Journal Description
Atmosphere
Atmosphere
is an international, peer-reviewed, open access journal of scientific studies related to the atmosphere published monthly online by MDPI. The Italian Aerosol Society (IAS) and Working Group of Air Quality in European Citizen Science Association (ECSA) are affiliated with Atmosphere and their members receive a discount on the article processing charges.
- Open Access— free for readers, with article processing charges (APC) paid by authors or their institutions.
- High Visibility: indexed within Scopus, SCIE (Web of Science), Ei Compendex, GEOBASE, GeoRef, Inspec, CAPlus / SciFinder, Astrophysics Data System, and other databases.
- Journal Rank: CiteScore - Q2 (Environmental Science (miscellaneous))
- Rapid Publication: manuscripts are peer-reviewed and a first decision is provided to authors approximately 17.7 days after submission; acceptance to publication is undertaken in 2.8 days (median values for papers published in this journal in the second half of 2023).
- Recognition of Reviewers: reviewers who provide timely, thorough peer-review reports receive vouchers entitling them to a discount on the APC of their next publication in any MDPI journal, in appreciation of the work done.
- Testimonials: See what our editors and authors say about the Atmosphere.
- Companion journal: Meteorology.
Impact Factor:
2.9 (2022);
5-Year Impact Factor:
3.0 (2022)
Latest Articles
Seasonal Variation in Short-Term Ambient Air Pollutants and ST-Elevation Myocardial Infarction Admissions: An Innovative Exploration of Air Pollution’s Health Consequences
Atmosphere 2024, 15(5), 590; https://doi.org/10.3390/atmos15050590 (registering DOI) - 12 May 2024
Abstract
Cardiovascular diseases (CVDs) persist as a significant contributor to global morbidity and mortality despite advances in medical technology. Air pollution has emerged as a significant contemporary challenge due to increased energy consumption and rapid economic development. The study utilized multivariable Poisson regression and
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Cardiovascular diseases (CVDs) persist as a significant contributor to global morbidity and mortality despite advances in medical technology. Air pollution has emerged as a significant contemporary challenge due to increased energy consumption and rapid economic development. The study utilized multivariable Poisson regression and Distributed Lag Models (DLM) to assess the link between brief exposure to outdoor air pollutants (PM10—particulate matter with a diameter ≤ 10 μm, NO2—nitrogen dioxide, and O3—ozone) and the risk of acute myocardial infarction with ST-segment elevation (STEMI) hospitalization, stratified by season. The research was conducted from January 2019 to December 2021 at the University Hospital in Timisoara, Romania, and daily records were collected for STEMI admissions, atmospheric pollutant levels, and meteorological parameters. The most pronounced impacts were observed with each 10 μg/m3 increase at lag 07 for PM10 during summer, leading to a 2% increase in STEMI admissions, and for NO2 during spring at lag 07, resulting in a 0.9% rise in CVD incidence. Men, middle-aged adults, and older adults exhibited greater susceptibility to elevated NO2 and PM10 concentrations than women and younger individuals. Brief exposure to diverse air pollutants heightens the likelihood of hospitalization due to STEMI, particularly among men and adults over 45. Effective measures must be implemented to mitigate these impacts, especially for vulnerable populations.
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(This article belongs to the Special Issue New Insights into Exposure and Health Impacts of Air Pollution)
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Protective Effects of Resveratrol on Cytotoxicity of Mouse Hepatic Stellate Cells Induced by PM2.5
by
Mei Zhang, Shanshan Chen, Lirong Bai, Wenqi Chen and Ruijin Li
Atmosphere 2024, 15(5), 588; https://doi.org/10.3390/atmos15050588 (registering DOI) - 12 May 2024
Abstract
The atmosphere’s fine particulate matter (PM2.5) can enter the liver through the circulatory system, leading to hepatic inflammation and fibrosis. As a non-flavonoid polyphenolic compound, resveratrol (RES) has anti-oxidant, anti-inflammatory and hepatoprotective effects, but the molecular mechanisms of liver fibrosis induced
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The atmosphere’s fine particulate matter (PM2.5) can enter the liver through the circulatory system, leading to hepatic inflammation and fibrosis. As a non-flavonoid polyphenolic compound, resveratrol (RES) has anti-oxidant, anti-inflammatory and hepatoprotective effects, but the molecular mechanisms of liver fibrosis induced by PM2.5 exposure are still limited. In this study, we established an in vitro cell model to investigate the intervention effect of RES with different concentrations (5 and 20 μmol/mL) on mouse hepatic stellate cells (mHSCs) injury induced by PM2.5 (100 μg/mL). We determined the cell viability in mHSCs after treatment with PM2.5 or/and RES for 24 h. We investigated the intracellular oxidative stress by detecting the changes in reactive oxygen species (ROS), malondialdehyde (MDA), superoxide dismutase (SOD) and lactate dehydrogenase (LDH) levels. We also measured the protein expressions of fibrosis-related genes (α-SMA, Collagen I and Collagen III) and key genes (SIRT1, NF-κB, NLRP3, Cleaved-Caspase1, IL-1β) in the NLRP3 pathway in mHSCs exposed to PM2.5 with or without RES. The results showed that (1) PM2.5 has cytotoxic effects on mHSCs, whereas RES (5 μmol/L and 20 μmol/L) inhibited PM2.5-induced cytotoxicity and LDH leakage; (2) RES effectively reduces ROS and MDA production caused by PM2.5 while concurrently enhancing SOD levels, thereby improving cellular anti-oxidant capacity; (3) the expression of α-SMA, Collagen I and Collagen III were notably downregulated in the PM2.5 plus RES treatment group compared to the PM2.5-exposed group; (4) RES significantly increased SIRT1 expression and decreased the expression of NF-κB, NLRP3, Cleaved-Caspase1 and IL-1β in mHSCs exposure to PM2.5 compared to the PM2.5 group. These results demonstrate that RES can up-regulate SIRT1 and mitigate PM2.5-induced fibrosis by suppressing oxidative stress in mHSCs and the SIRT1/NF–κB/NLRP3 pathway activated by PM2.5.
