3.1. Magnetization Curves
The three aforementioned techniques for characterizing the magnetization properties of Wiegand wires differ fundamentally in their underlying operating principles:
The MOKE detects changes in the polarization state (Kerr rotation angle and ellipticity) of linearly polarized light reflected from the wire surface, enabling characterization of the near-surface magnetization state. This technique provides sensitive detection of surface domain structures and dynamic magnetic behavior in Wiegand wires [
13].
The VSM measures voltage signals induced in detection coils as the sample undergoes mechanical vibration under an applied magnetic field. Utilizing lock-in amplification techniques, it precisely determines material hysteresis loops, making it particularly suitable for analyzing the stepped magnetization reversal behavior associated with the bistable magnetic structure of Wiegand wires. This method effectively characterizes the large Barkhausen jump phenomena arising from the hard/soft magnetic composite architecture.
The excitation coil method detects Wiegand pulses induced in a pick-up coil through rapid flux changes (dΦ/dt) generated by large Barkhausen jumps. This approach directly probes the microscopic dynamics of domain wall pinning–depinning processes. The underlying physical mechanism involves the nonlinear breakdown of pinning potentials at hard/soft magnetic interfaces, revealing the discrete nature of irreversible domain wall motion during magnetization reversal.
The fundamental differences in the measurement principles of the three aforementioned techniques result in distinctive magnetization curves for the Wiegand wire, as shown in
Figure 5.
In our previous studies, we utilized First-Order Reversal Curves (FORCs) analysis and FORC diagrams to investigate the coercivity distribution and magnetic structure of Wiegand wires, establishing the absence of a distinct boundary between the soft and hard magnetic phases while demonstrating a radially graded, continuously increasing coercivity distribution from surface to core [
12]. To further elucidate the mechanism responsible for large Barkhausen jumps in Wiegand wires, the present study utilizes samples with systematically varying diameters to propose a novel five-layer magnetic structure model with corresponding coercivity distribution. This model architecture, shown schematically in
Figure 6, consists of the following layers arranged sequentially from the surface inward: soft-lock layer, soft-jump layer, intermediate-1 layer, intermediate-2 layer, and hard core.
The original Wiegand wire sample has a diameter of 0.23 mm. As successive etching removes the outer layers, the diameter decreases correspondingly: when the diameter is reduced to 0.18 mm, the Soft-jump layer becomes exposed; at 0.14 mm, the Intermediate-1 layer is revealed; at 0.10 mm, the Intermediate-2 layer is reached; and at 0.06 mm, only the Hard core remains present.
For the unetched 0.23 mm sample (possessing the complete five-layer structure), the three measurement methods reveal substantial differences, as shown in
Figure 5a.
The magnetization curve obtained by MOKE measurements exhibits sharp, large Barkhausen jumps in applied magnetic fields of 5–15 mT. These jumps correspond to rapid magnetization reversal in the soft-lock layer at the Wiegand wire surface and abrupt transitions in the magnetic domain structure.
When a maximum applied field of 3 mT was used, the minor hysteresis loop measured by VSM shows distinct large Barkhausen jumps. The switching field for this jump was measured at approximately 0.8 mT. which are attributed to the outermost soft-lock layer of the Wiegand wire. This layer has a coercivity of approximately 2 mT, meaning that an external maximum applied field of 3 mT is sufficient to induce rapid magnetization reversal. This process leads to the formation of magnetic locking coupling with the underlying soft transition layer, followed by sudden collapse of this magnetic lock.
The magnetization curve derived from Wiegand pulse measurements also exhibits large Barkhausen jumps when external maximum applied field was 3 mT. These jumps result from abrupt magnetic flux changes caused by rapid magnetization reversal in the soft-lock layer, followed by the formation and subsequent sudden collapse of magnetic locking coupling with the soft-jump layer. This behavior corresponds well with the characteristic voltage pulses detected by the pick-up coils.
