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Keywords = radiation of ultrafast laser

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13 pages, 11188 KB  
Article
Two-Way Shape Memory Effect Driven Solar Sails for Active Solar Radiation Pressure Modulation
by Peidong Jia, Ruilei Chen, Zhongjing Ren, Chengyang Li, Zizhan Tu, Boyang Jiang, Xu Zhang, Ziran Wang, Dakai Liu and Erchao Li
Aerospace 2026, 13(1), 14; https://doi.org/10.3390/aerospace13010014 - 24 Dec 2025
Viewed by 243
Abstract
Solar sailing has proven to be an effective solution for cost-effective and long-term space missions due to its fuel-free propulsion. While multiple large-scale solar sails based on kilogram-class satellites have been developed and tested in space, solar sails created for lightweight chip-scale satellites [...] Read more.
Solar sailing has proven to be an effective solution for cost-effective and long-term space missions due to its fuel-free propulsion. While multiple large-scale solar sails based on kilogram-class satellites have been developed and tested in space, solar sails created for lightweight chip-scale satellites are much less. To enable the gram-class satellite of solar sailing for active attitude adjustment and orbital maneuvers, a novel solar sail driven by two-way shape memory effect (TWSME) was proposed in this work. The solar sail base was made of rectangular Al-Kapton thin films, while a U-shaped NiTi beam was developed by 50 μm thin Ni50.6Ti49.4 foils. Both of the U-shaped NiTi beam and rectangular Al-Kapton thin films were manufactured by the ultra-fast femtosecond laser cutting machine. Finite element modeling of single U-shaped NiTi beam and assembled solar sail were built to validate that an 80 mm-long TWSME NiTi beam with a curvature of 37.31 m−1 were sufficient to drive the solar sail for solar radiation pressure modulation. A solar sail prototype was developed, and an in situ experiment test of the prototype was conducted with infrared imaging, showing efficient bending behaviors by application of a 0.5 A direct current across the U-shape NiTi beam. These findings reveal that U-shaped TWSME NiTi foils provide an effective driving strategy for lightweight chip-scale satellites, and thus dramatically broaden the space application of the gram-scale satellite. Full article
(This article belongs to the Section Astronautics & Space Science)
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16 pages, 11356 KB  
Article
Extraction of Electron and Hole Drift Velocities in Thin 4H-SiC PIN Detectors Using High-Frequency Readout Electronics
by Andreas Gsponer, Sebastian Onder, Stefan Gundacker, Jürgen Burin, Matthias Knopf, Daniel Radmanovac, Simon Waid and Thomas Bergauer
Sensors 2025, 25(23), 7196; https://doi.org/10.3390/s25237196 - 25 Nov 2025
Viewed by 441
Abstract
Silicon carbide (SiC) has been widely adopted in the semiconductor industry, particularly in power electronics, because of its high temperature stability, high breakdown field, and fast switching speeds. Its wide bandgap makes it an interesting candidate for radiation-hard particle detectors in high-energy physics [...] Read more.
Silicon carbide (SiC) has been widely adopted in the semiconductor industry, particularly in power electronics, because of its high temperature stability, high breakdown field, and fast switching speeds. Its wide bandgap makes it an interesting candidate for radiation-hard particle detectors in high-energy physics and medical applications. Furthermore, the high electron and hole drift velocities in 4H-SiC enable devices suitable for ultra-fast particle detection and timing applications. However, currently, the front-end readout electronics used for 4H-SiC detectors constitute a bottleneck in investigations of the charge carrier drift. To address these limitations, a high-frequency readout board with an intrinsic bandwidth of 10 GHz was developed. With this readout, the transient current signals of a 4H-SiC diode with a diameter of 141 μm and a thickness of 50 μm upon UV laser, alpha particle, and high-energy proton beam excitation were recorded. In all three cases, the electron and hole drift can clearly be separated, which enables the extraction of the charge carrier drift velocities as a function of the electric field. These velocities, directly measured for the first time, provide a valuable comparison to Monte Carlo-simulated literature values and constitute an essential input for TCAD simulations. Finally, a complete simulation environment combining TCAD, the Allpix2 framework, and SPICE simulations is presented, which is in good agreement with the measured data. Full article
(This article belongs to the Section Physical Sensors)
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20 pages, 7163 KB  
Article
Glass-Forming Ionic Liquid Crystal Gold–Carbon Nanocomposites with Ultrafast Optical Nonlinearity Sign Reversal
by Valentyn Rudenko, Anatolii Tolochko, Svitlana Bugaychuk, Dmytro Zhulai, Gertruda Klimusheva, Galina Yaremchuk, Tatyana Mirnaya and Yuriy Garbovskiy
J. Compos. Sci. 2025, 9(9), 472; https://doi.org/10.3390/jcs9090472 - 2 Sep 2025
Viewed by 1495
Abstract
The development of new types of nanocomposites capable of manipulating light is critical for various modern photonics applications. Recently, we proposed the use of overlooked glass-forming ionic liquid crystals made of cadmium octanoate containing gold, carbon, or both carbon and gold nanoparticles as [...] Read more.