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(This article belongs to the Special Issue Composition Analysis and Health Effects of Atmospheric Particulate Matter)
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Development of a Refrigerant-Free Cryotrap Unit for Pre-Concentration of Biogenic Volatile Organic Compounds in Air
by
Xiaoxiao Ding, Daocheng Gong, Qinqin Li, Shiwei Liu, Shuo Deng, Hao Wang, Hongjie Li and Boguang Wang
Atmosphere 2024, 15(5), 587; https://doi.org/10.3390/atmos15050587 (registering DOI) - 11 May 2024
Abstract
Biogenic volatile organic compounds (BVOCs) are key compounds in atmospheric chemistries, but difficult to measure directly. In this study, a pre-concentration unit combined with gas chromatography-mass spectrometry (GC-MS) was developed for the quantitative analysis of 18 BVOCs in ambient air. The analytes are
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Biogenic volatile organic compounds (BVOCs) are key compounds in atmospheric chemistries, but difficult to measure directly. In this study, a pre-concentration unit combined with gas chromatography-mass spectrometry (GC-MS) was developed for the quantitative analysis of 18 BVOCs in ambient air. The analytes are trapped on an empty silonite-coated tube, which is cooled by a thermoacoustic cooler to cryotrap at −150 °C, and then desorbed by rapid heating to 200 °C. The set-up involves neither the exchange of solid adsorbents nor any further condensation or refocusing steps. Reliable operation is ensured by the thermoacoustic cooler, which neither contains a liquid refrigerant nor requires refilling a cryogen. The pre-concentration unit parameters such as water removal temperature, desorption temperature and desorption time were optimized. All compounds had correlation coefficients that were better than 0.95, and the detection limits were 0.005–0.009 ppbv when the injection volume is 400 mL. The repeatability ranges were 0.9–5.8%. The recoveries were ranged from 81.8% to 93.2%. This new method was applied for the first time to measure ambient BVOCs in suburb Guangzhou in summer 2022. Isoprene concentrations ranged from 0.375 ppbv to 2.98 ppbv. In addition, several extremely low-level monoterpenes (e.g., α-pinene, β-pinene, and D-limonene) were also detected by the method.
Full article
(This article belongs to the Special Issue State-of-the-Art Detection and Analysis of Atmospheric Volatile Organic Compounds (VOCs))
Open AccessArticle
Evaluation of Air Quality and Thermal Comfort in University Dormitories in China
by
Yanpeng Wu, Xiaoyu Li, Sheng Zhao, Qianglong Wang, Shanxin Wang, Liyang Yu and Faming Wang
Atmosphere 2024, 15(5), 586; https://doi.org/10.3390/atmos15050586 (registering DOI) - 11 May 2024
Abstract
Most studies on Chinese dormitories are carried out in summer, while few focus on a transition season or winter. This study evaluated the air quality of a student dormitory in a university in the Beijing area by using a questionnaire survey and on-site
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Most studies on Chinese dormitories are carried out in summer, while few focus on a transition season or winter. This study evaluated the air quality of a student dormitory in a university in the Beijing area by using a questionnaire survey and on-site measurements. The CO2 concentration was used as an indoor air quality evaluation index to characterize the freshness of the air, and different window opening conditions in the dormitory were simulated, with corresponding improvement plans proposed. The results of this study revealed that the air quality and thermal comfort of the student dormitories during a transition season and winter fell short of expectations. According to the survey, students who opened their windows frequently had a better subjective perception of the air quality. However, due to the large temperature difference between day and night, more than 80% of the students felt too cold when opening the windows. For daytime conditions, the area of unilateral ventilation window opening should not be less than 0.39 m2, the area of bilateral ventilation window opening should not be less than 0.13 m2, and the time taken to close the windows and doors should not exceed the maximum ventilation interval. Empirical equations were fitted for nighttime conditions based on the CO2 concentration, number of people in the room, and window opening area, resulting in a reasonable window opening area of 0.349 m2~0.457 m2. In sum, this study assessed the air quality status within typical university dormitories across varying seasons, gaining a clear understanding of how different ventilation strategies and occupant densities influence air freshness and thermal comfort. Based on these insights, a practical and optimized window area recommendation was formulated to enhance the indoor environmental quality in these dormitories.
