Search Results (613)

We report on the welding of optical borosilicate glass to an unpolished copper substrate (surface Ra of 0.27 µm and Rz of 1.89 µm) using bursts of femtosecond laser pulses. The present paper puts forth the hypothesis that glass–metal welding with a gap is contingent upon the ejection of molten jets of glass. We have ascertained the impact of pulse energy and focal position on weldability. This finding serves to substantiate our initial hypothesis and provides a framework for understanding the conditions under which this hypothesis is applicable. Under optimal conditions, but without the assistance of any clamping system, our welded samples maintained a breaking resistance of up to 10.9 MPa. Full article

Stress fields imparted with an ultrafast laser can correct low spatial frequency surface figure error of mirrors through ultrafast laser stress figuring (ULSF): the formation of nanograting structures within the bulk substrate generates localized stress, creating bending moments that equilibrize via wafer deformation. For ULSF to be used as an optical figuring process, the ultrafast laser generated stress must be effectively permanent or risk unwanted figure drift. Two isochronal annealing experiments were performed to measure ultrafast laser-generated stress stability in fused silica and Corning ultra-low expansion (ULE) wafers. The first experiment tracked changes to induced astigmatism up to 1000 °C on 25.4 mm-diameter wafers. Only small changes were measured after each thermal cycle up to 500 °C for both materials, but significant changes were observed at higher temperatures. The second experiment tracked stress changes in fused silica and ULE up to 500 °C but with 4 to 16× higher signal-to-noise ratio. Change in trefoil on 100 mm-diameter wafers was measured, and the induced stress in fused silica and ULE was found to be stable after thermal cycling up to 300 °C and 200 °C, respectively, with larger changes at higher temperatures. Full article

Glass enjoys a wide range of applications thanks to its superior optical properties and chemical stability. Conventional glass bonding techniques suffer from low efficiency, limited precision, and high cost. Moreover, for multilayer glass bonding, repeated alignment is often required, further complicating the process. These limitations have become major constraints on the advancement of microfluidic chip technologies. Laser bonding of microfluidic chips offers high precision and efficiency. This research first uses an ultrafast laser system to investigate how processing parameters affect weld morphology, identifying the optimal parameter range. Then, this paper proposes two methods for ultrafast-laser bonding of multilayer glass with different thicknesses and performs preliminary experiments to demonstrate their feasibility. The research in this paper could expand the fabrication method of microfluidic chips and lay a foundation for the wider application of microfluidic chips. Full article

In this paper, we develop a peridynamic computational framework to analyze thermomechanical interactions in fractured thin films subjected to ultrashort-pulsed laser excitation, employing nonlocal discrete material point discretization to eliminate mesh dependency artifacts. The generalized Cattaneo–Fourier thermal flux formulation uncovers contrasting dynamic responses: hyperbolic heat propagation ($F_T=0$) generates intensified temperature localization and elevates transient crack-tip stress concentrations relative to classical Fourier diffusion ($F_T=1$). A GSSSS (Generalized Single Step Single Solve) i-Integration temporal scheme achieves oscillation-free numerical solutions across picosecond-level laser–matter interactions, effectively resolving steep thermal fronts through adaptive stabilization. These findings underscore hyperbolic conduction’s essential influence on stress-mediated fracture evolution during ultrafast laser processing, providing critical guidelines for thermal management in micro-/nano-electromechanical systems. Full article

Chemically strengthened glass is widely used for its remarkable fracture strength, mechanical performance, and scratch resistance. Assessing its hardness is crucial to evaluating improvements from chemical tempering. However, conventional methods like Vickers hardness tests are destructive, altering the sample surface. This study presents a novel, rapid, and nondestructive testing (NDT) approach by correlating the nonlinear refractive index (n₂) with surface hardness. Using ultrafast laser pulses, we measured the n₂ cross-section via the nonlinear ellipse rotation (NER) signal in Gorilla^®-type glass subjected to ion exchange (Na⁺ by K⁺). A microscope objective lens provided a penetration resolution of ≈5.5 μm, enabling a localized NER signal analysis. We demonstrate a correlation between the NER signal and hardness, offering a promising pathway for advanced, noninvasive characterization. This approach provides a reliable alternative to traditional destructive techniques, with potential applications in industrial quality control and material science research. Full article

Optically pumped semiconductor disk lasers—known as vertical-external-cavity surface-emitting lasers (VECSELs)—are promising devices for ultrashort pulse formation. For it, a “SESAM-free” approach labeled “self-mode-locking” received considerable attention in the past decade, relying solely on a chip-related nonlinear optical property which can establish adequate pulsing conditions—thereby suggesting a reduced reliance on a semiconductor saturable-absorber mirror (the SESAM) in the cavity. Self-mode-locked (SML) VECSELs with sub-ps pulse durations were reported repeatedly. This motivated investigations on a Kerr-lensing type effect acting as an artificial saturable absorber. So-called Z-scan and ultrafast beam-deflection experiments were conducted to emphasize the role of nonlinear lensing in the chip for pulse formation. Recently, in addition to allowing stable ultrashort pulsed operation, self-starting mode-locked operation gave rise to another emission regime related to frequency comb formation. While amplitude-modulated combs relate to signal peaks in time, providing a so-called pulse train, a frequency-modulated comb is understood to cause quasi continuous-wave output with its sweep of instantaneous frequency over the range of phase-locked modes. With gain-bandwidth-enhanced chips, as well as with an improved understanding of the impacts of dispersion and nonlinear lensing properties and cavity configurations on the device output, an enhanced employment of SML VECSELs is to be expected. Full article

