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Keywords = soft X-ray transients

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13 pages, 1895 KB  
Article
Class-Dependent Solar Flare Effects on Mars’ Upper Atmosphere: MAVEN NGIMS Observations of X8.2 and M6.0 from September 2017
by Junaid Haleem and Shican Qiu
Universe 2025, 11(8), 245; https://doi.org/10.3390/universe11080245 - 25 Jul 2025
Viewed by 701
Abstract
Transient increments of X-ray radiation and extreme ultraviolet (EUV) during solar flares are strong drivers of thermospheric dynamics on Mars, yet their class-dependent impacts remain poorly measured. This work provides the first direct, side-by-side study of Martian thermospheric reactions to flares X8.2 on [...] Read more.
Transient increments of X-ray radiation and extreme ultraviolet (EUV) during solar flares are strong drivers of thermospheric dynamics on Mars, yet their class-dependent impacts remain poorly measured. This work provides the first direct, side-by-side study of Martian thermospheric reactions to flares X8.2 on 10 September 2017 and M6.0 on 17 September 2017. This study shows nonlinear, class-dependent effects, compositional changes, and recovery processes not recorded in previous investigations. Species-specific responses deviated significantly from irradiance proportionality, even though the soft X-ray flux in the X8.2 flare was 13 times greater. Argon (Ar) concentrations rose 3.28× (compared to 1.13× for M6.0), and radiative cooling led CO2 heating to approach a halt at ΔT = +40 K (X8.2) against +19 K (M6.0) at exobase altitudes (196–259 km). N2 showed the largest class difference, where temperatures rose by +126 K (X8.2) instead of +19 K (M6.0), therefore displaying flare-magnitude dependent thermal sensitivity. The 1.95× increase in O concentrations during X8.2 and the subsequent decrease following M6.0 (−39 K cooling) illustrate the contradiction between photochemical production and radiative loss. The O/CO2 ratio at 225 km dropped 46% during X8.2, revealing compositional gradients boosted by flares. Recovery timeframes varied by class; CO2 quickly re-equilibrated because of effective cooling, whereas inert species (Ar, N2) stabilized within 1–2 orbits after M6.0 but needed >10 orbits of the MAVEN satellite after the X8.2 flare. The observations of the X8.2 flare came from the western limb of the Sun, but the M6.0 flare happened on the far side. The CME shock was the primary driver of Mars’ EUV reaction. These findings provide additional information on atmospheric loss and planetary habitability by indicating that Mars’ thermosphere has a saturation threshold where strong flares induce nonlinear energy partitioning that encourages the departure of lighter species. Full article
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18 pages, 934 KB  
Article
Evidence of Gapless Superfluidity in MXB 1659-29 With and Without Late Time Cooling
by Valentin Allard and Nicolas Chamel
Universe 2025, 11(5), 140; https://doi.org/10.3390/universe11050140 - 27 Apr 2025
Cited by 1 | Viewed by 523
Abstract
The interpretation of the thermal relaxation of some transiently accreting neutron stars in quasipersistent soft X-ray transients, especially MXB 1659-29, has been found to be challenging within the traditional deep crustal heating paradigm. Due to the pinning of quantized vortices, the neutron superfluid [...] Read more.
