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Search Results (522)

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Keywords = polymer actuator

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21 pages, 7773 KiB  
Article
Dynamic Properties and Vibration Control of Additively Manufactured Carbon and Glass Fiber Reinforced Polymer Composites Using MFC: A Numerical Study with Experimental Validation
by Ali Raza, Magdalena Mieloszyk, Rūta Rimašauskienė, Vytautas Jūrėnas, Nabeel Maqsood, Marius Rimašauskas and Tomas Kuncius
J. Manuf. Mater. Process. 2025, 9(7), 235; https://doi.org/10.3390/jmmp9070235 - 8 Jul 2025
Viewed by 385
Abstract
With the growing need for lightweight, durable, and high-performance structures, additively manufactured (AM) polymer composite structures have captured significant attention in the engineering community. These structures offer considerable advantages in various dynamic engineering sectors including automotive, aviation, and military. Thus, this investigation emphasizes [...] Read more.
With the growing need for lightweight, durable, and high-performance structures, additively manufactured (AM) polymer composite structures have captured significant attention in the engineering community. These structures offer considerable advantages in various dynamic engineering sectors including automotive, aviation, and military. Thus, this investigation emphasizes the numerical analysis of the dynamic properties and vibration control of AM polylactic acid (PLA) composite structures reinforced with continuous glass fibers (CGFR-PLA) and carbon fibers (CCFR-PLA), with 0°–0° and 0°–90° layer orientations. The findings of this numerical study are compared and validated against earlier published experimental results. Initially, the numerical models were created using the Abaqus CAE 2024, replicating the actual experimental models. The numerical bending modal frequency of each numerical model is determined, and the 0°–0° oriented models exhibited considerably higher values compared to the corresponding 0°–90° models. Significant differences were noted between the numerical and experimental values in the higher modes, mainly due to existence of voids and misalignment in the actual models that were not considered in numerical models. Following this, a numerical amplitude frequency response (AFR) analysis was conducted to observe vibration amplitude variations as a function of frequency. The AFR numerical results demonstrated consistent trends with the experimental results despite differences between the absolute values of both scenarios. Afterwards, vibration amplitude control analysis was performed under the influence of a macro fiber composite (MFC) actuator. The findings from both numerical and experimental cases revealed that vibration control was noticeably higher in 0°–0° oriented structures compared to 0°–90° structures. Experimental models demonstrated higher vibration control effectiveness than the corresponding numerical models. Although significant differences between the numerical and experimental vibration response values were observed in each composite structure, the numerical results exhibited consistent trends with the experiments. This discrepancy is attributed to the challenge of capturing all boundary conditions of the experimental scenario and incorporating them into the numerical simulation. Full article
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18 pages, 2880 KiB  
Article
Novel Magnetically Charged Grafts for Vascular Repair: Process Optimization, Mechanical Characterization and In Vitro Validation
by Iriczalli Cruz-Maya, Roberto De Santis, Luciano Lanotte and Vincenzo Guarino
Polymers 2025, 17(13), 1877; https://doi.org/10.3390/polym17131877 - 5 Jul 2025
Viewed by 480
Abstract
In the last decade, magnetic nanoparticles (MNPs) have attracted much attention for the implementation of non-invasive approaches suitable for the diagnosis and treatment of vascular diseases. In this work, the optimization of novel vascular grafts loaded with Nickel-based nanoparticles via electrospinning is proposed. [...] Read more.
