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27 pages, 949 KB  
Systematic Review
Material Reuse in the European Union Construction Sector: A Review
by Inês Silva, Graça Martinho and Mário Ramos
Recycling 2026, 11(4), 79; https://doi.org/10.3390/recycling11040079 - 16 Apr 2026
Abstract
The progression towards a circular economy in the construction sector has gained attention as a response to rising resource consumption and construction and demolition waste generation, with material reuse playing a central role. In this context, this study analyses the literature on reuse [...] Read more.
The progression towards a circular economy in the construction sector has gained attention as a response to rising resource consumption and construction and demolition waste generation, with material reuse playing a central role. In this context, this study analyses the literature on reuse in the construction sector, examining its investigation over time and its relation to European regulatory frameworks and policy strategies. A systematic literature review was conducted using a structured search across the B-on, Scopus, and Web of Science databases. The search targeted peer-reviewed journal articles in English, published between 2008 and 2023, focusing on titles, abstracts, and keywords with predefined terms. A total of 78 articles met the inclusion criteria and were analysed. Research activity has increased in recent years, reflecting growing European policy attention, particularly the Waste Framework Directive, its 2018 amendment, and the Circular Economy Action Plan. Most studies address strategies to promote the circular economy, waste management practices, life cycle assessments, and the identification of barriers and opportunities to reuse. Despite the expanding literature, reuse remains insufficiently addressed. These findings underline the need for more targeted research and stronger integration between policy and practice to support effective reuse in the construction sector. Full article
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20 pages, 3146 KB  
Article
Dewatering of Short-Fibre Digestates from Paper Recycling Mills: Liquid Fraction and Mass Distribution Profiles
by Dheeraja Winter, Svea Ziegner, Simone Krafft, Markus Grömping and Silvio Beier
Recycling 2026, 11(4), 78; https://doi.org/10.3390/recycling11040078 - 15 Apr 2026
Viewed by 192
Abstract
The paper sector is characterised by high freshwater consumption and a strong need for improved resource efficiency. In this context, industrial digestates derived from short-fibre residues in paper recycling mills represent a promising substrate for water recovery within a circular economy framework. This [...] Read more.
The paper sector is characterised by high freshwater consumption and a strong need for improved resource efficiency. In this context, industrial digestates derived from short-fibre residues in paper recycling mills represent a promising substrate for water recovery within a circular economy framework. This study investigated the dewatering of short-fibre digestates as a pre-treatment for downstream membrane processes, aiming to maximise the liquid fraction (LF) recovery while minimising dry matter (DM) content. Seven scenarios were studied: sedimentation (S0); pre-sedimentation with chemical addition using iron(III) chloride (FeCl3) + polydiallyldimethylammonium chloride (polyDADMAC) (S1), FeCl3 + starch (S2), Nanofloc® (S3), and polyDADMAC (S4); and direct dewatering without pre-sedimentation using polyDADMAC with cloth filtration (S5) and centrifugation (S6). With reference to the sedimentation supernatant, S4 achieved the highest DM separation efficiency of 76%, followed by S1 (64%), whereas S2 and S3 were below 40%. However, LF recovery relative to the initial digestate was limited in scenarios S1–S4 to 17% (170 g/kgdigestate), with DM concentrations of 2.0–4.8 g/kgLF. In contrast, direct dewatering increased LF recovery substantially, with centrifugation (S6) achieving up to 690 gLF/kgdigestate and cloth filtration (S5) 420 g/kgdigestate, while maintaining a low DM (1.7 g/kgLF). Chemical oxygen demand (COD) and phosphorus (Ptot) were largely separated from the liquid fractions in all the scenarios. Nitrogen (Ntot) and ammonium (NH4-N) in the LF remained more variable, ranging from 22 to 153 and 5 to 22 mg/kgdigestate, respectively. These results indicate that centrifugation with polyDADMAC is the most effective approach, suggesting that mechanical force with a chemical additive can be used for the efficient dewatering of short-fibre digestates. Full article
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12 pages, 490 KB  
Article
Citrus Waste as a Source of High-Value Compounds: Effect of Solvent System and Extraction Time on Bioactive Compound Recovery
by Noemi García-Gomez, Roifer Pérez-Vásquez, José Luis Pasquel-Reátegui, Manuel Fernando Coronado-Jorge, Enrique Navarro-Ramírez, Karen Gabriela Documet-Petrlik, Pierre Vidaurre-Rojas, Keller Sánchez-Dávila and Ángel Cárdenas-García
Recycling 2026, 11(4), 77; https://doi.org/10.3390/recycling11040077 - 12 Apr 2026
Viewed by 304
Abstract
Orange waste, generally discarded, is a source of many bioactive compounds that could be used for the development of high-value-added products in the food, cosmetic, and pharmaceutical industries. The objective of this study was to evaluate the influence of extraction method (automated Soxhlet [...] Read more.
