessArticle
Thermally Enhanced Bioremediation of NAPL Polluted Soil-Water Resources
Pollutants 2022, 2(1), 32-41; https://doi.org/10.3390/pollutants2010005 - 08 Feb 2022
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The use of conventional techniques for physico-chemical remediation of hydrocarbon such non-aqueous phase liquids (NAPL)-polluted sites may disturb the natural biotic settings of the (sub)-surface. However, natural attenuation has been reported very slow and sometime results as incomplete removal under prevailing site conditions.
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The use of conventional techniques for physico-chemical remediation of hydrocarbon such non-aqueous phase liquids (NAPL)-polluted sites may disturb the natural biotic settings of the (sub)-surface. However, natural attenuation has been reported very slow and sometime results as incomplete removal under prevailing site conditions. In particular, microbial growth is quite slow in cold regions, which reduces the applicability of bioremediation in treating NAPL-polluted soil-water. Thus, this study aims to evaluate the thermally enhanced bioremediation techniques to treat NAPL-polluted soil-water using practical experiments. A one-dimensional large column setup was designed and fabricated for this purpose. The column was integrated with automatic temperature controlling baths to maintain different soil-water temperatures (4 °C, 20 °C, 28 °C, and 36 °C), which was circulated through the porous media filled in the column setup. Results show a high dissolution rate of toluene, the selected light NAPL, at an elevated temperature of 28–36 °C. The biodegradation rates of the NAPL were found to be 0.002 mg L/h, 0.008 mg L/h, 0.012 mg L/h, and 0.015 mg L/h at soil-water temperature levels of 4 °C, 20 °C, 28 °C, and 36 °C, respectively. It was found that at high soil-water temperature (28 °C and 36 °C), a significant increment in microbial actions accelerates the biodegradation rate of NAPL in the subsurface system. The outcomes of this study may help in treating NAPL-polluted sites using solar or geo-thermal based heating systems for thermally enhanced bioremediation.
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Open AccessArticle
Transfer of 7 Organic UV Filters from Sediment to the Ragworm Hediste diversicolor: Bioaccumulation of Benzophenone-3 and Further Proof of Octocrylene Metabolism
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, , , , and
Pollutants 2022, 2(1), 23-31; https://doi.org/10.3390/pollutants2010004 - 04 Feb 2022
Cited by 1
Abstract
Organic UV filters are continuously released in aquatic ecosystems due to their widespread use, especially in touristic coastal environments. Generally, organic UV filters are poorly soluble in water and tend to accumulate in the sediment compartment. This represents a conceivable risk for sediment-dwelling
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Organic UV filters are continuously released in aquatic ecosystems due to their widespread use, especially in touristic coastal environments. Generally, organic UV filters are poorly soluble in water and tend to accumulate in the sediment compartment. This represents a conceivable risk for sediment-dwelling organisms and a potential for transfer of the UV filters up the food chain. This study aimed to assess the potential transfer of seven UV filters including benzophenone-3 (BP3), bis-ethylhexyloxyphenol methoxyphenyl triazine (BEMT), butyl methoxydibenzoylmethane (BM), methylene bis-benzotriazolyl tetramethylbutylphenol (MBBT), 2-ethylhexyl salicylate (ES), diethylhexyl butamido triazone (DBT), and octocrylene (OC) from artificial spiked sediment (10 µg.g−1 dry weight) to sediment-dwelling worms. All UV filters were detected in the worms after 28 days of exposure, but only BP3 was apparently bioaccumulated, with a biota sediment accumulation factor (BSAF) of 12.38 ± 4.65. However, metabolomic profiling revealed that OC was metabolized by the worms into 11 fatty acid conjugates, demonstrating that OC did also accumulate in the worms in the form of OC–fatty acid conjugates. Here, the sole quantification of the parent organic UV filter underestimated the accumulation factor and the exposure of organisms. In general, it is therefore important to pair the conventional method (BSAF calculus) with other techniques, such as metabolomics, to assess the actual potential for bioaccumulation of xenobiotics including transformed xenobiotics.
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(This article belongs to the Section Impact Assessment of Environmental Pollution)
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Acknowledgment to Reviewers of Pollutants in 2021
Pollutants 2022, 2(1), 21-22; https://doi.org/10.3390/pollutants2010003 - 27 Jan 2022
Abstract
Rigorous peer-reviews are the basis of high-quality academic publishing [...]