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(This article belongs to the Special Issue Contributions of Emission Inventory to Air Quality)
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Marine Stratus—A Boundary-Layer Model
by
Peter A. Taylor
Atmosphere 2024, 15(5), 585; https://doi.org/10.3390/atmos15050585 (registering DOI) - 11 May 2024
Abstract
A relatively simple 1D RANS model of the time evolution of the planetary boundary layer is extended to include water vapor and cloud droplets plus transfers between them. Radiative fluxes and flux divergence are also included. An underlying ocean surface is treated as
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A relatively simple 1D RANS model of the time evolution of the planetary boundary layer is extended to include water vapor and cloud droplets plus transfers between them. Radiative fluxes and flux divergence are also included. An underlying ocean surface is treated as a source of water vapor and as a sink for cloud or fog droplets. With a constant sea surface temperature and a steady wind, initially dry or relatively dry air will moisten, starting at the surface. Turbulent boundary layer mixing will then lead towards a layer with a well-mixed potential temperature (and so temperature decreasing with height) and well-mixed water vapor mixing ratio. As a result, the air will, sooner or later, become saturated at some level, and a stratus cloud will form.
Full article
(This article belongs to the Special Issue Aerosol-Cloud Interactions in Marine Warm Clouds)
Open AccessArticle
Influence of Spring Precipitation over Maritime Continent and Western North Pacific on the Evolution and Prediction of El Niño–Southern Oscillation
by
Yifan Ma, Fei Huang and Ruihuang Xie
Atmosphere 2024, 15(5), 584; https://doi.org/10.3390/atmos15050584 (registering DOI) - 10 May 2024
Abstract
Previous studies suggested that spring precipitation over the tropical western Pacific Ocean can influence the development of El Niño–Southern Oscillation (ENSO). To identify crucial precipitation patterns for post-spring ENSO evolution, a singular value decomposition (SVD) method was applied to spring precipitation and sea
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Previous studies suggested that spring precipitation over the tropical western Pacific Ocean can influence the development of El Niño–Southern Oscillation (ENSO). To identify crucial precipitation patterns for post-spring ENSO evolution, a singular value decomposition (SVD) method was applied to spring precipitation and sea surface temperature (SST) anomalies, and three precipitation and ENSO types were obtained with each highlighting precipitation over the Maritime Continent (MC) or western north Pacific (WNP). High MC spring precipitation corresponds to the slow decay of a multi-year La Niña event. Low MC spring precipitation is associated with a rapid El Niño-to-La Niña transition. High WNP spring precipitation is related to positive north Pacific meridional mode and induces the El Niño initiation. Among the three ENSO types, ocean current and heat content behave differently. Based on these spring precipitation and oceanic factors, a statistical model was established aimed at predicting winter ENSO state. Compared to a full dynamical model, this model exhibits higher prediction skills in the winter ENSO phase and amplitude for the period of 1980–2022. The explained total variance of the winter Niño-3.4 index increases from 43% to 75%, while the root-mean-squared error decreases from 0.82 °C to 0.53 °C. The practical utility and limitations of this model are also discussed.
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(This article belongs to the Section Meteorology)
Open AccessArticle
A Decadal Change in Atmospheric Nitrogen Deposition at a Rural Site in Southern China
by
Kaige Ren, Yalan Zhou, Jiarui Liu, Ziyin Yu, Xin Ma, Ruotong Si, Zhang Wen, Wen Xu, Aohan Tang, Jianlin Shen, Keith Goulding and Xuejun Liu
Atmosphere 2024, 15(5), 583; https://doi.org/10.3390/atmos15050583 (registering DOI) - 10 May 2024
Abstract
Elevated atmospheric reactive nitrogen (Nr) emissions and the subsequent nitrogen (N) deposition have negatively impacted the global environment, particularly in China. In order to assess the long-term trends in atmospheric N deposition in the south of China, Taojiang County in Hunan Province was
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Elevated atmospheric reactive nitrogen (Nr) emissions and the subsequent nitrogen (N) deposition have negatively impacted the global environment, particularly in China. In order to assess the long-term trends in atmospheric N deposition in the south of China, Taojiang County in Hunan Province was selected as a representative rural area for study. We analyzed interannual variation in atmospheric Nr, including gaseous ammonia (NH3), nitrogen dioxide (NO2), nitrate acid (HNO3) vapor, particulate ammonium (NH4+), and nitrate (NO3−) in air and NH4+-N and NO3−-N in precipitation from 2011 to 2020. The 10-year average atmospheric wet-plus-dry N deposition was 41.9 kg N ha−1 yr−1, which decreased by approximately 24% after 2012, indicating that NH3 and NOx emissions were effectively reduced by emission controls introduced in 2013. Wet deposition accounted for approximately 74% of the total N deposition and was significantly influenced by annual precipitation amount. Reduced N (NH3, pNH4+, and NH4+ in rainwater) was the dominant form, comprising approximately 58% of the total N deposition, while oxidized N (pNO3−, NO2, HNO3, and NO3− in rainwater) accounted for 42% of the total N deposition. Atmospheric HNO3, NO2, and NH3 concentrations and deposition declined by 30–80% over the decade, while particulate NH4+ and NO3− concentrations and deposition remained at relatively stable levels, which suggests that ongoing research and policy should focus on rural particulate pollution. Future strategies must concentrate on the integrated control of NH3 and NOx emissions to mitigate air pollution and protect human health, particularly in rural areas because current abatement efforts are primarily directed toward urban areas and the industrial sector, whereas non-point source NH3 pollution, influenced mainly by agricultural activities, dominates in rural regions.
