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Keywords = flexible operation of carbon capture unit

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22 pages, 1921 KiB  
Article
Cooperative Game-Theoretic Scheduling for Low-Carbon Integrated Energy Systems with P2G–CCS Synergy
by Huijia Liu, Sheng Ye, Chengkai Yin, Lei Wang and Can Zhang
Energies 2025, 18(15), 3942; https://doi.org/10.3390/en18153942 - 24 Jul 2025
Viewed by 286
Abstract
In the context of the dual-carbon goals, this study proposes a cooperative game-theoretic optimization strategy to enhance the energy utilization efficiency, operational efficiency, and cost-effectiveness of integrated energy systems (IESs) while simultaneously reducing carbon emissions, improving operational flexibility, and mitigating renewable energy variability. [...] Read more.
In the context of the dual-carbon goals, this study proposes a cooperative game-theoretic optimization strategy to enhance the energy utilization efficiency, operational efficiency, and cost-effectiveness of integrated energy systems (IESs) while simultaneously reducing carbon emissions, improving operational flexibility, and mitigating renewable energy variability. To achieve these goals, an IES framework integrating power-to-gas (P2G) technology and carbon capture and storage (CCS) facilities is established to regulate carbon emissions. The system incorporates P2G conversion units and thermal components—specifically, hydrogen fuel cells, electrolyzers, reactors, and electric boilers—aiming to maximize energy conversion efficiency and asset utilization. A cooperative game-theoretic optimization model is developed to facilitate collaboration among multiple stakeholders within the coalition, which employs the Shapley value method to ensure equitable distribution of the cooperative surplus, thereby maximizing collective benefits. The model is solved using an improved gray wolf optimizer (IGWO). The simulation results demonstrate that the proposed strategy effectively coordinates multi-IES scheduling, significantly reduces carbon emissions, facilitates the efficient allocation of cooperation gains, and maximizes overall system utility. Full article
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15 pages, 2000 KiB  
Article
A Bench-Scale Demonstration of Direct Air Capture Using an Enhanced Electrochemical System
by Jinwen Wang, Xin Gao, Adam Berger, Ayokunle Omosebi, Tingfei Chen, Aron Patrick and Kunlei Liu
Clean Technol. 2025, 7(2), 50; https://doi.org/10.3390/cleantechnol7020050 - 16 Jun 2025
Viewed by 578
Abstract
The bench-scale demonstration of the UKy-IDEA process for direct air capture (DAC) technology combines solvent-aided CO2 capture with electrochemical regeneration (ER) through a pH swing process, enabling efficient CO2 capture and simultaneous solvent regeneration, producing high-purity hydrogen as a valuable co-product. [...] Read more.
The bench-scale demonstration of the UKy-IDEA process for direct air capture (DAC) technology combines solvent-aided CO2 capture with electrochemical regeneration (ER) through a pH swing process, enabling efficient CO2 capture and simultaneous solvent regeneration, producing high-purity hydrogen as a valuable co-product. The system shows stable performance with over 90% CO2 capture efficiency and approximately 80% CO2 recovery, handling ambient air at 280 L/min. During testing, the unit captured 1 kg of CO2 over 100 h, with a concentrated CO2 output purity of around 70%. Operating efficiently at low voltage (<3 V), the system supports flexible and remote operation without AC/DC converters when using intermittent renewable energy. Techno-economic analysis (TEA) and Life Cycle Assessment (LCA) highlight its minimized required footprint and cost-effectiveness. Marketable hydrogen offsets capture costs, and compatibility with renewable DC power enhances appeal. Hydrogen production displacing CO2 produced via electrolysis achieves 0.94 kg CO2 abated per kg CO2 captured. The project would be economic, with USD 26 per ton of CO2 from the federal 45Q tax credit for carbon utilization, and USD 5 to USD 12 per kg for H2. Full article
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22 pages, 2052 KiB  
Article
Optimization Scheduling of Carbon Capture Power Systems Considering Energy Storage Coordination and Dynamic Carbon Constraints
by Tingling Wang, Yuyi Jin and Yongqing Li
Processes 2025, 13(6), 1758; https://doi.org/10.3390/pr13061758 - 3 Jun 2025
Cited by 1 | Viewed by 557
Abstract
To achieve low-carbon economic dispatch and collaborative optimization of carbon capture efficiency in power systems, this paper proposes a flexible carbon capture power plant and generalized energy storage collaborative operation model under a dynamic carbon quota mechanism. First, adjustable carbon capture devices are [...] Read more.
