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Keywords = PEMFC diagnosis

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17 pages, 2886 KB  
Article
Online Pre-Diagnosis of Multiple Faults in Proton Exchange Membrane Fuel Cells by Convolutional Neural Network Based Bi-Directional Long Short-Term Memory Parallel Model with Attention Mechanism
by Junyi Chen, Huijun Ran, Ziyang Chen, Trevor Hocksun Kwan and Qinghe Yao
Energies 2025, 18(10), 2669; https://doi.org/10.3390/en18102669 - 21 May 2025
Viewed by 509
Abstract
Proton exchange membrane fuel cell (PEMFC) fault diagnosis faces two critical limitations: conventional offline methods lack real-time predictive capability, while existing prediction approaches are confined to single fault types. To address these gaps, this study proposes an online multi-fault prediction framework integrating three [...] Read more.
Proton exchange membrane fuel cell (PEMFC) fault diagnosis faces two critical limitations: conventional offline methods lack real-time predictive capability, while existing prediction approaches are confined to single fault types. To address these gaps, this study proposes an online multi-fault prediction framework integrating three novel contributions: (1) a sensor fusion strategy leveraging existing thermal/electrochemical measurements (voltage, current, temperature, humidity, and pressure) without requiring embedded stack sensors; (2) a real-time sliding window mechanism enabling dynamic prediction updates every 1 s under variable load conditions; and (3) a modified CNN-based Bi-LSTM parallel model with attention mechanism (ConvBLSTM-PMwA) architecture featuring multi-input multi-output (MIMO) capability for simultaneous flooding/air-starvation detection. Through comparative analysis of different neural architectures using experimental datasets, the optimized ConvBLSTM-PMwA achieved 96.49% accuracy in predicting dual faults 64.63 s pre-occurrence, outperforming conventional LSTM models in both temporal resolution and long-term forecast reliability. Full article
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22 pages, 899 KB  
Article
Square Root Unscented Kalman Filter-Based Multiple-Model Fault Diagnosis of PEM Fuel Cells
by Abdulrahman Allam, Michael Mangold and Ping Zhang
Sensors 2025, 25(1), 29; https://doi.org/10.3390/s25010029 - 24 Dec 2024
Viewed by 907
Abstract
Harsh operating conditions imposed by vehicular applications significantly limit the utilization of proton exchange membrane fuel cells (PEMFCs) in electric propulsion systems. Improper/poor management and supervision of rapidly varying current demands can lead to undesired electrochemical reactions and critical cell failures. Among other [...] Read more.
Harsh operating conditions imposed by vehicular applications significantly limit the utilization of proton exchange membrane fuel cells (PEMFCs) in electric propulsion systems. Improper/poor management and supervision of rapidly varying current demands can lead to undesired electrochemical reactions and critical cell failures. Among other failures, flooding and catalytic degradation are failure mechanisms that directly impact the composition of the membrane electrode assembly and can cause irreversible cell performance deterioration. Due to the functional significance and high manufacturing costs of the catalyst layer, monitoring internal fuel cell states is crucial. For this purpose, a diagnostic-oriented multi-scale PEMFC catalytic degradation model is developed which incorporates the failure effects of catalytic degradation on cell dynamics and global stack performance. Embedded to the multi-scale model is a square root unscented Kalman filter (SRUKF)-based multiple-model fault diagnosis scheme. In this approach, multiple models are used to estimate specific internal PEMFC system parameters, such as the mass transfer coefficient of the gas diffusion layer or the exchange current density, which are treated as additional system states. Online state estimates are provided by the SRUKF, which additionally propagates model-conditioned statistical information to update a Bayesian framework for model selection. The Bayesian model selection method carries fault indication signals that are interpreted by a derived decision logic to obtain reliable information on the current-operating system regime. The proposed diagnosis scheme is evaluated through simulations using the LA 92 and NEDC driving cycles. Full article
(This article belongs to the Section Fault Diagnosis & Sensors)
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15 pages, 4167 KB  
Article
Real-Time Impedance Detection for PEM Fuel Cell Based on TAB Converter Voltage Perturbation
by Jialong Zhou, Jinhai Jiang, Fulin Fan, Chuanyu Sun, Zhen Dong and Kai Song
Energies 2024, 17(17), 4320; https://doi.org/10.3390/en17174320 - 29 Aug 2024
Cited by 1 | Viewed by 1604
Abstract
Fuel cells, as clean and efficient energy conversion devices, hold great potential for applications in the fields of hydrogen-based transportation and stand-alone power systems. Due to their sensitivity to load parameters, environmental parameters, and gas supply, the performance monitoring and fault diagnosis of [...] Read more.