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(This article belongs to the Topic Accessing and Analyzing Air Quality and Atmospheric Environment)
Open AccessArticle
Analysis of Near-Surface Wind Shear Characteristics over Land in China
by
Ling Yuan, Fengzhi Yang, Xia Ruan, Feng Zou and Qi Luo
Atmosphere 2024, 15(5), 582; https://doi.org/10.3390/atmos15050582 (registering DOI) - 10 May 2024
Abstract
Wind shear is one of the crucial parameters in wind resource assessment and also serves as a vital parameter and basis for determining wind turbines’ selection and hub height. Existing studies have only focused on typical underlying surface areas, but a relatively limited
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Wind shear is one of the crucial parameters in wind resource assessment and also serves as a vital parameter and basis for determining wind turbines’ selection and hub height. Existing studies have only focused on typical underlying surface areas, but a relatively limited comprehensive analysis of wind shear characteristics in different complex environments remains. This study analyzes the daily and monthly variations in wind shear index (α) at the station scale based on the observations from 754 wind measurement towers across land surfaces in China. The distribution and empirical values of wind shear in different wind regions and underlying surface types are also investigated. The research findings indicate that the wind shear index derived from fitting the complete annual average wind speeds at multiple height levels of meteorological towers can accurately characterize the stratification state of the atmospheric boundary layer. The variation pattern of solar radiation influences the daily α value in typical regions. In mountainous and desert areas, the monthly variation tends to be higher in autumn and winter and lower in spring and summer. However, its monthly variation shows relatively smaller fluctuations in plain regions. The comprehensive α value over land regions in China is 0.135. The α values for I, II, III, and IV wind fields are 0.111, 0.163, 0.1, and 0.153, respectively. Its values for mountainous, plains, grassland, and desert regions are 0.12, 0.273, 0.123, and 0.104, respectively. By conducting statistical analysis on α values across different wind regions, guidance is provided for extrapolating surface wind speeds to hub-height wind speeds. This serves as a reference for wind energy resource assessment, wind turbine selection, and hub height determination in the atmospheric boundary layer of China.
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(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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Rainfall Potential and Consequences on Structural Soil Degradation of the Most Important Agricultural Region of Mexico
by
Mariano Norzagaray Campos, Patricia Muñoz Sevilla, Jorge Montiel Montoya, Omar Llanes Cárdenas, María Ladrón de Guevara Torres and Luz Arcelia Serrano García
Atmosphere 2024, 15(5), 581; https://doi.org/10.3390/atmos15050581 (registering DOI) - 9 May 2024
Abstract
This study investigates the historical variability in annual average precipitation in the northwest region of Mexico, aiming to evaluate the cumulative impact of precipitation on soil degradation and associated risks posed by rainfall. Despite being known as “The Agricultural Heart of Mexico
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This study investigates the historical variability in annual average precipitation in the northwest region of Mexico, aiming to evaluate the cumulative impact of precipitation on soil degradation and associated risks posed by rainfall. Despite being known as “The Agricultural Heart of Mexico”, the region’s soil has experienced significant damage to its granulometric structure due to unpredictable rainfall patterns attributed to climate change. Sixteen historical series of average annual rainfall were analyzed as stationary stochastic processes for spectral analysis. The results revealed exponential decay curves in each radial spectrum, indicating a linear relationship between frequency and amplitude. These curves identified initial impulses correlated with moments of severity for structural damages caused by rainfall-induced degradation. The degradation process, exacerbated by water stress, accelerates, as evidenced by maps illustrating approximately 75% soil damage. In the context of climate change and the uncertainty surrounding soil responses to extreme meteorological events, understanding this phenomenon becomes crucial. Recognizing the dynamic nature of soil responses to environmental stressors is essential for effective soil management. Emphasizing the need to employ numerical processes tailored to new environmental considerations related to observed soil damages is crucial for sustainable soil management practices in any region.
