Search Results (61)

High-purity germanium (HPGe) gamma-ray detectors are core instruments in nuclear physics and astrophysics experiments, where long-term stability and reliable extraction of decay parameters are essential. However, the standard exponential decay analyses of the detector time-series data are often affected by the strong correlations between the fitted parameters and the sensitivity to detector-related fluctuations and outliers. In this study, we present a robust analysis framework for HPGe detector decay data based on pairwise ratios and the Steiner’s most frequent value (MFV) statistic. By forming point-to-point ratios of background-subtracted net counts, the dependence on the absolute detector response is eliminated, removing the amplitude–lifetime correlation that is inherent to conventional regression. The resulting pairwise lifetime estimates exhibit heavy-tailed behavior, which is efficiently summarized using the MFV, a robust estimator designed for such distributions. For the case study, a long and stable dataset from an HPGe detector was used. This data was gathered during a low-temperature nuclear physics experiment focused on observing the 216 keV gamma-ray line in ⁹⁷Ru. Using measurements spanning approximately 10 half-lives, we obtain a mean lifetime of $\tau =4.0959\pm 0.{0007}_{\mathrm{stat}}\pm 0.{0110}_{\mathrm{syst}}\mathrm{d}$, corresponding to a half-life of $T_{1/2}=2.8391\pm 0.{0005}_{\mathrm{stat}}\pm 0.{0076}_{\mathrm{syst}}\mathrm{d}$. These results demonstrate that the pairwise–MFV approach provides a robust and reproducible tool for analyzing long-duration HPGe detector data in nuclear physics and nuclear astrophysics experiments, particularly for precision decay measurements, detector-stability studies, and low-background monitoring. Full article

In recent years, polymer-based hybrid nanocomposites have emerged as promising alternatives to traditional heavy metal shields due to their low density, flexibility, and environmental safety. In this study, the synthesis of PS-PEG copolymers and the gamma radiation-shielding properties of PS-PEG/As₂O₃, PS-PEG/BN, and PS-PEG/As₂O₃/BN nanocomposites with different compositions are investigated. The goal is to find the optimal nanocomposite composition for gamma radiation shielding and dosimetry. Therefore, the mass attenuation coefficient (MAC), linear attenuation coefficient (LAC), half-value layer (HVL), tenth-value layer (TVL), effective atomic number, mean free path (MFP), radiation shielding efficiency (RPE), electron density, and specific gamma-ray constant were presented. Gamma rays emitted by the Eu source were detected by a high-purity germanium (HPGe) detector device. GammaVision was used to analyze the given data. Photon energy was in the vicinity of 121.8–1408.0 keV. The MAC values in XCOM simulation tools were used to compute. Gamma-shielding efficiency was increased by an increased number of NPs at a smaller photon energy. At 121.8 keV, the HVL of a composite with 70 wt% As₂O₃ NPs is 2.00 cm, which is comparable to the HVL of lead (0.56 cm) at the same energy level. Due to the increasing need for lightweight, flexible, and lead-free shielding materials, PS-b-PEG copolymer-based nanocomposites reinforced with arsenic oxide and BN NPs will be materials of significant interest for next-generation radiation protection applications. Full article

Multinuclide calibration sources, consisting of mixtures of gamma-emitting radionuclides, are commonly used for detector efficiency calibration in gamma-ray spectrometry. While they enable fast and accurate calibration, they have certain drawbacks, such as high cost and relatively short usable lifespans. This paper presents a simplified and cost-effective method for the efficiency calibration of cylindrical high-purity germanium (HPGe) detectors, which relies on the use of certified reference materials containing natural radionuclides. The method is based on selected gamma lines from natural radionuclides that are practically unaffected by the true coincidence summing (TCS) effect, enabling reasonably accurate calibration for multiple measurement geometries at energies above 200 keV. The main limitation of the method is its applicability only to energies higher than 200 keV; however, this range is sufficient for most routine environmental measurements. Verification measurements conducted for cylindrical geometry showed that detector efficiency values obtained using the proposed method (with IAEA RGK, RGU, and RGTh certified reference materials) differed by less than approximately 4% from those obtained using a commercial multinuclide calibration source. Full article

