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Keywords = magnetorheological elastomer device

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62 pages, 4192 KiB  
Review
Advancements in Magnetorheological Foams: Composition, Fabrication, AI-Driven Enhancements and Emerging Applications
by Hesamodin Khodaverdi and Ramin Sedaghati
Polymers 2025, 17(14), 1898; https://doi.org/10.3390/polym17141898 - 9 Jul 2025
Viewed by 709
Abstract
Magnetorheological (MR) foams represent a class of smart materials with unique tunable viscoelastic properties when subjected to external magnetic fields. Combining porous structures with embedded magnetic particles, these materials address challenges such as leakage and sedimentation, typically encountered in conventional MR fluids while [...] Read more.
Magnetorheological (MR) foams represent a class of smart materials with unique tunable viscoelastic properties when subjected to external magnetic fields. Combining porous structures with embedded magnetic particles, these materials address challenges such as leakage and sedimentation, typically encountered in conventional MR fluids while offering advantages like lightweight design, acoustic absorption, high energy harvesting capability, and tailored mechanical responses. Despite their potential, challenges such as non-uniform particle dispersion, limited durability under cyclic loads, and suboptimal magneto-mechanical coupling continue to hinder their broader adoption. This review systematically addresses these issues by evaluating the synthesis methods (ex situ vs. in situ), microstructural design strategies, and the role of magnetic particle alignment under varying curing conditions. Special attention is given to the influence of material composition—including matrix types, magnetic fillers, and additives—on the mechanical and magnetorheological behaviors. While the primary focus of this review is on MR foams, relevant studies on MR elastomers, which share fundamental principles, are also considered to provide a broader context. Recent advancements are also discussed, including the growing use of artificial intelligence (AI) to predict the rheological and magneto-mechanical behavior of MR materials, model complex device responses, and optimize material composition and processing conditions. AI applications in MR systems range from estimating shear stress, viscosity, and storage/loss moduli to analyzing nonlinear hysteresis, magnetostriction, and mixed-mode loading behavior. These data-driven approaches offer powerful new capabilities for material design and performance optimization, helping overcome long-standing limitations in conventional modeling techniques. Despite significant progress in MR foams, several challenges remain to be addressed, including achieving uniform particle dispersion, enhancing viscoelastic performance (storage modulus and MR effect), and improving durability under cyclic loading. Addressing these issues is essential for unlocking the full potential of MR foams in demanding applications where consistent performance, mechanical reliability, and long-term stability are crucial for safety, effectiveness, and operational longevity. By bridging experimental methods, theoretical modeling, and AI-driven design, this work identifies pathways toward enhancing the functionality and reliability of MR foams for applications in vibration damping, energy harvesting, biomedical devices, and soft robotics. Full article
(This article belongs to the Section Polymer Composites and Nanocomposites)
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22 pages, 9995 KiB  
Article
Skin-Inspired Magnetoresistive Tactile Sensor for Force Characterization in Distributed Areas
by Francisco Mêda, Fabian Näf, Tiago P. Fernandes, Alexandre Bernardino, Lorenzo Jamone, Gonçalo Tavares and Susana Cardoso
Sensors 2025, 25(12), 3724; https://doi.org/10.3390/s25123724 - 13 Jun 2025
Cited by 1 | Viewed by 856
Abstract
Touch is a crucial sense for advanced organisms, particularly humans, as it provides essential information about the shape, size, and texture of contacting objects. In robotics and automation, the integration of tactile sensors has become increasingly relevant, enabling devices to properly interact with [...] Read more.
