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Keywords = fast Joule heating

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15 pages, 2181 KB  
Article
A Flexible and Thermally Uniform TiO2/Ag/SiO2 Transparent Heater for Skin-Integrated Applications
by Jaejeong Jo, Geonwoo Kang, Chankyoung Lee, Tran Thi Bao Vo and Dooho Choi
J. Funct. Biomater. 2026, 17(3), 151; https://doi.org/10.3390/jfb17030151 - 18 Mar 2026
Viewed by 829
Abstract
Transparent heaters intended for skin-contacting applications must simultaneously satisfy optical transparency, mechanical compliance, thermal uniformity, and operational safety under biologically relevant temperature ranges. Here, we evaluate the applicability of a TiO2/Ag/SiO2 (TAS) dielectric–metal–dielectric transparent heater as a functional biomaterial platform [...] Read more.
Transparent heaters intended for skin-contacting applications must simultaneously satisfy optical transparency, mechanical compliance, thermal uniformity, and operational safety under biologically relevant temperature ranges. Here, we evaluate the applicability of a TiO2/Ag/SiO2 (TAS) dielectric–metal–dielectric transparent heater as a functional biomaterial platform for wearable and skin-integrated thermal systems. By systematically optimizing each layer thickness of the TAS structure, the heater achieves high visible-light transmittance (average of 86.6%) together with low sheet resistance on the order of 7.7 Ω/sq for low-voltage operation. The TAS heater demonstrates rapid and reproducible Joule-heating behavior, showing fast thermal response with short thermal time constants and spatially homogeneous temperature distributions without localized hot spots. Stable electrothermal performance is maintained under repeated on/off cycling and during cyclic mechanical bending down to small radii, confirming excellent mechanical stability under repeated bending relevant to wearable applications. Importantly, direct on-skin evaluations conducted by attaching the device to a human elbow reveal conformal contact, uniform heating at therapeutically relevant temperatures (50–70 °C), and stable operation under dynamic bending and extension. The absence of thermal inhomogeneity during motion highlights the intrinsic stability of the TAS architecture for skin-interfaced use. Given the high optical visibility, mechanical compliance, thermal uniformity, and electrothermal stability, the proposed TAS architecture represents a promising functional biomaterial platform for wearable thermotherapy, skin-mounted healthcare devices, and human-interactive thermal systems operating under continuous mechanical deformation and direct skin contact. Full article
(This article belongs to the Special Issue Advanced Materials and Devices for Medical Interventions)
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19 pages, 4323 KB  
Article
Synthesis of Turbostratic Graphene with Micron-Sized Domains from Activated Charcoal by Fast Joule Heating
by Aisen Ruslanovich Prokopiev, Nikolay Nikolaevich Loskin and Pavel Vasilievich Vinokurov
Nanomaterials 2025, 15(24), 1885; https://doi.org/10.3390/nano15241885 - 15 Dec 2025
Viewed by 2175
Abstract
The development of economical and scalable methods for synthesizing high-quality graphene remains a pivotal challenge in materials science. This study presents an efficient approach for synthesizing turbostratic graphene with micron-sized domains from an accessible bioprecursor-activated charcoal—using fast Joule heating. We demonstrate that ultra-rapid [...] Read more.
The development of economical and scalable methods for synthesizing high-quality graphene remains a pivotal challenge in materials science. This study presents an efficient approach for synthesizing turbostratic graphene with micron-sized domains from an accessible bioprecursor-activated charcoal—using fast Joule heating. We demonstrate that ultra-rapid thermal annealing (~16.2 kJ/g, up to 3000 K) triggers a phase transition from amorphous carbon to a highly graphitized structure. Comprehensive characterization via SEM, AFM, Raman spectroscopy, and XRD revealed the formation of large flakes with lateral dimensions up to 1.5 µm and thicknesses ranging from 4 to 200 nm. Raman mapping further uncovered a heterogeneous structure with alternating regions exhibiting different degrees of interlayer coupling, characteristic of turbostratic stacking. The key feature of the material is its turbostratic layer stacking, confirmed by the combination of XRD data showing an interlayer distance of 3.436 Å and Raman spectra characteristic of decoupled graphene layers. The synthesized material exhibits excellent electrical transport properties, with a bulk resistivity of 0.51 Ω·cm—an order of magnitude lower than that of the initial charcoal. These findings highlight the potential of the developed method for producing electrode materials for energy storage devices and conductive composites. Full article
(This article belongs to the Section 2D and Carbon Nanomaterials)
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15 pages, 5168 KB  
Article
The Anisotropic Electrothermal Behavior and Deicing Performance of a Self-Healing Epoxy Composite Reinforced with Glass/Carbon Hybrid Fabrics
by Ting Chen and Xusheng Du
Molecules 2025, 30(13), 2794; https://doi.org/10.3390/molecules30132794 - 28 Jun 2025
Viewed by 1100
Abstract
Hybrid fiber-reinforced polymer-laminated composites are often used under icy conditions (such as for reinforcing parts in aircraft frames and bridge beams), where there is an urgent demand for deicing. In this paper, besides the different mechanical properties of laminates along the longitudinal carbon [...] Read more.