Orange waste, generally discarded, is a source of many bioactive compounds that could be used for the development of high-value-added products in the food, cosmetic, and pharmaceutical industries. The objective of this study was to evaluate the influence of extraction method (automated Soxhlet extraction and temperature-controlled maceration), solvent system, and extraction time on the recovery of bioactive compounds from Valencia orange (Citrus sinensis) by-products. Proximate characterization of the dried orange residue (DOR) was performed prior to extraction. The type of solvent (ethanol and methanol), solvent:water ratio (50, 75, and 100%), and extraction time (60 and 120 min) were evaluated in terms of total extraction yield (TEY), total phenolic content (TPC), and antioxidant capacity determined by ABTS and DPPH assays, for each extraction method. ASE generally provided higher extraction yield and total phenolic content, particularly with 75:25 ethanol:water at 120 min, whereas TCM combined with methanol produced the highest antioxidant capacity. Extracts with up to 46.32% TEY, 5.57 mg GAE/g dm, and antioxidant capacities of 66.49 and 11.10 µmol TE/g dm determined by ABTS and DPPH assays, respectively, were obtained. The results demonstrated that Valencia orange by-products are a source of phenolic compounds and antioxidants with potential for product development across different industrial sectors. Full article
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18 pages, 7475 KB  
Article
Comparative Analysis of Industrial Waste as Supplementary Cementitious Materials—A Preliminary Study
by Pauls P. Argalis, Kristers Gelzis, Ralfs K. Valdovskis and Laura Vitola
Recycling 2026, 11(4), 75; https://doi.org/10.3390/recycling11040075 - 8 Apr 2026
Viewed by 258
Abstract
This preliminary study investigates the viability of substituting high-performance Aalborg white Portland cement (CEM I 52.5 R) with five diverse industrial byproducts: wood ash, silica waste, clay brick, glass fibre, and calcined sewage sludge ash. Sewage sludge ash was produced in a laboratory [...] Read more.
This preliminary study investigates the viability of substituting high-performance Aalborg white Portland cement (CEM I 52.5 R) with five diverse industrial byproducts: wood ash, silica waste, clay brick, glass fibre, and calcined sewage sludge ash. Sewage sludge ash was produced in a laboratory from two different sludges from wastewater treatment plants in the Latvian cities of Jelgava and Liepaja. The research evaluates the influence of substitution levels ranging from 5% to 20% on the rheology of fresh material and its early-age mechanical performance (day 7). Results indicate that particle morphology largely dictates workability; porous and angular materials, such as wood ash, clay brick, and sewage sludge ash, reduce flowability, whereas non-absorbent milled glass fibres unexpectedly improve spread diameter. Regarding mechanical performance, glass fibre and clay brick waste demonstrated the highest potential, exceeding the 48–62 MPa reference compressive strengths by achieving up to 69 MPa at a 10% substitution level. Conversely, wood ash and silica waste exhibited significant strength degradation at higher substitution levels, due to agglomeration and high water demand. This approach not only identifies viable waste streams for cement substitution but also diverts significant industrial waste from landfills, thereby reducing CO2e emissions and advancing more sustainable construction practices. Full article
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19 pages, 1204 KB  
Article
Bioprocess Valorization of Brazilian Agro-Industrial Wastes for Enzyme Synthesis in Protease Production
by Rhudson Fellipy de Oliveira Almeida, Ivaldo Itabaiana and Maria Alice Zarur Coelho
Recycling 2026, 11(4), 76; https://doi.org/10.3390/recycling11040076 - 8 Apr 2026
Viewed by 218
Abstract
Proteases are key biocatalysts widely applied in the food, pharmaceutical, detergent, and environmental industries. One of the most costly steps in large-scale enzyme production is the preparation of the culture medium, making agro-industrial wastes attractive as low-cost nutrient sources and potential inducers. The [...] Read more.