The interpretation of the thermal relaxation of some transiently accreting neutron stars in quasipersistent soft X-ray transients, especially MXB 1659-29, has been found to be challenging within the traditional deep crustal heating paradigm. Due to the pinning of quantized vortices, the neutron superfluid is not expected to remain at rest in the crust, as was generally assumed. We have recently shown that for sufficiently large relative superflows, the neutron superfluid could become gapless. This dynamical phase could naturally explain the late-time cooling of MXB 1659-29. However, the interpretation of the last observation of MXB 1659-29 in 2013 before its second accretion phase in 2015 remains debated, with some spectral fits being consistent with no further temperature decline. Here, we revisit the cooling of this neutron star considering the different fits. New simulations of the crust cooling are performed, accounting for neutron diffusion and allowing for gapless superfluidity. In all cases, gapless superfluidity is found to provide the best fit to observations. Full article
(This article belongs to the Special Issue Challenges and Future Directions in Neutron Star Research)
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23 pages, 2586 KB  
Review
IXPE View of BH XRBs during the First 2.5 Years of the Mission
by Michal Dovčiak, Jakub Podgorný, Jiří Svoboda, James F. Steiner, Philip Kaaret, Henric Krawczynski, Adam Ingram, Vadim Kravtsov, Lorenzo Marra, Fabio Muleri, Javier A. García, Guglielmo Mastroserio, Romana Mikušincová, Ajay Ratheesh and Nicole Rodriguez Cavero
Galaxies 2024, 12(5), 54; https://doi.org/10.3390/galaxies12050054 - 25 Sep 2024
Cited by 11 | Viewed by 2896
Abstract
Accreting stellar-mass black holes represent unique laboratories for studying matter and radiation under the influence of extreme gravity. They are highly variable sources going through different accretion states, showing various components in their X-ray spectra from the thermal emission of the accretion disc [...] Read more.
Accreting stellar-mass black holes represent unique laboratories for studying matter and radiation under the influence of extreme gravity. They are highly variable sources going through different accretion states, showing various components in their X-ray spectra from the thermal emission of the accretion disc dominating in the soft state to the up-scattered Comptonisation component from an X-ray corona in the hard state. X-ray polarisation measurements are particularly sensitive to the geometry of the X-ray scatterings and can thus constrain the orientation and relative positions of the innermost components of these systems. The IXPE mission has observed about a dozen stellar-mass black holes with masses up to 20 solar masses in X-ray binaries with different orientations and in various accretion states. The low-inclination sources in soft states have shown a low fraction of polarisation. On the other hand, several sources in soft and hard states have revealed X-ray polarisation higher than expected, which poses significant challenges for theoretical interpretation, with 4U 1630–47 being one of the most puzzling sources. IXPE has measured the spin of three black holes via the measurement of their polarisation properties in the soft emission state. In each of the three cases, the new results agree with the constraints from the spectral observations. The polarisation observations of the black hole X-ray transient Swift J1727.8–1613 across its entire outburst has revealed that the soft-state polarisation is much weaker than the hard-state polarisation. Remarkably, the observations furthermore show that the polarisation of the bright hard state and that of the 100 times less luminous dim hard state are identical within the accuracy of the measurement. For sources with a radio jet, the electric field polarisation tends to align with the radio jet, indicating the equatorial geometry of the X-ray corona, e.g., in the case of Cyg X–1. In the unique case of Cyg X–3, where the polarisation is perpendicular to the radio jet, the IXPE observations reveal the presence and geometry of obscuring material hiding this object from our direct view. The polarisation measurements acquired by the IXPE mission during its first 2.5 years have provided unprecedented insights into the geometry and physical processes of accreting stellar-mass black holes, challenging existing theoretical models and offering new avenues for understanding these extreme systems. Full article
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31 pages, 2024 KB  
Article
Prospects for Time-Domain and Multi-Messenger Science with AXIS
by Riccardo Arcodia, Franz E. Bauer, S. Bradley Cenko, Kristen C. Dage, Daryl Haggard, Wynn C. G. Ho, Erin Kara, Michael Koss, Tingting Liu, Labani Mallick, Michela Negro, Pragati Pradhan, J. Quirola-Vásquez, Mark T. Reynolds, Claudio Ricci, Richard E. Rothschild, Navin Sridhar, Eleonora Troja and Yuhan Yao
Universe 2024, 10(8), 316; https://doi.org/10.3390/universe10080316 - 2 Aug 2024
Cited by 9 | Viewed by 3322
Abstract
The Advanced X-ray Imaging Satellite (AXIS) promises revolutionary science in the X-ray and multi-messenger time domain. AXIS will leverage excellent spatial resolution (<1.5 arcsec), sensitivity (80× that of Swift), and a large collecting area (5–10× that of Chandra) across a 24-arcmin [...] Read more.