Hybrid fiber-reinforced polymer-laminated composites are often used under icy conditions (such as for reinforcing parts in aircraft frames and bridge beams), where there is an urgent demand for deicing. In this paper, besides the different mechanical properties of laminates along the longitudinal carbon fiber (CF) and glass fiber (GF) directions, the anisotropic electrothermal behavior of a hybrid glass/carbon fiber-reinforced epoxy (GCF/EP) is also investigated, as well as its deicing performance and self-repairing capability. The surface equilibrium temperature of GCF/EP composites can conveniently be adjusted by tuning the current magnitude and its flow direction. Compared to the longitudinal CF direction of the GCF/EP, where 0.3 A was loaded to achieve a surface equilibrium temperature of 122.8 °C, a much weaker current (0.03 A) was needed to load along the longitudinal GF direction to reach almost the same temperature. However, besides the higher flexural strength and fast temperature response, along the longitudinal CF direction, the GCF/EP exhibited excellent deicing performance, including a shorter time and larger energy efficiency. Furthermore, the self-repairing ability of the GCF/EP and its effect on the deicing performance of the composite were characterized. Studying the Joule heating effect of GCF/EP composite laminates and their corresponding deicing performance lays the foundation for their design and practical application in icy environments. Full article
(This article belongs to the Special Issue Micro/Nano-Materials for Anti-Icing and/or De-Icing Applications)
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18 pages, 5262 KB  
Article
A Novel Microelectrode Based on Joule Heating and Impedance Spectroscopy for Inducing and Monitoring the Aggregation of HCV-Specific Probes
by Reda Abdelbaset, Omar E. Morsy, Mariam Hossam Eldin, Sherif M. Shawky, Yehya H. Ghallab and Yehea Ismail
Sensors 2025, 25(11), 3312; https://doi.org/10.3390/s25113312 - 24 May 2025
Viewed by 1397
Abstract
The world urgently needs new methods to quickly and efficiently detect mutated viruses. An RNA-AuNP-based colorimetric biosensor is a highly sensitive, specific, and cost-effective tool that enables rapid, visual detection of target molecules for applications in disease diagnostics, environmental monitoring, and forensic analysis. [...] Read more.
The world urgently needs new methods to quickly and efficiently detect mutated viruses. An RNA-AuNP-based colorimetric biosensor is a highly sensitive, specific, and cost-effective tool that enables rapid, visual detection of target molecules for applications in disease diagnostics, environmental monitoring, and forensic analysis. An RNA-AuNP-based colorimetric biosensor requires precise control over nanoparticle dispersion and aggregation, which can be achieved using temperature regulation. A novel on-chip microelectrode is proposed to induce and monitor the aggregation of RNA-attached gold nanoparticles (AuNPs) through Joule heating and impedance spectroscopy. The proposed platform is implemented based on printed circuit board (PCB) technology, which has many advantages, such as fast and easy design and fabrication, low power consumption, and low costs. Joule heating is the process in which the energy of an electric current is converted into heat as it flows through a resistance. Impedance spectroscopy is an analytical technique that measures a system’s electrical response to an applied AC signal across a range of frequencies, providing insights into a sample’s dielectric properties. The results validate that the fabricated microelectrode is capable of heating a 20 µL droplet to 75 °C within 30 s, utilizing a low power input of only 3.75 watts and successfully inducing a color change based on the presence of hepatitis C virus (HCV) RNA, while impedance readings are used to monitor the aggregation. Full article
(This article belongs to the Special Issue Advances in Energy Harvesting and Sensor Systems)
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25 pages, 2513 KB  
Review
Protein Manipulation via Dielectrophoresis: Theoretical Principles and Emerging Microfluidic Platforms
by Zuriel Da En Shee, Ervina Efzan Mhd Noor and Mirza Farrukh Baig
Micromachines 2025, 16(5), 531; https://doi.org/10.3390/mi16050531 - 29 Apr 2025
Cited by 1 | Viewed by 2034
Abstract
Dielectrophoresis (DEP) has been widely employed in microfluidic platforms for particle or cell manipulation in biomedical science applications due to its accurate, fast, label-free, and low-cost diagnostic technique. However, the application of the DEP technique towards protein manipulation has yet to be extensively [...] Read more.