Touch is a crucial sense for advanced organisms, particularly humans, as it provides essential information about the shape, size, and texture of contacting objects. In robotics and automation, the integration of tactile sensors has become increasingly relevant, enabling devices to properly interact with their environment. This study aimed to develop a biomimetic, skin-inspired tactile sensor device capable of sensing applied force, characterizing it in three dimensions, and determining the point of application. The device was designed as a 4 × 4 matrix of tunneling magnetoresistive sensors, which provide a higher sensitivity in comparison to the ones based on the Hall effect, the current standard in tactile sensors. These detect magnetic field changes along a single axis, wire-bonded to a PCB and encapsulated in epoxy. This sensing array detects the magnetic field from an overlayed magnetorheological elastomer composed of Ecoflex and 5 µm neodymium–iron–boron ferromagnetic particles. Structural integrity tests showed that the device could withstand forces above 100 N, with an epoxy coverage of 0.12 mL per sensor chip. A 3D movement stage equipped with an indenting tip and force sensor was used to collect device data, which was then used to train neural network models to predict the contact location and 3D magnitude of the applied force. The magnitude-sensing model was trained on 31,260 data points, being able to accurately characterize force with a mean absolute error ranging between 0.07 and 0.17 N. The spatial sensitivity model was trained on 171,008 points and achieved a mean absolute error of 0.26 mm when predicting the location of applied force within a sensitive area of 25.5 mm × 25.5 mm using sensors spaced 4.5 mm apart. For points outside the testing range, the mean absolute error was 0.63 mm. Full article
(This article belongs to the Special Issue Smart Magnetic Sensors and Application)
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24 pages, 6799 KiB  
Article
Design and Analysis of Combined Vibration Absorbers for Ship Propulsion Shaft Systems
by Dongdong Luo, Qing Ouyang and Hongsheng Hu
Actuators 2025, 14(1), 41; https://doi.org/10.3390/act14010041 - 20 Jan 2025
Viewed by 1124
Abstract
The vibration of a ship’s propulsion shaft system directly affects the ship’s lifespan, and many studies have designed vibration absorbers only for one of the natural frequencies of a ship’s propulsion shaft system without considering the influence of multiple low-order resonance frequencies. In [...] Read more.
The vibration of a ship’s propulsion shaft system directly affects the ship’s lifespan, and many studies have designed vibration absorbers only for one of the natural frequencies of a ship’s propulsion shaft system without considering the influence of multiple low-order resonance frequencies. In this paper, a vibration absorber combined with a magnetorheological elastomer vibration absorber and a rubber vibration absorber in series is designed, and it can cover two torsional natural frequency band ranges to achieve better vibration reduction performances in multiple different torsional natural frequencies. The torsional natural frequency of the propulsion shafting of a 45 m fishing vessel is determined based on a multiple-degrees-of-freedom equivalent discretization model. Two natural frequencies, 22.4 Hz and 131.4 Hz, of a ship propulsion shaft system are selected as the design goal parameters of the combined vibration absorber. The magnetic field is simulated to ensure that the magnetic field generated by an energized coil can meet requirements. Then, a dynamic simulation of the ship propulsion shaft system with a combined vibration absorber is conducted via co-simulation. Afterward, the device is installed on the intermediate shaft of the ship propulsion shaft system for simulation, and the vibration reduction effect of the device is analyzed at different frequencies by controlling the current. When the device is controlled to operate at the optimal frequency point, the results show that the angular acceleration vibration amplitude reduction around the first and third torsional natural frequencies of the propulsion shaft system reaches 90% and 18%, respectively. This study provides new ideas for the intelligent and controllable vibration damping of ship propulsion shaft systems, especially for the development trend of intelligent ship equipment under complex working conditions. Full article
(This article belongs to the Section Control Systems)
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11 pages, 3375 KiB  
Article
A Pressure Sensor Based on the Interaction between a Hard Magnet Magnetorheological Elastomer and a Hall Effect Structure
by Onejae Sul, Sung Joong Choo, In-Sik Jee, Jeengi Kim and Hyeong-Jun Kim
Micromachines 2024, 15(10), 1221; https://doi.org/10.3390/mi15101221 - 30 Sep 2024
Viewed by 1280
Abstract
In this article, we report a novel pressure sensing method based on the Hall effect and a hard magnet magnetorheological elastomer (hmMRE). The elastic property of the MRE under pressure was used to generate spatial variation in the magnetic flux density around the [...] Read more.
In this article, we report a novel pressure sensing method based on the Hall effect and a hard magnet magnetorheological elastomer (hmMRE). The elastic property of the MRE under pressure was used to generate spatial variation in the magnetic flux density around the MRE, and the variation was detected by the Hall effect device underneath. As the first development in this kind of pressure sensing mechanism, we conducted research for the following three purposes: (1) to verify the Hall effect on the output signal, (2) to understand the sensor output variations under different modes of operation, and (3) to utilize the mechanism as a pressure sensor. We characterized the sensor with its operation parameters, such as signal polarity switching depending on wiring directions, signal amplitude, and offset shift depending on the input voltage. Based on the analyses, we concluded that the Hall voltage represents the pressure applied on the hmMRE, and the new pressure sensing mechanism was devised successfully. Full article
(This article belongs to the Special Issue Magnetorheological Materials and Application Systems)
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12 pages, 5354 KiB  
Article
Magnetically Actuated Transport Pipeline with Self-Perception
by Quan Shu, Shaolin Ge, Yanfang Li and Shouhu Xuan
Actuators 2024, 13(6), 199; https://doi.org/10.3390/act13060199 - 22 May 2024
Cited by 1 | Viewed by 1218
Abstract
Soft transportation devices with high flexibility, good stability, and quick controllability have attracted increasing attention. However, a smart soft transportation device with tactile perception and a non-contact actuating mode remains a challenge. This work reports a magnetic soft pipeline (MSP) composed of sensor [...] Read more.