As the outer layers of the Wiegand wire are progressively etched away and the diameter decreases, the resulting evolution of the magnetic structure significantly influences the measurement outcomes, as demonstrated in
Figure 5b–e.
Figure 5b displays the magnetization curves of the 0.18 mm sample. In comparison with
Figure 5a, these curves resemble those of the unetched 0.23 mm sample, except that no distinct large Barkhausen jumps are detected in the MOKE-measured magnetization curve. Notably, pronounced large Barkhausen jumps are observed at 3 mT and 5 mT in both the minor hysteresis loop measured by VSM and the magnetization curve derived from Wiegand pulse measurements.
This phenomenon occurs because the outermost layer—specifically, the soft-lock layer of the original Wiegand wire—has been etched away, which alters the magnetic structure. The newly exposed surface layer (formerly the soft-jump layer) exhibits a coercivity of approximately 3.5 mT, requiring stronger external magnetic fields to undergo rapid magnetization reversal. Following this reversal, it forms magnetic locking coupling with the adjacent Intermediate-1 layer.
This magnetic locking coupling builds up energy as it resists the external magnetic field until the applied field strength becomes sufficient to overcome the pinning potential. The subsequent sudden collapse of this coupling releases the stored magnetostatic energy and triggers two simultaneous phenomena:
Rapid magnetization reversal within the Intermediate-1 layer, resulting in large Barkhausen jumps observable in VSM-measured minor hysteresis loops;
Abrupt changes in magnetic flux around the wire, which induce characteristic Wiegand voltage pulses in the pick-up coils.
Figure 5c,d present the magnetization curves for the 0.14 mm and 0.10 mm samples, respectively. Distinct large Barkhausen jumps are observed at 3 mT, 5 mT, 7 mT, and 10 mT in both the minor hysteresis loops measured by VSM and the magnetization curves derived from Wiegand pulse measurements. This behavior follows a mechanism similar to that observed in the 0.18 mm sample, which exhibited jumps at 3 mT and 5 mT, but requires stronger external magnetic fields to induce these jumps due to the higher coercivity of the newly exposed surface layers in the progressively etched samples.
Figure 5e presents the magnetization curves of the 0.06 mm sample (hard core only). Based on our previous FORC analysis of these differentially etched samples [
12], the 0.06 mm specimen is confirmed to have all outer layers removed, retaining only the hard magnetic core. The MOKE-measured magnetization curves show nearly complete overlap, demonstrating the homogenization of the surface magnetic structure after removal of the layered architecture.
Due to the absence of both the outer soft layers and intermediate transition layers, the formation of magnetic locking coupling under external fields is precluded, and interlayer magnetic interactions are eliminated. The monolithic hard magnetic core undergoes magnetization reversal solely in response to external field variations. Consequently, no large Barkhausen jumps are observed in either the minor hysteresis loops measured by VSM or the magnetization curves derived from Wiegand pulse measurements. However, the VSM minor loop still reveals small-scale jumps, suggesting possible nanoscale magnetic domain reorganization within the hard core.
The higher apparent switching field observed via MOKE for the 0.23 mm wire, compared to VSM and coil measurements, resolves the distinction between the initial onset of reversal and the large Barkhausen jump. VSM and coil detect the early, gradual onset of reversal in the soft-lock layer. In contrast, MOKE specifically captures the later, abrupt collapse of the magnetic lock between the soft-lock and soft-jump layers, which triggers the rapid, collective reversal of the soft-jump layer and constitutes the large jump itself, occurring at a higher critical field as predicted by the simulation.
Based on a comparative analysis of the experimental results, we conclude that the formation and subsequent abrupt collapse of magnetic locking coupling between the outermost layer and adjacent layers is the fundamental mechanism responsible for large Barkhausen jumps in Wiegand wires. Essentially, the multilayered magnetic architecture of Wiegand wires is crucial for generating these pronounced jumps. Experimental samples with monolithic magnetic structures lack this characteristic layered configuration and consequently fail to produce large Barkhausen jumps. This explanation accounts for why such jumps are observed in
Figure 5c,d but are absent in
Figure 5e.