Proteases are key biocatalysts widely applied in the food, pharmaceutical, detergent, and environmental industries. One of the most costly steps in large-scale enzyme production is the preparation of the culture medium, making agro-industrial wastes attractive as low-cost nutrient sources and potential inducers. The non-conventional yeast Yarrowia lipolytica stands out in bioprocess engineering due to its high secretion capacity, GRAS status, and ability to metabolize diverse industrial residues. In this study, Brazilian agro-industrial by-products, namely Corn steep liquor (CSL), brewer’s yeast residue (BYR), and okara, were evaluated as alternative nitrogen sources for protease production by Y. lipolytica IMUFRJ 50678. Enzyme activity was quantified by the azocasein method at optimized conditions (40 °C, 40 min, pH 5 and 8). After an initial exploratory screening (n = 1), brewer’s yeast residue (BYR) and okara were identified as promising candidates for protease production. These preliminary findings guided subsequent experiments performed in biological triplicate (n = 3), which confirmed the reproducibility and comparative performance of these substrates, showing higher acid protease (AXP) activity in the BYR medium ((5.4 ± 0.3) U/mL), whereas alkaline protease (AEP) activities were comparable between the BYR ((8.4 ± 0.6) U/mL) and okara ((7.5 ± 0.9) U/mL) media. CSL was associated with higher lipase activity ((11.7 ± 0.9) × 103 U/L), while esterase activity was higher in the BYR medium. These findings indicate that agro-industrial residues, particularly BYR and okara, can serve as effective nitrogen sources for protease production by Y. lipolytica IMUFRJ 50678, supporting their use in waste valorization and sustainable bioprocesses. Full article
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15 pages, 1249 KB  
Article
Effect of Water Treatment Plant Sludge Addition on the Composting Efficiency, Quality, and Environmental Sustainability of Sewage Sludge, Food Waste, and Agro-Industrial Waste
by Daví Matos Lopes, Monica Luci Oliveira de Brito, Josiel Isaac Domingues de Almeida, Danilo Corado de Melo, Jhon Adno de Almeida Santana, Manoel Ferreira Lima Neto and Maico Chiarelotto
Recycling 2026, 11(4), 74; https://doi.org/10.3390/recycling11040074 - 7 Apr 2026
Viewed by 336
Abstract
This study aimed to evaluate the effects of adding sludge generated in water treatment plants on the composting of sewage sludge, urban organic waste, and agroindustrial waste. Four treatments were conducted with different proportions of water treatment plant sludge (WTS). Four treatments were [...] Read more.
This study aimed to evaluate the effects of adding sludge generated in water treatment plants on the composting of sewage sludge, urban organic waste, and agroindustrial waste. Four treatments were conducted with different proportions of water treatment plant sludge (WTS). Four treatments were conducted with 0%, 10%, 20%, and 30% proportions of WTS. The different proportions allowed for the evaluation of the effects of WTS addition on composting. The study was carried out in composting reactors. Kinetic models were applied to study the degradation of organic matter. Physicochemical and microbiological parameters were analyzed. During the process, temperature variation and basal respiration exhibited similar patterns. Principal component analysis showed that the 30WTS (32.2% water treatment sludge) treatment presented higher values of cation exchange capacity (CEC)/total organic carbon (TOC) ratio (3.83), and germination index (94.35%), and lower values of TOC (23.67%) and C/N (carbon/nitrogen) ratio (14.45). The composts produced in all treatments complied with Brazilian regulations for the environmental and agronomic quality of organic composts. It was concluded that the inclusion of up to 30% of WTS in composting did not negatively affect the composting process and did not compromise the environmental or agronomic quality of the final organic composts. Full article
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38 pages, 1809 KB  
Review
A Review of Organic Municipal Waste Management in Medium Cities in Latin America
by Linda Y. Pérez-Morales, Adriana Guzmán-López, Rita Miranda-López, Micael Gerardo Bravo-Sánchez and José E. Botello-Álvarez
Recycling 2026, 11(4), 73; https://doi.org/10.3390/recycling11040073 - 5 Apr 2026
Viewed by 614
Abstract
Latin America faces growing challenges in the management of municipal solid waste (MSW). This is particularly evident in medium-sized and metropolitan cities where rapid urbanization, limited infrastructure, and high proportions of organic waste (40–70%) converge. This review synthesizes the most recent advances in [...] Read more.
