Photocatalytic Properties and Chemical Durability of CaO-B2O3-V2O5 Borovanadate Glasses
Abstract
:1. Introduction
2. Experimental Procedures
2.1. Sample Preparation
2.2. Durability Testing
2.3. Photocatalyic Activity
3. Results and Discussion
3.1. Chemical Durability
3.1.1. Variation in Weight Loss and Dissolution Rate (DR)
- The weight loss of sample A4 rapidly increased to reach 11% in 120 h.
- The sample A1 showed a very low weight loss of nearly 1% in 120 h.
- A similar weight loss of 5% was recorded for A2 and A3 samples.
3.1.2. Variation of the pH
3.2. Photocatalytic Activity
3.2.1. Effect of V2O5 and Modeling of Photodegradation Kinetics
3.2.2. Effect of Catalyst Loading and of Initial MB Concentration
4. Conclusions
Supplementary Materials
Author Contributions
Funding
Data Availability Statement
Acknowledgments
Conflicts of Interest
References
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Glass No. | CaO | B2O3 | V2O5 | ρ [12] | Tg ± 6° [12] | DR (pH = 7) | DR (pH = 4) |
---|---|---|---|---|---|---|---|
A1 | 40 | 60 | 0 | 2.603 | 650 | (3.76 ± 0.20) × 10−7 | (4.74 ± 0.20) × 10−7 |
A2 | 40 | 50 | 10 | 2.669 | 570 | (1.58 ± 0.20) × 10−6 | (4.18 ± 0.20) × 10−6 |
A3 | 40 | 40 | 20 | 2.749 | 480 | (2.05 ± 0.20) × 10−6 | (6.74 ± 0.20) × 10−6 |
A4 | 40 | 30 | 30 | 2.853 | 430 | (5.48 ± 0.20) × 10−6 | (8.95 ± 0.20) × 10−6 |
Catalyst | Concentration of Catalyst | Concentration of Dye | Light Source | Photocatalytique Degradation | Ref |
---|---|---|---|---|---|
Zn3(VO4)2/BiVO4 | 0.7 g/L | - | Visible light | 98% at 90 min | [73] |
CuO-BiVO4 | 0.6 g/L | 10 mg/L | Visible light | 92% at 240 min | [74] |
SrBi3VO8 | 0.17 g/L | 10 mg/L | Visible light | 80% at 180 min | [75] |
2Bi2O3–B2O3 (BBO) glass | 50 mg/L | UV light | 25% at 180 min | [36] | |
Fe doped TiO2 | 1 g/L | 10 mg/L | UV light | 38% at 120min | [64] |
CdS-Borosilicate glass (SiO2-B2O3-Na2O-ZnO) | 1 g/L | 10 mg/L | sunlight | 68% at 270 min | [34] |
titanium-doped hydroxyapatite | 0.5 g/L | 10 mg/L | UV light | 99% at 240 min | [76] |
SnO2/CdSe/Bi2S3 composite | 0.5 g/L | 30 mg/L | Visible light | 99% at 60 min | [77] |
Tin Oxide (SnO2) | 0.5 g/L | 30 mg/L | Visible light | 53% at 60 min | [77] |
CeO2–Fe2O3–NiO nanocomposite | 0.6 g/L | 5 mg/L | sunlight | 73% at 50 min | [78] |
Fe2O3 nanoparticles | 0.4 g/L | 10 mg/L | sunlight | 53% at 50 min | [79] |
40CaO–30 B2O3-30 V2O5 | 0.5 g/L | 10 mg/L | UV light | 99% at 180 min | Present work |
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Kaaouass, A.; Ben Ali, A.; Ait Ahsaine, H.; Kaichouh, G.; Zarrouk, A.; Saadi, M. Photocatalytic Properties and Chemical Durability of CaO-B2O3-V2O5 Borovanadate Glasses. Catalysts 2023, 13, 512. https://doi.org/10.3390/catal13030512
Kaaouass A, Ben Ali A, Ait Ahsaine H, Kaichouh G, Zarrouk A, Saadi M. Photocatalytic Properties and Chemical Durability of CaO-B2O3-V2O5 Borovanadate Glasses. Catalysts. 2023; 13(3):512. https://doi.org/10.3390/catal13030512
Chicago/Turabian StyleKaaouass, Ayoub, Abdelkader Ben Ali, Hassan Ait Ahsaine, Ghizlaine Kaichouh, Abdelkader Zarrouk, and Mohamed Saadi. 2023. "Photocatalytic Properties and Chemical Durability of CaO-B2O3-V2O5 Borovanadate Glasses" Catalysts 13, no. 3: 512. https://doi.org/10.3390/catal13030512