The Advanced X-ray Imaging Satellite (AXIS) promises revolutionary science in the X-ray and multi-messenger time domain. AXIS will leverage excellent spatial resolution (<1.5 arcsec), sensitivity (80× that of Swift), and a large collecting area (5–10× that of Chandra) across a 24-arcmin diameter field of view at soft X-ray energies (0.3–10.0 keV) to discover and characterize a wide range of X-ray transients from supernova-shock breakouts to tidal disruption events to highly variable supermassive black holes. The observatory’s ability to localize and monitor faint X-ray sources opens up new opportunities to hunt for counterparts to distant binary neutron star mergers, fast radio bursts, and exotic phenomena like fast X-ray transients. AXIS will offer a response time of <2 h to community alerts, enabling studies of gravitational wave sources, high-energy neutrino emitters, X-ray binaries, magnetars, and other targets of opportunity. This white paper highlights some of the discovery science that will be driven by AXIS in this burgeoning field of time domain and multi-messenger astrophysics. This White Paper is part of a series commissioned for the AXIS Probe Concept Mission; additional AXIS White Papers can be found at the AXIS website. Full article
(This article belongs to the Section Galaxies and Clusters)
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15 pages, 4117 KB  
Article
A Study of Interstellar Medium in the Line of Sight of Transient Neutron Star Low-Mass X-ray Binary, MXB 1659-298, by Timing and Spectral Analysis
by Rabindra Mahato, Parag Bhattacharya and Monmoyuri Baruah
Galaxies 2024, 12(4), 41; https://doi.org/10.3390/galaxies12040041 - 31 Jul 2024
Viewed by 1597
Abstract
This work is dedicated to the study of interstellar medium (ISM) along the line of sight (LOS) of the transient low-mass X-ray binary, MXB 1659-298, capitalizing the high resolving power of XMM-Newton in the soft energy range. We emphasized the analysis of reflection [...] Read more.
This work is dedicated to the study of interstellar medium (ISM) along the line of sight (LOS) of the transient low-mass X-ray binary, MXB 1659-298, capitalizing the high resolving power of XMM-Newton in the soft energy range. We emphasized the analysis of reflection grating spectrometer (RGS) data in the energy range 0.5–2.15 keV, suitable for the study of ISM. The paper includes an explanation of why, in the soft X-ray energy range, only two observations (out of seven) were deemed eligible for analysis. Three absorption lines associated with highly ionized Fe XX (1s22p2-2p2 (3p) 4d), Si XIV (1s2-1s2p), and Mg XI (1s2-1s6p) were identified in the observations, with IDs of 8620701(2001) and 748391601(2015). These new absorption lines and the absorption edge due to the neutral oxygen K edge seen in the spectra validate the multiphase structure of ISM. The predominance of interstellar medium over the ionized absorber is established along the direction of the source. The equivalent hydrogen column density measured is nearly equal to the galactic HI value derived previously. The small value of the ionic column density of Fe, Si, and Mg in the site of the high-temperature region resembles previous findings. Full article
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24 pages, 4719 KB  
Review
Mechanisms of Nanoscale Radiation Enhancement by Metal Nanoparticles: Role of Low Energy Electrons
by Yi Zheng and Léon Sanche
Int. J. Mol. Sci. 2023, 24(5), 4697; https://doi.org/10.3390/ijms24054697 - 28 Feb 2023
Cited by 14 | Viewed by 2905
Abstract
Metal nanoparticles are considered as highly promising radiosensitizers in cancer radiotherapy. Understanding their radiosensitization mechanisms is critical for future clinical applications. This review is focused on the initial energy deposition by short-range Auger electrons; when high energy radiation is absorbed by gold nanoparticles [...] Read more.