The development of new types of nanocomposites capable of manipulating light is critical for various modern photonics applications. Recently, we proposed the use of overlooked glass-forming ionic liquid crystals made of cadmium octanoate containing gold, carbon, or both carbon and gold nanoparticles as promising optical and nonlinear optical materials. These were characterized using nanosecond laser pulses at a wavelength of 532 nm. In this paper, femtosecond radiation at different wavelengths (600 nm and 800 nm) is employed to study ultrafast electronic nonlinear optical processes in mesomorphic glass nanocomposites. The observed nonlinear optical response probed at the femtosecond time scale dramatically differs from that at the nanosecond time scale reported previously. The intensity-dependent effective nonlinear absorption coefficient of all studied samples remains positive due to the dominant reverse saturable absorption effect, while the nonlinear refractive index exhibits a sign reversal depending on the intensity and wavelength of laser pulses. The strategy for producing glass-forming ionic liquid crystal gold–carbon nanocomposites with an ultrafast nonlinear optical response is of high interest for modern applications in advanced photonics, and it can also be applied to other types of glass-forming metal alkanoates and nanomaterials. Full article
(This article belongs to the Special Issue Recent Progress in Hybrid Composites)
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42 pages, 5853 KB  
Review
Harnessing Ultra-Intense Long-Wave Infrared Lasers: New Frontiers in Fundamental and Applied Research
by Igor V. Pogorelsky and Mikhail N. Polyanskiy
Photonics 2025, 12(3), 221; https://doi.org/10.3390/photonics12030221 - 28 Feb 2025
Cited by 2 | Viewed by 2505 | Correction
Abstract
This review explores two main topics: the state-of-the-art and emerging capabilities of high-peak-power, ultrafast (picosecond and femtosecond) long-wave infrared (LWIR) laser technology based on CO2 gas laser amplifiers, and the current and advanced scientific applications of this laser class. The discussion is [...] Read more.
This review explores two main topics: the state-of-the-art and emerging capabilities of high-peak-power, ultrafast (picosecond and femtosecond) long-wave infrared (LWIR) laser technology based on CO2 gas laser amplifiers, and the current and advanced scientific applications of this laser class. The discussion is grounded in expertise gained at the Accelerator Test Facility (ATF) of Brookhaven National Laboratory (BNL), a leading center for ultrafast, high-power CO2 laser development and a National User Facility with a strong track record in high-intensity physics experiments. We begin by reviewing the status of 9–10 μm CO2 laser technology and its applications, before exploring potential breakthroughs, including the realization of 100 terawatt femtosecond pulses. These advancements will drive ongoing research in electron and ion acceleration in plasma, along with applications in secondary radiation sources and atmospheric energy transport. Throughout the review, we highlight how wavelength scaling of physical effects enhances the capabilities of ultra-intense lasers in the LWIR spectrum, expanding the frontiers of both fundamental and applied science. Full article
(This article belongs to the Special Issue High-Power Ultrafast Lasers: Development and Applications)
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13 pages, 2725 KB  
Article
Scintillation Properties of β-Ga2O3 Under the Excitation of Ultra-High-Charge Electron Bunches
by Yulan Liang, Jianhan Sun, Chaoyi Zhang, Tianqi Xu, Haoran Chen, Huaqing Huang, Chenhao Hua, Pengying Wan, Chuanwei Dai, Qingfan Wu, Juntao Liu, Lin Huang, Lin Lin, Huili Tang, Jianming Xue, Jun Xu, Senlin Huang, Bo Liu and Wenjun Ma
Photonics 2025, 12(2), 149; https://doi.org/10.3390/photonics12020149 - 12 Feb 2025
Cited by 1 | Viewed by 1339
Abstract
The performance of ultrafast scintillators under ultrahigh dose rate is highly important for applications utilizing brilliant radiation sources. In this work, the scintillation properties of β-Ga2O3, a high-performance ultrafast wide-bandgap semiconductor scintillator, are systematically investigated under dose rates of [...] Read more.