In the last decade, magnetic nanoparticles (MNPs) have attracted much attention for the implementation of non-invasive approaches suitable for the diagnosis and treatment of vascular diseases. In this work, the optimization of novel vascular grafts loaded with Nickel-based nanoparticles via electrospinning is proposed. Two different polycarbonate urethanes—i.e., Corethane A80 (COT) and Chronoflex AL80 (CHF)—were used to fabricate 3D electrospun nanocomposite grafts. SEM analysis showed a homogeneous distribution of fibers, with slight differences in terms of average diameters as a function of the polymer used—(1.14 ± 0.18) µm for COT, and (1.33 ± 0.23) µm for CHF—that tend to disappear in the presence of MNPs—(1.26 ± 0.19) µm and (1.26 ± 0.213) µm for COT/NPs and CHF/NPs, respectively. TGA analyses confirmed the higher ability of CHF to entrap MNPs in the fibers—18.25% with respect to 14.63% for COT—while DSC analyses suggested an effect of MNPs on short-range rearrangements of hard/soft micro-domains of CHF. Accordingly, mechanical tests confirmed a decay of mechanical strength in the presence of MNPs with some differences depending on the matrix—from (6.16 ± 0.33) MPa to (4.55 ± 0.2) MPa (COT), and from (3.67 ± 0.18) MPa to (2.97 ± 0.22) MPa (CNF). The in vitro response revealed that the presence of MNPs did not negatively affect cell viability after 7 days in in vitro culture, suggesting a promising use of these materials as smart vascular grafts able to support the actuation function of vessel wall muscles. Full article
(This article belongs to the Section Polymer Applications)
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68 pages, 10407 KiB  
Review
Bioinspired Morphing in Aerodynamics and Hydrodynamics: Engineering Innovations for Aerospace and Renewable Energy
by Farzeen Shahid, Maqusud Alam, Jin-Young Park, Young Choi, Chan-Jeong Park, Hyung-Keun Park and Chang-Yong Yi
Biomimetics 2025, 10(7), 427; https://doi.org/10.3390/biomimetics10070427 - 1 Jul 2025
Viewed by 1067
Abstract
Bioinspired morphing offers a powerful route to higher aerodynamic and hydrodynamic efficiency. Birds reposition feathers, bats extend compliant membrane wings, and fish modulate fin stiffness, tailoring lift, drag, and thrust in real time. To capture these advantages, engineers are developing airfoils, rotor blades, [...] Read more.
Bioinspired morphing offers a powerful route to higher aerodynamic and hydrodynamic efficiency. Birds reposition feathers, bats extend compliant membrane wings, and fish modulate fin stiffness, tailoring lift, drag, and thrust in real time. To capture these advantages, engineers are developing airfoils, rotor blades, and hydrofoils that actively change shape, reducing drag, improving maneuverability, and harvesting energy from unsteady flows. This review surveys over 296 studies, with primary emphasis on literature published between 2015 and 2025, distilling four biological archetypes—avian wing morphing, bat-wing elasticity, fish-fin compliance, and tubercled marine flippers—and tracing their translation into morphing aircraft, ornithopters, rotorcraft, unmanned aerial vehicles, and tidal or wave-energy converters. We compare experimental demonstrations and numerical simulations, identify consensus performance gains (up to 30% increase in lift-to-drag ratio, 4 dB noise reduction, and 15% boost in propulsive or power-capture efficiency), and analyze materials, actuation, control strategies, certification, and durability as the main barriers to deployment. Advances in multifunctional composites, electroactive polymers, and model-based adaptive control have moved prototypes from laboratory proof-of-concept toward field testing. Continued collaboration among biology, materials science, control engineering, and fluid dynamics is essential to unlock robust, scalable morphing technologies that meet future efficiency and sustainability targets. Full article
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24 pages, 5782 KiB  
Article
Gamma Irradiation-Induced Synthesis of Nano Au-PNiPAAm/PVA Bi-Layered Photo-Thermo-Responsive Hydrogel Actuators with a Switchable Bending Motion
by Nikolina Radojković, Jelena Spasojević, Ivana Vukoje, Zorica Kačarević-Popović, Una Stamenović, Vesna Vodnik, Goran Roglić and Aleksandra Radosavljević
Polymers 2025, 17(13), 1774; https://doi.org/10.3390/polym17131774 - 26 Jun 2025
Viewed by 403
Abstract
In this study, we present bi-layered hydrogel systems that incorporate different sizes and shapes of gold nanoparticles (nanospheres and nanorods) for potential use in areas such as photoactuators, soft robotics, artificial muscles, drug delivery and tissue engineering. The synthesized nano Au-PNiPAAm/PVA bi-layered hydrogel [...] Read more.
