Atmospheric Composition and Cloud Cover Observations

A special issue of Atmosphere (ISSN 2073-4433). This special issue belongs to the section "Meteorology".

Deadline for manuscript submissions: closed (15 October 2019) | Viewed by 33202

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Department of Chemistry, Physics and Environment, Universitatea Dunarea de Jos Galati, 800008 Galați, Romania
Interests: atmospheric physics; climate variability; solar-terrestrial interactions; ionosphere and near-Earth environment; clouds
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Dear Colleagues,

This Special Issue of Atmosphere aims at presenting recent achievements in observations of clouds and atmospheric composition. The main focus is on remote sensing and in situ observations at local, regional, or global scale; however, these can be accompanied by modeling approaches and simulations. Scientific articles are invited that investigate the optical, chemical, and physical properties of clouds and cloud cover, and their relation to aerosol content, environmental conditions, or the more eccentric drivers of solar and electric origin. Contributions discussing the impact of cloud cover on atmospheric measurements or link of trace gases variability to natural and anthropogenic processes are equally welcome. We expect manuscripts that examine the progress of atmospheric trace gases retrieval, using data from various generations of space-based instruments, and ground-based measurements. Submission is open to manuscripts that discuss critical issues, e.g., separating between various cloud types, removal of artefacts, or accuracy of vertical profiles. We encourage the scientific community to present observational studies that improve the understanding of the complex feedback between clouds and processes involving various climate essential variables (CEV), e.g., surface radiation budget, water vapor, temperature, lightning, and aerosol properties. Studies that aim at understanding how meteorological conditions, circulation patterns, or teleconnections affect cloud formation mechanisms or the evolution of atmospheric composition are appreciated. Researchers are invited to present the results of the recent pan-European research initiative ACTRIS (Aerosols, Clouds, and Trace Gases Research Infrastructure).   

Prof. Mirela Voiculescu
Guest Editor

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Keywords

  • Clouds
  • Trace gases
  • Satellite retrieval
  • Ground-based observations
  • Atmospheric composition
  • Atmosphere remote sensing

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Published Papers (8 papers)

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Editorial

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2 pages, 168 KiB  
Editorial
Special Issue Atmospheric Composition and Cloud Cover Observations
by Mirela Voiculescu
Atmosphere 2021, 12(1), 56; https://doi.org/10.3390/atmos12010056 - 31 Dec 2020
Viewed by 1355
Abstract
A Special Issue of Atmosphere, “Atmospheric Composition and Cloud Cover Observations”, is focused on presenting some of the latest results of observations of clouds and atmospheric composition, mainly by referring to new equipment or experimental set-ups [...] Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)