We demonstrate a novel bidirectional mode-locked ultrafast fiber laser based on an asymmetric dual-cavity architecture that enables freely tunable repetition rate differentials at the kilohertz level, while maintaining inherent common-mode noise suppression through precision thermomechanical stabilization. Through cascaded amplification and nonlinear temporal compression, we obtained bidirectional pulse durations of 33.2 fs (clockwise) and 61.6 fs (counterclockwise), respectively. The developed source demonstrates exceptional capability for asynchronous optical sampling applications, particularly in enabling the compact implementation of real-time measurement systems such as terahertz time-domain spectroscopy (THz-TDS) systems. Full article

Laser-induced periodic surface structures (LIPSSs) produced via ultrafast laser-induced oxidation offer a promising route for high-quality nanostructuring, with reduced thermal damage compared to conventional ablation-based methods. However, the influence of laser repetition frequency on the formation and morphology of oxidized LIPSSs remains insufficiently explored. In this study, we systematically investigate the effects of varying the femtosecond laser repetition frequency from 1 kHz to 100 kHz while keeping the total pulse number constant on the oxidation-induced LIPSSs formed on amorphous silicon films. Scanning electron microscopy and Fourier analysis reveal a transition between two morphological regimes with increasing repetition frequency: at low frequencies, the long inter-pulse intervals result in irregular, disordered oxidation patterns; at high frequencies, closely spaced pulses promote the formation of highly ordered, periodic surface structures. Statistical measurements show that the laser-modified area decreases with frequency, while the LIPSS period remains relatively stable and the ridge width exhibits a peak at 10 kHz. Finite-difference time-domain (FDTD) and finite-element simulations suggest that the observed patterns result from a dynamic balance between light-field modulation and oxidation kinetics, rather than thermal accumulation. These findings advance the understanding of oxidation-driven LIPSS formation dynamics and provide guidance for optimizing femtosecond laser parameters for precise surface nanopatterning. Full article

In recent years, ultrafast bursts with high power have been applied in many significant fields. However, the peak power of the pulse train generated by fiber lasers is limited by fiber characteristics from nonlinear effects, which can only be at the level of milliwatt. In this research, the pulse frequency is reduced by an AOM pulse picker-integrated modulator. With M2 and pulse width guaranteed, the frequency of the reduced pulse train is amplified by a solid-state three-stage Nd:YVO₄ amplifier system. Finally, the peak power of the pulse train is increased. The final output pulse repetition rate of the experiment is 1 MHz with a pulse width of 8.09 picoseconds and a peak power of up to 3.7 MW. Full article

This fundamental understanding of molecular structure–NLO property relationships provides critical design principles for next-generation optical limiting materials, quantum photonic devices, and ultrafast nonlinear optical switches, addressing the growing demand for high-performance organic optoelectronic materials in laser protection and photonic computing applications. In this study, it was observed that selenophene-incorporated fused D-A-D architectures exhibit a remarkable enhancement in two-photon absorption characteristics. By strategically modifying the heteroatomic composition of the Y6-derived fused-ring core, replacing thiophene (BDS) with selenophene (BDSe), the optimized system achieves unprecedented NLO performance. BDSe displays a nonlinear absorption coefficient (β) of 3.32 × 10⁻¹⁰ m/W and an effective two-photon absorption cross-section (σ_TPA) of 2428.2 GM under 532 nm with ns pulse excitation. Comprehensive characterization combining Z-scan measurements, transient absorption spectroscopy, and DFT calculations reveals that the heavy atom effect of selenium induces enhanced spin–orbit coupling, optimized intramolecular charge transfer dynamics and stabilized excited states, collectively contributing to the superior reverse saturable absorption behavior. It is believed that this molecular engineering strategy establishes critical structure–property relationships for the rational design of organic NLO materials. Full article

This paper introduces a single-shot ultrafast imaging technique termed wavelength and polarization time-encoded ultrafast raster imaging (WP-URI). By integrating raster imaging principles with wavelength- and polarization-based temporal encoding, the system uses a spatial raster mask and time–space mapping to aggregate multiple two-dimensional temporal raster images onto a single detector plane, thereby enabling the effective spatial separation and extraction of target information. Finally, the target dynamics are recovered using a reconstruction algorithm based on the Nyquist–Shannon sampling theorem. Numerical simulations demonstrate the single-shot acquisition of four dynamic frames at 25 trillion frames per second (Tfps) with an intrinsic spatial resolution of 50 line pairs per millimeter (lp/mm) and a wide field of view. The WP-URI technique achieves unparalleled spatio-temporal resolution and frame rates, offering significant potential for investigating ultrafast phenomena such as matter interactions, carrier dynamics in semiconductor devices, and femtosecond laser–matter processes. Full article

