Advanced Coating Technology by Physical Vapor Deposition and Applications

A special issue of Coatings (ISSN 2079-6412). This special issue belongs to the section "Surface Characterization, Deposition and Modification".

Deadline for manuscript submissions: 20 September 2025 | Viewed by 17290

Special Issue Editor


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Guest Editor
Department of Electrical Engineering, Feng Chia University, Taichung 40724, Taiwan
Interests: optical design; optical thin film; residual stress; optical interferometry; fiber-optic sensors
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Special Issue Information

Dear Colleagues,

Physical vapor deposition (PVD) is a widely used technique used for the preparation of thin films and surface coatings. PVD has been widely used in industry and combined with different methods to produce film components with excellent performance. Uniform PVD coatings provide hard surfaces that can be applied to a variety of materials and substrates. The PVD process can also be used to form multilayer coatings, composite coatings, oblique coatings, and unique structures. The PVD multilayered film structure is beneficial for improving oxidation resistance, enhancing mechanical properties, reducing internal stress, inhibiting crack propagation, and improving fracture toughness. We sincerely invite you to contribute your original papers to this Special Issue. The topics of interest include (but are not limited to) the following topics:

  • Thin film coating techniques;
  • Characterization of thin films for micro-components;
  • Advanced sputtering coatings;
  • -Multilayer thin film preparation and applications;
  • Novel PVD coating techniques;
  • Optical interference coatings;
  • Mechanical stress in thin films and coatings;
  • Simulation and modeling in PVD processes.

Prof. Dr. Chuen-Lin Tien
Guest Editor

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Keywords

  • physical vapor deposition
  • coating technology
  • thin film
  • multilayer coatings
  • optical interference coatings
  • sputtering
  • evaporation

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Published Papers (7 papers)

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Editorial

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5 pages, 214 KiB  
Editorial
Special Issue “Advanced Coating Technology by Physical Vapor Deposition and Applications”
by Chuen-Lin Tien
Coatings 2023, 13(2), 467; https://doi.org/10.3390/coatings13020467 - 18 Feb 2023
Cited by 12 | Viewed by 4979
Abstract
Coating technology covers a wide range of fields [...] Full article