Dielectrophoresis (DEP) has been widely employed in microfluidic platforms for particle or cell manipulation in biomedical science applications due to its accurate, fast, label-free, and low-cost diagnostic technique. However, the application of the DEP technique towards protein manipulation has yet to be extensively explored due to the challenges of the complexity of protein itself, such as its complex morphologies, extremely minuscule particle size, inherent electrical properties, and temperature sensitivity, which make it relatively more challenging. Furthermore, given that protein DEP investigation requires entering the micro- to nano-scale level of DEP configuration, various challenging factors such as electrohydrodynamic effects, electrolysis, joule heating, and electrothermal force that emerge will make it more difficult in realizing protein DEP investigation. This review study has discussed the fundamental theory of DEP and considerations toward protein DEP manipulation. In particular, it focused on the DEP theoretical principle towards protein, protein DEP application challenges, microfluidic platform considerations, medium considerations, and a critically reviewed list of protein bioparticles that have been investigated were all highlighted. Full article
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24 pages, 6825 KB  
Article
Numerical Analysis on Cooling Performances for Connectors Using Immersion Cooling in Ultra-Fast Chargers for Electric Vehicles
by Seong-Guk Hwang, Moo-Yeon Lee and Beom-Seok Ko
Symmetry 2025, 17(4), 624; https://doi.org/10.3390/sym17040624 - 20 Apr 2025
Cited by 9 | Viewed by 2861
Abstract
The increasing demand for ultra-fast charging in electric vehicles (EVs) necessitates advancements in thermal management strategies to mitigate Joule heating, which arises due to electrical resistance in charging connectors and cable cores. This study presents a numerical analysis of immersion cooling performance for [...] Read more.
The increasing demand for ultra-fast charging in electric vehicles (EVs) necessitates advancements in thermal management strategies to mitigate Joule heating, which arises due to electrical resistance in charging connectors and cable cores. This study presents a numerical analysis of immersion cooling performance for ultra-fast chargers under realistic charging conditions. The simulated results are validated by experiments with a maximum deviation of 5.5% at 600 A and 700 A currents. The novelty of this work lies in the consideration of a realistic charging cable length of 5 m, the evaluation of temperature characteristics in the charger connector, and the analysis of geometric symmetry in the charging cable and coolant configuration to ensure uniform heat distribution. Key operating conditions were systematically analyzed, including applied currents, ambient temperatures, coolant flow rates, cable core cross-sectional areas, and different types of coolants. Results indicate that increasing the applied current from 400 A to 800 A raised the connector temperature from 60.73 °C to 97.33 °C. As the ambient temperature increased from 20 °C to 50 °C, the connector temperature rose significantly from 42.71 °C to 74.99 °C, while the maximum cable core temperature increased from 65.26 °C to 100.61 °C. Increasing the cable core cross-sectional area from 20 mm2 to 30 mm2 reduced the connector temperature from 77.20 °C to 74.99 °C. Meanwhile, increasing the coolant flow rate from 2 LPM to 5 LPM had a negligible effect on the connector temperature. Among the three tested coolants, Novec 7500 exhibited the highest cooling efficiency, achieving the lowest contact temperature (74.76 °C) and the highest performance evaluation criteria (PEC) value of 3.8. This study provides valuable guidelines for enhancing symmetry-driven thermal management systems and demonstrates the potential of immersion cooling to improve efficiency, safety, and operational reliability in next-generation high-power EV chargers. Full article
(This article belongs to the Special Issue Symmetry in Power Systems and Thermal Engineering)
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17 pages, 521 KB  
Article
Numerical Simulation and Parameter Estimation of the Space-Fractional Magnetohydrodynamic Flow and Heat Transfer Coupled Model
by Yi Liu, Xiaoyun Jiang and Junqing Jia
Fractal Fract. 2024, 8(10), 557; https://doi.org/10.3390/fractalfract8100557 - 26 Sep 2024
Cited by 3 | Viewed by 1378
Abstract
In this paper, a coupled model is built to research the space-fractional magnetohydrodynamic (MHD) flow and heat transfer problem. The fractional coupled model is solved numerically by combining the matrix function vector products method in the temporal direction with the spectral method in [...] Read more.