Fuel cells, as clean and efficient energy conversion devices, hold great potential for applications in the fields of hydrogen-based transportation and stand-alone power systems. Due to their sensitivity to load parameters, environmental parameters, and gas supply, the performance monitoring and fault diagnosis of fuel cell systems have become crucial research areas. Electrochemical impedance spectroscopy (EIS) is a widely applied analytical method in fuel cell systems. that can provide rich information about dynamic system responses, internal impedance, and transmission characteristics. Currently, EIS detection is primarily implemented by using simple topologies such as boost circuits. However, the injection of excitation signals often results in significant power fluctuations, leading to issues such as uneven temperature distributions within the cell, unstable gas supply, and damage to the proton exchange membrane. To address this issue, this paper proposes a real-time EIS detection technique for a proton exchange membrane fuel cell (PEMFC) system that connects a lithium-ion battery and injects the load voltage perturbation through a triple active bridge (TAB) converter. By applying the small-signal model of the TAB converter and designing a system controller using a decoupling control method, the PEMFC power remains stable after the disturbance injection across the entire frequency range under tests. Furthermore, the lithium-ion battery can instantly track load changes during fluctuations. The proposed EIS detection method can acquire EIS data in real time to monitor the state of the PEMFC. Simulation results validate the effectiveness and accuracy of the proposed method for EIS detection. Full article
(This article belongs to the Special Issue Renewable Energy and Hydrogen Energy Technologies)
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17 pages, 3461 KB  
Article
Dynamic Fractional-Order Model of Proton Exchange Membrane Fuel Cell System for Sustainability Improvement
by Yunjin Ao, Yong-Chao Liu, Salah Laghrouche and Denis Candusso
Sustainability 2024, 16(7), 2939; https://doi.org/10.3390/su16072939 - 1 Apr 2024
Cited by 2 | Viewed by 1496
Abstract
The proton exchange membrane fuel cell (PEMFC) stands at the forefront of advancing energy sustainability. Effective monitoring, control, diagnosis, and prognosis are crucial for optimizing the PEMFC system’s sustainability, necessitating a dynamic model that can capture the transient response of the PEMFC. This [...] Read more.
The proton exchange membrane fuel cell (PEMFC) stands at the forefront of advancing energy sustainability. Effective monitoring, control, diagnosis, and prognosis are crucial for optimizing the PEMFC system’s sustainability, necessitating a dynamic model that can capture the transient response of the PEMFC. This paper uses a dynamic fractional-order model to describe the behaviors of a stationary micro combined heat and power (mCHP) PEMFC stack. Based on the fractional-order equivalent circuit model, the applied model accurately represents the electrochemical impedance spectroscopy (EIS) and the dynamic voltage response under transient conditions. The applied model is validated through experiments on an mCHP PEMFC stack under various fault conditions. The EIS data is analyzed under different current densities and various fault conditions, including the stoichiometry of the anode and cathode, the stack temperature, and the relative humidity. The dynamic voltage response of the applied model shows good correspondence with experimental results in both phase and amplitude, thereby affirming the method’s precision and solidifying its role as a reliable tool for enhancing the sustainability and operational efficiency of PEMFC systems. Full article
(This article belongs to the Section Energy Sustainability)
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25 pages, 4191 KB  
Article
PEMFCs Model-Based Fault Diagnosis: A Proposal Based on Virtual and Real Sensors Data Fusion
by Eduardo Ariza, Antonio Correcher and Carlos Vargas-Salgado
Sensors 2023, 23(17), 7383; https://doi.org/10.3390/s23177383 - 24 Aug 2023
Cited by 9 | Viewed by 1883
Abstract
Proton Exchange Membrane Fuel Cells (PEMFCs) are critical components in renewable hybrid systems, demanding reliable fault diagnosis to ensure optimal performance and prevent costly damages. This study presents a novel model-based fault diagnosis algorithm for commercial hydrogen fuel cells using LabView. Our research [...] Read more.