This paper reports the levels of radon (Rn), thoron (Tn), and their progeny (TnP) concentrations in dwellings; studies factors influencing these concentrations; and assesses the associated lung cancer risk in Akonolinga’s area in Cameroon, where rutile deposits have been identified but are not yet industrially exploited. Indoor Rn and Tn were determined using CR39-based detectors. Additionally, Rn in soil gas, ²²⁶Ra, and ²³²Th concentrations in soil were measured using Markus 10, high purity germanium detector (HPGe), respectively. On average, indoor Rn, Tn concentration, and the equilibrium equivalent Thoron concentration (EETC) or TnP were 39.5, 68.1, and 5.0 Bq m⁻³, respectively. Average concentrations of Rn in soil gas, ²²⁶Ra, and ²³²Th in soil were 24.3 kBq m⁻³, 17 Bq kg⁻¹, and 27 Bq kg⁻¹, respectively. Correlation analysis indicates that indoor radon and thoron levels were tightly linked with factors such as their precursor concentrations in soil, the building materials, dwelling architecture, and inhabitant living habits. Furthermore, it was observed that Rn and TnP were the major contributors to the inhalation effective dose, accounting for 39.6% and 56.7% of the total, respectively. The estimated excess lifetime cancer risk (ELCR) from the exposition to Rn and TnP was found to be 2.93 × 10⁻³ and 4.36 × 10⁻³, respectively, exceeding the global average, raising health concerns. Full article

Laboratory magnetoplasmas can become an intriguing experimental environment for fundamental studies relevant to nuclear astrophysics processes. Theoretical predictions indicate that the ionization state of isotopes within the plasma can significantly alter their lifetimes, potentially due to nuclear and atomic mechanisms such as bound-state β-decay. However, only limited experimental evidence on this phenomenon has been collected. PANDORA (Plasmas for Astrophysics, Nuclear Decay Observations, and Radiation for Archaeometry) is a novel facility which proposes to investigate nuclear decays in high-energy-density plasmas mimicking some properties of stellar nucleosynthesis sites (Big Bang Nucleosynthesis, s-process nucleosynthesis, role of CosmoChronometers, etc.). This paper focuses on the case of ⁷Be electron capture (EC) decay into ⁷Li, since its in-plasma decay rate has garnered considerable attention, particularly concerning the unresolved Cosmological Lithium Problem and solar neutrino physics. Numerical simulations were conducted to assess the feasibility of this possible lifetime measurement in the plasma of PANDORA. Both the ionization and atomic excitation of the ⁷Be isotopes in a He buffer Electron Cyclotron Resonance (ECR) plasma within PANDORA were explored via numerical modelling in a kind of “virtual experiment” providing the expected in-plasma EC decay rate. Since the decay of ⁷Be provides γ-rays at 477.6 keV from the ⁷Li excited state, Monte-Carlo GEANT4 simulations were performed to determine the γ-detection efficiency by the HPGe detectors array of the PANDORA setup. Finally, the sensitivity of the measurement was evaluated through a virtual experimental run, starting from the simulated plasma-dependent γ-rate maps. These results indicate that laboratory ECR plasmas in compact traps provide suitable environments for β-decay studies of ⁷Be, with the estimated duration of experimental runs required to reach 3σ significance level being few hours, which prospectively makes PANDORA a powerful tool to investigate the decay rate under different thermodynamic conditions and related charge state distributions. Full article

Gamma-ray analysis is a widely used technique for radioactive element characterization in environmental samples, contributing significantly to natural and anthropogenic radioactivity evaluations, particularly in areas such as natural reservations or regions that have been affected by nuclear pollutants. As the Danube Delta belongs to both categories, we decided to conduct a study in order to find out whether gamma spectroscopy is suited for pattern identification in common biota constituents such as reed and whether anthropogenic tracers can still be found in the samples. The answer to both questions is affirmative, as shown by the pattern and cluster analyses. Furthermore, our conclusions point out that it would be interesting to extend the spectroscopy and correlation studies to sediment and trophic chains over a certain period in order to obtain the transfer factors and information on radionuclide dynamics. The HPGe detector used proves this is the best class of sensing devices for such purposes. Full article

Mushrooms are a significant component of human diets but can bioaccumulate hazardous substances, including both anthropogenic (¹³⁷Cs) and naturally occurring (²³⁸U, ²³²Th, and ⁴⁰K) radionuclides. This study quantified these radionuclides in 24 commonly consumed mushroom species collected in Amasya and Tekirdağ, provinces of Türkiye. Using a high-purity germanium (HPGe) detector, we found ¹³⁷Cs activity in the Tekirdağ samples ranging from 3.9 to 127.8 Bq/kg, while the ¹³⁷Cs activity in the Amasya samples ranged from 3.1 to 63.7 Bq/kg. In particular, Tricholoma terreum (Tekirdağ) and Tricholoma imbricatum (Amasya) exhibited notably higher ¹³⁷Cs concentrations. The concentration of ²³⁸U varied between 4.8 and 17.5 Bq/kg in the Tekirdağ samples and 6.5 and 16 Bq/kg in the Amasya samples, whereas the ²³²Th and ⁴⁰K values fluctuated across species and regions, with ⁴⁰K sometimes exceeding 1900 Bq/kg. These results highlight that mushrooms can serve as effective bioindicators for residual radioactive contamination and underline the need for periodic monitoring to assess potential public health risks associated with wild mushroom consumption. These findings also offer a valuable dataset for understanding post-Chernobyl fallout dynamics in the forest ecosystems of Türkiye. Full article

