Search Results (18)

The beam angle error of the pump light in a K-Rb-²¹Ne spin-exchange relaxation-free atomic co-magnetometer (SERFCM) significantly degrades the efficiency of optical pumping and the system’s ability to suppress magnetic field noise. In this work, a system response model that incorporates the pump beam alignment error (PBAE) is established. The influence of PBAE on the scale factor, bandwidth, and magnetic noise response of the inertial output is analyzed. Theoretical results show that PBAE increases the internal magnetic field gradient, reduces the efficiency of nuclear spin hyperpolarization, and increases the nuclear spin relaxation rate, ultimately degrading the system’s scale factor, bandwidth, and magnetic noise suppression capability. Experimental results demonstrate that, compared to the original SERFCM with PBAE, aligning the pump laser using the proposed method improves the polarization strength of nuclear spins by approximately 10% and enhances magnetic noise suppression by 40%. Full article

Optically pumped magnetometers (OPMs) functioning in the spin-exchange relaxation-free (SERF) regime have emerged as attractive options for measuring weak magnetic fields, owing to their portability and remarkable sensitivity. The operation of SERF-OPM critically relies on the ambient magnetic field; thus, a magnetic field compensation device is commonly employed to mitigate the ambient magnetic field to near zero. Nonetheless, the bias of the OPM may influence the compensation impact, a subject that remains unexamined. This paper introduced an innovative bias calibration technique for OPMs. The sensitivity of the OPM was altered by adjusting the cell temperature. The output of the OPM was then documented with varying sensitivity. It is assumed that the signal exhibits a linear correlation with the environmental magnetic field, and the statistical characteristics of the magnetic field are identical for both measurements, upon which the bias of the OPM is assessed. The bias was subsequently considered in the feedback magnetic field compensation mechanism. The results indicate that this technique might successfully reduce environmental magnetic fluctuations and enhance the sensitivity of the OPM. This technique measured the magnetic field produced by the human heart, confirming the viability of the ultra-weak biomagnetic field measurement approach. Full article

The spin-exchange-pumped nuclear magnetic resonance gyroscope (NMRG) is a pivotal tool in quantum navigation. The transverse relaxation of atoms critically impacts the NMRG’s performance parameters and is essential for judging normal operation. Conventional methods for measuring transverse relaxation typically use dual beams, which involves complex optical path and frequency stabilization systems, thereby complicating miniaturization and integration. This paper proposes a method to construct a ¹³³Cs parametric resonance magnetometer using a single-beam vertical-cavity surface-emitting laser (VCSEL) to measure the transverse relaxation of ¹²⁹Xe and ¹³¹Xe. Based on this method, the volume of the gyroscope probe is significantly reduced to 50 cm³. Experimental results demonstrate that the constructed Cs-Xe NMRG can achieve a transverse relaxation time (T₂) of 8.1 s under static conditions. Within the cell temperature range of 70 °C to 110 °C, T₂ decreases with increasing temperature, while the signal amplitude inversely increases. The research lays the foundation for continuous measurement operations of miniaturized NMRGs. Full article

A K–Rb–${}^{83}$Kr-based atomic comagnetometer for performing movement-related Magnetoencephalography (MEG) is theoretically studied in this paper. Parameters such as the spin-exchange rates, the spin-dephasing rates and the polarization of the nuclear spins are studied to configure the comagnetometer. The results show that the nuclear spin can generate a magnetic field of around 700 nT, at which the nuclear spin can compensate for a wide range of magnetic fields. In this paper, we also show the fabrication process for hybrid optical-pumping vapor cells, whereby alkali metals are mixed in a glove box that is then connected to the alkali vapor-cell fabrication system. Full article

The low-frequency fluctuations of the atomic density within the cell can induce the longterm drift of the K-Rb-²¹Ne spin-exchange relaxation-free (SERF) co-magnetometer output, such that the accurate measurement of in situ atomic density is of great significance for improving the performance of co-magnetometer. In this paper, the complex refractive index model of the spin ensembles under the hybrid optical pumping condition is established first, according to which the relation between atomic density and its complex refractive index is revealed and an optical heterodyne-based scheme for atomic density detection is proposed. The dependence of the atomic density on the demodulated phase signal from the optical heterodyne-based scheme is provided by numerical simulations. After that, a dual acousto-optics frequency shifter (AOFS)-based optical heterodyne interferometry is constructed with a noise level below 1 mrad/$\sqrt{\mathrm{Hz}}$ for frequencies > 1 Hz, and a compact SERF co-magnetometer is implemented as the testing medium, by which the atomic density detection with resolution of 0.40 K @ 473 K is reached and the experimental results agree well with theoretical simulations. Moreover, the detection scheme proposed in this paper has the properties of high detection sensitivity and immunity to laser power fluctuation, which are also proved experimentally. Full article