In this study, we present bi-layered hydrogel systems that incorporate different sizes and shapes of gold nanoparticles (nanospheres and nanorods) for potential use in areas such as photoactuators, soft robotics, artificial muscles, drug delivery and tissue engineering. The synthesized nano Au-PNiPAAm/PVA bi-layered hydrogel nanocomposites provide the unique ability to exhibit controlled motion upon light exposure, indicating that the above systems possess the capability of photo–thermal energy conversion. The chosen synthesis approach is a combination of chemical production of gold nanoparticles (AuNPs) followed by gamma radiation formation of crosslinked polymer networks around them, as the final step, which also allows for sterilization in a single technological step. According to the TEM analysis, the gold nanospheres (AuNSs) with mean diameters of around 17 and 30 nm, as well as nanorods (AuNRs) with an aspect ratio of around 4.5, were synthesized and used as nanofillers in the formation of nanocomposites. Their stability within the polymer matrix was confirmed by UV–Vis spectral studies, by the presence of local surface plasmon resonance (LSPR) bands, typical for nanoparticles of various shapes and sizes. Morphological studies (FE-SEM) of hydrogels revealed the formation of a porous structure with PNiPAAm hydrogel as an active layer and PVA hydrogel as a passive layer, as well as a stable interfacial layer with a thickness of around 80 μm. The synthesized bi-layered photoactuators showed a photo–thermal response upon exposure to irradiation of green lasers and lamps that simulate sunlight, resulting in bending motion. This bending response reveals the huge potential of the obtained materials as soft actuators, which are more flexible than rigid systems, making them effective for specific applications where controlled movement and flexibility are essential. Full article
(This article belongs to the Special Issue Polymer Hydrogels: Synthesis, Properties and Applications)
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18 pages, 2992 KiB  
Article
The Influence of Concentration and Type of Salts on the Behaviour of Linear Actuators Based on PVA Hydrogel Activated by AC Power
by Aleksey Maksimkin, Mikhail Zadorozhnyy, Kseniia V. Filippova, Lidiia D. Iudina, Dmitry V. Telyshev and Tarek Dayyoub
Gels 2025, 11(7), 484; https://doi.org/10.3390/gels11070484 - 23 Jun 2025
Viewed by 658
Abstract
The creation of quick-reacting electrically conductive polymers for use as actuators driven by low electrical currents is now seen as an important issue. Enhancing the electrical conductivity of hydrogels through the incorporation of conductive fillers, like salts, can reduce the necessary actuating voltage. [...] Read more.
The creation of quick-reacting electrically conductive polymers for use as actuators driven by low electrical currents is now seen as an important issue. Enhancing the electrical conductivity of hydrogels through the incorporation of conductive fillers, like salts, can reduce the necessary actuating voltage. However, several important questions arise about how the type of salt chosen and its concentration will affect not only the activation efficiency of the actuators but also the structure of the hydrogels utilized. In this study, to enhance the electrical conductivity of the hydrogel and lower the necessary activation voltage of the hydrogel actuators, lithium chloride (LiCl) and sodium chloride (NaCl) were incorporated as conductive fillers into the polyvinyl alcohol (PVA) polymer matrix. To determine the deformation of actuators, as well as the activation and relaxation times and efficiencies during activation, linear actuators capable of being activated through extension/contraction (swelling/shrinking) cycles were developed and examined based on the LiCl/NaCl content, applied voltage, and frequency. The main finding is that the required actuating voltage was lowered by up to 20 V by adding an equal mass of salt in relation to the PVA mass content. With a load of around 20 kPa, it was observed that the extension deformation for PVA/NaCl-based actuators can achieve 75%, while in contraction deformation, can reach 17%. Additionally, for the PVA/LiCl-based actuators, the extension deformation can reach 87%, while during contraction deformation, it can reach 22%. The degree of swelling in the PVA/NaCl hydrogels was generally less than that in the PVA/LiCl hydrogels, which was associated with the finding that the actuators prepared from PVA/NaCl hydrogels delivered an output that was 10–15% lower than those made from PVA/LiCl hydrogels across different testing cycles. Furthermore, adding salt increases the degree of crosslinking, which can explain why increased crosslinking leads to reduced deformation when exposed to AC voltage. These actuators can find extensive use in soft robotics, artificial muscles, medical applications, and aerospace industries. Full article
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19 pages, 997 KiB  
Review
A Review of Bio-Inspired Actuators and Their Potential for Adaptive Vehicle Control
by Vikram Mittal, Michael Lotwin and Rajesh Shah
Actuators 2025, 14(7), 303; https://doi.org/10.3390/act14070303 - 20 Jun 2025
Viewed by 1464
Abstract
Adaptive vehicle control systems are crucial for enhancing safety, performance, and efficiency in modern transportation, particularly as vehicles become increasingly automated and responsive to dynamic environments. This review explores the advancements in bio-inspired actuators and their potential applications in adaptive vehicle control systems. [...] Read more.