Proton Exchange Membrane Fuel Cells (PEMFCs) are critical components in renewable hybrid systems, demanding reliable fault diagnosis to ensure optimal performance and prevent costly damages. This study presents a novel model-based fault diagnosis algorithm for commercial hydrogen fuel cells using LabView. Our research focused on power generation and storage using hydrogen fuel cells. The proposed algorithm accurately detects and isolates the most common faults in PEMFCs by combining virtual and real sensor data fusion. The fault diagnosis process began with simulating faults using a validated mathematical model and manipulating selected input signals. A statistical analysis of 12 residues from each fault resulted in a comprehensive fault matrix, capturing the unique fault signatures. The algorithm successfully identified and isolated 14 distinct faults, demonstrating its effectiveness in enhancing reliability and preventing performance deterioration or system shutdown in hydrogen fuel cell-based power generation systems. Full article
(This article belongs to the Special Issue Sensors and Methods for Diagnostics and Early Fault Detection)
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16 pages, 6273 KB  
Article
Design of a Fuel Cell Test System with Fault Identification
by Shusheng Xiong, Zhankuan Wu and Junjie Cheng
Electronics 2023, 12(15), 3365; https://doi.org/10.3390/electronics12153365 - 7 Aug 2023
Cited by 2 | Viewed by 2870
Abstract
With the growing concerns over the energy crisis and environmental pollution, fuel cells have attracted increasing attention. Proton exchange membrane fuel cells (PEMFCs) have promising prospects due to their economic efficiency, low noise, and minimal environmental pollution. However, the existing commercial testing systems [...] Read more.
With the growing concerns over the energy crisis and environmental pollution, fuel cells have attracted increasing attention. Proton exchange membrane fuel cells (PEMFCs) have promising prospects due to their economic efficiency, low noise, and minimal environmental pollution. However, the existing commercial testing systems for PEMFCs suffer from limited functionalities and lack of scalability. In this study, we propose the design of a testing platform specifically tailored for water-cooled PEMFCs with a power greater than 1 kW. The functionality of the testing platform is verified through static and dynamic testing, demonstrating its compliance with the required standards. Furthermore, a fault diagnosis model for fuel cell stacks is developed based on the back-propagation (BP) neural network, achieving an overall accuracy rate of over 95% for fault classification. Full article
(This article belongs to the Section Electronic Materials, Devices and Applications)
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16 pages, 891 KB  
Review
Fault Detection for PEM Fuel Cells via Analytical Redundancy: A Critical Review and Prospects
by Mukhtar Sani, Maxime Piffard and Vincent Heiries
Energies 2023, 16(14), 5446; https://doi.org/10.3390/en16145446 - 18 Jul 2023
Cited by 7 | Viewed by 2349
Abstract
Decarbonization of the transport sector could be achieved through fuel cell technology. The candidature of this technology is motivated by its high current density and lack of emissions. However, its widespread deployment is restrained by durability and reliability constraints. During normal operation, the [...] Read more.
Decarbonization of the transport sector could be achieved through fuel cell technology. The candidature of this technology is motivated by its high current density and lack of emissions. However, its widespread deployment is restrained by durability and reliability constraints. During normal operation, the fuel cell system supplies stable power to the load. Contrarily, when it is operated under faulty conditions, the system’s output power deteriorates, leading to low durability. It is therefore of paramount importance to ensure that the system is operated in a non-faulty condition. In this paper, we provide a critical review of the analytical-redundancy-based fault diagnosis methods for proton exchange membrane fuel cells (PEMFCs). An in-depth analysis of the various methods has been presented in terms of accuracy, complexity, implementability, and robustness to aging and dynamic operating conditions. Full article
(This article belongs to the Collection Hydrogen Energy Reviews)
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19 pages, 9139 KB  
Article
A System-Level Modeling of PEMFC Considering Degradation Aspect towards a Diagnosis Process
by Antoine Bäumler, Jianwen Meng, Abdelmoudjib Benterki, Toufik Azib and Moussa Boukhnifer
Energies 2023, 16(14), 5310; https://doi.org/10.3390/en16145310 - 11 Jul 2023
Cited by 7 | Viewed by 2251
Abstract
This paper proposes a modular modeling towards a health system integration of fuel cells by considering not only the dynamics of the gases but also fault models that affect the PEMFC performances. The main goal is to simulate the faulty state in order [...] Read more.