A 1083 nm laser, corresponding to a characteristic spectral line of ³He 2³S₁-2³P, is the core light source for spin-exchange optical pumping-free technology, and thus has important developmental significance. In this paper, precise wavelength 1083.34 nm semiconductor lasers with 285 mW output power, −144.73 dBc/Hz RIN noise and 30.9952 kHz linewidth have been successfully achieved via reasonable chips design, high-quality epitaxial growth process and ultra-low reflectivity coating fabrication. All the results show the highest output power and ultra-narrow linewidth of the single-frequency 1083 nm DFB semiconductor laser achieved in this paper, which can fully satisfy the requirement of quantum magnetometers. Full article

In this paper, we describe a new approach to the continuous operation of a transverse spin-exchange optically pumped NMR gyroscope that utilizes modulation of both the applied bias field and the optical pumping. We demonstrate the simultaneous, continuous excitation of ${}^{131}$Xe and ${}^{129}$Xe using this hybrid modulation approach and the real-time demodulation of the Xe precession using a custom least-squares fitting algorithm. We present rotation rate measurements with this device, with a common field suppression factor of ∼1400, an angle random walk of 21 $\mathsf{\mu }\mathrm{Hz}$/$\sqrt{\mathrm{Hz}}$, and a bias instability of ∼480 nHz after ∼1000 s. Full article

Zero-field optically pumped magnetometers operating in the spin-exchange relaxation-free (SERF) regime have been extensively studied, and usually depend on zeroth-order parametric resonance to measure the magnetic field. However, the studies conducted on this topic lack thorough analyses and in-depth discussion of nonzero-order magnetic resonances in single-beam SERF magnetometers. In this paper, we analyzed the nonzero-order resonance, especially the first-order resonance, based on a single-beam SERF magnetometer, and discussed its various applications. A comprehensive theoretical analysis and experiments were conducted with respect to multiple functions, including nonzero finite magnetic field measurements, spin polarization measurement, and in situ coil constant calibration. The results showed that first-order resonance can be utilized for nonzerofinite magnetic field measurements, and the spin polarization of alkali-metal atoms can be determined by measuring the slowing-down factor using the resonance condition. Furthermore, acquiring the first-order resonance point at an equivalent zero pump light power through fitting offers an approach for quick and precise in situ coil constant calibration. This study contributes to the applications of SERF magnetometers in nonzero finite magnetic fields. Full article

Machine learning (ML) is an effective tool to interrogate complex systems to find optimal parameters more efficiently than through manual methods. This efficiency is particularly important for systems with complex dynamics between multiple parameters and a subsequent high number of parameter configurations, where an exhaustive optimisation search would be impractical. Here we present a number of automated machine learning strategies utilised for optimisation of a single-beam caesium (Cs) spin exchange relaxation free (SERF) optically pumped magnetometer (OPM). The sensitivity of the OPM ($\mathrm{T}/\sqrt{\mathrm{Hz}}$), is optimised through direct measurement of the noise floor, and indirectly through measurement of the on-resonance demodulated gradient (mV/nT) of the zero-field resonance. Both methods provide a viable strategy for the optimisation of sensitivity through effective control of the OPM’s operational parameters. Ultimately, this machine learning approach increased the optimal sensitivity from 500 $\mathrm{fT}/\sqrt{\mathrm{Hz}}$ to $<109\mathrm{fT}/\sqrt{\mathrm{Hz}}$. The flexibility and efficiency of the ML approaches can be utilised to benchmark SERF OPM sensor hardware improvements, such as cell geometry, alkali species and sensor topologies. Full article