To achieve low-carbon economic dispatch and collaborative optimization of carbon capture efficiency in power systems, this paper proposes a flexible carbon capture power plant and generalized energy storage collaborative operation model under a dynamic carbon quota mechanism. First, adjustable carbon capture devices are integrated into high-emission thermal power units to construct carbon–electricity coupled operation modules, enabling a dynamic reduction of carbon emission intensity and enhancing low-carbon performance. Second, a time-varying carbon quota allocation mechanism and a dynamic correction model for carbon emission factors are designed to improve the regulation capability of carbon capture units during peak demand periods. Furthermore, pumped storage systems and price-guided demand response are integrated to form a generalized energy storage system, establishing a “source–load–storage” coordinated peak-shaving framework that alleviates the regulation burden on carbon capture units. Finally, a multi-timescale optimization scheduling model is developed and solved using the GUROBI algorithm to ensure the economic efficiency and operational synergy of system resources. Simulation results demonstrate that, compared with the traditional static quota mode, the proposed dynamic carbon quota mechanism reduces wind curtailment cost by 9.6%, the loss of load cost by 48.8%, and carbon emission cost by 15%. Moreover, the inclusion of generalized energy storage—including pumped storage and demand response—further decreases coal consumption cost by 9% and carbon emission cost by 17%, validating the effectiveness of the proposed approach in achieving both economic and environmental benefits. Full article
(This article belongs to the Section Energy Systems)
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27 pages, 947 KiB  
Article
Low-Carbon Economic Scheduling of Hydrogen-Integrated Energy Systems with Enhanced Bilateral Supply–Demand Response Considering Vehicle to Grid Under Power-to-Gas–Carbon Capture System Coupling
by Yulong Dang and Weiqing Wang
Processes 2025, 13(3), 636; https://doi.org/10.3390/pr13030636 - 24 Feb 2025
Cited by 2 | Viewed by 892
Abstract
Hydrogen-Integrated energy systems (HIESs) are pivotal in driving the transition to a low-carbon energy structure in China. This paper proposes a low-carbon economic scheduling strategy to improve the operational efficiency and reduce the carbon emissions of HIESs. The approach begins with the implementation [...] Read more.
Hydrogen-Integrated energy systems (HIESs) are pivotal in driving the transition to a low-carbon energy structure in China. This paper proposes a low-carbon economic scheduling strategy to improve the operational efficiency and reduce the carbon emissions of HIESs. The approach begins with the implementation of a stepwise carbon trading framework to limit the carbon output of the system. This is followed by the development of a joint operational model that combines hydrogen energy use and carbon capture. To improve the energy supply flexibility of HIESs, modifications to the conventional combined heat and power (CHP) unit are made by incorporating a waste heat boiler and an organic Rankine cycle. This results in a flexible CHP response model capable of adjusting both electricity and heat outputs. Furthermore, a comprehensive demand response model is designed to optimize the flexible capacities of electric and thermal loads, thereby enhancing demand-side responsiveness. The integration of electric vehicles (EVs) into the system is analyzed with respect to their energy consumption patterns and dispatch capabilities, which improves their potential for flexible scheduling and enables an optimized synergy between the demand-side flexibility and system operations. Finally, a low-carbon economic scheduling model for the HIES is developed with the objective of minimizing system costs. The results show that the proposed scheduling method effectively enhances the economy, low-carbon performance, and flexibility of HIES operation while promoting clean energy consumption, deep decarbonization of the system, and the synergistic complementarity of flexible supply–demand resources. In the broader context of expanding clean energy and growing EV adoption, this study demonstrates the potential of energy-saving, emission-reduction systems and vehicle-to-grid (V2G) strategies to contribute to the sustainable and green development of the energy sector. Full article
(This article belongs to the Section Energy Systems)
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20 pages, 2496 KiB  
Article
Optimal Scheduling of the Microgrid Based on the Dynamic Characteristics of the Natural Gas Pipeline Network and the Thermal Network Along with P2G-CCS
by Fangzong Wang and Zhenghong Tu
Processes 2025, 13(2), 324; https://doi.org/10.3390/pr13020324 - 24 Jan 2025
Viewed by 612
Abstract
In the power system, the integration of power-to-gas and carbon capture systems (P2G-CCS) within the microgrid enables the conversion of electrical energy into hydrogen or methane while simultaneously capturing CO2 emissions from power generation units. This approach significantly mitigates carbon emissions and [...] Read more.