Research

Jump to: Editorial

14 pages, 4190 KiB  
Article
Multi-Sensor Observation of a Saharan Dust Outbreak over Transylvania, Romania in April 2019
by Nicolae Ajtai, Horațiu Ștefănie, Alexandru Mereuță, Andrei Radovici and Camelia Botezan
Atmosphere 2020, 11(4), 364; https://doi.org/10.3390/atmos11040364 - 9 Apr 2020
Cited by 13 | Viewed by 3247
Abstract
Mineral aerosols are considered to be the second largest source of natural aerosol, the Saharan desert being the main source of dust at global scale. Under certain meteorological conditions, Saharan dust can be transported over large parts of Europe, including Romania. The aim [...] Read more.
Mineral aerosols are considered to be the second largest source of natural aerosol, the Saharan desert being the main source of dust at global scale. Under certain meteorological conditions, Saharan dust can be transported over large parts of Europe, including Romania. The aim of this paper is to provide a complex analysis of a Saharan dust outbreak over the Transylvania region of Romania, based on the synergy of multiple ground-based and satellite sensors in order to detect the dust intrusion with a higher degree of certainty. The measurements were performed during the peak of the outbreak on April the 24th 2019, with instruments such as a Cimel sun-photometer and a multi-wavelength Raman depolarization lidar, together with an in-situ particle counter measuring at ground level. Remote sensing data from MODIS sensors on Terra and Aqua were also analyzed. Results show the presence of dust aerosol layers identified by the multi-wavelength Raman and depolarization lidar at altitudes of 2500–4000 m, and 7000 m, respectively. The measured optical and microphysical properties, together with the HYSPLIT back-trajectories, NMMB/BSC dust model, and synoptic analysis, confirm the presence of lofted Saharan dust layers over Cluj-Napoca, Romania. The NMMB/BSC dust model predicted dust load values between 1 and 1.5 g/m2 over Cluj-Napoca at 12:00 UTC for April the 24th 2019. Collocated in-situ PM monitoring showed that dry deposition was low, with PM10 and PM2.5 concentrations similar to the seasonal averages for Cluj-Napoca. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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17 pages, 47895 KiB  
Article
Cloud Occurrence Frequency at Puy de Dôme (France) Deduced from an Automatic Camera Image Analysis: Method, Validation, and Comparisons with Larger Scale Parameters
by Jean-Luc Baray, Asmaou Bah, Philippe Cacault, Karine Sellegri, Jean-Marc Pichon, Laurent Deguillaume, Nadège Montoux, Vincent Noel, Geneviève Seze, Franck Gabarrot, Guillaume Payen and Valentin Duflot
Atmosphere 2019, 10(12), 808; https://doi.org/10.3390/atmos10120808 - 13 Dec 2019
Cited by 8 | Viewed by 3596
Abstract
We present a simple algorithm that calculates the cloud occurrence frequency at an altitude site using automatic camera image analysis. This algorithm was applied at the puy de Dôme station (PUY, 1465 m. a.s.l., France) over 2013–2018. Cloud detection thresholds were determined by [...] Read more.
We present a simple algorithm that calculates the cloud occurrence frequency at an altitude site using automatic camera image analysis. This algorithm was applied at the puy de Dôme station (PUY, 1465 m. a.s.l., France) over 2013–2018. Cloud detection thresholds were determined by direct comparison with simultaneous in situ cloud probe measurements (particulate volume monitor (PVM) Gerber). The cloud occurrence frequency has a seasonal cycle, with higher values in winter (60%) compared to summer (24%). A cloud diurnal cycle is observed only in summer. Comparisons with the larger scale products from satellites and global model reanalysis are also presented. The NASA cloud-aerosol transport system (CATS) cloud fraction shows the same seasonal and diurnal variations and is, on average, 11% higher. Monthly variations of the ECMWF ERA-5 fraction of cloud cover are also highly correlated with the camera cloud occurrence frequency, but the values are 19% lower and up to 40% for some winter months. The METEOSAT-SEVIRI cloud occurrence frequency also follows the same seasonal cycle but with a much smaller decrease in summer. The all-sky imager cloud fraction (CF) presents larger variability than the camera cloud occurrence but also follows similar seasonal variations (67% in winter and 44% in summer). This automatic low-cost detection of cloud occurrence is of interest in characterizing altitude observation sites, especially those that are not yet equipped with microphysical instruments and can be deployed to other high-altitude sites equipped with cameras. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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14 pages, 29312 KiB  
Article
An Exceptional Case of Freezing Rain in Bucharest (Romania)
by Simona Andrei, Bogdan Antonescu, Mihai Boldeanu, Luminiţa Mărmureanu, Cristina Antonia Marin, Jeni Vasilescu and Dragoş Ene
Atmosphere 2019, 10(11), 673; https://doi.org/10.3390/atmos10110673 - 1 Nov 2019
Cited by 7 | Viewed by 4415
Abstract