Inside a spin-exchange relaxation-free (SERF) co-magnetometer with a high-pressure buffer gas atomic cell, the magnetic field gradient causes the decoherence of atomic spins to produce magnetic-field gradient relaxation. This paper presents a new method for the accurate measurement of magnetic field gradient relaxation of alkali metal atoms and inert atoms of strongly coupled spin systems under triaxial magnetic field gradients in the K-Rb-²¹Ne co-magnetometer. The magnetic field gradient relaxation of alkali metal atoms is measured using a step magnetic field modulation method, and the magnetic field gradient relaxation of inert atoms is measured using a combined free induction decay and spin growth method. The method does not require the use of large background magnetic fields and RF fields to maintain the atoms in the SERF state, does not require additional optics, and is not affected by the pumping or detecting of optical power. A kinetic model that considers a large electron-equivalent magnetic field was designed and a gradient relaxation model was developed. The quadratic coefficients of the experimentally measured gradient relaxation curves fit the theoretical model well over the range of the applied magnetic field gradients, confirming the validity of the proposed method. Full article

The measurement of atomic spin polarization distribution in spin-exchange relaxation free (SERF) magnetometer is an important topic for improving the sensitivity and consistency of multi-channel magnetic field measurement applications. A novel spin polarization spatial distribution measurement method is presented based on the transient response of the magnetometer after modulating the pumped light with a chopper. Polarization is obtained by a slow-down factor based on the fast spin-exchange interaction effects. Longitudinal and transverse polarization distributions are measured simultaneously without interrupting the operation of the SERF status. Under different oscillating magnetic fields, the spin polarization is measured at the cell centroid. Residual magnetic field inside the magnetometer is obtained from the linear relationship between the precession frequency and the oscillating magnetic field. The one-dimensional polarization distributions in the x, y, and z axes are measured using a digital micromirror device with a resolution of 0.25 cm. The measurement results conform to the Lambert-Bier absorption law and the Gaussian distribution law. Furthermore, 7 × 7 two-dimensional spatial distribution measurements of polarization on the xy and yz planes are performed. Nonuniformity of 1.04 in the xy plane and 1.82 in the yz plane in the built magnetometer. Compared with other measurement methods, the distribution measurement method proposed is independent of optical depth and suitable for low polarization and high polarization applications. Based on the results of the proposed measurement method of spin polarization spatial distribution, further compensation can improve the application consistency of multi-channel magnetic field measurements and improve the sensitivity of single-channel differential measurements. Full article

Accurate knowledge of the rubidium (Rb) vapor density, $\left[\mathrm{Rb}\right]$, is necessary to correctly model the spin dynamics of ${}^{129}$Xe-Rb spin-exchange optical pumping (SEOP). Here we present a systematic evaluation of $\left[\mathrm{Rb}\right]$ within a high-throughput ${}^{129}$Xe-Rb hyperpolarizer during continuous-flow SEOP. Near-infrared ($5^2{S}_{1/2}\to 5^2{P}_{1/2}$ (D${}_1$)/5${}^2{P}_{3/2}$ (D${}_2$)) and violet ($5^2{S}_{1/2}\to 6^2{P}_{1/2}$/6${}^2{P}_{3/2}$) atomic absorption spectroscopy was used to measure $\left[\mathrm{Rb}\right]$ within 3.5 L cylindrical SEOP cells containing different spatial distributions and amounts of Rb metal. We were able to quantify deviation from the Beer-Lambert law at high optical depth for D${}_2$ and 6${}^2{P}_{3/2}$ absorption by comparison with measurements of the D${}_1$ and 6${}^2{P}_{1/2}$ absorption lines, respectively. D${}_2$ absorption deviates from the Beer-Lambert law at ${\left[\mathrm{Rb}\right]}_{D_2}>4\times {10}^{17}$ m${}^{-3}$ whilst 5${}^2$S${}_{1/2}\to 6^2{P}_{3/2}$ absorption deviates from the Beer-Lambert law at ${\left[\mathrm{Rb}\right]}_{6P_{3/2}}>(4.16\pm 0.01)\times {10}^{19}$ m${}^{-3}$. The measured $\left[\mathrm{Rb}\right]$ was used to estimate a ${}^{129}$Xe-Rb spin exchange cross section of ${\gamma }^{\prime }=(1.2\pm 0.1)\times {10}^{-21}$ m${}^3$ s${}^{-1}$, consistent with spin-exchange cross sections from the literature. Significant $\left[\mathrm{Rb}\right]$ heterogeneity was observed in a SEOP cell containing 1 g of Rb localized at the back of the cell. While $\left[\mathrm{Rb}\right]$ homogeneity was improved for a greater surface area of the Rb source distribution in the cell, or by using a Rb presaturator, the measured $\left[\mathrm{Rb}\right]$ was consistently lower than that predicted by saturation Rb vapor density curves. Efforts to optimize $\left[\mathrm{Rb}\right]$ and thermal management within spin polarizer systems are necessary to maximize potential future enhancements of this technology. Full article

