Food Gel-Based Systems: Gel-Forming and Food Applications

A special issue of Gels (ISSN 2310-2861). This special issue belongs to the section "Gel Applications".

Deadline for manuscript submissions: closed (30 August 2025) | Viewed by 7196

Special Issue Editors


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Guest Editor
Environmental Sustainability and Health Institute, Technological University Dublin, D24FKT9 Dublin, Ireland
Interests: hydrocolloids; food chemistry; food rheology; food gels
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Guest Editor
Department of Food Science, Purdue University, West Lafayette, IN 47907, USA
Interests: food gels; rheology; gel microstructure; plant and dairy proteins

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Guest Editor
Faculty of Food Technology Osijek, Josip Juraj Strossmayer University of Osijek, F. Kuhača 18, HR-31000 Osijek, Croatia
Interests: bioactive compounds; extraction; encapsulation; food gels; bioaccessibility of phenolic compounds; upcycling of by-products from the agro-food industry
Special Issues, Collections and Topics in MDPI journals

Special Issue Information

Dear Colleagues,

Recent innovations in modern processing technology have transformed a number of scientific and industrial areas, including the food industry. Gels have attracted increasing interest in the food discipline due to their good biocompatibility, biodegradability, nutritional properties, and edibility. These food colloids exhibit applicative potential in domains where gel-based systems play a crucial role, such as encapsulation and the controlled release of bioactive compounds, the bioaccessibility of bioactive compounds during digestion, the structuring and stabilization of emulsions and foams, the development of meat substitutes, plant-based protein gels, dairy products, confectioneries, bakery products, and novel gel-based food products. The mechanism of gelation is determined by the gelling agent(s) and the conditions of gel formation. The incorporation of plant-based proteins, plant-based hydrocolloids, gums, and fibers to create healthier and sustainable gel-based products is explored. Novel formulations with enhanced functional properties, nutritional profiles, and reduced allergenicity are also investigated.

This Special Issue invites authors to contribute high-quality original research or review articles on the utilization of novel ingredients and formulations in the development of versatile food gels.

Dr. Buliyaminu Adegbemiro Alimi
Dr. Da Chen
Prof. Dr. Ana Bucić-Kojić
Guest Editors

Manuscript Submission Information

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Keywords

  • novel food-derived gels
  • encapsulation and delivery of bioactive compounds using gels
  • bioaccessibility of bioactive compounds
  • gel-based packaging and edible coatings
  • structure
  • processing technologies

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Related Special Issue

Published Papers (6 papers)

