Search Results (467)

The rapid advancement of flexible electronics technology has endowed flexible sensors with significant application potential in fields such as wearable sensors, bionic skin, and human–machine interaction, owing to their excellent conformability, stretchability, and comfort. However, as application scenarios continue to expand and deepen, higher requirements are imposed on sensor performance in terms of sensitivity, stability, biocompatibility, environmental friendliness, and multifunctional integration. Polyurethane composites, leveraging their intrinsic characteristics, including tunable molecular structure, superior flexibility, and good biocompatibility, can effectively impart properties such as electrical conductivity, self-healing capability, and high sensitivity through compositing with various functional materials, thereby precisely aligning with the diverse demands of next-generation flexible sensors. This article systematically reviews the synthesis strategies of polyurethane composites; provides a detailed analysis of the roles of fillers—including carbon-based materials, polymers, and metal nanoparticles/nanowires—in enhancing the mechanical, electrical, and functional properties of the composites; and further summarizes the research progress of polyurethane composite-based flexible sensors in cutting-edge areas such as eco-friendly sensing, human motion monitoring, health monitoring, and bionic electronic skin. Future development trends are also discussed, aiming to provide insights for the design and development of high-performance flexible sensors. Full article

Gel-based flexible electronic sensors have emerged as a transformative class of materials for next-generation applications. These applications are wearable electronics, soft robotics, electronic skin (e-skin), and healthcare monitoring systems. Owing to their intrinsic softness, stretchability, and biocompatibility, gels provide an ideal platform for constructing highly deformable and skin-conformable sensing devices. This paper provides insight into emerging fabrication techniques, including 3D printing, bioprinting, and microfabrication. These techniques have facilitated the creation of complex architectures with improved sensitivity and scalability. The review also focuses on recent advancements that have focused on overcoming traditional limitations. These limitations are poor mechanical strength, dehydration, limited environmental stability, and low sensitivity. In particular, the incorporation of conductive fillers and ionic species has enabled a range of sensing mechanisms. These mechanisms include piezoresistive, capacitive, piezoelectric, and ionotronic responses. Therefore, it allows for the accurate detection of strain, pressure, temperature, and biochemical signals. Finally, this review provides a summary of future research, which is expected to focus on multifunctional integration, sustainable materials, and intelligent data processing. It provides pathways to the widespread adoption of gel-based flexible electronic sensors in both consumer and clinical applications. Full article

With the rapid advancement of artificial intelligence and wearable technologies, the demand for soft, multifunctional electronic materials has grown substantially. Hydrogels have emerged as a promising platform due to their intrinsic softness, stretchability, and biocompatibility. Among them, cellulose-based conductive hydrogels uniquely integrate the sustainability of natural polymers with tunable electrical functionality, offering significant potential for flexible and biointegrated electronics. This review provides a comprehensive and critical perspective on the recent progress in cellulose-based conductive hydrogels. We systematically summarize key design strategies, including physical and chemical crosslinking and interpenetrating network engineering. More importantly, we present a comparative analysis of distinct conductive mechanisms, including ionic conduction, conductive polymers, metallic nanostructures, and carbon-based fillers, highlighting the inherent trade-offs among electrical conductivity, mechanical robustness, and environmental stability. Emerging applications in flexible electronics, energy storage, bioelectronics, and self-powered systems are discussed through structure–property relationships. Finally, we outline current challenges and future directions, emphasizing multifunctional integration, scalable fabrication, and long-term operational stability, thereby providing a framework for the rational design of next-generation sustainable electronic materials. Full article