Research

Jump to: Editorial

19 pages, 14017 KiB  
Article
Multi-Step Simulations of Ionized Metal Physical Vapor Deposition to Enhance the Plasma Formation Uniformity
by Cheongbin Cheon, Min Young Hur, Ho Jun Kim and Hae June Lee
Coatings 2025, 15(1), 11; https://doi.org/10.3390/coatings15010011 - 25 Dec 2024
Viewed by 840
Abstract
Ionized metal physical vapor deposition (IMPVD), which is operated at a very low pressure to take advantage of the metal sputtering effect on the target surface, has unique properties compared with conventional DC magnetron sputtering. In this study, we investigated the effect of [...] Read more.
Ionized metal physical vapor deposition (IMPVD), which is operated at a very low pressure to take advantage of the metal sputtering effect on the target surface, has unique properties compared with conventional DC magnetron sputtering. In this study, we investigated the effect of the rotating magnetic field on the plasma formation of IMPVD to enhance the deposition uniformity. This was accomplished through a multi-step simulation, which enabled plasma analysis, sputtered particle and chemical reaction analysis, and deposition profile analysis. A two-dimensional particle-in-cell Monte Carlo simulation utilizes the exact cross-section data of the Cu ion collisions and calculates the particle trajectories under specific magnetic field profiles. This new methodology gives guidance for the design of the magnetic field profiles of IMPVD and an understanding of the physical mechanism. Full article
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13 pages, 4907 KiB  
Article
Tribological Comparison of Coatings Produced by PVD Sputtering for Application on Combustion Piston Rings
by Ney Francisco Ferreira, Filipe Fernandes, Patric Daniel Neis, Jean Carlos Poletto, Talha Bin Yaqub, Albano Cavaleiro, Luis Vilhena and Amilcar Ramalho
Coatings 2024, 14(9), 1109; https://doi.org/10.3390/coatings14091109 - 2 Sep 2024
Viewed by 1480
Abstract
This article compares the tribological performance of coatings produced by PVD sputtering. Transition metal dichalcogenide (TMD) coatings doped with carbon (WSC and MoSeC) and nitrogen (WSN and MoSeN) and a conventional diamond-like carbon (DLC) coating are compared. The tribological evaluation was oriented towards [...] Read more.
This article compares the tribological performance of coatings produced by PVD sputtering. Transition metal dichalcogenide (TMD) coatings doped with carbon (WSC and MoSeC) and nitrogen (WSN and MoSeN) and a conventional diamond-like carbon (DLC) coating are compared. The tribological evaluation was oriented towards the use of coatings on piston rings. Block-on-ring tests in a condition lubricated with an additive-free polyalphaolefin (PAO 8) and at temperatures of 30, 60, and 100 °C were carried out to evaluate the coatings in boundary lubrication conditions. A load scanner test was used to evaluate dry friction and scuffing propensity. In addition to WSN, all other TMD coatings (WSC, MoSeC, and MoSeN) exhibited lower friction than DLC in dry and lubricated conditions. The study reveals that WSC, among TMD coatings, offers promising results, with significantly lower friction levels than DLC, while demonstrating reduced wear and a lower risk of metal adhesion. These findings suggest that WSC may be a viable alternative to DLC in piston rings, with potential benefits for reducing fuel consumption and increasing engine durability. Full article
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19 pages, 21066 KiB  
Article
The Influence of Bias Voltage and Gas Pressure on Edge Covering during the Arc-PVD Deposition of Hard Coatings
by Otmar Zimmer, Tim Krülle and Thomas Litterst
Coatings 2024, 14(6), 732; https://doi.org/10.3390/coatings14060732 - 7 Jun 2024
Cited by 1 | Viewed by 1525
Abstract
The edge area is especially essential for cutting tools, since this is the contact zone between the work piece and the tool. Hard coatings (PVD or CVD coatings) can protect the edge against wear and they are commonly used. The geometries of the [...] Read more.
The edge area is especially essential for cutting tools, since this is the contact zone between the work piece and the tool. Hard coatings (PVD or CVD coatings) can protect the edge against wear and they are commonly used. The geometries of the cutting edges change during the coating process, with the edge radius increasing. Therefore, the film thickness is limited and the initial radius of the uncoated tool must be smaller than the target radius of the coated edge. A new coating process based on vacuum arc PVD was developed to overcome this limitation. The film growth at the edges can be properly controlled by means of selected coating materials and process conditions. Thus, it is possible to grow edges sharper than the initial edge geometry. Different substrates were coated with different coating systems. Parameters such as the bias voltage, coating pressure, and initial radius were varied within this work. It was found that the application of a bias voltage is crucial for the generation of sharp edges. It was also found that the edge sharpening caused by coatings works best on samples with an initial radius of around 15 µm. Full article
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14 pages, 3669 KiB  
Article
Optical Interference Filters Combined with Thin Film Residual Stress Compensation for Image Contrast Enhancement
by Chuen-Lin Tien, Shu-Hui Su, Ching-Ying Cheng, Yuan-Ming Chang and Dong-Han Mo
Coatings 2023, 13(5), 857; https://doi.org/10.3390/coatings13050857 - 30 Apr 2023
Cited by 3 | Viewed by 2171
Abstract