Latin America faces growing challenges in the management of municipal solid waste (MSW). This is particularly evident in medium-sized and metropolitan cities where rapid urbanization, limited infrastructure, and high proportions of organic waste (40–70%) converge. This review synthesizes the most recent advances in organic waste management, valorization strategies, environmental performance, and policy frameworks in Mexico and Latin America. To provide a comprehensive overview, evidence from studies on informal recycling systems, route optimization, sustainable landfill siting, food waste valorization, life cycle assessments (LCAs), and biogas production is integrated. Techno-economic analyses of energy recovery from organic fractions are specifically reviewed. This review highlights that valorization of organic waste through composting, anaerobic digestion, food supplementation, and bioproduct generation can reduce greenhouse gas emissions by 40–70% compared to landfilling, with AD–composting hybrids achieving the highest reductions of 60–70%. Community composting achieved moderate reductions, 30–50%, but at significantly lower cost and with greater social co-benefits. These alternatives for valorizing the organic fraction extend the lifespan of both confined and open landfills. It also contributes to mitigating the public health impacts related to open dumping, disease vectors, and contaminated leachate. In short, this review also highlights shortcomings in policy coherence, financial mechanisms, source separation, and technology adoption. A strategic framework is proposed that prioritizes decentralized treatment systems, the integration of informal recyclers, tax incentives, community-based waste separation, and planning based on Life Cycle Assessment (LCA). The findings point to a viable strategy for transitioning from landfill dependency to circular waste management systems that improve the quality of life for the population of Latin America and the Caribbean. Full article
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19 pages, 581 KB  
Article
Research on Producing Boiler Fuel from Sunflower Oil Wastes
by Denis Miroshnichenko, Yurii Parkhomov, Yurii Lypko, Vladislav Reivi, Yurii Rohovyi, Mariia Shved, Bohdan Korchak and Serhiy Pyshyev
Recycling 2026, 11(4), 72; https://doi.org/10.3390/recycling11040072 - 2 Apr 2026
Viewed by 339
Abstract
The effective utilization and effective valorization of various organic industrial wastes have become increasingly important issues. One significant area for enhancing the circular economy is the processing of waste generated from vegetable oils and animal fats. This article focuses on the processing and [...] Read more.
The effective utilization and effective valorization of various organic industrial wastes have become increasingly important issues. One significant area for enhancing the circular economy is the processing of waste generated from vegetable oils and animal fats. This article focuses on the processing and use of soapstocks, which result from the chemical reaction between fatty acids and alkali. These soapstocks represent the most significant portion (approximately 70–90 wt% by weight) of waste produced by the oil and fat industry. The raw material for this study was soapstock obtained from the neutralization of sunflower oil at the PJSC “Zaporizhzhya Oil and Fat Plant,” designed by the Belgian company “De Smet.” The soapstock yield was found to be 9.95 wt% based on 100 wt% oil. Through a series of treatments involving water, acid, and multiple washes, a low-sulfur fuel component was produced that nearly meets the standards for boiler fuels as outlined in DSTU 4058-2001 and PN-C-96024:2020, except for the heat of combustion. It fully complies with the requirements specified in ISO 8217:2024. The sulfur content of the final product was determined to be 0.12 wt%. Additionally, the fuels produced contained 75.33 wt% carbon, 11.64 wt% hydrogen, and 12.00 wt% oxygen. Due to the relatively low oxygen content, the resulting product exhibits approximately twice the heat of combustion of similar fuels derived from other waste streams in the oil and fat industry. Full article
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17 pages, 7972 KB  
Article
Thermal Recycling of Gypsum–Hemp Bio-Concrete: Experimental Evaluation of Dehydration Conditions and Properties Evolution
by Placide Uwizeyimana, Tania Lopes, Rodolphe Sonnier, Anthony Burlet, Mohammed Rakkane, Wissal Bouamri and Marc Potin
Recycling 2026, 11(4), 71; https://doi.org/10.3390/recycling11040071 - 2 Apr 2026
Viewed by 368
Abstract
The building sector is a major source of CO2 emissions and construction waste, motivating the development of sustainable materials and end-of-life recycling strategies. Bio-concretes, combining mineral binders with plant-based aggregates, offer low density and favorable hygrothermal performance but remain insufficiently studied with [...] Read more.