This paper proposes a modular modeling towards a health system integration of fuel cells by considering not only the dynamics of the gases but also fault models that affect the PEMFC performances. The main goal is to simulate the faulty state in order to overcome data scarcity, since running a fuel cell to generate a database under faulty conditions is a costly process in time and resources. The degradation processes detailed in this paper allow to introduce a classification of faults that can occur, giving a better understanding of the performance losses necessary to simulate them. The faults that are detailed and modeled are the flooding, drying and aging processes. This modeling is based on a system approach, so it runs faster than real-time degradation tests, allowing the training and validation of online supervisors, such as the energy management strategy (EMS) method or diagnosis. The faults are reproduced according to the study requirements to be a very effective support tool to help design engineers to include faulty conditions in early design stages toward a diagnosis process and health-conscious energy management strategies. Full article
(This article belongs to the Special Issue Hydrogen and Fuel Cell Technology, Modelling and Simulation II)
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16 pages, 3699 KB  
Article
State Estimation of Membrane Water Content of PEMFC Based on GA-BP Neural Network
by Haibo Huo, Jiajie Chen, Ke Wang, Fang Wang, Guangzhe Jin and Fengxiang Chen
Sustainability 2023, 15(11), 9094; https://doi.org/10.3390/su15119094 - 5 Jun 2023
Cited by 6 | Viewed by 2703
Abstract
Too high or too low water content in the proton exchange membrane (PEM) will affect the output performance of the proton exchange membrane fuel cell (PEMFC) and shorten its service life. In this paper, the mathematical mechanisms of cathode mass flow, anode mass [...] Read more.
Too high or too low water content in the proton exchange membrane (PEM) will affect the output performance of the proton exchange membrane fuel cell (PEMFC) and shorten its service life. In this paper, the mathematical mechanisms of cathode mass flow, anode mass flow, water content in the PEM and stack voltage of the PEMFC are deeply studied. Furthermore, the dynamic output characteristics of the PEMFC under the conditions of flooding and drying membrane are reported, and the influence of water content in PEM on output performance of the PEMFC is analyzed. To effectively diagnose membrane drying and flooding faults, prolong their lifespan and thus to improve operation performance, this paper proposes the state assessment of water content in the PEM based on BP neural network optimized by genetic algorithm (GA). Simulation results show that compared with LS-SVM, GA-BP neural network has higher estimation accuracy, which lays a foundation for the fault diagnosis, life extension and control scheme design of the PEMFC. Full article
(This article belongs to the Special Issue Development Trends of New Energy Materials and Devices)
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20 pages, 3172 KB  
Article
An Innovative PEMFC Magnetic Field Emulator to Validate the Ability of a Magnetic Field Analyzer to Detect 3D Faults
by Ali Bawab, Stefan Giurgea, Daniel Depernet and Daniel Hissel
Hydrogen 2023, 4(1), 22-41; https://doi.org/10.3390/hydrogen4010003 - 5 Jan 2023
Cited by 6 | Viewed by 2662
Abstract
An original non-invasive methodology of the fuel cell diagnosis is proposed to identify different positions of the faults in Proton Exchange Membrane Fuel Cell (PEMFC) stacks from external magnetic field measurements. The approach is based on computing the external magnetic field difference between [...] Read more.