The performance of ultrafast scintillators under ultrahigh dose rate is highly important for applications utilizing brilliant radiation sources. In this work, the scintillation properties of β-Ga2O3, a high-performance ultrafast wide-bandgap semiconductor scintillator, are systematically investigated under dose rates of 107 to 109 Gy/s for the first time by employing ultrashort high-charge electron bunches (bunch charge from 500 fC to 50 pC) generated from a superconducting radio-frequency accelerator. Our results show that in spite of the ultrahigh dose rate, the scintillation intensity was still linearly proportional to the electron bunch charge. Lifetime analysis reveals a fast decay component ranging from 3 to 4 ns, along with an average lifetime of 20 ns. These findings establish a solid foundation for the application of β-Ga2O3 as the scintillation material for high-charge electron sources such as laser-wakefield accelerated electrons. Full article
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28 pages, 10257 KB  
Article
Thomson Scattering and Radiation Reaction from a Laser-Driven Electron
by Ignacio Pastor, Luis Roso, Ramón F. Álvarez-Estrada and Francisco Castejón
Photonics 2024, 11(10), 971; https://doi.org/10.3390/photonics11100971 - 17 Oct 2024
Viewed by 2284
Abstract
We investigate the dynamics of electrons initially counter-propagating to an ultra-fast ultra-intense near-infrared laser pulse using a model for radiation reaction based on the classical Landau–Lifshitz–Hartemann equation. The electrons, with initial energies of 1 GeV, interact with laser fields of up to [...] Read more.
We investigate the dynamics of electrons initially counter-propagating to an ultra-fast ultra-intense near-infrared laser pulse using a model for radiation reaction based on the classical Landau–Lifshitz–Hartemann equation. The electrons, with initial energies of 1 GeV, interact with laser fields of up to 1023 W/cm2. The radiation reaction effects slow down the electrons and significantly alter their trajectories, leading to distinctive Thomson scattering spectra and radiation patterns. It is proposed to use such spectra, which include contributions from harmonic and Doppler-shifted radiation, as a tool to measure laser intensity at focus. We discuss the feasibility of this approach for state-of-the-art and near-future laser technologies. We propose using Thomson scattering to measure the impact of radiation reaction on electron dynamics, thereby providing experimental scenarios for validating our model. This work aims to contribute to the understanding of electron behavior in ultra-intense laser fields and the role of radiation reaction in such extreme conditions. The specific properties of Thomson scattering associated with radiation reaction, shown to be dominant at the intensities of interest here, are highlighted and proposed as a diagnostic tool, both for this phenomenon itself and for laser characterization in a non-intrusive way. Full article
(This article belongs to the Special Issue Extreme Lasers)
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11 pages, 3470 KB  
Article
The EuAPS Betatron Radiation Source: Status Update and Photon Science Perspectives
by Federico Galdenzi, Maria Pia Anania, Antonella Balerna, Richard J. Bean, Angelo Biagioni, Claudio Bortolin, Luca Brombal, Francesco Brun, Marcello Coreno, Gemma Costa, Lucio Crincoli, Alessandro Curcio, Martina Del Giorno, Enrico Di Pasquale, Gianluca di Raddo, Valentina Dompè, Sandro Donato, Zeinab Ebrahimpour, Antonio Falone, Andrea Frazzitta, Mario Galletti, Andrea Ghigo, Stefano Lauciani, Andrea Liedl, Valerio Lollo, Augusto Marcelli, Emiliano Principi, Andrea R. Rossi, Federica Stocchi, Fabio Villa, Marco Zottola, Alessandro Cianchi, Francesco Stellato and Massimo Ferrarioadd Show full author list remove Hide full author list
Condens. Matter 2024, 9(3), 30; https://doi.org/10.3390/condmat9030030 - 22 Jul 2024
Cited by 2 | Viewed by 2164
Abstract
The EuPRAXIA EU project is at the forefront of advancing particle accelerator research and the development of photon sources through innovative plasma acceleration approaches. Within this framework, the EuAPS project aims to exploit laser wakefield acceleration to build and operate a betatron radiation [...] Read more.