Conductive hydrogels are attractive for flexible electronics, but their practical use is often limited by resistance drift during repeated deformation and performance degradation at low temperatures. Here, core–shell polyaniline-coated polyacrylonitrile (PANi@PAN) electrospun nanofibers were incorporated into a polyacrylamide/hydroxypropyl cellulose (PAM/HPC) hydrogel matrix to construct a hybrid conductive network. The PANi shell serves as an electronic pathway alongside ionic conduction in the hydrated polymer network, leading to markedly improved electromechanical stability. The resistance drift is about 11% after 2000 stretching–relaxation cycles at 0–100% strain, about 12 times lower than that of the nanofiber-free hydrogel. Stable electrical responses are maintained under large deformation, with a resistance drift as low as 3.3% over a strain range of 0–400%. The hydrogels show a conductivity of 0.32 S m⁻¹ while retaining high stretchability (>600%). An ethylene glycol/water binary solvent is used to suppress ice formation and improve moisture retention, allowing stable electromechanical performance at −15 °C over 500 cycles. The hydrogel also adheres reliably to human skin (about 10.25 kPa) and functions as a conformal strain sensor without extra fixation. Full article

Respiratory rate (RR) is a critical indicator of physiological status, yet unobtrusive and continuous RR monitoring remains challenging, particularly in wearable applications that require soft, lightweight, and low-power sensing systems. This paper presents an integrated approach that combines a textile-embedded embroidered strain-gauge sensor with Tiny Machine Learning (TinyML) to enable real-time, on-device RR estimation. The sensing platform consists of a textile-integrated meander-pattern strain gauge and a fabric-mounted analog readout circuit, which together capture thoracic expansion during breathing. Two lightweight neural network models—a convolutional neural network (CNN) operating on raw respiratory waveforms and a dense neural network (DNN) operating on wavelet features—were developed and trained using a public strain-sensor dataset and a custom dataset collected with the textile system (TexHype dataset). Both models were optimized through 8-bit quantization and deployed to an STM32L4 microcontroller, where end-to-end on-device preprocessing, filtering, segmentation, normalization, and inference were performed. The CNN achieved the highest accuracy, with a mean absolute error (MAE) of 1.23 breaths per minute (BPM) on the TexHype dataset, but exhibited substantial inference latency (5.8–6.2 s) due to its computational complexity. In contrast, the wavelet-based DNN demonstrated lower accuracy (MAE 2.21 BPM) but achieved real-time performance with inference times of 18–96 ms, and a power overhead ($\Delta P=P_{\mathrm{active}}-P_{\mathrm{idle}}$) of approximately 3.3 mW during inference. Cross-dataset testing revealed limited generalization between different strain-sensor platforms. The findings highlight key trade-offs between accuracy, latency, and energy efficiency, and illustrate the potential of combining stretchable electronics with embedded intelligence to enable next-generation wearable respiratory monitoring systems. Full article

Printed electronics have emerged as a versatile manufacturing platform for next-generation biosensors, enabling on-demand and low-cost fabrication of functional devices on flexible, stretchable, and unconventional substrates. One major challenge in this field lies in the sintering of printed features, as conventional high-temperature processing is incompatible with polymeric substrates and thermally sensitive biological components. Low-temperature sintering inks, typically processed below 200 °C or even at room temperature, have become a critical enabling technology for bio-integrated electronics. This review provides an overview of the current state-of-the-art and key challenges associated with low-temperature sintering inks for printed bioelectronics. We discuss inks based on metal nanoparticles, metal–organic decomposition precursors, metal oxides, chalcogenides, and hybrid material systems. The emphasis is on how ink chemistry, ligand selection, and precursor structure govern rheology, stability, and sintering behavior. In addition, key low-temperature sintering and curing strategies, including thermal, photonic, laser, plasma, microwave, and chemical sintering, are compared in terms of energy delivery, densification mechanisms, and substrate compatibility. Finally, we outline emerging directions towards low temperature and room-temperature sintering inks, and sustainable biobased ink formulations, and discuss their applications for wearable, implantable, and soft biosensing platforms. Full article