Metal nanoparticles are considered as highly promising radiosensitizers in cancer radiotherapy. Understanding their radiosensitization mechanisms is critical for future clinical applications. This review is focused on the initial energy deposition by short-range Auger electrons; when high energy radiation is absorbed by gold nanoparticles (GNPs) located near vital biomolecules; such as DNA. Auger electrons and the subsequent production of secondary low energy electrons (LEEs) are responsible for most the ensuing chemical damage near such molecules. We highlight recent progress on DNA damage induced by the LEEs produced abundantly within about 100 nanometers from irradiated GNPs; and by those emitted by high energy electrons and X-rays incident on metal surfaces under differing atmospheric environments. LEEs strongly react within cells; mainly via bound breaking processes due to transient anion formation and dissociative electron attachment. The enhancement of damages induced in plasmid DNA by LEEs; with or without the binding of chemotherapeutic drugs; are explained by the fundamental mechanisms of LEE interactions with simple molecules and specific sites on nucleotides. We address the major challenge of metal nanoparticle and GNP radiosensitization; i.e., to deliver the maximum local dose of radiation to the most sensitive target of cancer cells (i.e., DNA). To achieve this goal the emitted electrons from the absorbed high energy radiation must be short range, and produce a large local density of LEEs, and the initial radiation must have the highest possible absorption coefficient compared to that of soft tissue (e.g., 20–80 keV X-rays). Full article
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12 pages, 2764 KB  
Article
Breakthrough Multi-Messenger Astrophysics with the THESEUS Space Mission
by Giulia Stratta, Lorenzo Amati, Marica Branchesi, Riccardo Ciolfi, Nial Tanvir, Enrico Bozzo, Diego Götz, Paul O’Brien and Andrea Santangelo
Galaxies 2022, 10(3), 60; https://doi.org/10.3390/galaxies10030060 - 21 Apr 2022
Cited by 6 | Viewed by 3673
Abstract
The mission concept THESEUS (Transient High Energy Sky and Early Universe Surveyor) aims at exploiting Gamma-Ray Bursts (GRB) to explore the early Universe, as well as becoming a cornerstone of multi-messenger and time-domain astrophysics. To achieve these goals, a key feature is the [...] Read more.
The mission concept THESEUS (Transient High Energy Sky and Early Universe Surveyor) aims at exploiting Gamma-Ray Bursts (GRB) to explore the early Universe, as well as becoming a cornerstone of multi-messenger and time-domain astrophysics. To achieve these goals, a key feature is the capability to survey the soft X-ray transient sky and to detect the faint and soft GRB population so far poorly explored. Among the expected transients there will be high-redshift GRBs, nearby low-luminosity, X-ray Flashes and short GRBs. Our understanding of the physics governing the GRB prompt emission will benefit from the 0.3 keV–10 MeV simultaneous observations for an unprecedented large number of hundreds of events per year. In particular the mission will provide the identification, accurate sky localisation and characterization of electromagnetic counterparts to sources of gravitational wave and neutrino sources, which will be routinely detected during the 2030s by the upgraded second generation and third generation Gravitational Wave (GW) interferometers and next generation neutrino detectors. Full article
(This article belongs to the Special Issue Gamma-Ray Burst Science in 2030)
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18 pages, 1270 KB  
Article
Small Spacecraft Payload Study for X-ray Astrophysics including GRB Science
by Vladimír Dániel, Veronika Maršíková, Rene Hudec, Ladislav Pína, Adolf Inneman and Karel Pelc
Universe 2022, 8(3), 144; https://doi.org/10.3390/universe8030144 - 23 Feb 2022
Cited by 14 | Viewed by 3514
Abstract
This paper presents microsatellite spacecraft payload study for prompt observation of transient astrophysical objects in X-ray energy range. By combining telescope concepts and miniaturized detectors, the small spacecraft will be able to probe the X-ray temporal emissions of bright events such as Gamma-Ray [...] Read more.