An original non-invasive methodology of the fuel cell diagnosis is proposed to identify different positions of the faults in Proton Exchange Membrane Fuel Cell (PEMFC) stacks from external magnetic field measurements. The approach is based on computing the external magnetic field difference between normal and faulty PEMFC operating conditions. To evaluate the external magnetic field distribution, in this paper, we propose an improved design of the magnetic field analyzer. This analyzer amplifies the magnetic field around the cell to perform an accurate detection of the fault position. Moreover, the main contribution of this work is represented by conceiving and implementing a 3D multi-physical current distribution emulator of a proton exchange membrane fuel cell. The new concept of a proton exchange membrane fuel cell emulator has been specially designed to emulate the magnetic field of a real fuel cell stack. This emulator concept is also beneficial for a new model of the fuel cell, which implies a multi-physical coupling between electrochemical electric conduction and the generated magnetic field. Finally, finally, the numerical model and the emulator have been involved in the realization of numerical simulations and experimental analysis to prove the ability of the system to detect and localize 3D faults. Full article
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12 pages, 5413 KB  
Article
Modelling of Proton Exchange Membrane Fuel Cells with Sinusoidal Approach
by Catalina González-Castaño, Yahya Aalaila, Carlos Restrepo, Javier Revelo-Fuelagán and Diego Hernán Peluffo-Ordóñez
Membranes 2022, 12(11), 1056; https://doi.org/10.3390/membranes12111056 - 28 Oct 2022
Cited by 2 | Viewed by 2386
Abstract
This paper validates a sinusoidal approach for the proton-exchange membrane fuel cell (PEMFC) model as a supplement to experimental studies. An FC simulation or hardware emulation is necessary for prototype design, testing, and fault diagnosis to reduce the overall cost. For this objective, [...] Read more.
This paper validates a sinusoidal approach for the proton-exchange membrane fuel cell (PEMFC) model as a supplement to experimental studies. An FC simulation or hardware emulation is necessary for prototype design, testing, and fault diagnosis to reduce the overall cost. For this objective, a sinusoidal model that is capable of accurately estimating the voltage behavior from the operating current value of the DC was developed. The model was tested using experimental data from the Ballard Nexa 1.2 kW fuel cell (FC). This methodology offers a promising approach for static and current-voltage, characteristic of the three regions of operation. A study was carried out to evaluate the effectiveness and superiority of the proposed FC Sinusoidal model compared with the Diffusive Global model and the Evolution Strategy. Full article
(This article belongs to the Special Issue Progress in Proton Exchange Membrane Fuel Cells (PEMFCs))
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15 pages, 11057 KB  
Article
A 2D Multi-Layer Model to Study the External Magnetic Field Generated by a Polymer Exchange Membrane Fuel Cell
by Antony Plait and Frédéric Dubas
Mathematics 2022, 10(20), 3883; https://doi.org/10.3390/math10203883 - 19 Oct 2022
Cited by 3 | Viewed by 1781
Abstract
An original innovative two-dimensional (2D) multi-layer model based on the Maxwell–Fourier method for the diagnosis of a polymer exchange membrane (PEM) fuel cell (FC) stack is presented. It is possible to determine the magnetic field distribution generated around the PEMFC stack from the [...] Read more.
An original innovative two-dimensional (2D) multi-layer model based on the Maxwell–Fourier method for the diagnosis of a polymer exchange membrane (PEM) fuel cell (FC) stack is presented. It is possible to determine the magnetic field distribution generated around the PEMFC stack from the (non-)homogenous current density distribution inside the PEMFC stack. Analysis of the magnetic field distribution can indicate whether the FC is healthy or faulty. In this way, an explicit, accurate and fast analytical model can allow the health state of an FC to be studied. To evaluate the capacity and the efficiency of the 2D analytical model, the distribution of local quantities (i.e., magnetic vector potential and magnetic field) in a PEMFC stack has been validated with those obtained by the 2D finite-element analysis (FEA). The comparisons demonstrate excellent results both in terms of amplitude and waveform. The validation of this 2D analytical model is essential for the subsequent generation of an inverse model useful for the diagnosis of a PEMFC. Full article
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16 pages, 5140 KB  
Article
A Closed-Loop Water Management Methodology for PEM Fuel Cell System Based on Impedance Information Feedback
by Xinjie Xu, Kai Li, Zhenjie Liao, Jishen Cao and Renkang Wang
Energies 2022, 15(20), 7561; https://doi.org/10.3390/en15207561 - 13 Oct 2022
Cited by 10 | Viewed by 2999
Abstract
Water management is an important issue for proton exchange membrane fuel cells (PEMFC). The research mainly focuses on the diagnosis and treatment of faults. However, faults harm PEMFC and cause its durability decay, whatever duration they last. This study designs a closed-loop water [...] Read more.