Elastomer-based nanocomposites combining polymer flexibility with conductive nanofillers provide lightweight, stretchable systems with tunable electromechanical properties for wearable electronics, soft robotics, and self-powered sensors. However, predicting their nonlinear response remains challenging because the observed piezoelectric-like response arises from strain-dependent interfacial polarization and evolving piezoresistive conduction pathways within heterogeneous microstructures. We introduce a continuum electro-hyperelastic framework combining the Mooney–Rivlin model for large-strain elasticity with a Helmholtz free-energy approach for electrostatic coupling. Analytical expressions for stress, electric displacement, and apparent piezoelectric coefficients are derived and implemented in finite element simulations. The model accurately reproduces the experimental mechanical, dielectric, and electromechanical behaviour of polydimethylsiloxane (PDMS) nanocomposites with 0.1–1 wt% graphene. These show increased stiffness, relative permittivity (from 3.4 to 4.0, ≈18%), and quasi-static d₃₃ coefficients (from −5.6 to −10.0 pC N⁻¹, ≈80% enhancement). Analytical and finite element method (FEM) results show consistent trends across the full deformation range, with Maxwell stress agreement within 10% at lower deformation levels, while deviations of 33–40% for coupled electromechanical quantities at an axial displacement u_z = ~−1 mm (~16.7% compressive strain) are attributable to three-dimensional shear effects absent from the uniaxial analytical assumption. Simulations reveal that graphene boosts Maxwell stress, yielding a four-fold increase at lower stretch ratios. This reframes PDMS–graphene composites as electro-hyperelastic materials, offering a predictive, extensible framework. It highlights apparent piezoelectricity as an emergent, tunable effect from charge redistribution in a compliant hyperelastic matrix—guiding the design of next-generation flexible devices leveraging field-induced coupling over intrinsic polarization. Full article

Flexible skin electronics are increasingly sought after for their potential in sensing and drug delivery within wearable human–machine interfaces. However, developing multifunctional applications that maintain biocompatibility and stable electrical performance under various mechanical deformations remains a challenge. Here, we introduce tattoo paper-based graphene–gold conductors that are approximately 0.04 mm thick and feature a dual conductive pathway within the graphene–gold film. By integrating a folding structure with this dual conductive pathway, we can mitigate the strain effects on the electrical resistance of film-based conductors, resulting in wider areas of stable resistance. In addition, we have designed film conductors with a kirigami structure, which achieves a high initial conductivity of 1.5 × 10³ S cm⁻¹ and exhibits negligible resistance changes across a broad strain range of 0 to 130%. We utilize these conductors to develop waterproof on-skin patches that incorporate electrically and optically active heaters for body heating and drug delivery. Furthermore, we have created an on-skin dialing interface using these conductors, which enables users to make telephone calls based on triboelectric nanogenerators. Full article

With the rapid development of artificial intelligence and wearable electronics, there is an increasing demand for skin-like, flexible, and self-powered sensors capable of continuously perceiving mechanical stimuli and human motions. Triboelectric nanogenerator (TENG)-based sensors incorporating stretchable conductive gels represent a promising approach to meet these requirements by combining soft mechanical compliance with efficient electromechanical signal transduction. However, conventional metallic or composite electrodes often suffer from mechanical mismatch with soft skin-like systems, motivating the exploration of intrinsically soft and stretchable conductive gels. In this review, we present a comprehensive and structured overview with comparative perspectives of stretchable skin-like conductive gel-based triboelectric devices. First, different classes of conductive gels, including hydrogels, organogels, ionogels, and other emerging gel systems, are systematically summarized and compared in terms of their composition, crosslinking strategies, conductivity, and mechanical characteristics. Next, the pivotal role of conductive gels in bridging skin-like sensing functions and triboelectric applications is elucidated, highlighting how their intrinsic softness, stretchability, self-healing capability, and interfacial conformability enable intimate skin contact and reliable electromechanical coupling. The key performance attributes of gel-based skin-like triboelectric sensors, including stretchability, self-healing behavior, optical and thermal tolerance, electrical durability, and environmental stability, are critically discussed with representative examples and comparative analysis. Typical device configurations, such as thin-film, fiber-shaped, and textile-based architectures, are further reviewed to illustrate structure–function relationships and application-oriented design strategies. Finally, current challenges, limitations, and future research directions for stretchable conductive gel-based triboelectric systems are outlined, aiming to provide practical guidelines and insights for the rational design of high-performance skin-like triboelectric sensors based on conductive gels. Full article