This paper presents microsatellite spacecraft payload study for prompt observation of transient astrophysical objects in X-ray energy range. By combining telescope concepts and miniaturized detectors, the small spacecraft will be able to probe the X-ray temporal emissions of bright events such as Gamma-Ray Bursts (GRBs), X-ray transients or the electromagnetic counterparts of Gravitational Wave Events (GWEs), but also short and long term observations of other types of variable X-ray sources. The spacecraft is based on the CubeSat nanosatellite platform with a volume of 16U. The spacecraft carries two types of X-ray telescopes onboard. The first is intended for X-ray transient monitoring and localization, and the second for detailed spectroscopic observation. The X-ray monitor/localization telescope with wide field of view of several arc degrees is used for localization and flux measurement of X-ray transients, as well as for permanent monitoring of Galactic center area. This telescope is based on Lobster Eye X-ray optics together with pixel detector based on the Timepix3 Quad detector. Rapid follow-up observation by soft X-ray spectroscopy is enabled by a second X-ray spectroscopic telescope with limited FOV (Field of View) of several arcmins with no spatial and/or angular resolution. The spectroscopic telescope uses condenser optics based on replicated parabolic total reflection system (or, alternatively, Wolter system) and a Ketek X-ray SDD detector with energy resolution of about 130 eV as a detector. In addition to technical and instrumental aspects, observational strategy and astrophysical issues and justifications are also addressed in the paper. Full article
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18 pages, 3719 KB  
Article
Towards Understanding Excited-State Properties of Organic Molecules Using Time-Resolved Soft X-ray Absorption Spectroscopy
by Holger Stiel, Julia Braenzel, Adrian Jonas, Richard Gnewkow, Lisa Theresa Glöggler, Denny Sommer, Thomas Krist, Alexei Erko, Johannes Tümmler and Ioanna Mantouvalou
Int. J. Mol. Sci. 2021, 22(24), 13463; https://doi.org/10.3390/ijms222413463 - 15 Dec 2021
Cited by 10 | Viewed by 4267
Abstract
The extension of the pump-probe approach known from UV/VIS spectroscopy to very short wavelengths together with advanced simulation techniques allows a detailed analysis of excited-state dynamics in organic molecules or biomolecular structures on a nanosecond to femtosecond time level. Optical pump soft X-ray [...] Read more.
The extension of the pump-probe approach known from UV/VIS spectroscopy to very short wavelengths together with advanced simulation techniques allows a detailed analysis of excited-state dynamics in organic molecules or biomolecular structures on a nanosecond to femtosecond time level. Optical pump soft X-ray probe spectroscopy is a relatively new approach to detect and characterize optically dark states in organic molecules, exciton dynamics or transient ligand-to-metal charge transfer states. In this paper, we describe two experimental setups for transient soft X-ray absorption spectroscopy based on an LPP emitting picosecond and sub-nanosecond soft X-ray pulses in the photon energy range between 50 and 1500 eV. We apply these setups for near-edge X-ray absorption fine structure (NEXAFS) investigations of thin films of a metal-free porphyrin, an aggregate forming carbocyanine and a nickel oxide molecule. NEXAFS investigations have been carried out at the carbon, nitrogen and oxygen K-edge as well as on the Ni L-edge. From time-resolved NEXAFS carbon, K-edge measurements of the metal-free porphyrin first insights into a long-lived trap state are gained. Our findings are discussed and compared with density functional theory calculations. Full article
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24 pages, 1561 KB  
Review
A Review of Semiconductor Based Ionising Radiation Sensors Used in Harsh Radiation Environments and Their Applications
by Arijit Karmakar, Jialei Wang, Jeffrey Prinzie, Valentijn De Smedt and Paul Leroux
Radiation 2021, 1(3), 194-217; https://doi.org/10.3390/radiation1030018 - 20 Aug 2021
Cited by 53 | Viewed by 15704
Abstract
This article provides a review of semiconductor based ionising radiation sensors to measure accumulated dose and detect individual strikes of ionising particles. The measurement of ionising radiation (γ-ray, X-ray, high energy UV-ray and heavy ions, etc.) is essential in several critical [...] Read more.