High-purity germanium (HPGe) detectors occupy a prominent position in fields such as radiation detection and aerospace because of their excellent energy resolution and wide detection range. To achieve a broader detection range, conventional HPGe detectors often need to be expanded to cubic-centimeter-scale volumes. However, this increase in volume leads to a large detector area, which in turn increases the detector capacitance, affecting the detector’s noise level and performance. To address this issue, this study proposes a novel high-purity germanium drift detector (HPGeDD). The design features a small-area central collecting cathode surrounded by concentric anode rings, with a resistive chain interposed between the anode rings to achieve self-dividing voltage. This design ensures that the detector’s capacitance is only related to the area of the central collecting cathode, independent of the overall active area, thus achieving a balance between a small capacitance and large active area. Electrical performance simulations of the novel detector were conducted using the semiconductor simulation software Sentaurus TCAD (P-2019.03). The results show a smooth electric potential distribution within the detector, forming a lateral electric field, as well as a lateral hole drift channel precisely directed toward the collecting cathode. Furthermore, simulations of heavy ion incidence were performed to investigate the detector’s carrier collection characteristics. The simulation results demonstrate that the HPGeDD exhibits advantages such as fast signal response and short collection time. The design proposal presented in this study offers a new solution to the problem of excessive capacitance in conventional HPGe detectors, expands their application scope, and provides theoretical guidance for subsequent improvements, optimizations, and practical manufacturing. Full article

Naturally occurring radionuclides are ubiquitous at various levels of concentration, while exposure to ionizing radiation by humans is of global concern. Radiological health risk assessment due to the consumption of natural spring mineral water is critical for ensuring public health and safety. This study aims at investigating the radioactivity concentration levels of natural radionuclides ²²⁶Ra, ²³²Th and ⁴⁰K and the associated radiological health risk in commercial natural spring bottled water in South Africa. A total of 21 of the most-consumed bottled drinking water brands from grocery stores, were analysed using the HPGe gamma detector. The results indicate that the range of radioactivity concentrations is from 1.060 ± 0.067 to 2.571 ± 0.143 BqL⁻¹, with a mean of 1.766 ± 0.399 BqL⁻¹ for ²²⁶Ra; 1.736 ± 0.112 to 7.807 ± 0.099 BqL⁻¹, with a mean of 3.688 ± 1.371 BqL⁻¹ for ²³²Th and 149.000 ± 38.480 to 242.900 ± 59.700 BqL⁻¹ with a mean of 220.229 ± 22.297 BqL⁻¹ for ⁴⁰K. The potential radiological health risks evaluated show mean values for Ra_eq, D_Ab, AEID and AGED as 23.976 ± 0.446 BqL⁻¹, 12.232 ± 1.445 nGyh⁻¹, 0.060 ± 0.007 mSvy⁻¹ and 0.090 ± 0.027 mSvy⁻¹, respectively. The radiation dose based on age group is in the order of infants (≤1 year) > teenagers (12–17 years) > children (1–12 years) > adults (>17 years). The activity concentrations of radionuclides in bottled water are ranked in the order of ⁴⁰K > ²³²Th > ²²⁶Ra, with ²³²Th contributing the highest radiation dose, consistent with findings reported in previous studies. The findings reveal that the activity concentration levels and estimated radiological health risks are within the permissible limits set by UNSCEAR guidelines. Therefore, the consumption of bottled water is radiologically safe. However, the findings also suggest that 12 out of 1000 individuals may suffer cancer fatality, while 6 out of 1 million individuals may experience hereditary effects over their lifetime from the consumption of bottled water. Regular monitoring and stringent regulatory controls are recommended to ensure the radiological safety of bottled drinking water in South Africa. Full article