In this paper, a coupled model is built to research the space-fractional magnetohydrodynamic (MHD) flow and heat transfer problem. The fractional coupled model is solved numerically by combining the matrix function vector products method in the temporal direction with the spectral method in the spatial direction. A fast method based on the numerical scheme is established to reduce the computational time. With the help of the Bayesian method, the space-fractional orders of the coupled model are estimated, and the problem of multi-parameter estimation in the coupled model is solved. Finally, a numerical example is carried out to verify the stability of the numerical methods and the effectiveness of the parameter estimation method. Results show that the numerical method is stable, which converges with an accuracy of O(τ2+Nr). The fast method is efficient in reducing the computational time, and the parameter estimation method can effectively estimate parameters in the space-fractional coupled model. The numerical solutions are discussed to describe the effects of several important parameters on the velocity and the temperature. Results indicate that the Lorentz force produced by the MHD flow blocks the movement of the fluid and prolongs the time for the fluid to reach a stable state. But the Hall parameter m weakens this hindrance. The Joule heating effects play a negative role in heat transfer. Full article
(This article belongs to the Special Issue New Advances and Applications of Fractional Oscillate System)
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9 pages, 8889 KB  
Article
Bimetallic Fe, Co-Modified TiO2 Derived from NH2-MIL-125(Ti) as an Efficient Photocatalyst for N2 Fixation
by Huiying Yang and Xiangchao Meng
Processes 2024, 12(9), 1879; https://doi.org/10.3390/pr12091879 - 2 Sep 2024
Viewed by 1948
Abstract
The conversion of nitrogen (N2) and water (H2O) into NH3 by photocatalysis under ambient conditions has been considered an environmentally friendly strategy. However, developing effective catalysts for N2 fixation is still challenging. Herein, we report a bimetallic [...] Read more.
The conversion of nitrogen (N2) and water (H2O) into NH3 by photocatalysis under ambient conditions has been considered an environmentally friendly strategy. However, developing effective catalysts for N2 fixation is still challenging. Herein, we report a bimetallic JH Fe, Co/TiO2 derived from NH2-MIL-125(Ti) by the fast Joule heating (FJH) method for visible–light–driven catalytic N2 fixation. It was found that the photocatalytic N2 reduction efficiency of bimetallic FC@TiO2-JH was improved, enabling an NH3 yield rate of 110.14 µmol g−1 h−1 without any sacrificial agents. Furthermore, the rate was higher than those of Fe@TiO2-JH and Co@TiO2-JH, suggesting that the synergistic effect between Fe and Co broke the electronic equilibrium and increased the center of its d-band, enhancing electronic feedback to the antibonding π* orbitals of N2 while weakening the bonding energy of N≡N. Meanwhile, the rate was about 2.75 times higher than that of FC@TiO2-TF, which was calcined in a tube furnace. It is assumed that FJH might lead to the formation of lattice defects, leading to localized charge deficiency, enhanced carrier separation, and transport. Thus, doping of Fe and Co synergistically interacted with the defects produced from FJH, facilitating the photocatalytic reduction process. As detected, it had a greater ability to separate hole–electron pairs and transferred electrons to adsorbed N2 at faster rates. Our work demonstrates a prospective strategy for designing bimetallic catalysts derived from NH2-MIL-125(Ti) for N2 fixation. Full article
(This article belongs to the Special Issue Photocatalysts: Synthesis, Mechanisms and Applications)
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14 pages, 4480 KB  
Article
Nacre-like Anisotropic Multifunctional Aramid Nanofiber Composites for Electromagnetic Interference Shielding, Thermal Management, and Strain Sensing
by Jin Dong, Jing Lin, Hebai Zhang, Jun Wang, Ye Li, Kelin Pan, Haichen Zhang and Dechao Hu
Molecules 2024, 29(17), 4000; https://doi.org/10.3390/molecules29174000 - 23 Aug 2024
Cited by 1 | Viewed by 2522
Abstract
Developing multifunctional flexible composites with high-performance electromagnetic interference (EMI) shielding, thermal management, and sensing capacity is urgently required but challenging for next-generation smart electronic devices. Herein, novel nacre-like aramid nanofibers (ANFs)-based composite films with an anisotropic layered microstructure were prepared via vacuum-assisted filtration [...] Read more.