We propose two single-wavelength notch filters and one dual-wavelength (480 and 620 nm) notch filter to enhance image contrast. The stack structure of the notch filters was designed as (Ta2O5/SiO2)4Ta2O5 in Essential [...] Read more.
We propose two single-wavelength notch filters and one dual-wavelength (480 and 620 nm) notch filter to enhance image contrast. The stack structure of the notch filters was designed as (Ta2O5/SiO2)4Ta2O5 in Essential Macleod thin film simulation software. Dual-electron-beam evaporation with ion beam-assisted deposition was used to prepare optical interference filters with different center wavelengths. A multilayer notch filter with a center wavelength of 620 nm was deposited on the front surface of the glass, and then a notch filter with a center wavelength of 480 nm was coated on the rear surface of the same glass. The proposed dual-wavelength (480 and 620 nm) notch filter is a combination of two single-wavelength notch filters coated on a double-sided glass substrate to compensate for residual stress. The transmittance, residual stress, and surface roughness of the proposed notch filter were evaluated using different measuring instruments. The experimental results show that the residual stress of the dual-wavelength notch filter could be reduced to 10.8 MPa by using a double-sided coating technique. The root-mean-square (RMS) surface roughness of the notch filters was measured by using a Linnik microscopic interferometer. The RMS surface roughness was 1.80 for the 620 nm notch filter and 2.09 for the 480 nm notch filter. The image contrast obtained with the three different notch filters was measured using an optical microscope and a CMOS camera. The contrast value could be increased from 0.328 (without a filter) to 0.696 (dual-wavelength notch filter). Full article
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16 pages, 5290 KiB  
Article
Effect of Gradient Multilayer Design on Tribological Performance of TiN/TiSiN Coatings Prepared by Cathodic Arc Ion Plating
by Rong Tu, Jiao Jiao, Mingquan Jiang, Mai Yang, Baifeng Ji, Tenghua Gao, Qizhong Li, Song Zhang and Lianmeng Zhang
Coatings 2023, 13(5), 836; https://doi.org/10.3390/coatings13050836 - 26 Apr 2023
Cited by 5 | Viewed by 2650
Abstract
Hard coatings, such as transition metal nitrides, have been widely applied to improve the mechanical properties and tribological performance of cutting tools. The coatings in various multilayered or gradient structures have been designed to meet the demands of more severe service environments and [...] Read more.
Hard coatings, such as transition metal nitrides, have been widely applied to improve the mechanical properties and tribological performance of cutting tools. The coatings in various multilayered or gradient structures have been designed to meet the demands of more severe service environments and more precise processing requirements. In this work, TiN/TiSiN coatings in several gradient and multilayered structures were deposited on cemented carbides by cathodic arc ion plating using Ti and TiSi alloy targets. The modulation period (Λ) of the multilayer gradually varies with thickness, ranging from 6 to 46 nm. The gradient multilayer coatings consist of a nanocrystalline-amorphous composite with compact growth. The coating with a modulation period first increasing and then decreasing has the highest hardness of 38 GPa, and the maximum residual compressive stress of −2.71 GPa, as well as the minimum coefficient of friction (COF) and wear rate. Gradient and multilayer structures moderate the brittleness caused by the presence of amorphous SiNx phase and optimize the mechanical properties and tribological performances of the coatings. Full article
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9 pages, 4431 KiB  
Article
Direct Current Reactive Sputtering Deposition and Plasma Annealing of an Epitaxial TiHfN Film on Si (001)
by Ping-Hsun Wu, Kun-An Chiu, Fu-Han Shih, Yu-Siang Fang, Thi-Hien Do, Wei-Chun Chen and Li Chang
Coatings 2023, 13(1), 183; https://doi.org/10.3390/coatings13010183 - 14 Jan 2023
Cited by 1 | Viewed by 2083
Abstract
Deposition of a heteroepitaxial TiHfN film with a growth rate of about 1 μm/h was successfully achieved on a Si (001) substrate at a temperature above 700 °C by direct current magnetron reactive sputtering of a Ti0.6Hf0.4 (in atomic fraction) [...] Read more.
Deposition of a heteroepitaxial TiHfN film with a growth rate of about 1 μm/h was successfully achieved on a Si (001) substrate at a temperature above 700 °C by direct current magnetron reactive sputtering of a Ti0.6Hf0.4 (in atomic fraction) target with an Ar/N2 gas mixture. Annealing of the as-deposited TiHfN/Si sample at a temperature above 1000 °C using microwave plasma with H2/N2 gas was performed to further improve the TiHfN film’s quality. X-ray diffraction results show that the heteroepitaxial TiHfN film on Si exhibits a cube-on-cube relationship as {001}TiHfN//{001}Si and <110>TiHfN//<110>Si. X-ray rocking curve measurements show that the full width at half maximum of (200)TiHfN is 1.36° for the as-deposited TiHfN film, while it is significantly reduced to 0.53° after microwave plasma annealing. The surface morphologies of the as-deposited and annealed TiHfN films are smooth, with a surface roughness of around ~2 nm. Cross-sectional scanning/transmission electron microscopy (S/TEM) shows a reduction in defects in the annealed film, and X-ray photoelectron spectroscopy shows that the film composition remains unchanged. Additionally, S/TEM examinations with atomic resolution illustrate domain matching epitaxy (DME) between TiHfN and Si at the interface. The TiHfN films have good electrical conducting properties with resistivities of 40–45 μΩ·cm. Full article
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