The concentration of natural radionuclides ²²⁶Ra, ²³²Th and ⁴⁰K in ceramic tiles manufactured in Poland is presented in this paper. The concentration of natural radioactive isotopes in the tested samples was determined using a low-level digital gamma ray spectrometer equipped with an HPGe semiconductor detector. The mean concentrations of ²²⁶Ra, ²³²Th and ⁴⁰K in the analyzed samples were found to be 48 ± 3 Bq∙kg⁻¹, 49 ± 3 Bq∙kg⁻¹ and 476 ± 23 Bq∙kg⁻¹, respectively. The world mean concentrations of these radionuclides (50 Bq·kg⁻¹, 50 Bq·kg⁻¹ and 500 Bq·kg⁻¹, respectively) were not exceeded. Furthermore, in order to ascertain the level of gamma radiation exposure, fundamental radiation protection parameters were established: radioactivity concentration indicator/gamma ray indicator (I_γ), indoor dose rate (D_in) and annual indoor effective dose (E_in). In the case of the investigated ceramic tiles, it was established that the parameters were not higher than the limit values, except the indoor gamma radiation dose rate which was found to be 1.5 times higher than the world average. Therefore, the findings of this study indicate that the utilization of the examined ceramic tiles in constructions should be approached with a degree of caution. Full article

Ionizing radiation plays an essential role across various fields but also poses significant health risks, requiring effective shielding solutions. This study focuses on the photon shielding properties of PbO-reinforced composites, specifically PbO-0, PbO-2, PbO-4, PbO-6, PbO-8, and PbO-10, through experimental measurements of photon energies ranging from 59.5 keV to 1408.0 keV. The measurements were taken using an HPGe detector. Experimental results were compared to theoretical calculations. Among the tested composites, PbO-10, which contains the highest concentration of lead oxide (PbO), provided the most effective radiation shielding. This sample demonstrated superior mass and linear attenuation coefficients, offering excellent protection at low photon energies. Furthermore, PbO-10 exhibited the lowest half-value layer (HVL) and tenth-value layer (TVL) values, indicating its efficiency in reducing radiation intensity with thinner material layers. It was determined that the experimental TVL results for PbO-O, PbO-2, PbO-4, PbO-6, PbO-8, and PbO-10 at 59.5 keV photon energy were 9.95, 5.98, 4.77, 3.67, 3.22, and 2.71 cm, respectively. With these outstanding attenuation capabilities, PbO-10 is deemed highly suitable for use in medical, industrial, and radiation-heavy environments. In summary, this research emphasizes the effectiveness of PbO-reinforced composites in gamma-ray shielding, with PbO-10 emerging as the top performer, demonstrating great potential for applications that require durable and efficient radiation protection. Full article

Modeling the response of gamma detectors has long been a challenge within the nuclear community. Significant research has been conducted to digitally replicate instruments that can cost over USD 100,000 and are difficult to operate outside of a laboratory setting. The large cost and availability prevent some from making use of such equipment. Subsequently, there have been multiple attempts to create cost-effective codes that replicate the response of sodium-iodide and high-purity germanium detectors for data derivation related to gamma-ray interaction with matter. While robust programs do exist, they are often subject to export controls and/or they are not intuitive to use. Through the use of hybrid Monte Carlo methods, MATLAB can be used to produce a fast first-order response of various gamma-ray detectors. The combination of a graphical user interface with a numerical-based script allows for open-source and intuitive code. When benchmarked with experimental data from Co-60, Cs-137, and Na-22, the code can numerically calculate a response comparable to experimental and industry-standard response codes. Evidence supports both savings in computational requirements and the inclusion of an intuitive user experience that does not heavily compromise data when compared to other standard codes, such as MCNP and GADRAS, or experimental results. When the application is installed on a Dell Intel i7 computer with 16 cores, the average time to simulate the benchmarked isotopes is 0.26 s. Installation on an HP Intel i7 four-core machine runs the same isotopes in 1.63 s. The results indicate that simple gamma detectors can be modeled in an open-source format. The anticipation for the MATLAB application is to be a tool that can be easily accessible and provide datasets for use in an academic setting requiring gamma-ray detectors. Ultimately, this article provides evidence that hybrid Monte Carlo codes in an open-source format can benefit the nuclear community in both computational time and up-front cost for access. Full article

