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15 December 2025

Methodological Applicability of Ultra-Low Background Liquid Scintillation Counters in Low-Level Tritium Measurement

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1
School of Nuclear Science and Technology, University of South China, Hengyang 421001, China
2
Hunan Provincial Key Laboratory of Radon, Hengyang 421001, China
3
China State Key Laboratory of Advanced Environmental Technology, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510632, China
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Author to whom correspondence should be addressed.
This article belongs to the Special Issue Advances in Environmental Radioactivity Monitoring and Measurement

Abstract

Tritium (3H) is a low-energy β emitter commonly found in environmental water samples, and its routine monitoring requires highly sensitive techniques capable of achieving low detection limits. Liquid scintillation counting (LSC) is the standard method for low-level 3H analysis; however, quenching significantly affects detection efficiency and minimum detectable activity (MDA), and systematic evaluations across different quench levels and measurement approaches remain limited. This study evaluates quench-related uncertainties in low-level 3H measurement using two ultra-low background liquid scintillation counters, Quantulus 1220 and GCT 6220. High- and low-quench conditions were created by varying sample-to-cocktail ratios, and performance was assessed through detection efficiency, minimum detectable activity (MDA), and stability. Under the relative measurement method with limited quench variation, GCT 6220 achieved higher efficiency, lower background, and lower detection limits. Under the internal standard method with broader quench spans, Quantulus 1220 produced smoother efficiency–quench curves and more stable results. Thus, GCT 6220 is advantageous for sensitivity-demanding scenarios, while Quantulus 1220 is better suited for quench-correction applications.

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