Developing multifunctional flexible composites with high-performance electromagnetic interference (EMI) shielding, thermal management, and sensing capacity is urgently required but challenging for next-generation smart electronic devices. Herein, novel nacre-like aramid nanofibers (ANFs)-based composite films with an anisotropic layered microstructure were prepared via vacuum-assisted filtration and hot-pressing. The formed 3D conductive skeleton enabled fast electron and phonon transport pathways in the composite films. As a result, the composite films showed a high electrical conductivity of 71.53 S/cm and an outstanding thermal conductivity of 6.4 W/m·K when the mass ratio of ANFs to MXene/AgNWs was 10:8. The excellent electrical properties and multi-layered structure endowed the composite films with superior EMI shielding performance and remarkable Joule heating performance, with a surface temperature of 78.3 °C at a voltage of 2.5 V. Additionally, it was found that the composite films also exhibited excellent mechanical properties and outstanding flame resistance. Moreover, the composite films could be further designed as strain sensors, which show great promise in monitoring real-time signals for human motion. These satisfactory results may open up a new opportunity for EMI shielding, thermal management, and sensing applications in wearable electronic devices. Full article
(This article belongs to the Special Issue Recent Advances in Functional Composite Materials)
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14 pages, 3362 KB  
Article
A Rapid, Efficient Method for Anodic Aluminum Oxide Membrane Room-Temperature Multi-Detachment from Commercial 1050 Aluminum Alloy
by Chin-An Ku, Chia-Wei Hung and Chen-Kuei Chung
Nanomaterials 2024, 14(14), 1216; https://doi.org/10.3390/nano14141216 - 17 Jul 2024
Cited by 6 | Viewed by 3504
Abstract
For commercial processes, through-hole AAO membranes are fabricated from high-purity aluminum by chemical etching. However, this method has the disadvantages of using heavy-metal solutions, creating large amounts of material waste, and leading to an irregular pore structure. Through-hole porous alumina membrane fabrication has [...] Read more.
For commercial processes, through-hole AAO membranes are fabricated from high-purity aluminum by chemical etching. However, this method has the disadvantages of using heavy-metal solutions, creating large amounts of material waste, and leading to an irregular pore structure. Through-hole porous alumina membrane fabrication has been widely investigated due to applications in filters, nanomaterial synthesis, and surface-enhanced Raman scattering. There are several means to obtain freestanding through-hole AAO membranes, but a fast, low-cost, and repetitive process to create complete, high-quality membranes has not yet been established. Here, we propose a rapid and efficient method for the multi-detachment of an AAO membrane at room temperature by integrating the one-time potentiostatic (OTP) method and two-step electrochemical polishing. Economical commercial AA1050 was used instead of traditional high-cost high-purity aluminum for AAO membrane fabrication at 25 °C. The OTP method, which is a single-step process, was applied to achieve a high-quality membrane with unimodal pore distribution and diameters between 35 and 40 nm, maintaining a high consistency over five repetitions. To repeatedly detach the AAO membrane, two-step electrochemical polishing was developed to minimize damage on the AA1050 substrate caused by membrane separation. The mechanism for creating AAO membranes using the OTP method can be divided into three major components, including the Joule heating effect, the dissolution of the barrier layer, and stress effects. The stress is attributed to two factors: bubble formation and the difference in the coefficient of thermal expansion between the AAO membrane and the Al substrate. This highly efficient AAO membrane detachment method will facilitate the rapid production and applications of AAO films. Full article
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10 pages, 5275 KB  
Article
Fast Joule Heating for the Scalable and Green Production of Graphene with a High Surface Area
by Zakhar Ivanovich Evseev, Aisen Ruslanovich Prokopiev, Petr Stanislavovich Dmitriev, Nikolay Nikolaevich Loskin and Dmitrii Nikolaevich Popov
Materials 2024, 17(3), 576; https://doi.org/10.3390/ma17030576 - 25 Jan 2024
Cited by 2 | Viewed by 3918
Abstract
The rapid development of electric vehicles, unmanned aerial vehicles, and wearable electronic devices has led to great interest in research related to the synthesis of graphene with a high specific surface area for energy applications. However, the problem of graphene synthesis scalability, as [...] Read more.