In the power system, the integration of power-to-gas and carbon capture systems (P2G-CCS) within the microgrid enables the conversion of electrical energy into hydrogen or methane while simultaneously capturing CO2 emissions from power generation units. This approach significantly mitigates carbon emissions and supports the transition to a low-carbon energy system. Concurrently, the dynamic properties of the gas–thermal network exert a critical influence on the flexibility of system scheduling and the regulation of multi-energy coupling. Hence, this paper puts forward an optimal configuration strategy for microgrids with consideration of the dynamic characteristics of the gas–thermal network. Firstly, mathematical models for the dynamic characteristics of the gas network and the heat network were established and incorporated into the microgrid system. Secondly, in conjunction with the P2G-CCS coupling system, an optimization scheduling strategy was formulated with the aim of minimizing the total operational costs of the power grid, the natural gas network, and the heat network. An enhanced African vultures optimization algorithm (AVOA) was put forward. In the end, by setting different scheduling scenarios for conducting a comparative analysis, an appropriate optimization configuration scheme was selected, and the validity of the proposed method was verified through simulation with the improved case study. Full article
(This article belongs to the Section Energy Systems)
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16 pages, 1696 KiB  
Article
Dynamic Carbon Emission Factors in Source–Network–Storage Power System Planning: A Focus on Inverse Modelling
by Yixin Li, Weijie Wu, Haotian Yang, Guoxian Gong, Yining Zhang, Shuxin Luo, Shucan Zhou and Peng Wang
Energies 2024, 17(24), 6346; https://doi.org/10.3390/en17246346 - 17 Dec 2024
Cited by 1 | Viewed by 846
Abstract
In light of global climate change, China has set strategic goals for carbon peaking by 2030 and carbon neutrality by 2060, emphasizing the necessity of constructing a new power system with a high proportion of renewable energy sources. As coal-fired power plants are [...] Read more.
In light of global climate change, China has set strategic goals for carbon peaking by 2030 and carbon neutrality by 2060, emphasizing the necessity of constructing a new power system with a high proportion of renewable energy sources. As coal-fired power plants are the main carbon emissions source in the power system, their low-carbon transition and morphology structure optimization is crucial. This paper explores the critical role of dynamic carbon emission factors within source–network–storage power system planning and proposes an innovative inverse dynamic carbon emission factor that effectively captures the nonlinear relationship between load rates and emissions. Comparative analyses using the HRP-38 test case demonstrate that the inverse model enhances computational efficiency, reduces solution times, and more accurately reflects the emissions characteristics of coal-fired units across varying operational conditions. Furthermore, the inverse model offers improved economic performance and broader flexibility in unit selection, highlighting its potential to balance carbon emissions control and economic optimization in future power system planning. Full article
(This article belongs to the Special Issue Simulation and Modeling for Low-Carbon Energy Systems)
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18 pages, 3550 KiB  
Article
Multi-Time Optimization Scheduling Strategy for Integrated Energy Systems Considering Multiple Controllable Loads and Carbon Capture Plants
by Zhe Han, Zehua Li, Wenbo Wang, Wei Liu, Qiang Ma, Sidong Sun, Haiyang Liu, Qiang Zhang and Yue Cao
Energies 2024, 17(23), 5995; https://doi.org/10.3390/en17235995 - 28 Nov 2024
Cited by 4 | Viewed by 1059
Abstract
In response to the dual carbon targets, it is necessary not only to reduce carbon emissions but also to increase the proportion of renewable energy generation capacity, thereby exacerbating the scarcity of flexible resources in the power system. Addressing these challenges, this study [...] Read more.