The EuPRAXIA EU project is at the forefront of advancing particle accelerator research and the development of photon sources through innovative plasma acceleration approaches. Within this framework, the EuAPS project aims to exploit laser wakefield acceleration to build and operate a betatron radiation source at the INFN Frascati National Laboratory. The EuAPS source will provide femtosecond X-ray pulses in the spectral region between about 1 and 10 keV, unlocking a realm of experimental ultrafast methodologies encompassing diverse imaging and X-ray spectroscopy techniques. This paper presents a description of the EuAPS betatron source, including simulations of the photon beam parameters, outlines the preliminary design of the dedicated photon beamline, and provides an insightful overview of its photon science applications. Full article
(This article belongs to the Section Spectroscopy and Imaging in Condensed Matter)
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10 pages, 2954 KB  
Communication
Polarization-Dependent Formation of Extremely Compressed Femtosecond Wave Packets and Supercontinuum Generation in Fused Silica
by Ilia Geints and Olga Kosareva
Photonics 2024, 11(7), 620; https://doi.org/10.3390/photonics11070620 - 28 Jun 2024
Cited by 1 | Viewed by 1267
Abstract
Previous studies of formation of extremely compressed wave packets during femtosecond filamentation in the region of anomalous group velocity dispersion in solid dielectrics mostly considered the case of linearly polarized laser pulses. However, recent results suggest potential applications of polarization state manipulation for [...] Read more.
Previous studies of formation of extremely compressed wave packets during femtosecond filamentation in the region of anomalous group velocity dispersion in solid dielectrics mostly considered the case of linearly polarized laser pulses. However, recent results suggest potential applications of polarization state manipulation for ultrafast laser writing of optical structures in bulk solid-state media. In the present work, evolution of radiation polarization parameters during formation of such extreme wave packets at the pump wavelength of 1900 nm in fused silica is studied numerically on the basis of the carrier-resolved unidirectional pulse propagation equation (UPPE). It was revealed that initial close-to-circular polarization leads to higher intensity of the anti-Stokes wing in the spectrum of the generated supercontinuum. Numerical simulations indicate a complex, space–time variant polarization state, and the resulting spatiotemporal electric field distribution exhibits a strong dependence on the initial polarization of the femtosecond pulse. At the same time, electric field polarization tends to linear one in the region with the highest field strength regardless of the initial parameters. The origin of this behavior is attributed to the properties of the supercontinuum components generation during filament-induced plasma formation. Full article
(This article belongs to the Special Issue Ultrafast Intense Laser Filamentation and Beyond)
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11 pages, 1993 KB  
Article
Thermal Lattice Field during Ultra-Short Laser Pulse Irradiation of Metal Targets: A Fokker–Planck Analytical Model
by Sinziana-Andreea Anghel, Mihai Oane, Cristian N. Mihăilescu, Bogdan A. Sava, Mihail Elişa, Natalia Mihăilescu, Dorina Ticoş, Alexandra M. I. Trefilov, Carmen Ristoscu, Ana V. Filip and Ion N. Mihăilescu
Metals 2023, 13(10), 1775; https://doi.org/10.3390/met13101775 - 20 Oct 2023
Cited by 3 | Viewed by 2028
Abstract
The ultrafast fs laser pulse heating of thin metal films is studied for the first time using the two-temperature model on the basis of the Fokker–Planck formalism. The incident laser radiation is multi-modal, while the electron temperature is described during the first 2 [...] Read more.