Adaptive vehicle control systems are crucial for enhancing safety, performance, and efficiency in modern transportation, particularly as vehicles become increasingly automated and responsive to dynamic environments. This review explores the advancements in bio-inspired actuators and their potential applications in adaptive vehicle control systems. Bio-inspired actuators, which mimic natural mechanisms such as muscle movement and plant tropism, offer unique advantages, including flexibility, adaptability, and energy efficiency. This paper categorizes these actuators based on their mechanisms, focusing on shape memory alloys, dielectric elastomers, ionic polymer–metal composites, polyvinylidene fluoride-based electrostrictive actuators, and soft pneumatic actuators. The review highlights the properties, operating principles, and potential applications for each mechanism in automotive systems. Additionally, it investigates the current uses of these actuators in adaptive suspension, active steering, braking systems, and human–machine interfaces for autonomous vehicles. The review further outlines the advantages of bio-inspired actuators, including their energy efficiency and adaptability to road conditions, while addressing key challenges like material limitations, response times, and integration with existing automotive control systems. Finally, this paper discusses future directions, including the integration of bio-inspired actuators with machine learning and advancements in material science, to enable more efficient and responsive adaptive vehicle control systems. Full article
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15 pages, 2804 KiB  
Article
Enhanced Flexibility and β-Phase Crystallization in PVDF/BaTiO3 Composites via Ionic Liquid Integration for Multifunctional Applications
by Ayda Bouhamed, Ahmed Attaoui, Fatma Mabrouki, Christoph Tegenkamp and Olfa Kanoun
J. Compos. Sci. 2025, 9(6), 302; https://doi.org/10.3390/jcs9060302 - 13 Jun 2025
Viewed by 1048
Abstract
Piezoelectric polymer composites, particularly polyvinylidene fluoride (PVDF) blended with barium titanate (BT), show promise for wearable technologies as both energy harvesters and haptic actuators. However, these composites typically exhibit limited electromechanical coupling and insufficient β-phase formation. This study presents a novel approach using [...] Read more.
Piezoelectric polymer composites, particularly polyvinylidene fluoride (PVDF) blended with barium titanate (BT), show promise for wearable technologies as both energy harvesters and haptic actuators. However, these composites typically exhibit limited electromechanical coupling and insufficient β-phase formation. This study presents a novel approach using ionic liquids (ILs) to enhance PVDF-based piezoelectric composite performance. Through solution-casting methods, we examined the effect of IL concentration on the structural, mechanical, and piezoelectric properties of PVDF/BT composites. Results demonstrate that the use of IL significantly improves β-phase crystallization in PVDF while enhancing electrical properties and mechanical flexibility, which are key requirements for effective energy harvesting and haptic feedback applications. The optimized composites show a 25% increase in β-phase content, enhanced flexibility, and a 100% improvement in piezoelectric voltage output compared to other more conventional PVDF/BT systems. The IL-modified composite exhibits superior piezoelectric response, generating an output voltage of 9 V and an output power of 40.1 µW under mechanical excitation and a displacement of 138 nm when subjected to 13 V peak-to-peak voltage, making it particularly suitable for haptic interfaces. These findings establish a pathway toward high-performance, flexible piezoelectric materials for multifunctional wearable applications in human–machine interfaces. Full article
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27 pages, 1091 KiB  
Review
Advances in Thermoregulating Textiles: Materials, Mechanisms, and Applications
by Kuok Ho Daniel Tang
Textiles 2025, 5(2), 22; https://doi.org/10.3390/textiles5020022 - 11 Jun 2025
Viewed by 1612
Abstract
Advancements in thermoregulating textiles have been propelled by innovations in nanotechnology, composite materials, and smart fiber engineering. This article reviews recent scholarly papers on experimental passive and active thermoregulating textiles to present the latest advancements in these fabrics, their mechanisms of thermoregulation, and [...] Read more.