Soft transportation devices with high flexibility, good stability, and quick controllability have attracted increasing attention. However, a smart soft transportation device with tactile perception and a non-contact actuating mode remains a challenge. This work reports a magnetic soft pipeline (MSP) composed of sensor film, a magnetorheological elastomer (MRE) cavity pipeline, and heater film, which can not only respond well to tactile compression stimuli but also be transported by magnetic actuation. Notably, the sensor film was integrated on the upper surface of an MRE pipeline, and the relative resistance change (∆R/R0) of the MSP was maintained at 55.8% under 2.2 mm compression displacement during 4000 loading cycles. Moreover, the heater film was integrated on the lower surface of the MRE pipeline, which endows the MSP with an electrothermal heating characteristic. The temperature of the MSP can be increased from 26.7 °C to 38.1 °C within 1 min under 0.6 V. Furthermore, the MSP was attracted and deformed under the magnetic field, and the ∆R/R0 of the MSP reached 69.1% under application of a 165 mT magnetic field density. Benefiting from the excellent perception and magnetic deformation performances, the magnetic actuate transportation of the MSP with self-sensing was successfully achieved. This multi-functional soft pipeline integrated with in situ self-sensing, electrothermal heating, and non-contact magnetic actuating transportation performance possess high potential in smart flexible electronic devices. Full article
(This article belongs to the Special Issue Advances in Smart Materials-Based Actuators)
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23 pages, 7408 KiB  
Systematic Review
Sensors and Sensing Devices Utilizing Electrorheological Fluids and Magnetorheological Materials—A Review
by Yu-Jin Park and Seung-Bok Choi
Sensors 2024, 24(9), 2842; https://doi.org/10.3390/s24092842 - 29 Apr 2024
Cited by 7 | Viewed by 2845
Abstract
This paper comprehensively reviews sensors and sensing devices developed or/and proposed so far utilizing two smart materials: electrorheological fluids (ERFs) and magnetorheological materials (MRMs) whose rheological characteristics such as stiffness and damping can be controlled by external stimuli; an electrical voltage for ERFs [...] Read more.
This paper comprehensively reviews sensors and sensing devices developed or/and proposed so far utilizing two smart materials: electrorheological fluids (ERFs) and magnetorheological materials (MRMs) whose rheological characteristics such as stiffness and damping can be controlled by external stimuli; an electrical voltage for ERFs and a magnetic field for MRMs, respectively. In this review article, the MRMs are classified into magnetorheological fluids (MRF), magnetorheological elastomers (MRE) and magnetorheological plastomers (MRP). To easily understand the history of sensing research using these two smart materials, the order of this review article is organized in a chronological manner of ERF sensors, MRF sensors, MRE sensors and MRP sensors. Among many sensors fabricated from each smart material, one or two sensors or sensing devices are adopted to discuss the sensing configuration, working principle and specifications such as accuracy and sensitivity. Some sensors adopted in this article include force sensors, tactile devices, strain sensors, wearable bending sensors, magnetometers, display devices and flux measurement sensors. After briefly describing what has been reviewed in a conclusion, several challenging future works, which should be undertaken for the practical applications of sensors or/and sensing devices, are discussed in terms of response time and new technologies integrating with artificial intelligence neural networks in which several parameters affecting the sensor signals can be precisely and optimally tuned. It is sure that this review article is very helpful to potential readers who are interested in creative sensors using not only the proposed smart materials but also different types of smart materials such as shape memory alloys and active polymers. Full article
(This article belongs to the Special Issue Feature Review Papers in Physical Sensors)
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18 pages, 8386 KiB  
Article
Fiber Jamming of Magnetorheological Elastomers as a Technique for the Stiffening of Soft Robots
by Taylan Atakuru, Fatih Kocabaş, Niccolò Pagliarani, Matteo Cianchetti and Evren Samur
Robotics 2024, 13(1), 16; https://doi.org/10.3390/robotics13010016 - 17 Jan 2024
Cited by 4 | Viewed by 3797
Abstract
There has been a notable focus on the adoption of jamming-based technologies, which involve increasing the friction between grains, layers, or fibers to achieve variable stiffness capability in soft robots. Additionally, magnetorheological elastomers (MREs) that show magnetic-field-dependent viscoelasticity have great potential as a [...] Read more.