The building sector is a major source of CO2 emissions and construction waste, motivating the development of sustainable materials and end-of-life recycling strategies. Bio-concretes, combining mineral binders with plant-based aggregates, offer low density and favorable hygrothermal performance but remain insufficiently studied with respect to recyclability, particularly for gypsum-based materials. This study experimentally investigates the thermal recycling of gypsum–hemp bio-concrete, in which gypsum acts as the binder and hemp shiv as the aggregate. Thermogravimetric analysis of individual constituents and the bio-concrete was conducted to identify a temperature range enabling gypsum dehydration without hemp degradation. Controlled oven treatments at selected temperature–time couples were then applied to determine optimal recycling conditions, followed by the bio-concrete remanufacturing using 100% recycled constituents. Physical, thermal, and mechanical properties were evaluated before and after recycling under controlled conditions. Results show that a treatment at 180 °C for 60 min enables effective gypsum dehydration (18–20% mass loss) while preserving hemp integrity. Recycled gypsum–hemp bio-concrete exhibits increased density (368 to 587 kg·m−3) and compressive strength (0.05 to 0.52 MPa), accompanied by a moderate increase in thermal conductivity (0.081 to 0.096 W·m−1·K−1). These findings demonstrate the feasibility of 100% thermal recycling of gypsum–hemp bio-concrete without constituent separation. Full article
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30 pages, 3692 KB  
Review
Crystallization Behavior of Recycled Semi-Crystalline Polymers in 3D Printing: Progress, Challenges, and Opportunities
by Zunaida Zakaria, Arif Rochman and Paul Refalo
Recycling 2026, 11(4), 70; https://doi.org/10.3390/recycling11040070 - 1 Apr 2026
Viewed by 386
Abstract
In recent years, plastic recycling has emerged as a critical concern in environmental protection and waste management. Among the various techniques for repurposing plastic waste into valuable products, extrusion of filaments for 3D printing has proven to be a highly effective method. A [...] Read more.
In recent years, plastic recycling has emerged as a critical concern in environmental protection and waste management. Among the various techniques for repurposing plastic waste into valuable products, extrusion of filaments for 3D printing has proven to be a highly effective method. A thorough understanding of the crystallization behavior of recycled plastics used in 3D printing is essential, as it significantly influences their final performance. This review provides an in-depth analysis of the crystallization behavior and crystallinity of recycled semi-crystalline polymers, with particular emphasis on recycled commodity plastics such as recycled polyethylene terephthalate (rPET), recycled polypropylene (rPP), and recycled high-density polyethylene (rHDPE). Recent research published between 2015 and 2025 was systematically synthesized and provides information on sources of plastic waste, additives employed, and recycling processes involved, with the findings summarized in a table that highlights their effects on polymer crystallinity. Furthermore, the key factors impacting the crystallinity of 3D-printed recycled plastics were examined, including the influence of additives, multiple processing cycles, printing parameters, and thermal treatments. Research gaps and the challenges faced during the printing process were also identified and discussed. By consolidating recent findings, this review provides a comprehensive understanding of the crystallization behavior of recycled plastics in 3D printing, thereby providing guidance for future research and developing strategies to optimize the performance of these materials. Full article
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13 pages, 4081 KB  
Article
Selective Recycling of Steel Sandwich Polyisocyanurate (PIR) Foam Insulation Cladding
by Diana Meza-Rojas, James Holliman, David Penney, Anthony R. Lewis and Peter J. Holliman
Recycling 2026, 11(4), 69; https://doi.org/10.3390/recycling11040069 - 1 Apr 2026
Viewed by 285
Abstract
A method has been developed to delaminate the organic components (paint, foam) from the steel skins of composite polyisocyanurate (PIR) steel insulation panels at ambient temperature and in 20 min using selected solvents combined with ultrasonication. Using this method, polyisocyanurate foam can be [...] Read more.