Advancements in thermoregulating textiles have been propelled by innovations in nanotechnology, composite materials, and smart fiber engineering. This article reviews recent scholarly papers on experimental passive and active thermoregulating textiles to present the latest advancements in these fabrics, their mechanisms of thermoregulation, and their feasibility for use. The review underscores that phase-change materials enhanced with graphene, boron nitride, and carbon nanofibers offer superior thermal conductivity, phase stability, and flexibility, making them ideal for wearable applications. Shape-stabilized phase-change materials and aerogel-infused fibers have shown promising results in outdoor, industrial, and emergency settings due to their durability and high insulation efficiency. Radiative cooling textiles, engineered with hierarchical nanostructures and Janus wettability, demonstrate passive temperature regulation through selective solar reflection and infrared emission, achieving substantial cooling effects without external energy input. Thermo-responsive, shape-memory materials, and moisture-sensitive polymers enable dynamic insulation and actuation. Liquid-cooling garments and thermoelectric hybrids deliver precise temperature control but face challenges in portability and power consumption. While thermoregulating textiles show promise, the main challenges include achieving scalable manufacturing, ensuring material flexibility, and integrating multiple functions without sacrificing comfort. Future research should focus on hybrid systems combining passive and active mechanisms, user-centric wearability studies, and cost-effective fabrication methods. These innovations hold significant potential for applications in extreme environments, athletic wear, military uniforms, and smart clothing, contributing to energy efficiency, health, and comfort in a warming climate. Full article
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23 pages, 2058 KiB  
Review
Alginate Sphere-Based Soft Actuators
by Umme Salma Khanam, Hyeon Teak Jeong, Rahim Mutlu and Shazed Aziz
Gels 2025, 11(6), 432; https://doi.org/10.3390/gels11060432 - 5 Jun 2025
Viewed by 861
Abstract
Alginate hydrogels offer distinct advantages as ionically crosslinked, biocompatible networks that can be shaped into spherical beads with high compositional flexibility. These spherical architectures provide isotropic geometry, modularity and the capacity for encapsulation, making them ideal platforms for scalable, stimuli-responsive actuation. Their ability [...] Read more.
Alginate hydrogels offer distinct advantages as ionically crosslinked, biocompatible networks that can be shaped into spherical beads with high compositional flexibility. These spherical architectures provide isotropic geometry, modularity and the capacity for encapsulation, making them ideal platforms for scalable, stimuli-responsive actuation. Their ability to respond to thermal, magnetic, electrical, optical and chemical stimuli has enabled applications in targeted delivery, artificial muscles, microrobotics and environmental interfaces. This review examines recent advances in alginate sphere-based actuators, focusing on fabrication methods such as droplet microfluidics, coaxial flow and functional surface patterning, and strategies for introducing multi-stimuli responsiveness using smart polymers, nanoparticles and biologically active components. Actuation behaviours are understood and correlated with physical mechanisms including swelling kinetics, photothermal effects and the field-induced torque, supported by analytical and multiphysics models. Their demonstrated functionalities include shape transformation, locomotion and mechano-optical feedback. The review concludes with an outlook on the existing limitations, such as the material stability, cyclic durability and integration complexity, and proposes future directions toward the development of autonomous, multifunctional soft systems. Full article
(This article belongs to the Special Issue Polysaccharide Gels for Biomedical and Environmental Applications)
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20 pages, 2425 KiB  
Review
A Review of Electroactive Polymers in Sensing and Actuator Applications
by Diana Narvaez and Brittany Newell
Actuators 2025, 14(6), 258; https://doi.org/10.3390/act14060258 - 23 May 2025
Viewed by 3818
Abstract
Electroactive polymers (EAPs) represent a versatile class of smart materials capable of converting electrical stimuli into mechanical motion and vice versa, positioning them as key components in the next generation of actuators and sensors. This review summarizes recent developments in both electronic and [...] Read more.
Electroactive polymers (EAPs) represent a versatile class of smart materials capable of converting electrical stimuli into mechanical motion and vice versa, positioning them as key components in the next generation of actuators and sensors. This review summarizes recent developments in both electronic and ionic EAPs, highlighting their activation mechanisms, material architectures, and multifunctional capabilities. Representative systems include dielectric elastomers, ferroelectric and conducting polymers, liquid crystal elastomers, and ionic gels. Advances in fabrication methods, such as additive manufacturing, nanocomposite engineering, and patternable electrode deposition, are discussed with emphasis on miniaturization, stretchability, and integration into soft systems. Applications span biomedical devices, wearable electronics, soft robotics, and environmental monitoring, with growing interest in platforms that combine actuation and sensing within a single structure. Finally, the review addresses critical challenges such as long-term material stability and scalability, and outlines future directions toward self-powered, AI-integrated, and sustainable EAP technologies. Full article
(This article belongs to the Special Issue Electroactive Polymer (EAP) for Actuators and Sensors Applications)
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38 pages, 2989 KiB  
Review
Electroactive Polymers for Self-Powered Actuators and Biosensors: Advancing Biomedical Diagnostics Through Energy Harvesting Mechanisms
by Nargish Parvin, Sang Woo Joo, Jae Hak Jung and Tapas Kumar Mandal
Actuators 2025, 14(6), 257; https://doi.org/10.3390/act14060257 - 23 May 2025
Viewed by 1258
Abstract
Electroactive polymers (EAPs) have emerged as versatile materials for self-powered actuators and biosensors, revolutionizing biomedical diagnostics and healthcare technologies. These materials harness various energy harvesting mechanisms, including piezoelectricity, triboelectricity, and ionic conductivity, to enable real-time, energy-efficient, and autonomous sensing and actuation without external [...] Read more.