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(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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Analysis of Diffusion Characteristics and Influencing Factors of Particulate Matter in Ship Exhaust Plume in Arctic Environment Based on CFD
by
Yuanqing Zhu, Qiqi Wan, Qichen Hou, Yongming Feng, Jia Yu, Jie Shi and Chong Xia
Atmosphere 2024, 15(5), 580; https://doi.org/10.3390/atmos15050580 - 9 May 2024
Abstract
The gradual opening of the Arctic shipping route has made navigation possible. However, the harm caused by ship exhaust emissions is increasingly severe. Therefore, it is necessary to study the diffusion characteristics of ship exhaust plumes during Arctic navigation. The study focuses on
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The gradual opening of the Arctic shipping route has made navigation possible. However, the harm caused by ship exhaust emissions is increasingly severe. Therefore, it is necessary to study the diffusion characteristics of ship exhaust plumes during Arctic navigation. The study focuses on a merchant vessel as the subject of investigation, employing computational fluid dynamics (CFD) simulation techniques to analyze the diffusion characteristics of particulate matter (PM) within ship exhaust plumes under Arctic environmental conditions. The diffusion law of ship exhaust plume PM is clarified, and the influence of three factors, synthetic wind speed, yaw angle and chimney angle, on the PM diffusion is analyzed. It was found that after the PM was discharged from the chimney, the majority of the PM dispersed directly backward along with the external flow field, while a minor fraction lingered at the stern of the ship for an extended period before eventually diffusing backward. Among them, 1235 particles were captured within a range of 200 m from the stern, with a capture rate of 0.6%. When the synthetic wind shows a yaw angle, the capture rate of PM in the interval increases rapidly with the increase of yaw angle, while other factors have less influence on the capture rate of PM. This study provides foundational guidance for predicting PM diffusion from ship exhaust plumes in Arctic environments, thereby enabling more effective strategies for managing such emissions.
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(This article belongs to the Special Issue Sources, Spatio-Temporal Distribution and Health Effects of Atmospheric Compositions (2nd Edition))
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Spatio-Temporal Changes of Vegetation Net Primary Productivity and Its Driving Factors on the Tibetan Plateau from 1979 to 2018
by
Mingwang Li, Qiong Li and Mingxing Xue
Atmosphere 2024, 15(5), 579; https://doi.org/10.3390/atmos15050579 - 9 May 2024
Abstract
The Net Primary Productivity (NPP) of the Tibetan Plateau (TP) has undergone significant changes since the 1980s. The investigation of the spatiotemporal changes of NPP and its driving factors is of significant importance. Here, we analyze the spatial and temporal trends of Net
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The Net Primary Productivity (NPP) of the Tibetan Plateau (TP) has undergone significant changes since the 1980s. The investigation of the spatiotemporal changes of NPP and its driving factors is of significant importance. Here, we analyze the spatial and temporal trends of Net Primary Production (NPP) and the effects of meteorological factors on the NPP change on the Tibetan Plateau (TP) using version 5.0 of the Community Land Model. The results showed that the average NPP was 256 (g C·m2·yr−1) over the past 40 years, with a continuously increasing trend of 2.38 (g C·m2·yr−1). Precipitation was the main factor affecting NPP changes, temperature had no significant effect on NPP changes, while radiation showed a negative trend. Changes in precipitation, temperature and radiation account for approximately 91%, 5.3%, and 3.8% of NPP variation, respectively. Based on grass coverage, we categorized alpine grasslands into three types: high, medium, and low coverage. Our findings indicate the NPP change of the high-coverage grasslands was mainly affected by precipitation, and then the temperature and radiation. Comparatively, the precipitation change is the driving factor of the increased NPP of low-coverage grasslands, but the temperature increase is the negative factor. Our studies have implications for assessing and predicting vegetation responses to future climate change.
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(This article belongs to the Special Issue Ocean–Atmosphere–Land Interactions and Their Roles in Climate Change)
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Enhancement of the Vegetation Carbon Uptake by the Synergistic Approach to Air Pollution Control and Carbon Neutrality in China
by
Xiao Qin, Guangming Shi and Fumo Yang
Atmosphere 2024, 15(5), 578; https://doi.org/10.3390/atmos15050578 - 9 May 2024
Abstract
Carbon sinks provided by land ecosystems play a crucial role in achieving carbon neutrality. However, the future potential of carbon sequestration remains highly uncertain. The impact of pollutant emission reduction (PER) introduced by the proposed synergistic approach to air pollution control and carbon
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Carbon sinks provided by land ecosystems play a crucial role in achieving carbon neutrality. However, the future potential of carbon sequestration remains highly uncertain. The impact of pollutant emission reduction (PER) introduced by the proposed synergistic approach to air pollution control and carbon neutrality on carbon sinks in China has not yet been fully evaluated. In this study, we analyzed the effects of regional carbon-neutral PER policies, global climate change, and their coupled effects on China’s terrestrial gross primary productivity (GPP) by conducting numerical experiments using the weather research and forecasting model coupled with chemistry (WRF-Chem) and the moderate resolution imaging spectroradiometer photosynthesis algorithm (MODIS-PSN). We found that carbon-neutral PER policies could promote GPP growth in most regions of China in 2060, particularly during April and October, resulting in a total increase of at least 21.84 TgC compared to that in 2016, which offset the adverse effects of global climate change up to fourfold. The aerosol radiative effects drive GPP growth under carbon-neutral PER policies, primarily through an increase in daily minimum temperature during winter and an increase in shortwave radiation during other seasons. Our research highlights that reducing pollutant emissions enhances future potential for carbon sequestration, revealing positive feedback towards achieving the target of carbon neutrality.
