Recent Applications of Low-Carbon Cementitious Materials and Coatings

A special issue of Coatings (ISSN 2079-6412). This special issue belongs to the section "Architectural and Infrastructure Coatings".

Deadline for manuscript submissions: 31 March 2027 | Viewed by 1038

Editors


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Guest Editor
Department of Civil Engineering, School of Urban Construction, Wuhan University of Science and Technology, Wuhan 430065, China
Interests: low-carbon cementitious materials; calcium sulfoaluminate cement; ferroaluminate cement; utilization of solid waste

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Guest Editor
School of Qilu Transportation, Shandong University, Jinan 250100, China
Interests: low-carbon cementitious materials; geopolymer; utilization of solid waste
Special Issues, Collections and Topics in MDPI journals

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Guest Editor
Spanish National Research Council (CSIC), 28006 Madrid, Spain
Interests: low-carbon civil engineering materials; solid waste valorization; digital modeling and simulation for sustainable construction

Special Issue Information

Dear Colleagues,

The production of ordinary Portland cement (OPC) is responsible for nearly 8% of global CO2 emissions, driven by limestone calcination and high-temperature combustion. In response, low-carbon cementitious materials (LCCMs)—including alkali-activated materials (geopolymers), limestone calcined clay cements (LC3), CO2-solidified carbonate materials (CSCMs), calcium sulfoaluminate cement (CSA), and supersulfated cements (SSCs)—have emerged as promising alternatives. These systems drastically reduce or eliminate clinker by leveraging industrial by-products (e.g., fly ash, slag, metakaolin) or CO2-curing reactions. From a materials science perspective, LCCMs exhibit fundamentally different phase assemblages (e.g., N-A-S-H vs. C-S-H gels), pore structures, surface chemistries, and ion transport mechanisms compared to OPC. These differences profoundly influence not only bulk durability but also interfacial properties critical to coating performance.

While extensive research has focused on the mechanical and durability characteristics of LCCMs, their surface and near-surface behavior—which governs coating adhesion, barrier effectiveness, and long-term protection—remains significantly underexplored. This knowledge gap is the primary motivation for this Special Issue.

This Special Issue aims to bridge cement chemistry, surface science, and coating technology. By highlighting recent applications of LCCMs and their interactions with protective and functional coatings, we aim to advance durable, sustainable, and fit-for-purpose construction solutions. Contributions addressing interfacial characterization, novel coating formulations, long-term performance, and life-cycle assessment are particularly welcome.

The scope of this Special Issue includes, but is not limited to, the following topics:

  • Alkali-activated materials (geopolymers);
  • Limestone calcined clay cements (LC3);
  • CO2-solidified carbonate materials (CSCM);
  • Calcium sulfoaluminate cement (CSA);
  • Supersulfated cements (SSC);
  • Other low-carbon cementitious materials (LCCMs).

We look forward to receiving your contributions.

Dr. Yishun Liao
Prof. Dr. Yifeng Ling
Dr. Yibing Zuo
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 250 words) can be sent to the Editorial Office for assessment.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-anonymized peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Coatings is an international peer-reviewed open access monthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2600 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • low-carbon cementitious materials for coatings
  • rapid-setting cementitious materials for coatings
  • ultra-high-strength cementitious materials for coatings
  • 3D printing of cementitious materials for coatings
  • coating materials under extreme environments

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Published Papers (1 paper)

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Review

43 pages, 3624 KB  
Review
Fiber–Matrix Interface Engineering in Cementitious Composites: Surface Modification, Durability and Emerging Trends
by Adriano Galvão Souza Azevedo, Katheryn Cecilia Pallares Córdoba, Juan Camilo Adrada Molano and Holmer Savastano
Coatings 2026, 16(8), 922; https://doi.org/10.3390/coatings16080922 - 3 Aug 2026
Viewed by 809
Abstract
Fiber-reinforced cementitious composites have become increasingly important in the development of durable and sustainable construction materials, particularly following the replacement of asbestos-based reinforcements. However, the long-term performance of these composites is strongly influenced by the characteristics of the fiber–matrix interface, where moisture transport, [...] Read more.
Fiber-reinforced cementitious composites have become increasingly important in the development of durable and sustainable construction materials, particularly following the replacement of asbestos-based reinforcements. However, the long-term performance of these composites is strongly influenced by the characteristics of the fiber–matrix interface, where moisture transport, interfacial degradation, and stress transfer mechanisms govern durability and mechanical behavior. Consequently, considerable efforts have been devoted to developing surface engineering strategies capable of improving fiber–matrix compatibility and enhancing composite performance. This review examines recent advances in surface modification and interfacial engineering approaches applied to fiber-reinforced cementitious composites. The discussion covers fiber–matrix bonding mechanisms and the main modification strategies, including alkali treatments, hornification, silane coupling agents, polymeric and hydrophobic coatings, nanomaterial-assisted modifications, and carbonation-induced surface engineering. The effects of these approaches on interfacial properties, durability, dimensional stability, and mechanical performance are critically assessed. The literature indicates that treatments combining surface chemistry modification, moisture control, and mineral-based densification provide more consistent improvements in durability than single-mechanism approaches. Future developments are expected to focus on scalable treatment methods, low-carbon cementitious systems, and advanced materials design strategies, enabling the development of next-generation fiber cement composites with enhanced durability, sustainability, and long-term performance. Full article
(This article belongs to the Special Issue Recent Applications of Low-Carbon Cementitious Materials and Coatings)
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