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Research

18 pages, 1534 KB  
Article
Designing Spoonable Milk Kefir Gels: From Fermentation Optimization to Clean-Label Gel Structuring with Psyllium
by María Cardenete-Fernández, Alicia Castillo-Rivas, M. Montaña Durán-Barrantes, Luis A. Trujillo-Cayado and Jenifer Santos
Gels 2025, 11(9), 693; https://doi.org/10.3390/gels11090693 - 1 Sep 2025
Viewed by 370
Abstract
Kefir is a fermented dairy product whose structural properties can be modified to enhance its nutritional and sensory profile. The objective of this study was to develop spoonable milk kefir gels by optimizing fermentation conditions and incorporating psyllium and calcium chloride as structuring [...] Read more.
Kefir is a fermented dairy product whose structural properties can be modified to enhance its nutritional and sensory profile. The objective of this study was to develop spoonable milk kefir gels by optimizing fermentation conditions and incorporating psyllium and calcium chloride as structuring agents. In the initial phase of the study, a full factorial design was employed to conduct a comparative analysis of whole milk and skimmed milk during the fermentation process of kefir. The study encompassed the evaluation of the impact of various parameters, including inoculum level, temperature, and fermentation time, on the acidification kinetics of the fermentation process. This evaluation was facilitated through the measurement of pH and total acidity levels. Skimmed milk demonstrated accelerated acidification, consistently attaining a final pH of 4.08 and a total acidity of 9.99 g·L−1 lactic acid equivalents under optimized conditions (5.5% weight:weight grains, 26 °C, 24 h). In the subsequent phase, kefir obtained under these conditions was gelled with varying concentrations of psyllium and calcium chloride. Rheological characterization revealed that psyllium markedly strengthened the gel network: at 3.06% w:w psyllium, the elastic modulus increased up to 209.6 Pa, while the critical stress improved from 0.64 Pa at low psyllium/Ca2+ to 10.42 Pa at high psyllium content. Furthermore, zero-shear viscosity increased substantially, exceeding 1500 Pa·s in high-psyllium, low-calcium formulations. The findings demonstrate that combining fermentation optimization with clean-label structuring agents enables the development of low-fat kefir gels with enhanced textural and processing properties, supporting their potential as synbiotic, functional dairy products. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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16 pages, 6809 KB  
Article
Flaxseed Fiber-Structured Nanoemulgels for Salad Dressing Applications: Processing and Stability
by María-Carmen Alfaro-Rodríguez, Fátima Vela, María-Carmen García-González and José Muñoz
Gels 2025, 11(9), 678; https://doi.org/10.3390/gels11090678 - 24 Aug 2025
Viewed by 391
Abstract
This study aimed to investigate the production of nanoemulgels structured with flaxseed fiber, designed to simulate salad dressings. For this purpose, the influence of microfluidizer passes (from one to four) on physicochemical and rheological properties was determined, followed by an assessment of thermal [...] Read more.
This study aimed to investigate the production of nanoemulgels structured with flaxseed fiber, designed to simulate salad dressings. For this purpose, the influence of microfluidizer passes (from one to four) on physicochemical and rheological properties was determined, followed by an assessment of thermal behavior. Rotor–stator homogenization followed by microfluidization were employed to produce nanoemulgels, which were characterized using laser diffraction, multiple light scattering, and rheological measurements. The resulting systems exhibited monomodal particle size distributions with mean diameters below 220 nm. Increasing the number of microfluidizer passes from one to four led to slight reductions in particle size, although they were not statistically significant. The formulation with two passes demonstrated superior physical stability during aging studies. Rheological evaluation indicated enhanced gel-like behavior with up to three passes, whereas excessive energy input (four passes) slightly compromised structural integrity. The linear viscoelastic region decreased notably after the first pass but remained relatively stable thereafter. The two-pass nanoemulgel, identified as the optimal formulation, was further tested for thermal stability. Temperature increases (5–20 °C) led to minor decreases in viscosity and firmness, yet the structure remained thermally stable. These findings support microfluidization as an effective strategy for developing stable flaxseed fiber-based nanoemulgels, with potential applications in functional food systems. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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13 pages, 1890 KB  
Article
Compound Salt-Based Coagulants for Tofu Gel Production: Balancing Quality and Protein Digestibility
by Zhaolu Li, Sisi Zhang, Zihan Gao, Xinyue Guo, Ruohan Wang, Maoqiang Zheng and Guangliang Xing
Gels 2025, 11(7), 524; https://doi.org/10.3390/gels11070524 - 6 Jul 2025
Viewed by 745
Abstract
Tofu quality is critically influenced by coagulants, though their impact on protein digestibility remains underexplored. This study aimed to investigate the effects of calcium sulfate (CaSO4), magnesium chloride (MgCl2), and their combination (CaSO4 + MgCl2) on [...] Read more.
Tofu quality is critically influenced by coagulants, though their impact on protein digestibility remains underexplored. This study aimed to investigate the effects of calcium sulfate (CaSO4), magnesium chloride (MgCl2), and their combination (CaSO4 + MgCl2) on the physicochemical properties and protein digestibility of tofu. Water-holding capacity, cooking loss, texture, protein composition, and protein digestibility were analyzed. The results showed that the CaSO4 + MgCl2 combination yielded a water-holding capacity of 99.16%, significantly higher than CaSO4 tofu (93.73%) and MgCl2 tofu (96.82%), while reducing cooking loss to 2.03% and yielding the highest hardness (897.27 g) and gumminess (765.72). Electrophoresis revealed distinct protein retention patterns, with MgCl2 (0.6% w/v) forming denser gels that minimized protein leakage into soy whey. During in vitro digestion, MgCl2-coagulated tofu exhibited superior soluble protein release (5.33 mg/mL after gastric digestion) and higher intestinal peptide (5.89 mg/mL) and total amino acid (123.06 μmol/mL) levels, indicating enhanced digestibility. Conversely, the CaSO4 + MgCl2 combination showed delayed proteolysis in electrophoresis analysis. These findings demonstrate that coagulant selection directly modulates tofu’s texture, water retention, and protein bioavailability, with MgCl2 favoring digestibility and the hybrid coagulant optimizing physical properties. This provides strategic insights for developing nutritionally enhanced tofu products. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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25 pages, 6040 KB  