Water management is an important issue for proton exchange membrane fuel cells (PEMFC). The research mainly focuses on the diagnosis and treatment of faults. However, faults harm PEMFC and cause its durability decay, whatever duration they last. This study designs a closed-loop water management system to control the water content in a reasonable range which can not only avoid the faults of hydration and flooding but also improve the performance and durability of PEMFC. The proposed system introduces the measurement methodology based on the phase of single-frequency impedance, which corresponds numerically well with the water content. Moreover, two preferred operating conditions, cathode air stoichiometry and stack temperature, are adopted to regulate the water content with a trade-off between the time cost and power loss. The open-loop characteristics of water content on the temperature and air stoichiometry are studied to design the corresponding control strategy. Findings suggest that air stoichiometry is suitable for large regulation requirements of water content, while the temperature is suitable to meet small demands. Finally, the proposed closed-loop water management system is validated by experiments in variable-load and constant-load with disturbance situations. The results indicate that the proposed system effectively controls the water content within a 3% deviation from the desired value. Full article
(This article belongs to the Special Issue Advanced Studies for PEM Fuel Cells in Hydrogen-Fueled Vehicles)
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20 pages, 3278 KB  
Article
Experimental Validation of an Active Fault Tolerant Control Strategy Applied to a Proton Exchange Membrane Fuel Cell
by Etienne Dijoux, Nadia Yousfi Steiner, Michel Benne, Marie-Cécile Péra and Brigitte Grondin-Perez
Electrochem 2022, 3(4), 633-652; https://doi.org/10.3390/electrochem3040042 - 8 Oct 2022
Cited by 6 | Viewed by 2725
Abstract
Reliability of proton exchange membrane fuel cells (PEMFCs) is a major issue for large industrialization and commercialization. Indeed, performance can be degraded due to abnormal operating conditions, namely, faults, which lead either to a transient decay of the fuel cell performance or to [...] Read more.
Reliability of proton exchange membrane fuel cells (PEMFCs) is a major issue for large industrialization and commercialization. Indeed, performance can be degraded due to abnormal operating conditions, namely, faults, which lead either to a transient decay of the fuel cell performance or to permanent damage that cannot be recovered. The literature shows that long-time exposure to faults leads to fuel cell degradation. Therefore, it is necessary to use tools that can not only diagnose these faulty conditions, but also modify the fuel cell operations to recover a healthy operating point. For that purpose, one approach is the Active Fault Tolerant Control (AFTC) strategy which is composed of three functions. First, a diagnosis part allows fault detection and identification. Then a decision part, which is an algorithm aiming at finding a new operating point that mitigates the occurring fault. Finally, a control part applies the mitigation strategy established by the decision algorithm. The present work focuses on the decision part. and aims to bring a new contribution to PEMFCs reliability improvement and address water management issues, namely, the cell flooding and membrane drying out with the developed AFTC tool. The strategy is tested and validated on a single PEMFC cell and results are presented, analyzed, and discussed. Full article
(This article belongs to the Special Issue Feature Papers in Electrochemistry)
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14 pages, 4700 KB  
Article
Fault Diagnosis for PEMFC Water Management Subsystem Based on Learning Vector Quantization Neural Network and Kernel Principal Component Analysis
by Shuna Jiang, Qi Li, Rui Gan and Weirong Chen
World Electr. Veh. J. 2021, 12(4), 255; https://doi.org/10.3390/wevj12040255 - 4 Dec 2021
Cited by 8 | Viewed by 3233
Abstract
To solve the problem of water management subsystem fault diagnosis in a proton exchange membrane fuel cell (PEMFC) system, a novel approach based on learning vector quantization neural network (LVQNN) and kernel principal component analysis (KPCA) is proposed. In the proposed approach, the [...] Read more.
To solve the problem of water management subsystem fault diagnosis in a proton exchange membrane fuel cell (PEMFC) system, a novel approach based on learning vector quantization neural network (LVQNN) and kernel principal component analysis (KPCA) is proposed. In the proposed approach, the KPCA method is used for processing strongly coupled fault data with a high dimension to reduce the data dimension and to extract new low-dimensional fault feature data. The LVQNN method is used to carry out fault recognition using the fault feature data. The effectiveness of the proposed fault detection method is validated using the experimental data of the PEMFC power system. Results show that the proposed method can quickly and accurately diagnose the three health states: normal state, water flooding failure and membrane dry failure, and the recognition accuracy can reach 96.93%. Therefore, the method proposed in this paper is suitable for processing the fault data with a high dimension and abundant quantities, and provides a reference for the application of water management subsystem fault diagnosis of PEMFC. Full article
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