A high-impact freezing rain event affected parts of southeastern Romania on 24–26 January 2019. The freezing rain caused extensive damages in Bucharest, the capital city of Romania. The meteorological analysis highlighted the presence of a particular synoptic pattern involving a high-pressure system advecting [...] Read more.
A high-impact freezing rain event affected parts of southeastern Romania on 24–26 January 2019. The freezing rain caused extensive damages in Bucharest, the capital city of Romania. The meteorological analysis highlighted the presence of a particular synoptic pattern involving a high-pressure system advecting cold air mass at low levels, while at mid-levels a warm and humid intrusion was associated with a low-pressure system of Mediterranean origin. At Bucharest, the vertical profiles from ERA5 and radiosondes emphasized the presence of a thick warm layer between 1000–1400 m above the re-freezing layer close to the surface. A climatology of freezing rain events in Bucharest was built to understand the frequency and intensity of this phenomenon. On average, there were approximately 5 observations of freezing rain in Bucharest per year between 1980–2018. The number of consecutive freezing rain days was used as a proxy for the event severity. Moderate-duration events (2 consecutive days) represented 16 periods of all 59 non-overlapping freezing rain periods in Bucharest and long-duration events (3 consecutive days) represented 3 periods. The monthly distribution showed that freezing rain occurs more frequently between December–February with a maximum in December. The moderate and long-duration freezing rain events were associated with two main sub-synoptic patterns related to the Carpathians lee cyclogenesis. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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16 pages, 3241 KiB  
Article
Estimation of CO2 Emissions from Wildfires Using OCO-2 Data
by Meng Guo, Jing Li, Lixiang Wen and Shubo Huang
Atmosphere 2019, 10(10), 581; https://doi.org/10.3390/atmos10100581 - 25 Sep 2019
Cited by 24 | Viewed by 8328
Abstract
The biomass burning model (BBM) has been the most widely used method for estimation of trace gas emissions. Due to the difficulty and variability in obtaining various necessary parameters of BBM, a new method is needed to quickly and accurately calculate the trace [...] Read more.
The biomass burning model (BBM) has been the most widely used method for estimation of trace gas emissions. Due to the difficulty and variability in obtaining various necessary parameters of BBM, a new method is needed to quickly and accurately calculate the trace gas emissions from wildfires. Here, we used satellite data from the Orbiting Carbon Observatory-2 (OCO-2) to calculate CO2 emissions from wildfires (the OCO-2 model). Four active wildfires in Siberia were selected in which OCO-2 points intersecting with smoke plumes identified by Aqua MODIS (MODerate-resolution Imaging Spectroradiometer) images. MODIS band 8, band 21 and MISR (Multi-angle Imaging SpectroRadiometer) data were used to identify the smoke plume area, burned area and smoke plume height, respectively. By contrast with BBM, which calculates CO2 emissions based on the bottom–top mode, the OCO-2 model estimates CO2 emissions based on the top–bottom mode. We used a linear regression model to compute CO2 concentration (XCO2) for each smoke plume pixel and then calculated CO2 emissions for each wildfire point. The CO2 mass of each smoke plume pixel was added to obtain the CO2 emissions from wildfires. After verifying our results with the BBM, we found that the biases were between 25.76% and 157.11% for the four active fires. The OCO-2 model displays the advantages of remote-sensing technology and is a useful tool for fire-emission monitoring, although we note some of its disadvantages. This study proposed a new perspective to estimate CO2 emissions from wildfire and effectively expands the applied range of OCO-2 satellite data. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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24 pages, 10386 KiB  
Article
Evaluation of Different WRF Parametrizations over the Region of Iași with Remote Sensing Techniques
by Iulian-Alin Roșu, Silvia Ferrarese, Irina Radinschi, Vasilica Ciocan and Marius-Mihai Cazacu
Atmosphere 2019, 10(9), 559; https://doi.org/10.3390/atmos10090559 - 18 Sep 2019
Cited by 9 | Viewed by 3386
Abstract
This article aims to present an evaluation of the Weather Research and Forecasting (WRF) model with multiple instruments when applied to a humid continental region, in this case, the region around the city of Iași, Romania. A series of output parameters are compared [...] Read more.