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(This article belongs to the Section Climatology)
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Examining UV Radiation Patterns in Relation to Particulate Matter and Atmospheric Conditions in Arid, Unclouded Skies
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Abdullrahman Maghrabi, Badr Alharbi and Abdulah Aldosari
Atmosphere 2024, 15(5), 577; https://doi.org/10.3390/atmos15050577 - 9 May 2024
Abstract
This study investigates the influences of air temperature (T), relative humidity (RH), wind speed (WS), clearance index (KT), particulate matter (PM) concentrations (PM10 and PM2.5), and aerosol optical depth (AOD) on ultraviolet (UV) radiation during clear skies in Riyadh, central
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This study investigates the influences of air temperature (T), relative humidity (RH), wind speed (WS), clearance index (KT), particulate matter (PM) concentrations (PM10 and PM2.5), and aerosol optical depth (AOD) on ultraviolet (UV) radiation during clear skies in Riyadh, central Saudi Arabia. The observational dataset utilized in this study comprises global solar radiation (G), UVA radiation, AOD measurements, and PM concentrations. The data were collected from 2014 to 2015 at the King Abdulaziz City for Science and Technology (KACST) campus in Riyadh. Regression analyses were conducted to investigate the relationships between UV radiation and the considered variables. The methodology is based on the least square method and associated statistical tests. The findings of this study provide valuable insights into the impacts of meteorological variables and aerosols on UV radiation, contributing to the understanding of environmental and industrial applications in the Arabian Peninsula. The analyses showed that the strengths and magnitudes differed from one variable to another. No significant correlations between UVA radiation (315–400 nm) and hourly and daily values of PM2.5 were found. Moreover, no significant correlations were seen between daily values of the UVA radiation and RH and between the UVB (280–315 nm) and PM10. The rest of the correlations (between UV radiation and the PM10 and meteorological variables) were found to be significant. While WS, the ratio of the PM concentrations (PM2.5/PM10), KT, and T exhibited positive correlations with UV radiation, the rest of the variables had anti-correlations with UV radiation. The influences of T, WS, and RH on ambient PM concentrations during the considered period were taken into account, and it was found that the PM concentrations correlate, with different magnitudes and strengths, positively with T and negatively with RH and WS.
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(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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Experimental Study of the Reaction of OH Radicals with Carbonyl Sulfide between 365 and 960 K: Kinetics and Products
by
Yuri Bedjanian
Atmosphere 2024, 15(5), 576; https://doi.org/10.3390/atmos15050576 - 8 May 2024
Abstract
Reaction OH + OCS ® products (1) has been studied in a discharge–flow reactor combined with modulated molecular beam mass spectrometry. The reaction rate constant has been determined under pseudo-first-order conditions through monitoring OH decays in a high excess of OCS: k1
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Reaction OH + OCS ® products (1) has been studied in a discharge–flow reactor combined with modulated molecular beam mass spectrometry. The reaction rate constant has been determined under pseudo-first-order conditions through monitoring OH decays in a high excess of OCS: k1 = (2.35 ± 0.25) × 10−12 exp(−(2144 ± 56)/T) cm3 molecule−1 s−1 at T = 365–960 K (the uncertainties represent precision at the 2σ level, the total 2σ relative uncertainty including statistical and systematic errors on the rate constant being 20% at all temperatures). The rate constant of reaction (1) was found to be similar at a total helium pressure of 1, 2, and 8 torr at around 500 K. The SH radical was identified as the primary product of the reaction, and its yield was determined to be about 100% at T = 500 and 750 K. The kinetic and mechanistic data from the present study are compared to previous experimental and theoretical work.
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(This article belongs to the Special Issue Reaction Mechanisms and Chemical Kinetics in Atmospheric Chemistry)
Open AccessArticle
Overheating in the Tree Shade of Urban Parks: A Field Study of Thermal Adaption in China
by
Zhongjun Zhang, Yaqian Wang and Dangwei Zhu
Atmosphere 2024, 15(5), 575; https://doi.org/10.3390/atmos15050575 - 8 May 2024
Abstract
With increased atmospheric temperature, temperatures in the shade of trees in parks also increase, and people are faced with high temperature challenges. In this study, thermal comfort in the shade of the trees of an urban park during summer in China was assessed.
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With increased atmospheric temperature, temperatures in the shade of trees in parks also increase, and people are faced with high temperature challenges. In this study, thermal comfort in the shade of the trees of an urban park during summer in China was assessed. The subjective responses of the respondents were recorded via questionnaires, and environment parameters were measured. The results show that the air temperature in the shade was 31.1 ± 3.0 °C during the day, and that it peaked at 36.9 °C; the globe temperature was 31.3 ± 3.1 °C, and it peaked at 40.1 ℃. Respondents’ clothing insulation was 0.31 ± 0.08 clo, and the effect of clothing adjustment on thermal adaptation was limited. Thermal sensation is linearly related to standard effective temperature (SET), and the upper limit of 80% acceptable SET was 32.1 °C. At different temperature values, the proportion of expected airflow enhancement exceeded 50%. The respondents preferred a neutral-warm sensation. Moreover, there was an obvious thermal adaptation, with thermal history and psychological adaptation being the main factors affecting thermal comfort. This study confirmed the value of shade and provided us with guidance for park planning and design.