In response to the dual carbon targets, it is necessary not only to reduce carbon emissions but also to increase the proportion of renewable energy generation capacity, thereby exacerbating the scarcity of flexible resources in the power system. Addressing these challenges, this study proposes an operational optimization framework for an integrated energy system. This system encompasses wind/solar power plants, coal-fired power plants, carbon capture power plants, gas turbines, energy storage systems, and controllable loads, including reducible power loads, transferable power loads, electrolytic aluminum loads, transferable heat loads, and reducible loads. This study employs a system combining carbon capture plants with thermal power stations to supply flexible resources to the integrated energy system while reducing carbon emissions during the generation process of the thermal power units. A multi-timescale optimization scheduling approach is adopted to manage the uncertainties in wind, photovoltaic, and electric/thermal loads within the integrated energy system. The operational costs of the integrated energy system consider the capacity degradation costs of energy storage systems, the solvent degradation costs of carbon capture, and carbon costs. Finally, the cplex solver was used to solve the above model. The simulation results show that the consideration of five controllable loads leads to an increase of 7.22% in the interactive benefits with the power grid; the difference between the complete cost model and the incomplete overall benefits is 94.35%. It can be seen that the dispatching method proposed in this study can take advantage of the dispatching advantages of source-load adjustable resources and achieve the goal of low-carbon economic dispatching of the power system. Full article
(This article belongs to the Section F1: Electrical Power System)
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15 pages, 7847 KiB  
Article
High-Capacity Energy Storage Devices Designed for Use in Railway Applications
by Krystian Woźniak, Beata Kurc, Łukasz Rymaniak, Natalia Szymlet, Piotr Pielecha and Jakub Sobczak
Energies 2024, 17(23), 5904; https://doi.org/10.3390/en17235904 - 25 Nov 2024
Viewed by 916
Abstract
This paper investigates the application of high-capacity supercapacitors in railway systems, with a particular focus on their role in energy recovery during braking processes. The study highlights the potential for significant energy savings by capturing and storing energy generated through electrodynamic braking. Experimental [...] Read more.
This paper investigates the application of high-capacity supercapacitors in railway systems, with a particular focus on their role in energy recovery during braking processes. The study highlights the potential for significant energy savings by capturing and storing energy generated through electrodynamic braking. Experimental measurements conducted on a diesel–electric multiple unit revealed that approximately 28.3% to 30.5% of the energy could be recovered from the traction network, regardless of the type of drive used—whether electric or diesel. This research also explores the integration of starch-based carbon as an electrode material in supercapacitors, offering an innovative, sustainable alternative to traditional graphite or graphene electrodes. The carbon material was obtained through a simple carbonization process, with experimental results demonstrating a material capacity of approximately 130 F/g. To quantify the energy recovery, calculations were made regarding the mass and power requirements of the supercapacitors. For the tested vehicle, it was estimated that around 28.7% of the energy could be recovered during the braking process. To store 15 kWh of energy, the total mass of the capacitors required is approximately 245.1 kg. The study emphasizes the importance of increasing voltage levels in railway systems, which can enhance energy transmission and utilization efficiency. Additionally, the paper discusses the necessity of controlled energy discharge, allowing for the flexible management of energy release to meet the varying power demands of trains. By integrating high-voltage supercapacitors and advanced materials like starch-based carbon, this research paves the way for more sustainable and efficient railway systems, contributing to the industry’s goals of reducing emissions and improving operational performance. The findings underscore the crucial role of these capacitors in modernizing railway infrastructure and promoting environmentally responsible transportation solutions. Full article
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17 pages, 3816 KiB  
Article
Study on the Economic Operation of a 1000 MWe Coal-Fired Power Plant with CO2 Capture
by Jinning Yang, Chaowei Wang, Dong Xu, Xuehai Yu, Yang Yang, Zhiyong Wang and Xiao Wu
Energies 2024, 17(19), 4986; https://doi.org/10.3390/en17194986 - 5 Oct 2024
Cited by 2 | Viewed by 2160
Abstract
The flexible operation of carbon capture units is crucial for the economic performance of coal-fired power plants equipped with CO2 capture systems. This paper aims to investigate the impact of electricity, CO2, and fuel prices on the economic operation of [...] Read more.
The flexible operation of carbon capture units is crucial for the economic performance of coal-fired power plants equipped with CO2 capture systems. This paper aims to investigate the impact of electricity, CO2, and fuel prices on the economic operation of such plants. A novel economic optimization model is proposed, integrating a static model of the carbon capture system with a particle swarm optimization algorithm. A new concept, the CO2 boundary price, is introduced as a key metric for determining the operating conditions of CO2 capture units. The CO2 boundary price rises when the power load decreases due to the decline in power generation efficiency, and it also increases with rising fuel prices, as the cost of steam for CO2 capture increases. Additionally, when the objective is to meet power load demand, CO2 prices have a great influence on the operation of CO2 capture units, assuming fixed coal and electricity prices. However, when the primary goal is to maximize plant profitability, the system’s operational conditions are strongly influenced by the relative prices of electricity and CO2. The proposed optimization model and the uncovered price-effect mechanisms provide valuable insights into the economic operation of carbon capture power plants. Full article
(This article belongs to the Topic CO2 Capture and Renewable Energy)
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20 pages, 2633 KiB  
Article
Deep Low-Carbon Economic Optimization Using CCUS and Two-Stage P2G with Multiple Hydrogen Utilizations for an Integrated Energy System with a High Penetration Level of Renewables
by Junqiu Fan, Jing Zhang, Long Yuan, Rujing Yan, Yu He, Weixing Zhao and Nang Nin
Sustainability 2024, 16(13), 5722; https://doi.org/10.3390/su16135722 - 4 Jul 2024
Cited by 6 | Viewed by 1885
Abstract
Integrating carbon capture and storage (CCS) technology into an integrated energy system (IES) can reduce its carbon emissions and enhance its low-carbon performance. However, the full CCS of flue gas displays a strong coupling between lean and rich liquor as carbon dioxide liquid [...] Read more.