Optically pumped magnetometers (OPMs) are new, room-temperature alternatives to superconducting quantum interference devices (SQUIDs) for measuring the brain’s magnetic fields. The most used OPM in MagnetoEncephaloGraphy (MEG) are based on alkali atoms operating in the spin-exchange relaxation-free (SERF) regime. These sensors do not require cooling but have to be heated. Another kind of OPM, based on the parametric resonance of ⁴He atoms are operated at room temperature, suppressing the heat dissipation issue. They also have an advantageous bandwidth and dynamic range more suitable for MEG recordings. We quantitatively assessed the improvement (relative to a SQUID magnetometers array) in recording the magnetic field with a wearable ⁴He OPM-MEG system through data simulations. The OPM array and magnetoencephalography forward models were based on anatomical MRI data from an adult, a nine-year-old child, and 10 infants aged between one month and two years. Our simulations showed that a ⁴He OPMs array offers markedly better spatial specificity than a SQUID magnetometers array in various key performance areas (e.g., signal power, information content, and spatial resolution). Our results are also discussed regarding previous simulation results obtained for alkali OPM. Full article

We present a pilot quality assurance (QA) study of a clinical-scale, automated, third-generation (GEN-3) ¹²⁹Xe hyperpolarizer employing batch-mode spin-exchange optical pumping (SEOP) with high-Xe densities (50% natural abundance Xe and 50% N₂ in ~2.6 atm total pressure sourced from Nova Gas Technologies) and rapid temperature ramping enabled by an aluminum heating jacket surrounding the 0.5 L SEOP cell. ¹²⁹Xe hyperpolarization was performed over the course of 700 gas loading cycles of the SEOP cell, simulating long-term hyperpolarized contrast agent production in a clinical lung imaging setting. High levels of ¹²⁹Xe polarization (avg. %P_Xe = 51.0% with standard deviation σ_PXe = 3.0%) were recorded with fast ¹²⁹Xe polarization build-up time constants (avg. T_b = 25.1 min with standard deviation σ_Tb = 3.1 min) across the first 500 SEOP cell refills, using moderate temperatures of 75 °C. These results demonstrate a more than 2-fold increase in build-up rate relative to previously demonstrated results in a comparable QA study on a second-generation (GEN-2) ¹²⁹Xe hyperpolarizer device, with only a minor reduction in maximum achievable %P_Xe and with greater consistency over a larger number of SEOP cell refill processes at a similar polarization lifetime duration (avg. T₁ = 82.4 min, standard deviation σ_T1 = 10.8 min). Additionally, the effects of varying SEOP jacket temperatures, distribution of Rb metal, and preparation and operation of the fluid path are quantified in the context of device installation, performance optimization and maintenance to consistently produce high ¹²⁹Xe polarization values, build-up rates (T_b as low as 6 min) and lifetimes over the course of a typical high-throughput ¹²⁹Xe polarization SEOP cell life cycle. The results presented further demonstrate the significant potential for hyperpolarized ¹²⁹Xe contrast agent in imaging and bio-sensing applications on a clinical scale. Full article

In order to improve the precision and beam quality of a pump laser for a spin exchange relaxation free inertial measurement device, we applied one scheme to achieve the square wave modulation and power stability control of the pump laser and another one to obtain the uniform intensity distribution of the laser beam, in which the acousto-optic modulator (AOM) and proportion integration differentiation (PID) controller were used to achieve the former, and the freeform surface lens was designed and optimized to achieve the latter based on the TracePro software. In experiments, the first-order diffraction light beam coming through the AOM had a spot size of about 1.1 × 0.7 mm², and a spherical vapor cell with a radius of 7 mm was placed behind the freeform surface lens. Results show that the uniformity of the reshaped intensity distribution is higher than 90% within the target area with a radius of 7 mm both in the simulation and the experiment, which ensure that the uniform laser beam covers the area of cell. On the other hand, the power stability of the pump laser is controlled to be less than 0.05%. Compared with traditional methods, the complicated calculation process in optical design is better solved, and a higher uniformity with slight energy loss is achieved. Full article