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(This article belongs to the Section Biometeorology)
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Application of Effective Conversion Rates between NO and NO2 in a Standard Airport Dispersion Model System
by
Ulf Janicke
Atmosphere 2024, 15(5), 574; https://doi.org/10.3390/atmos15050574 - 8 May 2024
Abstract
The NO/NO2/O3 reaction mechanism of the standard VDI 3783 Part 19 was coupled to the Lagrangian particle model LASAT and quasi-stationary, individual plumes were calculated for a point source under various conditions. First-order conversion rates between NO and NO2
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The NO/NO2/O3 reaction mechanism of the standard VDI 3783 Part 19 was coupled to the Lagrangian particle model LASAT and quasi-stationary, individual plumes were calculated for a point source under various conditions. First-order conversion rates between NO and NO2 were derived by fitting to these plumes and further simplified to sets of categorized conversion rates which depend on background NO2 concentration, atmospheric stability and time of the day. The rates were applied in the standard airport dispersion model system LASPORT and compared to measured NO2 concentrations at Los Angeles International Airport. The agreement between modelled and measured NO2 concentrations (weekly averages) and ratios NO2 over NOx at monitor stations dominated by airport emissions was in most cases better than a factor of 2 with a Pearson correlation coefficient of about 0.9 or above.
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(This article belongs to the Special Issue Atmospheric Dispersion and Chemistry Models: Advances and Applications (2nd Edition))
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Open AccessArticle
Modeling Yield of Irrigated and Rainfed Bean in Central and Southern Sinaloa State, Mexico, Based on Essential Climate Variables
by
Omar Llanes Cárdenas, Rosa D. Estrella Gastélum, Román E. Parra Galaviz, Oscar G. Gutiérrez Ruacho, Jeován A. Ávila Díaz and Enrique Troyo Diéguez
Atmosphere 2024, 15(5), 573; https://doi.org/10.3390/atmos15050573 - 7 May 2024
Abstract
The goal was to model irrigated (IBY) and rainfed (RBY) bean yields in central (Culiacán) and southern (Rosario) Sinaloa state as a function of the essential climate variables soil moisture, temperature, reference evapotranspiration, and precipitation. For Sinaloa, for the period 1982–2013 (October–March), the
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The goal was to model irrigated (IBY) and rainfed (RBY) bean yields in central (Culiacán) and southern (Rosario) Sinaloa state as a function of the essential climate variables soil moisture, temperature, reference evapotranspiration, and precipitation. For Sinaloa, for the period 1982–2013 (October–March), the following were calculated: (a) temperatures, (b) average degree days for the bean, (c) cumulative reference evapotranspiration, and (d) cumulative effective precipitation. For essential climate variables, (e) daily soil moisture obtained from the European Space Agency and (f) IBY and RBY from the Agrifood and Fisheries Information Service were used. Multiple linear regressions were significant for predicting IBY–RBY (dependent variables) as a function of essential climate variables (independent variables). The four models obtained were significantly predictive: IBY–Culiacán (Pearson correlation (PC) = 0.590 > Pearson critical correlation (CPC) = |0.349|), RBY–Culiacán (PC = 0.734 > CPC = |0.349|), IBY–Rosario (PC = 0.621 > CPC = |0.355|), and RBY–Rosario (PC = 0.532 > CPC = |0.349|). Due to the lack of irrigation depth data, many studies only focus on modeling RBY; this study is the first in Sinaloa to predict IBY and RBY based on essential climate variables, contributing to the production of sustainable food.