The rapid development of electric vehicles, unmanned aerial vehicles, and wearable electronic devices has led to great interest in research related to the synthesis of graphene with a high specific surface area for energy applications. However, the problem of graphene synthesis scalability, as well as the lengthy duration and high energy intensity of the activation processes of carbon materials, are significant disadvantages. In this study, a novel reactor was developed for the green, simple, and scalable electrochemical synthesis of graphene oxide with a low oxygen content of 14.1%. The resulting material was activated using the fast joule heating method. The processing of mildly oxidized graphene with a high-energy short electrical pulse (32 ms) made it possible to obtain a graphene-based porous carbon material with a specific surface area of up to 1984.5 m2/g. The increase in the specific surface area was attributed to the rupture of the original graphene flakes into smaller particles due to the explosive release of gaseous products. In addition, joule heating was able to instantly reduce the oxidized graphene and decrease its electrical resistance from >10 MΩ/sq to 20 Ω/sq due to sp2 carbon structure regeneration, as confirmed by Raman spectroscopy. The low energy intensity, simplicity, and use of environment-friendly chemicals rendered the proposed method scalable. The resulting graphene material with a high surface area and conductivity can be used in various energy applications, such as Li-ion batteries and supercapacitors. Full article
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9 pages, 3700 KB  
Communication
Solar-Powered Switch of Antiferromagnetism/Ferromagnetism in Flexible Spintronics
by Chenying Wang, Yujing Du, Yifan Zhao, Zhexi He, Song Wang, Yaxin Zhang, Yuxuan Jiang, Yongjun Du, Jingen Wu, Zhuangde Jiang and Ming Liu
Nanomaterials 2023, 13(24), 3158; https://doi.org/10.3390/nano13243158 - 17 Dec 2023
Cited by 3 | Viewed by 2007
Abstract
The flexible electronics have application prospects in many fields, including as wearable devices and in structural detection. Spintronics possess the merits of a fast response and high integration density, opening up possibilities for various applications. However, the integration of miniaturization on flexible substrates [...] Read more.
The flexible electronics have application prospects in many fields, including as wearable devices and in structural detection. Spintronics possess the merits of a fast response and high integration density, opening up possibilities for various applications. However, the integration of miniaturization on flexible substrates is impeded inevitably due to the high Joule heat from high current density (1012 A/m2). In this study, a prototype flexible spintronic with device antiferromagnetic/ferromagnetic heterojunctions is proposed. The interlayer coupling strength can be obviously altered by sunlight soaking via direct photo-induced electron doping. With the assistance of a small magnetic field (±125 Oe), the almost 180° flip of magnetization is realized. Furthermore, the magnetoresistance changes (15~29%) of flexible spintronics on fingers receiving light illumination are achieved successfully, exhibiting the wearable application potential. Our findings develop flexible spintronic sensors, expanding the vision for the novel generation of photovoltaic/spintronic devices. Full article
(This article belongs to the Special Issue Magnetic Nanostructured Materials and Spin Electronics)
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17 pages, 3956 KB  
Article
Positive and Negative Photoconductivity in Ir Nanofilm-Coated MoO3 Bias-Switching Photodetector
by Mohamed A. Basyooni-M. Kabatas, Redouane En-nadir, Khalid Rahmani and Yasin Ramazan Eker
Micromachines 2023, 14(10), 1860; https://doi.org/10.3390/mi14101860 - 28 Sep 2023
Cited by 4 | Viewed by 2341
Abstract
In this study, we delved into the influence of Ir nanofilm coating thickness on the optical and optoelectronic behavior of ultrathin MoO3 wafer-scale devices. Notably, the 4 nm Ir coating showed a negative Hall voltage and high carrier concentration of 1.524 × [...] Read more.