Stretchable semiconductors capable of maintaining electrical performance under large mechanical deformation are essential for reliable wearable electronic devices. However, polymer semiconductors often suffer from electrical degradation when subjected to tensile strain. In this study, electrical stability under strain was achieved by using a rubber-blended poly(2,5-bis(2-octyldodecyl)-3,6-di(thiophen-2-yl)diketopyrrolo[3,4-c]pyrrole-1,4-dione-alt-thieno[3,2-b]thiophene) (DPPT-TT) polymer semiconductor based on a conjugated polymer/elastomer phase separation-induced elasticity (CONPHINE) structure. Unlike most previous studies on fully stretchable thin-film transistors (TFTs), which primarily report overall performance changes under mechanical strain, this work systematically identifies the dominant origin of electrical performance degradation through a stepwise electrical analysis encompassing the gate insulating layer, the semiconductor layer, and complete devices. Bottom-gate top-contact (BGTC) and bottom-gate bottom-contact (BGBC) devices were fabricated on rigid Si/SiO₂ substrates to examine the intrinsic properties of the DPPT-TT/styrene-ethylene-butylene-styrene (SEBS) CONPHINE film. As a result, the device exhibits 90% mobility retention even at 100% tensile strain applied parallel to the charge transport direction. Quantitative resistance analysis using the Y-function method reveals that variations in channel resistance play a dominant role in strain-induced performance degradation, whereas changes in contact resistance contribute only marginally. These findings demonstrate that stabilizing channel resistance, rather than contact resistance, is important for achieving high mobility retention under large mechanical deformation, thereby providing concrete and quantitative design guidelines for reliable stretchable TFTs. Full article

The rapid advancement of flexible and stretchable electronics has raised new demands for conductive materials with high conductivity and excellent mechanical properties. Compared to traditional conductive materials, gallium-based liquid metals exhibit a compelling set of attributes—including intrinsic deformability, high conductivity, good thermal conductivity, and a liquid state at or near room temperature—that address the critical requirements for conductors in flexible and stretchable electronics. However, the broader application of gallium-based liquid metals is limited by intrinsic challenges, such as oxidation tendency and high surface tension, while their multifunctional potential remains to be fully explored and developed. This paper provides a comprehensive review of gallium-based liquid metals, spanning from their fundamental concepts including intrinsic properties and processing characteristics (oxidative layer/droplet engineering) and functionalization techniques to their diverse applications in flexible electronics. It concisely summarizes key factors, existing issues, and challenges encountered during the design, research, and application of gallium-based liquid metals, aiming to provide guidance and assistance for subsequent research and applications. Full article

Thin film/substrate structures based on the principle of buckling mechanics exhibit both excellent stretchability and mechanical stability, and they have been recognized as a critical configuration in the design of flexible electronic devices. During application, flexible electronic devices are usually subjected to complex dynamic environments. Therefore, it is of great significance to investigate the dynamic behavior of thin film/substrate structures for the design of flexible electronic devices. The bending energy, membrane energy, and kinetic energy of the thin film and the elastic energy of the substrate were calculated. On this basis, the dynamic equation of the thin film/substrate structure with a checkerboard wrinkled pattern was derived by applying the principle of minimum energy combined with the Lagrangian function. Numerical simulations were conducted on the system to analyze the effect of pre-strain and the Young’s modulus of substrate on the system’s potential energy function, simulate the temporal response of the system’s dynamic behavior, and investigate the influences of pre-strain and the Young’s modulus of substrate on system stability and the chaos critical value. Theoretical support is expected to be provided for the design of two-dimensional (2D) thin film/substrate structures through this research. Full article