High-order harmonic generation in atomic systems driven by laser fields with tailored symmetries provides a powerful approach for producing structured ultrafast light sources. In this work, we theoretically investigate the ellipticity control of high-order harmonics emitted from helium atoms exposed to orthogonally polarized two-color laser pulses with a 1:3 frequency ratio. The polarization properties of the harmonics are governed by the interplay between the spatial symmetry of the driving field and the atomic potential. By numerically solving the time-dependent Schrödinger equation, we show that fine-tuning the relative phase and amplitude ratio between the fundamental and third-harmonic components enables selective symmetry breaking, resulting in the emission of elliptically and circularly polarized harmonics. Remarkably, we achieve near-perfect circular polarization (ellipticity ≈ 0.995) for the 5th harmonic, as well as highly circularly polarized 17th (0.945), 21st (0.96), and 23rd (0.935) harmonics, demonstrating a level of polarization control and efficiency that exceeds previous schemes. Our results highlight the advantage of using a 1:3 frequency ratio orthogonally polarized two-color laser field over the conventional 1:2 configuration, offering a promising route toward tunable attosecond light sources with tailored polarization characteristics. Full article

Laser-generated structures have a huge potential to induce an alignment of biological cells, which may be important for various fields in medicine and biotechnology. We describe the formation of fs-laser-induced micro- and nanostructures for achieving the directed growth of Schwann cells, a type of glial cell that can support the regeneration of nerve pathways by guiding the neuronal axons in the direction of their alignment. Polymer surfaces, i.e., polycarbonate (PC) or cellulose acetate butyrate (CAB), were exposed to the beam of a 1040 nm Yb-based amplified fs-laser system with a pulse length of about 350 fs. With appropriate parameters, the laser exposure resulted in a surface topography with oriented micro-grooves, which, for PC, were covered with nano-ripples. Schwann cell growth on these substrates was inspected after 3 to 5 days of cultivation by means of scanning electron microscopy (SEM). We show that Schwann cells can grow in a certain direction, predetermined by micro-groove or nano-ripple orientation. In contrast, cells cultivated on randomly oriented nanofibers or unstructured surfaces show an omnidirectional growth behavior. This method may be used in the future to produce nerve conduits for the treatment of injuries to the peripheral nervous system. Full article

This article presents a novel method for fabricating repeatable and uniform surface-enhanced Raman scattering (SERS) substrates. The proposed method consists of two steps: (1) the fabrication of nanohole arrays using advanced femtosecond laser-induced two-photon polymerization (TPP) technology; and (2) the deposition of 9 nm thick silver nanoparticles on the nanohole arrays. The proposed nanohole arrays were optimized at the diameter, and the thickness of the silver film at two parameters. Regarding SERS substrates, a limit of detection of 10⁻¹⁰ M (rhodamine 6G) and analytical enhancement factors up to 3.5 × 10⁴ were achieved. At 1361 cm⁻¹, the relative standard deviation (RSD) of the characteristic peak was 5.5%, demonstrating a highly reproducible SERS substrate. Full article

This study introduces an innovative analytical solution to the time-fractional Cattaneo heat conduction equation, which models photothermal transport in metallic thin films subjected to short laser pulse irradiation. The model integrates the Caputo fractional derivative of order 0 < p ≤ 1, addressing non-Fourier heat conduction characterized by finite wave speed and memory effects. The equation is nondimensionalized through suitable scaling, incorporating essential elements such as a newly specified laser absorption coefficient and uniform initial and boundary conditions. A hybrid approach utilizing the finite Fourier cosine transform (FFCT) in spatial dimensions and the Laplace transform in temporal dimensions produces a closed-form solution, which is analytically inverted using the two-parameter Mittag–Leffler function. This function inherently emerges from fractional-order systems and generalizes traditional exponential relaxation, providing enhanced understanding of anomalous thermal dynamics. The resultant temperature distribution reflects the spatiotemporal progression of heat from a spatially Gaussian and temporally pulsed laser source. Parametric research indicates that elevating the fractional order and relaxation time amplifies temporal damping and diminishes thermal wave velocity. Dynamic profiles demonstrate the responsiveness of heat transfer to thermal and optical variables. The innovation resides in the meticulous analytical formulation utilizing a realistic laser source, the clear significance of the absorption parameter that enhances the temperature amplitude, the incorporation of the Mittag–Leffler function, and a comprehensive investigation of fractional photothermal effects in metallic nano-systems. This method offers a comprehensive framework for examining intricate thermal dynamics that exceed experimental capabilities, pertinent to ultrafast laser processing and nanoscale heat transfer. Full article