There has been a notable focus on the adoption of jamming-based technologies, which involve increasing the friction between grains, layers, or fibers to achieve variable stiffness capability in soft robots. Additionally, magnetorheological elastomers (MREs) that show magnetic-field-dependent viscoelasticity have great potential as a material for varying stiffness. This study proposes a hybrid method (magnetic jamming of MRE fibers) for enhancing the stiffness of soft robots, combining a jamming-based with a viscosity-based method. First, a fiber jamming structure is developed and integrated into a soft robot, the STIFF-FLOP manipulator, to prove the concept of the magnetic jamming of MRE fibers. Then, based on the proposed method, a variable stiffness device actuated by electro-permanent magnets is developed. The device is integrated into the same manipulator and the electronically controlled magnetic jamming and stiffening of the manipulator is demonstrated. The experimental results show that stiffness gain in bending and compression is achieved with the proposed method. The outcomes of this investigation demonstrate that the proposed hybrid stiffening technique presents a promising avenue for realizing variable and controllable stiffness in soft robots. Full article
(This article belongs to the Special Issue Editorial Board Members' Collection Series: "Soft Robotics")
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17 pages, 5409 KiB  
Article
The Magneto–Mechanical Hyperelastic Property of Isotropic Magnetorheological Elastomers with Hybrid-Size Magnetic Particles
by Leizhi Wang, Ke Zhang and Zhaobo Chen
Materials 2023, 16(23), 7282; https://doi.org/10.3390/ma16237282 - 23 Nov 2023
Viewed by 1708
Abstract
Isotropic magnetorheological elastomers (MREs) with hybrid-size particles are proposed to tailor the zero-field elastic modulus and the relative magnetorheological rate. The hyperelastic magneto–mechanical property of MREs with hybrid-size CIPs (carbonyl iron particles) was experimentally investigated under large strain, which showed differential hyperelastic mechanical [...] Read more.
Isotropic magnetorheological elastomers (MREs) with hybrid-size particles are proposed to tailor the zero-field elastic modulus and the relative magnetorheological rate. The hyperelastic magneto–mechanical property of MREs with hybrid-size CIPs (carbonyl iron particles) was experimentally investigated under large strain, which showed differential hyperelastic mechanical behavior with different hybrid-size ratios. Quasi-static magneto–mechanical compression tests corresponding to MREs with different hybrid size ratios and mass fractions were performed to analyze the effects of hybrid size ratio, magnetic flux density, and CIP mass fraction on the magneto–mechanical properties. An extended Knowles magneto–mechanical hyperelastic model based on magnetic energy, coupling the magnetic interaction, is proposed to predict the influence of mass fraction, hybrid size ratio, and magnetic flux density on the magneto–mechanical properties of isotropic MRE. Comparing the experimental and predicted results, the proposed model can accurately evaluate the quasi-static compressive magneto–mechanical properties, which show that the predicted mean square deviations of the magneto–mechanical constitutive curves for different mass fractions are all in the range of 0.9–1. The results demonstrate that the proposed hyperelastic magneto–mechanical model, evaluating the magneto–mechanical properties of isotropic MREs with hybrid-size CIPs, has a significant stress–strain relationship. The proposed model is important for the characterization of magneto–mechanical properties of MRE-based smart devices. Full article
(This article belongs to the Section Smart Materials)
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17 pages, 12842 KiB  
Article
A Novel Tactile Sensing System Utilizing Magnetorheological Structures for Dynamic Contraction and Relaxation Motions
by Yu-Jin Park, Bo-Gyu Kim, Eun-Sang Lee and Seung-Bok Choi
Sensors 2023, 23(22), 9035; https://doi.org/10.3390/s23229035 - 8 Nov 2023
Cited by 1 | Viewed by 2120
Abstract
It is well known that the rheological properties of magnetorheological (MR) material change under a magnetic field. So far, most works on MR materials have been oriented toward actuating characteristics instead of sensing functions. In this work, to realize dynamic tactile motion, a [...] Read more.