Electroactive polymers (EAPs) have emerged as versatile materials for self-powered actuators and biosensors, revolutionizing biomedical diagnostics and healthcare technologies. These materials harness various energy harvesting mechanisms, including piezoelectricity, triboelectricity, and ionic conductivity, to enable real-time, energy-efficient, and autonomous sensing and actuation without external power sources. This review explores recent advancements in EAP-based self-powered systems, focusing on their applications in biosensing, soft robotics, and biomedical actuation. The integration of nanomaterials, flexible electronics, and wireless communication technologies has significantly enhanced their sensitivity, durability, and multifunctionality, making them ideal for next-generation wearable and implantable medical devices. Additionally, this review discusses key challenges, including material stability, biocompatibility, and optimization strategies for enhanced performance. Future perspectives on the clinical translation of EAP-based actuators and biosensors are also highlighted, emphasizing their potential to transform smart healthcare and bioelectronic applications. Full article
(This article belongs to the Special Issue Electroactive Polymer (EAP) for Actuators and Sensors Applications)
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15 pages, 2205 KiB  
Article
Highly Stretchable, Low Hysteresis, and Transparent Ionogels as Conductors for Dielectric Elastomer Actuators
by Limei Zhang, Hong Li, Zhiquan Li, Weimin Pan, Yi Men, Niankun Zhang, Jing Xu and Xuewei Liu
Gels 2025, 11(5), 369; https://doi.org/10.3390/gels11050369 - 17 May 2025
Viewed by 635
Abstract
As conductive materials, ionogels have attracted significant attention for their potential applications in flexible wearable electronics. However, preparing an ionogel with mechanical properties akin to human skin while also achieving transparency, adhesion, and low hysteresis through simple processes remains challenging. Here, we introduce [...] Read more.
As conductive materials, ionogels have attracted significant attention for their potential applications in flexible wearable electronics. However, preparing an ionogel with mechanical properties akin to human skin while also achieving transparency, adhesion, and low hysteresis through simple processes remains challenging. Here, we introduce a multifunctional ionogel synthesized via a one-step photopolymerization method. By leveraging the good compatibility between the ionic liquid and the polymer network, as well as the hydrogen bonding and chemical crosslinking within the gel network, we achieved an ionogel with high transparency (>98%), stretchability (fracture strain of 19), low hysteresis (<5.83%), strong adhesion, robust mechanical stability, excellent electrical properties, a wide operating temperature range, and a tunable modulus (1–103 kPa) that matches human skin. When used as a conductor in soft actuators, the ionogel enabled a large area strain of 36% and a fast electromechanical conversion time of less than 1 s. The actuator demonstrated good actuation performance with voltage and frequency dependence, electrochemical stability, and outstanding durability over millions of cycles. This study provides a simple and effective method to produce multifunctional ionogels with tailored mechanical properties that match those of human skin, paving the way for their application in flexible wearable electronics. Full article
(This article belongs to the Section Gel Analysis and Characterization)
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28 pages, 17687 KiB  
Review
Research Status and Potential Direction for Thermoplastic Shape Memory Polymers and Composites: A Review
by Shuai Yang, Yang He, Zijian Song and Yingchun Li
Polymers 2025, 17(10), 1360; https://doi.org/10.3390/polym17101360 - 15 May 2025
Cited by 1 | Viewed by 745
Abstract
Shape memory polymers (SMPs), due to the programmable deformation and recovery ability, exhibit widespread potential in fields of biomedical devices, smart actuators, and engineering structures. Thermoplastic SMPs, which possess the intrinsic linear molecular chain structures, are able to be processed through diverse methods, [...] Read more.