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(This article belongs to the Section Climatology)
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Open AccessReview
Review on Sampling Methods and Health Impacts of Fine (PM2.5, ≤2.5 µm) and Ultrafine (UFP, PM0.1, ≤0.1 µm) Particles
by
Balendra V. S. Chauhan, Karina Corada, Connor Young, Kirsty L. Smallbone and Kevin P. Wyche
Atmosphere 2024, 15(5), 572; https://doi.org/10.3390/atmos15050572 - 7 May 2024
Abstract
Airborne particulate matter (PM) is of great concern in the modern-day atmosphere owing to its association with a variety of health impacts, such as respiratory and cardiovascular diseases. Of the various size fractions of PM, it is the finer fractions that are most
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Airborne particulate matter (PM) is of great concern in the modern-day atmosphere owing to its association with a variety of health impacts, such as respiratory and cardiovascular diseases. Of the various size fractions of PM, it is the finer fractions that are most harmful to health, in particular ultrafine particles (PM0.1; UFPs), with an aerodynamic diameter ≤ 100 nm. The smaller size fractions, of ≤2.5 µm (PM2.5; fine particles) and ≤0.1 µm (PM0.1; ultrafine particles), have been shown to have numerous linkages to negative health effects; however, their collection/sampling remains challenging. This review paper employed a comprehensive literature review methodology; 200 studies were evaluated based on the rigor of their methodologies, including the validity of experimental designs, data collection methods, and statistical analyses. Studies with robust methodologies were prioritised for inclusion. This review paper critically assesses the health risks associated with fine and ultrafine particles, highlighting vehicular emissions as the most significant source of particulate-related health effects. While coal combustion, diesel exhaust, household wood combustors’ emissions, and Earth’s crust dust also pose health risks, evidence suggests that exposure to particulates from vehicular emissions has the greatest impact on human health due to their widespread distribution and contribution to air pollution-related diseases. This article comprehensively examines current sampling technologies, specifically focusing on the collection and sampling of ultrafine particles (UFP) from ambient air to facilitate toxicological and physiochemical characterisation efforts. This article discusses diverse approaches to collect fine and ultrafine particulates, along with experimental endeavours to assess ultrafine particle concentrations across various microenvironments. Following meticulous evaluation of sampling techniques, high-volume air samplers such as the Chem Vol Model 2400 High Volume Cascade Impactor and low-volume samplers like the Personal Cascade Impactor Sampler (PCIS) emerge as effective methods. These techniques offer advantages in particle size fractionation, collection efficiency, and adaptability to different sampling environments, positioning them as valuable tools for precise characterisation of particulate matter in air quality research and environmental monitoring.
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(This article belongs to the Section Air Quality and Human Health)
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Open AccessArticle
Sand Supply Affects Wind Erosion Efficiency and Sand Transport on Sand-Cemented Body Mulch Bed
by
Jie Zhou, Haifeng Wang and Beibei Han
Atmosphere 2024, 15(5), 571; https://doi.org/10.3390/atmos15050571 - 7 May 2024
Abstract
Sand-cemented bodies (SCBs) are naturally distributed in some interdune corridors in the central Taklimakan Desert, northwest China. In this study, field-collected SCB particles were used as the experimental material, and wind tunnel experiments were conducted with different sand supplies, wind velocities, and SCB
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Sand-cemented bodies (SCBs) are naturally distributed in some interdune corridors in the central Taklimakan Desert, northwest China. In this study, field-collected SCB particles were used as the experimental material, and wind tunnel experiments were conducted with different sand supplies, wind velocities, and SCB coverages to evaluate SCB wind erosion efficiency and vertical mass flux. The results showed that wind erosion efficiency decreased as SCB coverage increased. When the SCB coverage was above 40%, sand deposition processes occurred only under saturated sand flow, while sand transport remained unaffected by increases in SCB coverage under unsaturated sand flow. Under saturated flow, the highest concentrations of transported sand were found at 0–6 cm above the surface, and the main sand bed process was deposition. The sand bed process changed from aeolian erosion to deposition with increasing SCB coverage and tended to remain stable until the SCB coverage exceeded 40%. By contrast, under unsaturated sand flow, the sand bed process was primarily aeolian erosion, and the highest concentrations of transported sand were found at 0–4 cm above the surface. At high SCB coverage levels (more than 40%), a general balance between aeolian erosion and deposition processes was reached. In summary, increasing SCB coverage had a significant impact on surface wind erosion processes. Thus, SCBs can be used as a novel sand retention material.
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(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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Open AccessArticle
Resolving the Loss of Intermediate-Size Speech Aerosols in Funnel-Guided Particle Counting Measurements
by
Tayeb Kakeshpour and Adriaan Bax
Atmosphere 2024, 15(5), 570; https://doi.org/10.3390/atmos15050570 - 7 May 2024
Abstract
Modeling of airborne virus transmission and protection against it requires knowledge of the amount of biofluid emitted into the atmosphere and its viral load. Whereas viral concentrations in biofluids are readily measured by quantitative PCR, the total volume of fluids aerosolized during speaking,
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Modeling of airborne virus transmission and protection against it requires knowledge of the amount of biofluid emitted into the atmosphere and its viral load. Whereas viral concentrations in biofluids are readily measured by quantitative PCR, the total volume of fluids aerosolized during speaking, as measured by different researchers using various technologies, differs by several orders of magnitude. We compared collection methods in which the aerosols first enter into a low-humidity chamber either by direct injection or via commonly used funnel and tubing arrangements, followed by standard optical particle sizer measurement. This “collect first, measure later” approach sacrifices the recording of the temporal correlation between aerosol generation and sound types such as plosives and vowels. However, the direct-injection mode prevents inertia deposition associated with the funnel arrangements and reveals far more intermediate-size (5–20 μm in diameter) particles that can dominate the total mass of ejected respiratory aerosol. The larger aerosol mass observed with our method partially reconciles the large discrepancy between the SARS-CoV-2 infectious dose estimated from superspreader event analyses and that from human challenge data. Our results also impact measures to combat airborne virus transmission because they indicate that aerosols that settle faster than good room ventilation rates can dominate this process.
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(This article belongs to the Special Issue Atmospheric Bioaerosols: Detection, Characterization and Modelling)
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