Integrating carbon capture and storage (CCS) technology into an integrated energy system (IES) can reduce its carbon emissions and enhance its low-carbon performance. However, the full CCS of flue gas displays a strong coupling between lean and rich liquor as carbon dioxide liquid absorbents. Its integration into IESs with a high penetration level of renewables results in insufficient flexibility and renewable curtailment. In addition, integrating split-flow CCS of flue gas facilitates a short capture time, giving priority to renewable energy. To address these limitations, this paper develops a carbon capture, utilization, and storage (CCUS) method, into which storage tanks for lean and rich liquor and a two-stage power-to-gas (P2G) system with multiple utilizations of hydrogen including a fuel cell and a hydrogen-blended CHP unit are introduced. The CCUS is integrated into an IES to build an electricity–heat–hydrogen–gas IES. Accordingly, a deep low-carbon economic optimization strategy for this IES, which considers stepwise carbon trading, coal consumption, renewable curtailment penalties, and gas purchasing costs, is proposed. The effects of CCUS, the two-stage P2G system, and stepwise carbon trading on the performance of this IES are analyzed through a case-comparative analysis. The results show that the proposed method allows for a significant reduction in both carbon emissions and total operational costs. It outperforms the IES without CCUS with an 8.8% cost reduction and a 70.11% reduction in carbon emissions. Compared to the IES integrating full CCS, the proposed method yields reductions of 6.5% in costs and 24.7% in emissions. Furthermore, the addition of a two-stage P2G system with multiple utilizations of hydrogen further amplifies these benefits, cutting costs by 13.97% and emissions by 12.32%. In addition, integrating CCUS into IESs enables the full consumption of renewables and expands hydrogen utilization, and the renewable consumption proportion in IESs can reach 69.23%. Full article
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20 pages, 2917 KiB  
Article
CO2 Removal in Hydrogen Production Plants
by Stefania Moioli and Laura A. Pellegrini
Energies 2024, 17(13), 3089; https://doi.org/10.3390/en17133089 - 22 Jun 2024
Cited by 2 | Viewed by 1963
Abstract
Hydrogen is an industrial raw material both for the production of chemicals and for oil refining with hydrotreating. It is the subject of increasing attention for its possible use as an energy carrier and as a flexible energy storage medium. Its production is [...] Read more.
Hydrogen is an industrial raw material both for the production of chemicals and for oil refining with hydrotreating. It is the subject of increasing attention for its possible use as an energy carrier and as a flexible energy storage medium. Its production is generally accomplished in Steam Methane Reforming (SMR) plants, where a gaseous mixture of CO and H2, with a limited number of other species, is obtained. The process of production and purification generates relevant amounts of carbon dioxide, which needs to be removed due to downstream process requirements or to limit its emissions to the atmosphere. A work by IEAGHG focused on the study of a state-of-the-art Steam Methane Reforming plant producing 100 kNm3/h of H2 and considered chemical absorption with MethylDiEthanolAmine (MDEA) solvent for removing carbon dioxide from the PSA tail gas in a baseline scheme composed of the absorber, one flash vessel and the regeneration column. This type of process is characterized by high energy consumption, in particular at the reboiler of the regeneration column, usually operated by employing steam, and modifications to the baseline scheme can allow for a reduction of the operating costs, though with an increase in the complexity of the plant. This work analyses three configurations of the treatment section of the off gas obtained after the purification of the hydrogen stream in the Pressure Swing Adsorption unit with the aim of selecting the one which minimizes the overall costs so as to further enhance Carbon Capture and Storage in non-power industries as well. Full article
(This article belongs to the Special Issue Advances in Hydrogen Energy III)
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23 pages, 3160 KiB  
Article
Decarbonization Analysis for Thermal Generation and Regionally Integrated Large-Scale Renewables Based on Minutely Optimal Dispatch with a Kentucky Case Study
by Donovin D. Lewis, Aron Patrick, Evan S. Jones, Rosemary E. Alden, Abdullah Al Hadi, Malcolm D. McCulloch and Dan M. Ionel
Energies 2023, 16(4), 1999; https://doi.org/10.3390/en16041999 - 17 Feb 2023
Cited by 8 | Viewed by 3898
Abstract
Decarbonization of existing electricity generation portfolios with large-scale renewable resources, such as wind and solar photo-voltaic (PV) facilities, is important for a transition to a sustainable energy future. This paper proposes an ultra-fast optimization method for economic dispatch of firm thermal generation using [...] Read more.