In this study, we delved into the influence of Ir nanofilm coating thickness on the optical and optoelectronic behavior of ultrathin MoO3 wafer-scale devices. Notably, the 4 nm Ir coating showed a negative Hall voltage and high carrier concentration of 1.524 × 1019 cm−3 with 0.19 nm roughness. Using the Kubelka–Munk model, we found that the bandgap decreased with increasing Ir thickness, consistent with Urbach tail energy suggesting a lower level of disorder. Regarding transient photocurrent behavior, all samples exhibited high stability under both dark and UV conditions. We also observed a positive photoconductivity at bias voltages of >0.5 V, while at 0 V bias voltage, the samples displayed a negative photoconductivity behavior. This unique aspect allowed us to explore self-powered negative photodetectors, showcasing fast response and recovery times of 0.36/0.42 s at 0 V. The intriguing negative photoresponse that we observed is linked to hole self-trapping/charge exciton and Joule heating effects. Full article
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14 pages, 2852 KB  
Article
Optimization of Magnetoimpedance Effect and Magnetic Properties of Fe-Rich Glass-Coated Microwires by Annealing
by Alvaro González, Alfonso García-Gomez, Valentina Zhukova, Paula Corte-Leon, Mihail Ipatov, Juan Maria Blanco, Julian Gonzalez and Arcady Zhukov
Sensors 2023, 23(17), 7481; https://doi.org/10.3390/s23177481 - 28 Aug 2023
Cited by 3 | Viewed by 2101
Abstract
As-prepared Fe-rich microwires with perfectly rectangular hysteresis loops present magnetization reversal through fast domain wall propagation, while the giant magnetoimpedance (GMI) effect in Fe-rich microwires is rather low. However, the lower cost of Fe-rich microwires makes them attractive for magnetic sensors applications. We [...] Read more.
As-prepared Fe-rich microwires with perfectly rectangular hysteresis loops present magnetization reversal through fast domain wall propagation, while the giant magnetoimpedance (GMI) effect in Fe-rich microwires is rather low. However, the lower cost of Fe-rich microwires makes them attractive for magnetic sensors applications. We studied the effect of conventional (furnace) annealing and Joule heating on magnetic-propertied domain wall (DW) dynamics and the GMI effect in two Fe microwires with different geometries. We observed that magnetic softness, GMI effect and domain wall (DW) dynamics can be substantially improved by appropriate annealing. Observed experimental results are discussed considering the counterbalance between the internal stresses relaxation and induced magnetic anisotropy associated with the presence of an Oersted magnetic field during Joule heating. Full article
(This article belongs to the Special Issue Recent Advances in Magnetic GSR Sensor)
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18 pages, 3061 KB  
Article
Free and Wire-Guided Spark Discharges in Water: Pre-Breakdown Energy Losses and Generated Pressure Impulses
by Yifan Chai, Igor V. Timoshkin, Mark P. Wilson, Martin J. Given and Scott J. MacGregor
Energies 2023, 16(13), 4932; https://doi.org/10.3390/en16134932 - 25 Jun 2023
Cited by 7 | Viewed by 3514
Abstract
Impulsive underwater discharges have been investigated for many decades, yet the complex pre-breakdown processes that underpin their development are not fully understood. Higher pre-breakdown energy losses may lead to significant reduction in the magnitude and intensity of the pressure waves generated by expanding [...] Read more.
Impulsive underwater discharges have been investigated for many decades, yet the complex pre-breakdown processes that underpin their development are not fully understood. Higher pre-breakdown energy losses may lead to significant reduction in the magnitude and intensity of the pressure waves generated by expanding post-breakdown plasma channels. Thus, it is important to characterize these losses for different discharge types and to identify approaches to their reduction. The present paper analyses thermal pre-breakdown processes in the case of free path and wire-guided discharges in water: fast joule heating of a small volume of water at the high-voltage electrode and joule heating and the melting of the wire, respectively. The energy required for joule heating of the water and metallic wire have been obtained from thermal models, analysed and compared with the experimental pre-breakdown energy losses. Pressure impulses generated by free path and by wire-guided underwater discharges have also been investigated. It was shown that wire-guided discharges support the formation of longer plasma channels better than free path underwater discharges for the same energy available per discharge. This results in stronger pressure impulses developed by underwater wire-guided discharges. It has been shown that the pressure magnitude in the case of both discharge types is inversely proportional to the observation distance which is a characteristic of a spherical acoustic wave. Full article
(This article belongs to the Topic High Voltage Systems and Smart Technologies)
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