This article provides a review of semiconductor based ionising radiation sensors to measure accumulated dose and detect individual strikes of ionising particles. The measurement of ionising radiation (γ-ray, X-ray, high energy UV-ray and heavy ions, etc.) is essential in several critical reliability applications such as medical, aviation, space missions and high energy physics experiments considering safety and quality assurance. In the last few decades, numerous techniques based on semiconductor devices such as diodes, metal-oxide-semiconductor field-effect transistors (MOSFETs) and solid-state photomultipliers (SSPMs), etc., have been reported to estimate the absorbed dose of radiation with sensitivity varying by several orders of magnitude from μGy to MGy. In addition, the mitigation of soft errors in integrated circuits essentially requires detection of charged particle induced transients and digital bit-flips in storage elements. Depending on the particle energies, flux and the application requirements, several sensing solutions such as diodes, static random access memory (SRAM) and NAND flash, etc., are reported in the literature. This article goes through the evolution of radiation dosimeters and particle detectors implemented using semiconductor technologies and summarises the features with emphasis on their underlying principles and applications. In addition, this article performs a comparison of the different methodologies while mentioning their advantages and limitations. Full article
(This article belongs to the Special Issue Feature Papers for Radiation in 2021)
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10 pages, 812 KB  
Article
Properties of Faint X-ray Activity of XTE J1908+094 in 2019
by Debjit Chatterjee, Arghajit Jana, Kaushik Chatterjee, Riya Bhowmick, Sujoy Kumar Nath, Sandip K. Chakrabarti, A. Mangalam and Dipak Debnath
Galaxies 2021, 9(2), 25; https://doi.org/10.3390/galaxies9020025 - 16 Apr 2021
Cited by 6 | Viewed by 2665
Abstract
We study the properties of the faint X-ray activity of Galactic transient black hole candidate XTE J1908+094 during its 2019 outburst. Here, we report the results of detailed spectral and temporal analysis during this outburst using observations from Nuclear Spectroscopic Telescope Array (NuSTAR) [...] Read more.
We study the properties of the faint X-ray activity of Galactic transient black hole candidate XTE J1908+094 during its 2019 outburst. Here, we report the results of detailed spectral and temporal analysis during this outburst using observations from Nuclear Spectroscopic Telescope Array (NuSTAR). We have not observed any quasi-periodic-oscillations (QPOs) in the power density spectrum (PDS). The spectral study suggests that the source remained in the softer (more precisely, in the soft–intermediate) spectral state during this short period of X-ray activity. We notice a faint but broad Fe Kα emission line at around 6.5 keV. We also estimate the probable mass of the black hole to be 6.50.7+0.5M, with 90% confidence. Full article
(This article belongs to the Special Issue Global Understanding of Accretion and Ejection around Black Holes)
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12 pages, 1189 KB  
Review
Transient Changes of Optical Properties in Semiconductors in Response to Femtosecond Laser Pulses
by Victor Tkachenko, Nikita Medvedev and Beata Ziaja
Appl. Sci. 2016, 6(9), 238; https://doi.org/10.3390/app6090238 - 24 Aug 2016
Cited by 10 | Viewed by 6606
Abstract
In this paper we present an overview of our theoretical simulations on the interaction of ultrafast laser pulses with matter. Our dedicated simulation tool, X-ray induced Thermal And Non-thermal Transitions (XTANT) can currently treat semiconductors irradiated with soft to hard X-ray femtosecond pulses. [...] Read more.