The ultrafast fs laser pulse heating of thin metal films is studied for the first time using the two-temperature model on the basis of the Fokker–Planck formalism. The incident laser radiation is multi-modal, while the electron temperature is described during the first 2 fs. The predictions are intended for use by experimentalists in optoelectronics, photonics, laser processing, electronics, and bio- and nanomedicine. The crucial role of the nano-sized spatial dimensions of the metal sample is highlighted. A significant result of this study is the interdependence between the target’s size, the phonon/lattice characteristics, and the coefficient β (the quotient of non-diffusive phenomena), which varies between zero (pure diffusive case) and one (pure non-diffusive case). Full article
(This article belongs to the Section Computation and Simulation on Metals)
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13 pages, 4712 KB  
Article
Surface Conditions after LASER Shock Peening of Steel and Aluminum Alloys Using Ultrafast Laser Pulses
by Jan Schubnell, Eva-Regine Carl, Ardeshir Sarmast, Manuel Hinterstein, Johannes Preußner, Marco Seifert, Christoph Kaufmann, Peter Rußbüldt and Jan Schulte
Materials 2023, 16(20), 6769; https://doi.org/10.3390/ma16206769 - 19 Oct 2023
Cited by 7 | Viewed by 1963
Abstract
Laser shock peening (LSP) is a mechanical surface treatment process to modify near-surface material properties. Compared to conventional shot peening (SP) the process parameters can be finely adjusted with greater precision and a higher penetration depth of compressive residual stresses could be reached. [...] Read more.
Laser shock peening (LSP) is a mechanical surface treatment process to modify near-surface material properties. Compared to conventional shot peening (SP) the process parameters can be finely adjusted with greater precision and a higher penetration depth of compressive residual stresses could be reached. However, high process times of LSP leads to high production costs. In this study, ultrafast LSP (U-LSP) with an ultrafast laser source (pulse time in the picosecond range) was applied on specimens made of X5CrNiCu15-5 and AlZnMgCu1.5. The surface characteristics (surface roughness) and surface-near properties (microstructure, residual stresses, and phase composition) were compared to the as-delivered condition, to conventional laser shock peening (C-LSP), and to SP, whereas metallographic analyses and X-ray and synchrotron radiation techniques were used. The process time was significantly lower via U-LSP compared to C-LSP. For X5CrNiCu15-5, no significant compressive residual stresses were induced via U-LSP. However, for AlZnMgCu1.5, similar compressive residual stresses were reached via C-LSP and U-LSP; however, with a lower penetration depth. A change in the phase portions in the surface layer of X5CrNiCu15-5 after C-LSP compared to SP were determined. Full article
(This article belongs to the Special Issue Advances in Laser Materials and Processing Technologies)
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12 pages, 745 KB  
Article
Valley-Selective High Harmonic Generation and Polarization Induced by an Orthogonal Two-Color Laser Field
by Xi Liu, Dongdong Liu, Yan Sun, Yujie Li and Cui Zhang
Photonics 2023, 10(10), 1126; https://doi.org/10.3390/photonics10101126 - 8 Oct 2023
Cited by 12 | Viewed by 2236
Abstract
The valley pseudospin properties of electrons in two-dimensional hexagonal materials result in many fascinating physical phenomena, which opens up the new field of valleytronics. The valley-contrasting physics aims at distinguishing the valley degree of freedom based on valley-dependent effects. Here, we theoretically demonstrate [...] Read more.