It is well known that the rheological properties of magnetorheological (MR) material change under a magnetic field. So far, most works on MR materials have been oriented toward actuating characteristics instead of sensing functions. In this work, to realize dynamic tactile motion, a spherical MR structure was designed as a sensor, incorporating a magnetic circuit core to provide maximum dynamic motion. After manufacturing a prototype (sample), a sinusoidal magnetic field of varying exciting frequency and magnitude was applied to the sample, and the dynamic contraction and relaxation motion depending on the exciting magnetic field was observed. Among the test results, when 10% deformation occurred, the instantaneous force generated was from 2.8 N to 8.8 N, and the force when relaxed was from 1.2 N to 3.5 N. It is also shown that the repulsive force within this range can be implemented using an acceptable input current. The special tactile sensing structure proposed in this work can be used as a sensor to measure the field-dependent viscoelastic properties of human tissues such as stomach, liver, and overall body. In addition, it could be usefully applied to robot surgery, because it can mimic the dynamic motions of various human organs under various surgical conditions. Full article
(This article belongs to the Special Issue Advances in Magnetic Sensors and Their Applications)
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15 pages, 4611 KiB  
Article
Hysteresis Behavior Modeling of Magnetorheological Elastomers under Impact Loading Using a Multilayer Exponential-Based Preisach Model Enhanced with Particle Swarm Optimization
by Alawiyah Hasanah Mohd. Alawi, Khisbullah Hudha, Zulkiffli Abd. Kadir and Noor Hafizah Amer
Polymers 2023, 15(9), 2145; https://doi.org/10.3390/polym15092145 - 30 Apr 2023
Cited by 4 | Viewed by 2026
Abstract
Magnetorheological elastomers (MREs) are a type of smart material that can change their mechanical properties in response to external magnetic fields. These unique properties make them ideal for various applications, including vibration control, noise reduction, and shock absorption. This paper presents an approach [...] Read more.
Magnetorheological elastomers (MREs) are a type of smart material that can change their mechanical properties in response to external magnetic fields. These unique properties make them ideal for various applications, including vibration control, noise reduction, and shock absorption. This paper presents an approach for modeling the impact behavior of MREs. The proposed model uses a combination of exponential functions arranged in a multi-layer Preisach model to capture the nonlinear behavior of MREs under impact loads. The model is trained using particle swarm optimization (PSO) and validated using experimental data from drop impact tests conducted on MRE samples under various magnetic field strengths. The results demonstrate that the proposed model can accurately predict the impact behavior of MREs, making it a useful tool for designing MRE-based devices that require precise control of their impact response. The model’s response closely matches the experimental data with a maximum prediction error of 10% or less. Furthermore, the interpolated model’s response is in agreement with the experimental data with a maximum percentage error of less than 8.5%. Full article
(This article belongs to the Special Issue Scientific Machine Learning for Polymeric Materials)
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15 pages, 2180 KiB  
Article
Magnetostriction Enhancement in Midrange Modulus Magnetorheological Elastomers for Sensor Applications
by Muhammad Asyraf Tasin, Siti Aishah Abdul Aziz, Saiful Amri Mazlan, Mohd Aidy Faizal Johari, Nur Azmah Nordin, Shahir Yasin Mohd Yusuf, Seung-Bok Choi and Irfan Bahiuddin
Micromachines 2023, 14(4), 767; https://doi.org/10.3390/mi14040767 - 29 Mar 2023
Cited by 13 | Viewed by 2561
Abstract
Magnetorheological elastomer (MRE), which is capable of exhibiting magnetostriction in the presence of a magnetic field, has a great potential to be used for the development of sensor devices. Unfortunately, to date, many works focused on studying low modulus of MRE (less than [...] Read more.