A method has been developed to delaminate the organic components (paint, foam) from the steel skins of composite polyisocyanurate (PIR) steel insulation panels at ambient temperature and in 20 min using selected solvents combined with ultrasonication. Using this method, polyisocyanurate foam can be selectively delaminated from polymer-based paint (PVC plastisol) and, in turn, the polymer paint can be selectively delaminated from the galvanised steel. Both the foam and paint are removed as intact layers, leaving the galvanised steel intact for the next steps of recycling, enabling the subsequent individualised recycling of each sub-component or layer. Several solvents have been tested, and the data show that H-bonding solvents (e.g., H2O, alcohols) are less effective at delaminating these polymers. Whilst high polarity, medium H-bonding acetonitrile and DMSO remove PVC paint and some PIR foam, the most effective solvent for both PIR foam and PVC paint removal is medium polarity, medium H-bonding acetone. Full article
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15 pages, 899 KB  
Article
Visitor Perceptions of Reusable Foodware Implementation at Grand Canyon National Park: A Pilot Study for Messaging and Graphic Design Considerations
by Megan Wagaman, Brendan Derrick Taff, Jeremy Shellhorn, Haven Everhart, Jennifer Carrigan, Melissa Jung and Elizabeth A. Himschoot
Recycling 2026, 11(4), 68; https://doi.org/10.3390/recycling11040068 - 1 Apr 2026
Viewed by 360
Abstract
The Grand Canyon National Park (GRCA) attracts roughly five million visitors annually, creating immense pressure on the waste stream managed in the park. To reduce environmental impacts, the National Park Service, collaborating organizations and concessionaires are in the process of implementing large-scale reusable [...] Read more.
The Grand Canyon National Park (GRCA) attracts roughly five million visitors annually, creating immense pressure on the waste stream managed in the park. To reduce environmental impacts, the National Park Service, collaborating organizations and concessionaires are in the process of implementing large-scale reusable foodware systems, replacing single-use plastics. This pilot study aimed to engage visitors in the design process to inform preferences and attitudes to further support management decision-making regarding the design and implementation of reusable foodware systems in the park. During September 2025, park visitors were intercepted at key concessionaire food vending locations and asked to complete a brief survey. The survey contained attitudinal questions, persuasive phrases, and potential logos and graphic designs that could be used with program implementation, which were evaluated via Likert scales by n = 164 respondents. Results suggest that respondents have overwhelmingly positive attitudes and norms towards reusing foodware at the park. Results highlight phrases and graphic designs that will be most effective as the program launches and can be used to inform future research. Full article
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14 pages, 670 KB  
Article
Advancing Plastic Waste Circularity Through Modular Portable Pyrolysis Systems
by Dimitrios-Aristotelis Koumpakis, Dimitrios Christoforidis, Vasileios Diamantis, Alexandra V. Michailidou and Christos Vlachokostas
Recycling 2026, 11(4), 67; https://doi.org/10.3390/recycling11040067 - 1 Apr 2026
Viewed by 480
Abstract
The lack of centralized waste management infrastructure in certain regions makes plastic waste an escalating environmental and economic problem. This research investigates how modular portable pyrolysis systems function as sustainable decentralized solutions. A standard shipping container houses a custom-designed pyrolysis unit which demonstrates [...] Read more.
The lack of centralized waste management infrastructure in certain regions makes plastic waste an escalating environmental and economic problem. This research investigates how modular portable pyrolysis systems function as sustainable decentralized solutions. A standard shipping container houses a custom-designed pyrolysis unit which demonstrates flexibility and adaptability. The system contains a batch rotary kiln reactor with a processing capacity of 750 kg per batch which is fed with urban plastic waste, to produce pyrolytic oil, syngas and char. The produced pyrolytic oil exhibits an energy content comparable to that of conventional diesel fuel. Additionally, the integration of biomass briquettes and recycled pyrolytic gas can reduce to a big extent the external energy requirements, improving the system’s overall energy autonomy. Therefore, the system becomes economically reliable due to its low operational expenses and the short cycle of approximately 7-h operation. The unit’s mobility enables on-site treatment operations which reduces both transportation emissions and expenses. The analysis includes technical design elements together with performance metrics for different plastics. This conceptual study demonstrates the feasibility of containerized pyrolysis as a practical method to enhance plastic waste chemical recycling rates while presenting a scalable framework for industrial symbiosis and local waste-to-energy conversion. Full article
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24 pages, 3334 KB  
Article
Effect of Multiple Extrusion Cycles on Particle and Chemical Emissions and Mechanical and Thermal Properties of High-Density Polyethylene 3D Printing Filaments Made from Virgin and Post-Consumer Waste Plastics
by Aleksandr B. Stefaniak, Lauren N. Bowers, Callee M. Walsh, Sonette Du Preez, Elizabeth D. Brusak, Jason E. Ham, Ryan F. LeBouf, M. Abbas Virji and Johan L. Du Plessis
Recycling 2026, 11(4), 66; https://doi.org/10.3390/recycling11040066 - 1 Apr 2026
Viewed by 376
Abstract
Distributed recycling of high-density polyethylene (HDPE) into filament for use in material extrusion 3D printing has been proposed as part of a circular economy. There is a gap in the understanding of the potential for HDPE to release contaminants that are potentially hazardous [...] Read more.