The valley pseudospin properties of electrons in two-dimensional hexagonal materials result in many fascinating physical phenomena, which opens up the new field of valleytronics. The valley-contrasting physics aims at distinguishing the valley degree of freedom based on valley-dependent effects. Here, we theoretically demonstrate that both of the valley-selective high harmonic generation and valley-selective electronic excitation can be achieved by using an orthogonal two-color (OTC) laser field in gapped graphene. It is shown that the asymmetry degrees of harmonic yields in the plateaus, cutoff energies of generated harmonics and electron populations from two different valleys can be precisely controlled by the relative phase of the OTC laser field. Thus, the selectivity of the dominant valley for the harmonic radiation and electronic polarization can be switched by adjusting the relative phase of the OTC laser field. Our work offers an all-optical route to produce the valley-resolved high harmonic emissions and manipulate the ultrafast valley polarization on a femtosecond timescale in condensed matter. Full article
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25 pages, 4830 KB  
Review
Semiconductor Characterization by Terahertz Excitation Spectroscopy
by Arūnas Krotkus, Ignas Nevinskas and Ričardas Norkus
Materials 2023, 16(7), 2859; https://doi.org/10.3390/ma16072859 - 3 Apr 2023
Cited by 9 | Viewed by 4226
Abstract
Surfaces of semiconducting materials excited by femtosecond laser pulses emit electromagnetic waves in the terahertz (THz) frequency range, which by definition is the 0.1–10 THz region. The nature of terahertz radiation pulses is, in the majority of cases, explained by the appearance of [...] Read more.
Surfaces of semiconducting materials excited by femtosecond laser pulses emit electromagnetic waves in the terahertz (THz) frequency range, which by definition is the 0.1–10 THz region. The nature of terahertz radiation pulses is, in the majority of cases, explained by the appearance of ultrafast photocurrents. THz pulse duration is comparable with the photocarrier momentum relaxation time, thus such hot-carrier effects as the velocity overshoot, ballistic carrier motion, and optical carrier alignment must be taken into consideration when explaining experimental observations of terahertz emission. Novel commercially available tools such as optical parametric amplifiers that are capable of generating femtosecond optical pulses within a wide spectral range allow performing new unique experiments. By exciting semiconductor surfaces with various photon energies, it is possible to look into the ultrafast processes taking place at different electron energy levels of the investigated materials. The experimental technique known as the THz excitation spectroscopy (TES) can be used as a contactless method to study the band structure and investigate the ultrafast processes of various technologically important materials. A recent decade of investigations with the THz excitation spectroscopy method is reviewed in this article. TES experiments performed on the common bulk A3B5 compounds such as the wide-gap GaAs, and narrow-gap InAs and InSb, as well as Ge, Te, GaSe and other bulk semiconductors are reviewed. Finally, the results obtained by this non-contact technique on low-dimensional materials such as ultrathin mono-elemental Bi films, InAs, InGaAs, and GaAs nanowires are also presented. Full article
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10 pages, 2210 KB  
Article
Terahertz Emission Spectroscopy of Ultrafast Coupled Spin and Charge Dynamics in Nanometer Ferromagnetic Heterostructures
by Zhangshun Li, Yexin Jiang, Zuanming Jin, Zhuoyi Li, Xianyang Lu, Zhijiang Ye, Jin-Yi Pang, Yongbing Xu and Yan Peng
Nanomaterials 2022, 12(23), 4267; https://doi.org/10.3390/nano12234267 - 30 Nov 2022
Cited by 6 | Viewed by 3312
Abstract
Due to its high sensitivity and because it does not rely on the magneto-optical response, terahertz (THz) emission spectroscopy has been used as a powerful time-resolved tool for investigating ultrafast demagnetization and spin current dynamics in nanometer-thick ferromagnetic (FM)/heavy metal (HM) heterostructures. Here, [...] Read more.
Due to its high sensitivity and because it does not rely on the magneto-optical response, terahertz (THz) emission spectroscopy has been used as a powerful time-resolved tool for investigating ultrafast demagnetization and spin current dynamics in nanometer-thick ferromagnetic (FM)/heavy metal (HM) heterostructures. Here, by changing the order of the conductive HM coating on the FM nanometer film, the dominant electric dipole contribution to the laser-induced THz radiation can be unraveled from the ultrafast magnetic dipole. Furthermore, to take charge equilibration into account, we separate the femtosecond laser-induced spin-to-charge converted current and the instantaneous discharging current within the illuminated area. The THz emission spectroscopy gives us direct information into the coupled spin and charge dynamics during the first moments of the light–matter interaction. Our results also open up new perspectives to manipulate and optimize the ultrafast charge current for promising high-performance and broadband THz radiation. Full article
(This article belongs to the Section Nanophotonics Materials and Devices)
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11 pages, 1965 KB  
Article
High Responsivity Vacuum Nano-Photodiode Using Single-Crystal CsPbBr3 Micro-Sheet
by Xiangjun Zeng, Shasha Li, Zairan Liu, Yang Chen, Jun Chen, Shaozhi Deng, Fei Liu and Juncong She
Nanomaterials 2022, 12(23), 4205; https://doi.org/10.3390/nano12234205 - 26 Nov 2022
Cited by 4 | Viewed by 2593
Abstract
Field electron emission vacuum photodiode is promising for converting free-space electromagnetic radiation into electronic signal within an ultrafast timescale due to the ballistic electron transport in its vacuum channel. However, the low photoelectric conversion efficiency still hinders the popularity of vacuum photodiode. Here, [...] Read more.