Decarbonization of existing electricity generation portfolios with large-scale renewable resources, such as wind and solar photo-voltaic (PV) facilities, is important for a transition to a sustainable energy future. This paper proposes an ultra-fast optimization method for economic dispatch of firm thermal generation using high granularity, one minute resolution load, wind, and solar PV data to more accurately capture the effects of variable renewable energy (VRE). Load-generation imbalance and operational cost are minimized in a multi-objective clustered economic dispatch problem with various generation portfolios, realistic generator flexibility, and increasing levels of VRE integration. The economic feasibility of thermal dispatch scenarios is evaluated through a proposed method of levelized cost of energy (LCOE) for clustered generation portfolios. Effective renewable economics is applied to assess resource adequacy, annual carbon emissions, renewable capacity factor, over generation, and cost to build between thermal dispatch scenarios with incremental increases in VRE penetration. Solar PV and wind generation temporally complement one another in the region studied, and the combination of the two is beneficial to renewable energy integration. Furthermore, replacing older coal units with cleaner and agile natural gas units increases renewable hosting capacity and provides further pathways to decarbonization. Minute-based chronological simulations enable the assessment of renewable effectiveness related to weather-related variability and of complementary technologies, including energy storage for which a sizing procedure is proposed. The generally applicable methods are regionally exemplified for Kentucky, USA, including eight scenarios with four major year-long simulated case studies and 176 subcases using high performance computing (HPC) systems. Full article
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21 pages, 6791 KiB  
Article
Dynamic Modeling of CO2 Absorption Process Using Hollow-Fiber Membrane Contactor in MEA Solution
by Alexandru-Constantin Bozonc, Ana-Maria Cormos, Simion Dragan, Cristian Dinca and Calin-Cristian Cormos
Energies 2022, 15(19), 7241; https://doi.org/10.3390/en15197241 - 2 Oct 2022
Cited by 10 | Viewed by 3282
Abstract
In this work, a comprehensive mathematical model was developed in order to evaluate the CO2 capture process in a microporous polypropylene hollow-fiber membrane countercurrent contactor, using monoethanolamine (MEA) as the chemical solvent. In terms of CO2 chemical absorption, the developed model [...] Read more.
In this work, a comprehensive mathematical model was developed in order to evaluate the CO2 capture process in a microporous polypropylene hollow-fiber membrane countercurrent contactor, using monoethanolamine (MEA) as the chemical solvent. In terms of CO2 chemical absorption, the developed model showed excellent agreement with the experimental data published in the literature for a wide range of operating conditions (R2 > 0.96), 1–2.7 L/min gas flow rates and 10–30 L/h liquid flow rates. Based on developed model, the effects of the gas flow rate, aqueous liquid absorbents’ flow rate and also inlet CO2 concentration on the removal efficiency of CO2 were determined. The % removal of CO2 increased while increasing the MEA solution flow rate; 81% of CO2 was removed at the high flow rate. The CO2 removal efficiency decreased while increasing the gas flow rate, and the residence time in the hollow-fiber membrane contactors increased when the gas flow rate was lower, reaching 97% at a gas flow rate of 1 L‧min−1. However, the effect was more pronounced while operating at high gas flow rates. Additionally, the influence of momentous operational parameters such as the number of fibers and module length on the CO2 separation efficiency was evaluated. On this basis, the developed model was also used to evaluate CO2 capture process in hollow-fiber membrane contactors in a flexible operation scenario (with variation in operating conditions) in order to predict the process parameters (liquid and gaseous flows, composition of the streams, mass transfer area, mass transfer coefficient, etc.). Full article
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