Article
Spray-Drying Microencapsulation of Grape Pomace Extracts with Alginate-Based Coatings and Bioaccessibility of Phenolic Compounds
by Josipa Martinović, Rita Ambrus, Mirela Planinić, Gabriela Perković, Gordana Šelo, Ana-Marija Klarić and Ana Bucić-Kojić
Gels 2025, 11(2), 130; https://doi.org/10.3390/gels11020130 - 11 Feb 2025
Viewed by 1868
Abstract
Spray-drying is a common technique for the microencapsulation of bioactive compounds, which is crucial for improving their stability and bioavailability. In this study, the encapsulation efficiency (EE), physicochemical properties and in vitro bioaccessibility of phenolic compounds from spray-dried encapsulated phenol-rich extracts [...] Read more.
Spray-drying is a common technique for the microencapsulation of bioactive compounds, which is crucial for improving their stability and bioavailability. In this study, the encapsulation efficiency (EE), physicochemical properties and in vitro bioaccessibility of phenolic compounds from spray-dried encapsulated phenol-rich extracts of grape pomace, a winery waste, were evaluated. Sodium alginate alone (SA) or in a mixture with gum Arabic (SA-GA) or gelatin (SA-GEL) was used as a coating. SA-GEL achieved the highest EE (95.90–98.01%) and outperformed the intestinal release of phenolics by achieving a bioaccessibility index (BI) for total phenolic compounds of 37.8–96.2%. The release mechanism of phenolics from the microcapsules adhered to Fickian diffusion. Encapsulation significantly improved the BI of individual phenolics, with the highest BI values for gallocatechin gallate (2028.7%), epicatechin gallate (476.4%) and o-coumaric acid (464.2%) obtained from the SA-GEL microcapsules. Structural analysis confirmed amorphous matrices in all systems, which improved solubility and stability. These results suggest that encapsulation by spray-drying effectively protects phenolics during digestion and ensures efficient release in the intestine, which improves bioaccessibility. This study contributes to the understanding of biopolymer-based encapsulation systems, but also to the valorisation of grape pomace as a high-value functional ingredient in sustainable food processing. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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13 pages, 1643 KB  
Article
Quality Characteristics and In Vitro Digestibility of Starch Gel in White Noodles Prepared with Short-Chain Glucan Aggregates (SCGA)
by Jae-Geun Park, Sang-Jin Ye, Seon-Min Oh, Jae-Sung Shin, Ji-Eun Bae, Hyun-Wook Choi and Moo-Yeol Baik
Gels 2025, 11(1), 6; https://doi.org/10.3390/gels11010006 - 26 Dec 2024
Cited by 1 | Viewed by 1246
Abstract
Short-chain glucan aggregates (SCGA), a type of resistant starch (RS) Ⅲ, is produced by debranching amylopectin with pullulanase and inducing self-assembly. Despite its low digestibility and high RS content, SCGA has not been applied to real food systems, especially noodles. The objective of [...] Read more.
Short-chain glucan aggregates (SCGA), a type of resistant starch (RS) Ⅲ, is produced by debranching amylopectin with pullulanase and inducing self-assembly. Despite its low digestibility and high RS content, SCGA has not been applied to real food systems, especially noodles. The objective of this study was to determine the feasibility of low-digestible noodles using SCGA and to evaluate their quality characteristics and in vitro digestibility of starch gel. SCGA-noodles (SN) were prepared by substituting 0, 10, 20, and 25% of wheat flour with SCGA, and non-digestible maltodextrin (NMD) replaced 7% of the flour for comparison. Adding SCGA increased L- and b-values of the dough, resulting in a brighter appearance, while the NMD increased a-values. The substitution with SCGA weakened the gluten network, reducing dough and texture properties. Notably, cooked SN25 broke immediately in the tensile test, indicating substitution up to 20% is feasible in noodles. NMD7 formed sticky dough and showed extensive elongation without breaking. SN20 and SN25 significantly increased RS content and decreased the estimated glycemic index (eGI) compared to the control. However, NMD7 did not significantly reduce in vitro starch digestibility. In conclusion, this research confirmed the potential of SCGA as a low-digestible ingredient for noodles and other food applications. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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21 pages, 2634 KB  
Article
Effect of the Ratio of Protein to Water on the Weak Gel Nonlinear Viscoelastic Behavior of Fish Myofibrillar Protein Paste from Alaska Pollock
by Timilehin Martins Oyinloye and Won Byong Yoon
Gels 2024, 10(11), 737; https://doi.org/10.3390/gels10110737 - 13 Nov 2024
Cited by 2 | Viewed by 1545
Abstract
The linear and nonlinear rheological behaviors of fish myofibrillar protein (FMP) paste with 75%, 82%, and 90% moisture content were evaluated using small-amplitude oscillatory shear (SAOS) and large-amplitude oscillatory shear (LAOS) tests. SAOS revealed pastes with 75% and 82% moisture exhibited solid-like behavior, [...] Read more.
The linear and nonlinear rheological behaviors of fish myofibrillar protein (FMP) paste with 75%, 82%, and 90% moisture content were evaluated using small-amplitude oscillatory shear (SAOS) and large-amplitude oscillatory shear (LAOS) tests. SAOS revealed pastes with 75% and 82% moisture exhibited solid-like behavior, characterized by higher storage modulus (G′) than loss modulus (G″), indicative of weak gel properties with a strong protein interaction. In contrast, the 90% moisture content showed more viscous behavior due to weakened protein–protein entanglements. The frequency exponent (n′ and n″) from the power law equation varied slightly (0.24 to 0.36), indicating limited sensitivity to changes in deformation rate during SAOS. LAOS tests revealed significant structural changes, with Lissajous–Bowditch curves revealing early nonlinearities at 10% strain for 90% moisture content. Decomposed Chebyshev coefficients (e3/e1, v3/v1, S, and T) indicated strain stiffening at lower strains for the 75% and 82% moisture pastes (i.e., < 50% strain for 75% and < 10% strain for 82%), transitioning to strain thinning at higher strains. Additionally, numerical model confirmed the predictability of the 3D printing process from the nonlinear rheological data, confirmed the suitability of the 75% and 82% moisture pastes for applications requiring structural integrity. These insights are essential for optimizing processing conditions in industrial applications. The findings suggest that the 75% and 82% moisture pastes are suitable for applications requiring structural integrity, while the 90% moisture paste is ideal for flow-based processes. These insights are essential for optimizing processing conditions in industrial applications. Full article
(This article belongs to the Special Issue Food Gel-Based Systems: Gel-Forming and Food Applications)
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