Field electron emission vacuum photodiode is promising for converting free-space electromagnetic radiation into electronic signal within an ultrafast timescale due to the ballistic electron transport in its vacuum channel. However, the low photoelectric conversion efficiency still hinders the popularity of vacuum photodiode. Here, we report an on-chip integrated vacuum nano-photodiode constructed from a Si-tip anode and a single-crystal CsPbBr3 cathode with a nano-separation of ~30 nm. Benefiting from the nanoscale vacuum channel and the high surface work function of the CsPbBr3 (4.55 eV), the vacuum nano-photodiode exhibits a low driving voltage of 15 V with an ultra-low dark current (50 pA). The vacuum nano-photodiode demonstrates a high photo responsivity (1.75 AW−1@15 V) under the illumination of a 532-nm laser light. The estimated external quantum efficiency is up to 400%. The electrostatic field simulation indicates that the CsPbBr3 cathode can be totally depleted at an optimal thickness. The large built-in electric field in the depletion region facilitates the dissociation of photoexcited electron–hole pairs, leading to an enhanced photoelectric conversion efficiency. Moreover, the voltage drop in the vacuum channel increases due to the photoconductive effect, which is beneficial to the narrowing of the vacuum barrier for more efficient electron tunneling. This device shows great promise for the development of highly sensitive perovskite-based vacuum opto-electronics. Full article
(This article belongs to the Special Issue The Research Related to Nanomaterial Cold Cathode)
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13 pages, 4059 KB  
Article
Coherent XUV Multispectral Diffraction Imaging in the Microscale
by Stylianos Petrakis, Alexandros Skoulakis, Yannis Orphanos, Anastasios Grigoriadis, Georgia Andrianaki, Dimitrios Louloudakis, Nathanail Kortsalioudakis, Athanasios Tsapras, Costas Balas, Dimitrios Zouridis, Efthymios Pachos, Makis Bakarezos, Vasilios Dimitriou, Michael Tatarakis, Emmanouil P. Benis and Nektarios A. Papadogiannis
Appl. Sci. 2022, 12(20), 10592; https://doi.org/10.3390/app122010592 - 20 Oct 2022
Cited by 1 | Viewed by 2793
Abstract
The rapid growth of nanotechnology has increased the need for fast nanoscale imaging. X-ray free electron laser (XFEL) facilities currently provide such coherent sources of directional and high-brilliance X-ray radiation. These facilities require large financial investments for development, maintenance, and manpower, and thus, [...] Read more.
The rapid growth of nanotechnology has increased the need for fast nanoscale imaging. X-ray free electron laser (XFEL) facilities currently provide such coherent sources of directional and high-brilliance X-ray radiation. These facilities require large financial investments for development, maintenance, and manpower, and thus, only a few exist worldwide. In this article, we present an automated table-top system for XUV coherent diffraction imaging supporting the capabilities for multispectral microscopy at high repetition rates, based on laser high harmonic generation from gases. This prototype system aims towards the development of an industrial table-top system of ultrafast soft X-ray multi-spectral microscopy imaging for nanostructured materials with enormous potential and a broad range of applications in current nanotechnologies. The coherent XUV radiation is generated in a semi-infinite gas cell via the high harmonic generation of the near-infrared femtosecond laser pulses. The XUV spectral selection is performed by specially designed multilayer XUV mirrors that do not affect the XUV phase front and pulse duration. Full article
(This article belongs to the Section Optics and Lasers)
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