In this work, we studied the effect of bismuth oxide particle size and its attenuation capacity as a filler additive in epoxy resins. Six samples were prepared according to the amount of microparticles and nanoparticles in the sample and were coded as ERB-1, ERB-2, ERB-3, ERB-4, ERB-5, and ERB-6. One of the composite epoxies contained Bi₂O₃ microparticles at a 50:50 ratio (ERB-6) and was chosen as the control composite, and the number of microparticles (MPs) was gradually decreased and replaced by nanoparticles (NPs) to produce epoxy-containing Bi₂O₃ nanoparticles at a 50:50 ratio (ERB-1). The morphological and thermal characteristics of the studied composites were tested. The attenuation capability of the prepared composites, which is determined by the Bi₂O₃ particle size, was determined experimentally using a semiconductor detector, an HPGe-detector, and three different gamma-ray point sources (Am-241, Co-60, and Cs-137). The linear attenuation coefficient (LAC) of ERB-3, which contained 30% nanoparticles and 20% microparticles, had the highest value compared to the other composites at all the energies discussed, while the ERB-6 composite had the lowest value at all energies. The radiation-shielding efficiency (RSE) of the prepared samples was determined at all discussed energies; at 662 keV, the radiation-shielding efficiency values were 15.97%, 13.94%, and 12.55% for ERB-3, ERB-1, and ERB-6, respectively. The statistics also proved that the attenuation capacities of the samples containing a combination of nanoparticles and microparticles were much superior to those of the samples containing only microparticles or nanoparticles. A ranking of the samples based on their attenuation capacity is as follows: ERB-3 > ERB-4 > ERB-2 > ERB-1 > ERB-5 > ERB-6. Full article

PANDORA (Plasmas for Astrophysics Nuclear Decays Observation and Radiation for Archaeometry) is an INFN project aiming at measuring, for the first time, possible variations in in-plasma $\beta$-decay lifetimes in isotopes of astrophysical interest as a function of thermodynamical conditions of the in-laboratory controlled plasma environment. Theoretical predictions indicate that the ionization state can dramatically modify the $\beta$-decay lifetime (even of several orders of magnitude). The PANDORA experimental approach consists of confining a plasma able to mimic specific stellar-like conditions and measuring the nuclear decay lifetime as a function of plasma parameters. The $\beta$-decay events will be measured by detecting the $\gamma$-ray emitted by the daughter nuclei, using an array of 12 HPGe detectors placed around the magnetic trap. In this frame, plasma parameters have to be continuously monitored online. For this purpose, an innovative, non-invasive multi-diagnostic system, including high-resolution time- and space-resolved X-ray analysis, was developed, which will work synergically with the $\gamma$-rays detection system. In this contribution, we will describe this multi-diagnostics system with a focus on spatially resolved high-resolution X-ray spectroscopy. The latter is performed by a pin-hole X-ray camera setup operating in the 0.5–20 keV energy domain. The achieved spatial and energy resolutions are 450 µm and 230 eV at 8.1 keV, respectively. An analysis algorithm was specifically developed to obtain SPhC (Single Photon-Counted) images and local plasma emission spectrum in High-Dynamic-Range (HDR) mode. Thus, investigations of image regions where the emissivity can change by even orders of magnitude are now possible. Post-processing analysis is also able to remove readout noise, which is often observable and dominant at very low exposure times (ms). Several measurements have already been used in compact magnetic plasma traps, e.g., the ATOMKI ECRIS in Debrecen and the Flexible Plasma Trap at LNS. The main outcomes will be shortly presented. The collected data allowed for a quantitative and absolute evaluation of local emissivity, the elemental analysis, and the local evaluation of plasma density and temperature. This paper also discusses the new plasma emission models, implemented on PIC-ParticleInCell codes, which were developed to obtain powerful 3D maps of the X-rays emitted by the magnetically confined plasma. These data also support the evaluation procedure of spatially resolved plasma parameters from the experimental spectra as well as, in the near future, the development of appropriate algorithms for the tomographic reconstruction of plasma parameters in the X-ray domain. The described setups also include the most recent upgrade, consisting of the use of fast X-ray shutters with special triggering systems that will be routinely implemented to perform both space- and time-resolved spectroscopy during transient, stable, and turbulent plasma regimes (in the ms timescale). Full article

This paper focuses on the research and development of high-purity germanium (HPGe) crystals for detector fabrication, specifically targeting applications in rare-event physics searches. The primary objective was to produce large-scale germanium crystals weighing >1 kg with a controlled diameter of ∼10 cm and an impurity range of approximately ${10}^{10}$/cm${ }^3$. Ensuring structural integrity and excellent crystalline quality requires a thorough assessment of dislocation density, a critical aspect of the crystal development process. Dislocation density measurements play a crucial role in maximizing the sensitivity of HPGe detectors, and our findings confirmed that the dislocation density fell within acceptable ranges for detector fabrication. Additionally, this paper examines the segregation coefficient of various contaminants during the crystal development process. Comprehensive analysis of impurity segregation is essential for reducing contaminant quantities in the crystal lattice and customizing purification processes. This, in turn, minimizes undesired background noise, enhancing signal-to-noise ratios for rare-event physics searches and overall detector performance. The investigation included the segregation coefficients of three major acceptors and one donor in crystals grown at the University of South Dakota, providing valuable insights for optimizing crystal purity and detector efficiency. Full article