3.2. Switching Fields and Coercive Fields
We further performed statistical analysis of switching fields and coercive fields for differentially etched Wiegand wire samples using data obtained from both VSM-measured minor hysteresis loops and Wiegand pulse-derived magnetization curves, as summarized in
Figure 7.
The switching field is defined as the magnetic field strength at which large Barkhausen jumps initiate during the magnetization reversal process after crossing the origin. The coercive field corresponds to the magnetic field strength at which the net magnetization of the sample reaches zero during the reverse field sweep after crossing the origin.
Our analysis reveals a significant inverse correlation between sample diameter and magnetic threshold parameters: reduced diameters correspond to systematically increased switching and coercive fields. These findings provide conclusive validation of the hypothesized radially graded coercivity distribution in Wiegand wires—demonstrating a progressive enhancement of coercivity from the surface layers toward the core region. This gradient-modulated coercivity profile represents both a fundamental magnetic characteristic unique to Wiegand wires and the essential mechanism enabling large Barkhausen jumps.
The divergent behavior observed via MOKE is not contradictory but highly instructive, as it underscores the radial inhomogeneity of the magnetic structure in our wires. As established, our Wiegand wires possess a soft magnetic outer layer. MOKE probes only the magnetization dynamics within the optical penetration depth (tens of nanometers) of this surface. For the standard 0.23 mm wire, the intact soft outer layer hosts the large Barkhausen jump, which dominates the MOKE signal and results in a high, sharp switching field. For the etched wires (0.18–0.06 mm), the chemical etching has progressively removed this specific soft outer layer responsible for the surface jump. Consequently, the MOKE signal from the etched surface originates from underlying magnetic layers with different reversal characteristics, leading to smaller, more gradual loops and an apparently lower coercive field.
3.3. Simulation Model and Simulation Results
A simulation model was developed using JMAG-Designer (JSOL Corp., Tokyo, Japan, ver. 20.0). The simulation model was designed with five concentric layers of equal radial thickness, maintaining the actual external dimensions of a standard Wiegand wire (length: 13 mm; diameter: 0.23 mm). The coercivity values for the five layers, from outermost to innermost, were set to 2 mT/μ
0, 3.5 mT/μ
0, 5 mT/μ
0, 6.5 mT/μ
0, and 8 mT/μ
0, respectively, to represent a continuous radially increasing coercivity profile. Note that due to the cylindrical geometry, the layers have different volumes. The subsequent analysis of simulated magnetization patterns and reversal sequences focuses on the interplay between the set coercivity gradient and interlayer magnetostatic coupling, which governs the observed phenomena (e.g., cascading unlock), rather than treating them as a simple consequence of volume-weighted magnetic moment dominance. Due to the axial symmetry of the Wiegand wire, the simulation displays the magnetization state of each layer using only the upper half of the cross-section, as shown in
Figure 8.
The simulation of the proposed five-layer magnetic structure model of the Wiegand wire, conducted at varying applied magnetic field strengths, begins by demagnetizing the model before applying an initial 15 mT magnetic field. After reaching stabilization, the magnetization state of each layer exhibits its simplest form, with uniform magnetization direction throughout. The outermost soft-lock layer, possessing the lowest coercivity, demonstrates the strongest magnetization intensity, which becomes progressively weaker in inner layers with higher coercivity values. Due to demagnetization field effects and static magnetic coupling interactions, weaker magnetization is observed at the ends of the model, particularly more pronounced near the core layer region, as shown in
Figure 9a.
When the applied magnetic field is reduced to 0 mT, the magnetization direction of each layer remains unchanged. The soft-lock and soft-jump layers, characterized by lower coercivity, exhibit a significant reduction in magnetization intensity. In contrast, the intermediate layers and hard core show increased magnetization due to the influence of the soft-layer magnetization. As the simulation proceeds, the magnetization distribution begins to exhibit increasing disorder, particularly in regions adjacent to the higher-coercivity core layer. This phenomenon is attributed to the combined effects of the demagnetization field and static magnetic coupling between layers, as illustrated in
Figure 9b. Note that the simulated continuous decrease in magnetization magnitude within a layer is a distributed relaxation process, which is typically not resolved as a discrete feature in spatially averaged surface measurements like MOKE.