Biomedical antennas are essential components in modern healthcare systems, supporting wireless communication, physiological monitoring, diagnostic imaging, and therapeutic energy delivery. Their performance is strongly influenced by proximity to the human body, creating challenges such as impedance detuning, signal absorption, and size constraints that motivate new materials and fabrication approaches. This work reviews recent advances enabling next-generation wearable and implantable antennas, with emphasis on printed electronics, additive manufacturing, flexible hybrid integration, and metamaterial design. Methods discussed include 3D printing and inkjet, aerosol jet, and screen printing for fabricating conductive traces on textiles, elastomers, and biodegradable substrates, as well as multilayer Flexible Hybrid Electronics that co-integrate sensing, power management, and RF components into thin, body-conforming assemblies. Key results highlight how metamaterial and metasurface concepts provide artificial control over dispersion, radiation, and near-field interactions, enabling antenna miniaturization, enhanced gain and focusing, and improved isolation from lossy biological tissue. These approaches reduce SAR, stabilize impedance under deformation, and support more efficient communication and energy transfer. The review concludes that the convergence of novel materials, engineered electromagnetic structures, and AI-assisted optimization is enabling biomedical antennas that are compact, stretchable, personalized, and highly adaptive, supporting future developments in unobtrusive monitoring, wireless implants, point-of-care diagnostics, and continuous clinical interfacing. Full article

Flexible sensors have emerged as critical interfaces for information exchange between soft biological tissues and machines. Here, we present a dual-mode stretchable sensor system capable of synchronous strain and electromyography (EMG) signal detection, integrated with wireless WIFI transmission for real-time joint movement monitoring. The system consists of two key components: (1) A multi-channel gel electrode array for high-fidelity EMG signal acquisition from target muscle groups, and (2) a novel capacitive strain sensor made of stretchable micro-cracked gold film based on Styrene Ethylene Butylene Styrene (SEBS) that exhibits exceptional performance, including >80% stretchability, >4000-cycle durability, and fast response time (<100 ms). The strain sensor demonstrates position-independent measurement accuracy, enabling robust joint angle detection regardless of placement variations. Through synchronized mechanical deformation and electrophysiological monitoring, this platform provides comprehensive movement quantification, with data visualization interfaces compatible with mobile and desktop applications. The proposed technology establishes a generalizable framework for multimodal biosensing in human motion analysis, robotics, and human–machine interaction systems. Full article

An alternative conductive ink based on carbon nanotubes (CNTs) was developed using a platinum-catalyzed silicone elastomer and isopropyl alcohol (IPA). The inclusion of IPA in the conductive CNT ink facilitated the optimization of its mechanical strength, electrical conductivity, and viscosity. Compared to conventional silicone rubber-based conductive polymers that often solidify in a few hours at room temperature or with heating, this liquid composite of CNT particles and IPA exhibited a prolonged duration of up to several months in a hermetic environment, maintaining chemical stability even with the elastomer and its curing agent. The gradual evaporation of IPA initiates a well-known cross-linking process, leading to stretchability and electrical conductivity derived from the silicone elastomer and CNT particles, respectively. The relationship between the mechanical strength and electrical conductivity of the hardened conductive CNT ink was studied, which helped determine the optimized concentration of CNT particles in the conductive CNT ink. Subsequently, a piezoresistive sensor was designed, fabricated, and evaluated. The conductive CNT ink-based piezoresistive sensor showed high sensitivity and good repeatability with respect to a wide range of external forces. The effect of the concentration of CNT particles on the viscosity of the conductive CNT ink was also investigated, providing a better understanding of the entanglement of CNT particles within the silicone elastomer. A coating test using the conductive CNT ink with a paper cutting machine demonstrated its potential for adaptation to various printing techniques, including screen printing. The proposed conductive CNT ink, characterized by a simple chemical composition, facile fabrication process, use of non-toxic elements, high electrical conductivity, and stretchability, combined with an extended duration, has the potential to be applied for multiple purposes, such as various types of flexible and wearable electronics. Full article