Magnetorheological elastomer (MRE), which is capable of exhibiting magnetostriction in the presence of a magnetic field, has a great potential to be used for the development of sensor devices. Unfortunately, to date, many works focused on studying low modulus of MRE (less than 100 kPa) which can hamper their potential application in sensors due to short lifespan and low durability. Thus, in this work, MRE with storage modulus above 300 kPa is to be developed to enhance magnetostriction magnitude and reaction force (normal force). To achieve this goal, MREs are prepared with various compositions of carbonyl iron particles (CIPs), in particular, MRE with 60, 70 and 80 wt.% of CIP. It is shown that both the magnetostriction percentage and normal force increment are achieved as the concentration of CIPs increases. The highest magnetostriction magnitude of 0.075% is obtained with 80 wt.% of CIP, and this increment is higher than that of moderate stiffness MRE developed in the previous works. Therefore, the midrange range modulus MRE developed in this work can copiously produce the required magnetostriction value and potentially be implemented for the design of forefront sensor technology. Full article
(This article belongs to the Special Issue Magnetic and Spin Devices, Volume II)
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34 pages, 8999 KiB  
Review
A Review on Vibration Control Strategies Using Magnetorheological Materials Actuators: Application Perspective
by Aji Masa’id, Bhre Wangsa Lenggana, U. Ubaidillah, Didik Djoko Susilo and Seung-Bok Choi
Actuators 2023, 12(3), 113; https://doi.org/10.3390/act12030113 - 3 Mar 2023
Cited by 22 | Viewed by 5746
Abstract
Magnetorheological (MR) materials are a group of smart materials used in new technologies with controlled reliability. The development of these materials is expanding, starting from MR fluids, elastomers, grease, and gel. This large number of material types further expands the various applications of [...] Read more.
Magnetorheological (MR) materials are a group of smart materials used in new technologies with controlled reliability. The development of these materials is expanding, starting from MR fluids, elastomers, grease, and gel. This large number of material types further expands the various applications of MR materials as a creative technology to support performance enhancement. For example, MR fluid is used to improve the performance of shock absorbers such as vehicle suspension, the damping of building structures, and polishing of the workpiece. MR elastomers are used for engine mounting, insulation base, and many other applications with intelligent material properties such as stiffness controllability. However, there are still complexities in the practical implementation of the control system beyond reliability. Many previous studies have focused on the performance improvement and reliability of MR materials as smart materials for application devices and systems. In this review article, the specific discussion related to vibration control strategies in MR material-based systems was thoroughly investigated. To discuss this point, many MR applications including transportation system and vibration isolation were adopted using different types of control strategies. Many different control strategies that have been used for MR applications such as fuzzy logic control, optimal control, and skyhook control are discussed in-depth in terms of the inherent control characteristics of merits and demerits. Full article
(This article belongs to the Section Actuator Materials)
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20 pages, 4618 KiB  
Review
Review of Soft Actuators Controlled with Electrical Stimuli: IPMC, DEAP, and MRE
by Jakub Bernat, Piotr Gajewski, Jakub Kołota and Agnieszka Marcinkowska
Appl. Sci. 2023, 13(3), 1651; https://doi.org/10.3390/app13031651 - 28 Jan 2023
Cited by 27 | Viewed by 4579
Abstract
Soft actuators have been developed for a variety of applications, including soft grippers, artificial muscles, wearables, tactile devices, and medical devices. In this review, we will discuss a group of chemical materials and their robotic applications in soft actuators controlled with electrical stimuli. [...] Read more.
Soft actuators have been developed for a variety of applications, including soft grippers, artificial muscles, wearables, tactile devices, and medical devices. In this review, we will discuss a group of chemical materials and their robotic applications in soft actuators controlled with electrical stimuli. Soft actuators provide a deformable body and allow interaction with the environment to achieve the desired actuation pattern. We will also discuss the principles of operation and functionality and focus on important real-life applications of three groups of soft actuators: ionic polymer–metal composites (IPMCs), dielectric electroactive polymers (DEAPs), and magnetorheological elastomers (MREs). This review article aims to provide researchers interested in the field of soft robotics with a guide to various state-of-the-art chemistry methods used in electrically activated soft actuators, as well as the application areas for such devices. Full article
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19 pages, 5819 KiB  
Article
Effect of Carbonyl Iron Particle Types on the Structure and Performance of Magnetorheological Elastomers: A Frequency and Strain Dependent Study
by Ayman M. H. Salem, Abdelrahman Ali, Rahizar Bin Ramli, Asan G. A. Muthalif and Sabariah Julai
Polymers 2022, 14(19), 4193; https://doi.org/10.3390/polym14194193 - 6 Oct 2022
Cited by 17 | Viewed by 3469
Abstract
Magnetorheological elastomers (MREs) are smart viscoelastic materials in which their physical properties can be altered when subjected to a varying magnetic field strength. MREs consist of an elastomeric matrix mixed with magnetic particles, typically carbonyl iron particles (CIPs). The magnetic field-responsive property of [...] Read more.