In this paper we present an overview of our theoretical simulations on the interaction of ultrafast laser pulses with matter. Our dedicated simulation tool, X-ray induced Thermal And Non-thermal Transitions (XTANT) can currently treat semiconductors irradiated with soft to hard X-ray femtosecond pulses. During the excitation and relaxation of solids, their optical properties such as reflectivity, transmission and absorption, are changing, affected by transient electron excitation and, at sufficiently high dose, by atomic relocations. In this review we report how the transient optical properties can be used for diagnostics of electronic and structural transitions occurring in irradiated semiconductors. The presented methodology for calculation of the complex dielectric function applied in XTANT proves to be capable of describing changes in the optical parameters, when the solids are driven out of equilibrium by intense laser pulses. Comparison of model predictions with the existing experimental data shows a good agreement. Application of transient optical properties to laser pulse diagnostics is indicated. Full article
(This article belongs to the Special Issue Ultrashort Optical Pulses)
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12 pages, 1058 KB  
Article
X-ray Chirped Pulse Amplification: towards GW Soft X-ray Lasers
by Philippe Zeitoun, Eduardo Oliva, Thi Thu Thuy Le, David Ros, Stéphane Sebban, Lu Li, Pedro Velarde and Marta Fajardo
Appl. Sci. 2013, 3(3), 581-592; https://doi.org/10.3390/app3030581 - 12 Jul 2013
Cited by 4 | Viewed by 12131
Abstract
Extensive modeling of the seeding of plasma-based soft X-ray lasers is reported in this article. Seminal experiments on amplification in plasmas created from solids have been studied in detail and explained. Using a transient collisional excitation scheme, we show that a 18 µJ, [...] Read more.
Extensive modeling of the seeding of plasma-based soft X-ray lasers is reported in this article. Seminal experiments on amplification in plasmas created from solids have been studied in detail and explained. Using a transient collisional excitation scheme, we show that a 18 µJ, 80 fs fully coherent pulse is achievable by using plasmas pumped by a compact 10 Hz laser. We demonstrate that direct seeding of plasmas created by nanosecond lasers is not efficient. Therefore, we propose and fully study the transposition to soft X-rays of the Chirped Pulse Amplification (CPA) technique. Soft X-ray pulses with energy of 6 mJ and 200 fs duration are reachable by seeding plasmas pumped by compact 100 J, sub-ns, 1 shot/min lasers. These soft X-ray lasers would reach GW power, corresponding to an increase of 100 times as compared to the highest peak power achievable nowadays in the soft X-ray region (30 eV–1 keV). X-ray CPA is opening new horizon for soft x-ray ultra-intense sources. Full article
(This article belongs to the Special Issue Ultraintense Ultrashort Pulse Lasers)
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18 pages, 1285 KB  
Article
Time-Resolved Soft X-ray Diffraction Reveals Transient Structural Distortions of Ternary Liquid Crystals
by Wilson Quevedo, Christian Peth, Gerhard Busse, Mirko Scholz, Klaus Mann and Simone Techert
Int. J. Mol. Sci. 2009, 10(11), 4754-4771; https://doi.org/10.3390/ijms10114754 - 4 Nov 2009
Cited by 5 | Viewed by 13975
Abstract
Home-based soft X-ray time-resolved scattering experiments with nanosecond time resolution (10 ns) and nanometer spatial resolution were carried out at a table top soft X-ray plasma source (2.2–5.2 nm). The investigated system was the lyotropic liquid crystal C16E7/paraffin/glycerol/formamide/IR 5. [...] Read more.
Home-based soft X-ray time-resolved scattering experiments with nanosecond time resolution (10 ns) and nanometer spatial resolution were carried out at a table top soft X-ray plasma source (2.2–5.2 nm). The investigated system was the lyotropic liquid crystal C16E7/paraffin/glycerol/formamide/IR 5. Usually, major changes in physical, chemical, and/or optical properties of the sample occur as a result of structural changes and shrinking morphology. Here, these effects occur as a consequence of the energy absorption in the sample upon optical laser excitation in the IR regime. The liquid crystal shows changes in the structural response within few hundred nanoseconds showing a time decay of 182 ns. A decrease of the Bragg peak diffracted intensity of 30% and a coherent macroscopic movement of the Bragg reflection are found as a response to the optical pump. The Bragg reflection movement is established to be isotropic and diffusion controlled (1 μs). Structural processes are analyzed in the Patterson analysis framework of the time-varying diffraction peaks revealing that the inter-lamellar distance increases by 2.7 Å resulting in an elongation of the coherently expanding lamella crystallite. The present studies emphasize the possibility of applying TR-SXRD techniques for studying the mechanical dynamics of nanosystems. Full article
(This article belongs to the Special Issue Liquid Crystals)
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