Shape memory polymers (SMPs), due to the programmable deformation and recovery ability, exhibit widespread potential in fields of biomedical devices, smart actuators, and engineering structures. Thermoplastic SMPs, which possess the intrinsic linear molecular chain structures, are able to be processed through diverse methods, in addition to being re-processed after process-forming, compared with thermoset SMPs. The environmental recycling characteristics for thermoplastic SMPs describe their wide use potential and prospect. In this paper, a comprehensive description of mechanism, matrix polymers, actuations, and applications for thermoplastic SMPs and composites was reviewed. Furthermore, two promising potential developing directions, 4D printing metamaterial and dynamic covalent networks, were proposed. The multifunctionality and enhanced performances of thermoplastic SMPs and composites exhibited excellent application value, which is significant for future advancements. Full article
(This article belongs to the Section Polymer Applications)
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17 pages, 6284 KiB  
Article
Study on the Energy Storage and Driving Performance of IPMC with Laminated Structure Electrodes
by Jintao Zhao, Yanqi Dong, Zhenjie Zhang, Dongyu Yang, Siyan Zhang and Mingchuan Jia
Coatings 2025, 15(5), 577; https://doi.org/10.3390/coatings15050577 - 13 May 2025
Viewed by 465
Abstract
Ionic polymer–metal composites (IPMC) have the advantages of a large driving mass ratio, low driving voltage, and high current sensitivity, but their low electrode continuity, low energy storage, and unclear driving response mechanisms limit further application and development. In this study, Nafion is [...] Read more.
Ionic polymer–metal composites (IPMC) have the advantages of a large driving mass ratio, low driving voltage, and high current sensitivity, but their low electrode continuity, low energy storage, and unclear driving response mechanisms limit further application and development. In this study, Nafion is used as the base film and metallic silver is used as the electrode material to modify IPMC electrodes. The physical and electrochemical properties of silver-based IPMC with three electrode preparation processes are tested, and the effects of different electrode preparation processes and structures on the energy storage performance and driving performance of IPMC are analyzed. The results show that the electrode coating effect of the Hot Press Chemical Plating method (HPCP) is good and maintains better continuity, and the formed layer electrode can improve the energy storage performance of IPMC, and the enhancement of energy storage performance can improve the driving performance of IPMC. This study enhances the energy storage performance and driving performance of IPMC from the perspective of electrode process and structure and provides a basis for the study of the enhancement of energy storage performance of IPMC by the HPCP electrode preparation process. Full article
(This article belongs to the Special Issue Cutting Performance of Coated Tools)
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13 pages, 2237 KiB  
Article
Biomimetic Soft Actuator with Deformation and Motion Driven by Near-Infrared Light
by Mei Li and Yubai Ma
Polymers 2025, 17(10), 1315; https://doi.org/10.3390/polym17101315 - 12 May 2025
Viewed by 438
Abstract
Restricted by the inherent low sensitivity of materials and complex integration technology, it is difficult for existing soft actuators (s-actuators) to simultaneously possess the advantages of flexibility, fast response, and simple manufacturing, which greatly limits their practical applications. Herein, a stretchable (ε = [...] Read more.
Restricted by the inherent low sensitivity of materials and complex integration technology, it is difficult for existing soft actuators (s-actuators) to simultaneously possess the advantages of flexibility, fast response, and simple manufacturing, which greatly limits their practical applications. Herein, a stretchable (ε = 200%) nanocomposite film capable of deformation and motion driven by near infrared light (NIR) was developed using multi-walled carbon nanotubes (MWCNTs) as the light absorption–photothermal conversion nanonetwork, and liquid crystal polymer (LCP) as an elastic matrix featured reversible phase transition. Furthermore, s-actuators with various deformation and motion modes have been realized employing MWCNT/LCP nanocomposite film. Based on the mechanism that photothermal-effect-regulated liquid crystal–isotropic phase transition in LCP can induce macroscopic deformation of nanocomposites, MWCNT/LCP s-actuators have completed a series of complex deformation and motion tasks such as opening the knot, “V”-shape reversible deformation (30 s per cycle), the “spring” rotating and unfolding, imitating a “caterpillar” walking in a straight line (the average speed is 13 s/mm), etc. This work provides an effective strategy for the intelligent development of s-actuators. Full article
(This article belongs to the Section Polymer Composites and Nanocomposites)
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