This article aims to present an evaluation of the Weather Research and Forecasting (WRF) model with multiple instruments when applied to a humid continental region, in this case, the region around the city of Iași, Romania. A series of output parameters are compared with observed data, obtained on-site, with a focus on the Planetary Boundary Layer Height (PBLH) and on PBLH-related parametrizations used by the WRF model. The impact of each different parametrization on physical quantities is highlighted during the two chosen measurement intervals, both of them in the warm season of 2016 and 2017, respectively. The instruments used to obtain real data to compare to the WRF simulations are: a lidar platform, a photometer, and ground-level (GL) meteorological instrumentation for the measurement of temperature, average wind speed, and pressure. Maps of PBLH and 2   m above ground-level (AGL) atmospheric temperature are also presented, compared to a topological and relief map of the inner nest of the WRF simulation. Finally, a comprehensive simulation performance evaluation of PBLH, temperature, wind speed, and pressure at the surface and total precipitable water vapor is performed. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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19 pages, 4384 KiB  
Article
Multiyear Typology of Long-Range Transported Aerosols over Europe
by Victor Nicolae, Camelia Talianu, Simona Andrei, Bogdan Antonescu, Dragoș Ene, Doina Nicolae, Alexandru Dandocsi, Victorin-Emilian Toader, Sabina Ștefan, Tom Savu and Jeni Vasilescu
Atmosphere 2019, 10(9), 482; https://doi.org/10.3390/atmos10090482 - 22 Aug 2019
Cited by 21 | Viewed by 3730
Abstract
In this study, AERONET (Aerosol Robotic Network) and EARLINET (European Aerosol Research Lidar Network) data from 17 collocated lidar and sun photometer stations were used to characterize the optical properties of aerosol and their types for the 2008–2018 period in various regions of [...] Read more.
In this study, AERONET (Aerosol Robotic Network) and EARLINET (European Aerosol Research Lidar Network) data from 17 collocated lidar and sun photometer stations were used to characterize the optical properties of aerosol and their types for the 2008–2018 period in various regions of Europe. The analysis was done on six cluster domains defined using circulation types around each station and their common circulation features. As concluded from the lidar photometer measurements, the typical aerosol particles observed during 2008–2018 over Europe were medium-sized, medium absorbing particles with low spectral dependence. The highest mean values for the lidar ratio at 532 nm were recorded over Northeastern Europe and were associated with Smoke particles, while the lowest mean values for the Angstrom exponent were identified over the Southwest cluster and were associated with Dust and Marine particles. Smoke (37%) and Continental (25%) aerosol types were the predominant aerosol types in Europe, followed by Continental Polluted (17%), Dust (10%), and Marine/Cloud (10%) types. The seasonal variability was insignificant at the continental scale, showing a small increase in the percentage of Smoke during spring and a small increase of Dust during autumn. The aerosol optical depth (AOD) slightly decreased with time, while the Angstrom exponent oscillated between “hot and smoky” years (2011–2015) on the one hand and “dusty” years (2008–2010) and “wet” years (2017–2018) on the other hand. The high variability from year to year showed that aerosol transport in the troposphere became more and more important in the overall balance of the columnar aerosol load. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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14 pages, 11247 KiB  
Article
Wintertime Variations of Gaseous Atmospheric Constituents in Bucharest Peri-Urban Area
by Cristina Antonia Marin, Luminiţa Mărmureanu, Cristian Radu, Alexandru Dandocsi, Cristina Stan, Flori Ţoancă, Liliana Preda and Bogdan Antonescu
Atmosphere 2019, 10(8), 478; https://doi.org/10.3390/atmos10080478 - 20 Aug 2019
Cited by 9 | Viewed by 4011
Abstract
An intensive winter campaign was organized for measuring the surface air pollutants in southeastern Europe. For a three months period, the gas concentrations of NO x , SO 2 , CO, O 3 , and CH 4 as well as meteorological parameters were [...] Read more.
An intensive winter campaign was organized for measuring the surface air pollutants in southeastern Europe. For a three months period, the gas concentrations of NO x , SO 2 , CO, O 3 , and CH 4 as well as meteorological parameters were simultaneously sampled to evaluate the variations and characteristic reactions between the gases during winter at the measuring site. The photochemical production of the ozone was observed through the diurnal variation of ozone and the solar radiation, the maximum concentration for ozone being reached one hour after the maximum value for solar radiation. A non-parametric wind regression method was used to highlight the sources of the air pollutants. The long-range transport of SO 2 and two hotspots for CO from traffic and from residential heating emissions were emphasized. The traffic hotspot situated north of the measuring site, close to the city ring road, is also a hotspot for NO x . The air quality during the cold season was evaluated by comparing the measured gas concentration with the European limits. During the measuring period, the values for NO 2 , CO, and SO 2 concentration were at least two times lower than the European Union pollution limits. Only twice during the study period was the concentration of O 3 higher than the established limits. Full article
(This article belongs to the Special Issue Atmospheric Composition and Cloud Cover Observations)
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