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Removal of Volatile Toluene Using K2CO3-Activated Carbon Adsorbents Prepared from Buckwheat Hull
Pollutants 2022, 2(1), 12-20; https://doi.org/10.3390/pollutants2010002 - 04 Jan 2022
Abstract
Carbon adsorbents for use in the removal of gaseous toluene from the air were prepared from buckwheat (Fagopyrum esculentum Moench) hull. A chemically-activated adsorbent was prepared via the impregnation of raw hull powder with potassium carbonate, followed by thermal decomposition. The chemically-activated
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Carbon adsorbents for use in the removal of gaseous toluene from the air were prepared from buckwheat (Fagopyrum esculentum Moench) hull. A chemically-activated adsorbent was prepared via the impregnation of raw hull powder with potassium carbonate, followed by thermal decomposition. The chemically-activated adsorbent exhibited improved adsorption capacity for toluene compared to the adsorbent prepared without chemical activation. Toluene concentration in the air decreased from 220 ppm to 160 ppm during 24 h of adsorption using unactivated adsorbent. Only a trace amount of toluene remained after the adsorption under the same conditions using K2CO3-activated adsorbent. This improvement was explained based on experimental results, specifically, iodine adsorption tests, methylene blue adsorption tests, and microscopic observations. Chemical activation dramatically increased the specific surface area of the adsorbent and created mesopores capable of adsorbing toluene. This study revealed that a mesoporous adsorbent for use in volatile toluene removal can be prepared from waste biomass (buckwheat hull) by chemical activation using potassium carbonate.
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(This article belongs to the Section Pollution Removal)
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Open AccessArticle
The Evaluation of the Impact of a Saharan Event on Particulate Matter Using Compositional Data Analysis
Pollutants 2022, 2(1), 1-11; https://doi.org/10.3390/pollutants2010001 - 04 Jan 2022
Abstract
The proposed approach based on compositional data analysis was applied on simultaneous measurements of the mineral element concentrations of PM10 and PM2.5 from a typical suburban site with and without a Saharan event. The suburban site is located in the city
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The proposed approach based on compositional data analysis was applied on simultaneous measurements of the mineral element concentrations of PM10 and PM2.5 from a typical suburban site with and without a Saharan event. The suburban site is located in the city of Rome. The selected mineral elements were Al, Si, Ca, Fe, Ti, Mg, and Sr. The data relating to these elements are reported in a previous study. The considered elements are mainly related to mineral matter. The proposed approach allows statistically validating that the mineral element concentrations of PM during days with a Saharan event differ from those without a Saharan event in terms of mineral element composition and size distribution. In particular, the results showed that the compositional data analysis applied to simultaneous measurements of mineral element concentrations of PM10 and PM2.5 is a helpful technique that can be used to study environmental sites affected by natural sources such as Saharan events. Moreover, the presented technique can be handy in all those conditions where it is important to discriminate whether the occurrence of an exceedance or a violation of the daily limit value established for PM could also be due to natural sources.
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(This article belongs to the Section Air Pollution)
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Open AccessArticle
Quantification of Platinum in Edible Mushrooms Using Voltammetric Techniques
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Pollutants 2021, 1(4), 270-277; https://doi.org/10.3390/pollutants1040021 - 20 Dec 2021
Abstract
Edible mushrooms are a food source with interesting nutritional values. The chief objective of this research was to develop a consistent method for the quantitative ultra-trace analysis of Pt in mushrooms, which is complex because it cannot be readily quantified by common analytical
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Edible mushrooms are a food source with interesting nutritional values. The chief objective of this research was to develop a consistent method for the quantitative ultra-trace analysis of Pt in mushrooms, which is complex because it cannot be readily quantified by common analytical procedures. This research is one of the first analytical methods to establish Pt amount in these vegetables. In this research, 28 different edible mushroom samples from Italy were investigated. Determination of Pt in mushrooms was completed using Differential Pulse Voltammetry (DPV). In this study, we applied the standard addition method because there are no certified reference mushrooms containing platinum group elements on the market. The platinum quantification limit was 0.03 µg kg−1 d.w. In the analyzed samples, platinum amount was in the range of 0.03–73 µg kg−1. Our mushroom samples had a Pt content lower than the concentrations recommended by international establishments for other foodstuffs. In the future, the optimized method could be used for the analysis of plant and animal matrices intended for food supply.