Magnetorheological elastomers (MREs) are smart viscoelastic materials in which their physical properties can be altered when subjected to a varying magnetic field strength. MREs consist of an elastomeric matrix mixed with magnetic particles, typically carbonyl iron particles (CIPs). The magnetic field-responsive property of MREs have led to their wide exposure in research. The potential development and commercialization of MRE-based devices requires extensive investigation to identify the essential factors that can affect their properties. For this reason, this research aims to investigate the impact of CIPs’ type, concentration and coating on the rheological and mechanical properties of MREs. Isotropic MREs are fabricated with four different CIP compositions differing between hard or soft, and coated or uncoated samples. Each MRE composition have three different concentrations, which is 5%, 10%, and 20% by volume. The dynamic properties of the fabricated samples are tested by compression oscillations on a dynamic mechanical analyzer (DMA). Frequency and strain dependent measurements are performed to obtain the storage and loss modulus under different excitation frequencies and strain amplitudes. The emphasis is on the magnetorheological (MR) effect and the Payne effect which are an intrinsic characteristics of MREs. The effect of the CIPs’ type, coating, and concentration on the MR and Payne effect of MREs are elucidated. Overall, it is observed that, the storage and loss modulus exhibit a strong dependence on both the frequency excitations and the strain amplitudes. Samples with hard and coated CIPs tend to have a higher MR effect than other samples. A decrease in the storage modulus and non-monotonous behavior of the loss modulus with increasing strain amplitude are observed, indicating the Payne effect. The results of this study can aid in the characterization of MREs and the proper selection of CIPs grades based on the application. Full article
(This article belongs to the Section Polymer Analysis and Characterization)
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12 pages, 2199 KiB  
Article
Enhancement of Magneto-Induced Modulus by the Combination of Filler and Plasticizer Additives-Based Magnetorheological Elastomer
by Muntaz Hana Ahmad Khairi, Ervina Efzan Mhd Noor, Ubaidillah Ubaidillah, Siti Aishah Abdul Aziz, Saiful Amri Mazlan, Siti Maisarah Ahmad Tarmizi and Nur Azmah Nordin
Materials 2022, 15(18), 6396; https://doi.org/10.3390/ma15186396 - 15 Sep 2022
Cited by 8 | Viewed by 1942
Abstract
Filler additive is used to provide superior bonding in rubber matrix to enhance the storage modulus of magnetorheological elastomer (MRE). However, the magneto-induced modulus is reduced as the initial storage modulus increases. Therefore, this paper aims to increase the magneto-induced modulus and maintain [...] Read more.
Filler additive is used to provide superior bonding in rubber matrix to enhance the storage modulus of magnetorheological elastomer (MRE). However, the magneto-induced modulus is reduced as the initial storage modulus increases. Therefore, this paper aims to increase the magneto-induced modulus and maintain the initial storage modulus by combining filler and plasticizer additives. Both types of additives have different functions, where cobalt ferrite (CoFe2O4) is capable of enhancing the maximum storage modulus and silicone oil (SO) reduces the initial storage modulus. Thus, four MRE samples have been fabricated using (a) no additive, (b) CoFe2O4, (c) SO, and (d) a combination of CoFe2O4 and SO. The sample’s hardness and magnetic properties were investigated via Durometer Shore A and Vibrating Sample Magnetometer (VSM), respectively. Furthermore, the rheological properties of MRE samples in terms of storage modulus were investigated upon the frequency and magnetic field sweep using a rheometer. The results demonstrated that the storage modulus of the MRE samples has increased with increasing the oscillation frequency from 0.1 to 50 Hz. Interestingly, the combination of additives has produced the largest value of magneto-induced modulus of 0.90 MPa as compared to other samples. Furthermore, their initial storage modulus was in between samples with SO (lowest) and without additive (highest). Therefore, fundamental knowledge in adding the combination of additives can offer solutions for a wide range of stiffness in MR device applications such as vibration and noise control devices, sensing devices, and actuators. Full article
(This article belongs to the Special Issue Advances in Electromagnetic Properties of Magnetic Materials)
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