When the applied magnetic field is reduced to 0 mT and then a reverse magnetic field is gradually increased, a decrease in magnetization is observed throughout the entire model at −1.19 mT. At this field strength, the outermost soft-lock layer begins to reverse its magnetization direction. Partial magnetization reversal is also observed at the ends of the other layers due to demagnetization field effects and magnetostatic coupling interactions. As a result, the soft-lock and soft-jump layers become magnetically anti-parallel, forming a stable magnetic lock through magnetostatic coupling, as demonstrated in
Figure 9c.
In the simulation model, as the external magnetic field strength increases, the magnetization of the outermost soft-lock layer correspondingly rises. This leads to a progressive strengthening of the magnetic locking coupling between the soft-lock and soft-jump layers, as demonstrated in
Figure 9d.
Simultaneously, the energy barrier for magnetization reversal in the soft-jump layer increases, creating a competitive interplay between these two opposing forces. When the reverse magnetic field strength reaches −2.74 mT, significant magnetization reversal occurs in the central region of the soft-jump layer, as shown in
Figure 9e.
The collapse of magnetic locking coupling between the soft-lock and soft-jump layers triggers the rapid reversal of magnetization in the soft-jump layer, resulting in the large Barkhausen jump observed in the Wiegand wire. This simulation result corresponds closely with our experimental measurements of leakage magnetic flux density in a standard 0.23 mm diameter Wiegand wire, where complete magnetization reversal occurred at an external magnetic field of −3 mT under identical experimental conditions.
Furthermore, when the magnetic field strength reaches −4.04 mT, the soft-jump layer completes its magnetization reversal and establishes a new magnetic locking coupling with the intermediate-1 layer, as shown in
Figure 9f. As the magnetic field strength continues to increase, this magnetic locking coupling progressively strengthens.
At a field strength of −5.12 mT, the magnetic locking coupling between the soft-jump and intermediate-1 layers collapses, leading to the establishment of a new magnetic locking coupling between the intermediate-1 and intermediate-2 layers, as shown in
Figure 9g. With further increase in magnetic field strength to −6.99 mT, this newly formed magnetic lock between the intermediate-1 and intermediate-2 layers also collapses, simultaneously resulting in the formation of a new magnetic locking coupling between the intermediate-2 layer and the hard core, as demonstrated in
Figure 9h.
Finally, when the applied magnetic field reaches the same magnitude but in the opposite direction to the initial applied magnetic field, the magnetization state of the simulated model closely resembles the initial configuration, though with the magnetization of each layer reversed in direction, as presented in
Figure 9i.
The JMAG simulation of the Wiegand wire’s five-layer magnetic structure fundamentally reveals that large Barkhausen jumps originate from the synchronized collapse of interfacial magnetic locking coupling between layers, rather than from independent magnetization reversal within individual layers. Specifically, the abrupt rupture of magnetostatic coupling between the soft-lock and soft-jump layers at −2.74 mT triggers rapid magnetization reversal in the soft-jump layer, generating the characteristic jump—a finding consistent with experimental observations at −3 mT in 0.23 mm diameter wires. This process initiates a cascade of energy transfer: each coupling collapse (e.g., between soft-jump and intermediate-1 layers at −5.12 mT, and between intermediate-1 and intermediate-2 layers at −6.99 mT) releases stored magnetostatic energy, propagating the reversal process inward while simultaneously establishing new locking coupling with deeper layers. Crucially, the radially graded coercivity profile (2–8 mT/μ0) enables this sequential establishment and rupture of magnetic locking coupling, demonstrating that interlayer magnetostatic interactions—rather than isolated soft-layer dynamics—govern the Wiegand effect.