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(This article belongs to the Special Issue Analysis of Trace Pollutants in Complex Matrices)
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Use of Clay Minerals to Control Radioactive Cesium Leaching from Municipal Solid Waste Incineration Ash in Fukushima Prefecture in Summer and Winter
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and
Pollutants 2021, 1(4), 253-269; https://doi.org/10.3390/pollutants1040020 - 03 Dec 2021
Abstract
Radioactive cesium (r-Cs) released from the 2011 Fukushima Daiichi Nuclear Power Plant attaches to vegetation/soil and is collected as municipal solid waste (MSW) for incineration, being concentrated in incineration ash (bottom ash [BA], fly ash [FA], and chelate-treated FA [TFA]). r-Cs in FA
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Radioactive cesium (r-Cs) released from the 2011 Fukushima Daiichi Nuclear Power Plant attaches to vegetation/soil and is collected as municipal solid waste (MSW) for incineration, being concentrated in incineration ash (bottom ash [BA], fly ash [FA], and chelate-treated FA [TFA]). r-Cs in FA and TFA can easily leach upon contact with moisture. It is important to prevent further contamination, as r-Cs has negative effects on ecosystems and the human body. Naturally available clay minerals, considered effective for capturing r-Cs, are a good alternative. Here, we sampled ash from MSW incineration facilities in Fukushima in August 2016 and February 2017. We used energy dispersive X-ray fluorescence spectroscopy and Ge semiconductor detector to determine elemental composition and r-Cs concentration in the samples and conducted leaching tests. We also determined the extent of leaching suppression by zeolite, acidic clay, and vermiculite. Chloride contents and r-Cs leaching rates were higher in FA and TFA than in BA, regardless of the season. Prior direct addition and mixing of clay minerals (5 to 20 wt.%) effectively prevented r-Cs leaching. This study is the first to examine r-Cs leaching inhibition by clay mineral direct addition and mixing to MSW incineration ash.
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(This article belongs to the Section Radioactive Pollution)
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Open AccessArticle
Environmental Impact Assessment of Remediation Strategy in an Oil Spill in the Ecuadorian Amazon Region
by
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Pollutants 2021, 1(4), 234-252; https://doi.org/10.3390/pollutants1040019 - 28 Nov 2021
Abstract
Past petroleum-extraction activities in Ecuador have contaminated its Amazon region. To assess the environmental impact attributed to remediation activities regarding the cleanup of these oil spills, two scenarios were studied according to Life Cycle Analysis methodology: (1) No-action, which means to leave the
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Past petroleum-extraction activities in Ecuador have contaminated its Amazon region. To assess the environmental impact attributed to remediation activities regarding the cleanup of these oil spills, two scenarios were studied according to Life Cycle Analysis methodology: (1) No-action, which means to leave the contamination in place without any further action and (2) Environmental remediation, where the environmental-load attributed to the remediation of the representative oil spill was studied. Results indicated that the no-action scenario presented a higher environmental impact for 12 out of the 16 environmental categories evaluated (climate change, ozone depletion, human toxicity non-cancer effects, particulate matter, ionizing radiation human health, ionizing radiation ecosystem, photochemical ozone formation, acidification, terrestrial eutrophication, marine eutrophication, freshwater ecotoxicity, mineral, fossil and renewable resource depletion). Moreover, the no-action scenario presented a global weighted score of contamination of 5.45 points, while the remediation scenario got a score of 3.3 points, which means that the remediation decreased by 39% of the global environmental impact due to the remediation activity applied, showing the positive influence of environmental remediation to mitigate the effects attributed to the presence of pollution sources associated to the petroleum industry in the Ecuadorian Amazon region.
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(This article belongs to the Section Impact Assessment of Environmental Pollution)
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Open AccessArticle
Understanding Land Changes for Sustainable Environmental Management: The Case of Basilicata Region (Southern Italy)
Pollutants 2021, 1(4), 217-233; https://doi.org/10.3390/pollutants1040018 - 28 Nov 2021
Abstract
Sustainable land management is one of the key actions for the achievement of objectives set by the 2030 Agenda for Sustainable Development. In particular, land represents a fundamental resource to address issues of climate change, biodiversity preservation, maintaining ecosystem services, and at the
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Sustainable land management is one of the key actions for the achievement of objectives set by the 2030 Agenda for Sustainable Development. In particular, land represents a fundamental resource to address issues of climate change, biodiversity preservation, maintaining ecosystem services, and at the same time ensuring shared prosperity and well-being. Therefore, it is necessary to activate strategies to monitor changes in land use and land cover in order to evaluate strategies for proper management. To do this, the new open source geospatial analysis tools and the increasing availability of remote sensed open data can allow the activation of methodologies for monitoring changes in land use and land cover in order to provide data usable in other research areas or, for example, to implement a decision support system for environmental sustainability. In this study, a GIS approach based on open remote sensing data has been used to perform a spatial analysis of land cover changes within the Basilicata region (Southern Italy) that is spatially expeditious yet accurate. The results showed a very evident land transformation with important repercussions on the environmental components. The ease of use of techniques makes this methodology replicable in other territory and can be used as a preliminary approach to sustainable development model.
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(This article belongs to the Special Issue A New Development Model for a More Sustainable, Resilient and Fairer world)
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