Distributed recycling of high-density polyethylene (HDPE) into filament for use in material extrusion 3D printing has been proposed as part of a circular economy. There is a gap in the understanding of the potential for HDPE to release contaminants that are potentially hazardous to human health during reuse. Herein, HDPE from post-consumer packaging waste was sorted into food and non-food (NF) streams and virgin HDPE was taken as a benchmark material. All materials were extruded into filaments and recycled multiple times while monitoring emissions. In general, particle and organic chemical emissions decreased by 93 to 99% and 73 to 99%, respectively, with increased reprocessing cycle without appreciable decline in mechanical (Young’s modulus decreased by 5 to 16%), processability (melt flow index stable from 0.2 to 0.7 g/10 min for waste plastics), and thermal properties (crystallinity ranged from a 6% decrease to a 9% increase) of plastics. An exception was a sub-stream of NF plastic that had increased particle emissions (up to 3100%) with reprocessing cycle. Reductions in emissions during filament extrusion appeared to be more influenced by reprocessing cycle than by any specific process step (grinding, etc.). The progressive decline in emissions without appreciable loss of polymer integrity could be exploited to pre-condition HDPE to reduce potential hazardous emissions prior to extruding into filament. This work helps fill the knowledge gap on approaches to recycling plastics in distributed settings such as home-based businesses, which is critical for developing effective recommendations for controls to enable safe work practices such as the use of ventilation to minimize exposures. Full article
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23 pages, 1107 KB  
Systematic Review
Technological Pathways for Rare Earth Elements Recovery from WEEE: A Systematic Mapping Review
by Luca Taglieri, Pietro Romano, Francesco Vegliò, Alberto Gallifuoco and Luciano Fratocchi
Recycling 2026, 11(4), 65; https://doi.org/10.3390/recycling11040065 - 1 Apr 2026
Viewed by 591
Abstract
Rare earth elements (REEs) are essential to many low-carbon and digital technologies, yet the primary supply is geographically concentrated; waste electrical and electronic equipment (WEEE) could act as an “urban mine”, but recovery pathways remain fragmented. We synthesize the evidence through a structured [...] Read more.
Rare earth elements (REEs) are essential to many low-carbon and digital technologies, yet the primary supply is geographically concentrated; waste electrical and electronic equipment (WEEE) could act as an “urban mine”, but recovery pathways remain fragmented. We synthesize the evidence through a structured literature review of Scopus and Web of Science indexed studies focusing on WEEE-derived feedstocks for REE recovery: 148 records were screened and 51 papers met the inclusion criteria. Reporting of the search and study selection process follows PRISMA 2020. We coded each study by WEEE source/fraction, core technology family, and process configuration, target REEs, performance reporting, environmental proxies, and maturity, and discussed gaps against circularity goals. Results show an intense concentration on a few feedstocks, permanent magnets (22 studies), fluorescent lamps (16), and batteries (6), with only limited attention to multi-source streams. Hydrometallurgical routes dominate, while biometallurgical options are less explored. Recovery is more frequently reported than selectivity and environmental indicators, and most solutions remain at proof-of-concept maturity. Due to the heterogeneity of feedstocks, process configurations, and reported metrics, the findings were synthesized qualitatively (no meta-analysis). This review highlights priorities for future work: multi-source and heavy rare earth elements focused feedstocks, more selective and intensified flowsheets, harmonized performance reporting, and scale-up supported by life-cycle and cost assessments. Full article
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