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Keywords = X-ray and gamma ray detectors

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13 pages, 3451 KB  
Article
Performance Degradation of Ga2O3-Based X-Ray Detector Under Gamma-Ray Irradiation
by Xiao Ouyang, Silong Zhang, Tao Bai, Zhuo Chen, Yuxin Deng, Leidang Zhou, Xiaojing Song, Hao Chen, Yuru Lai, Xing Lu, Liang Chen, Liangliang Miao and Xiaoping Ouyang
Micromachines 2025, 16(3), 339; https://doi.org/10.3390/mi16030339 - 14 Mar 2025
Cited by 3 | Viewed by 958
Abstract
X-ray response performances of a p-NiO/β-Ga2O3 hetero-junction diode (HJD) X-ray detector were studied before and after γ-ray irradiation at −200 V, with a total dose of 13.5 kGy(Si). The response performances of the HJD X-ray detector were influenced [...] Read more.
X-ray response performances of a p-NiO/β-Ga2O3 hetero-junction diode (HJD) X-ray detector were studied before and after γ-ray irradiation at −200 V, with a total dose of 13.5 kGy(Si). The response performances of the HJD X-ray detector were influenced by the trap-assistant conductive process of the HJD under reverse bias, which exhibited an increasing net (response) current, nonlinearity, and a long response time. After irradiation, the Poole–Frenkel emission (PFE) dominated the leakage current of HJDs due to the higher electric field caused by the increased net carrier concentration of β-Ga2O3. This conductive process weakened the performance of the HJD X-ray detector in terms of sensitivity, output linearity, and response speed. This study provided valuable insights into the radiation damage and performance degradation mechanisms of Ga2O3-based radiation detectors and offered guidance on improving the reliability and stability of these radiation detectors. Full article
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28 pages, 1881 KB  
Review
Applications of Cd(Zn)Te Radiation Detectors in Non-Destructive Testing and Evaluation
by Anthony R. Whittemore and Elena Maria Zannoni
Sensors 2025, 25(6), 1776; https://doi.org/10.3390/s25061776 - 13 Mar 2025
Cited by 1 | Viewed by 2046
Abstract
This review explores the applications of room temperature semiconductor detectors, with a focus on Cd(Zn)Te based detection systems, in non-destructive testing and evaluation (NDT&E). Cd(Zn)Te detectors, which operate efficiently at ambient temperatures, eliminate the need for cryogenic cooling systems and offer high energy [...] Read more.
This review explores the applications of room temperature semiconductor detectors, with a focus on Cd(Zn)Te based detection systems, in non-destructive testing and evaluation (NDT&E). Cd(Zn)Te detectors, which operate efficiently at ambient temperatures, eliminate the need for cryogenic cooling systems and offer high energy and spatial resolution, making them ideal for a wide range of NDT&E applications. Key performance parameters such as energy resolution, spatial resolution, time resolution, detector efficiency, and form factor are discussed. The paper highlights the utilization of Cd(Zn)Te detectors in various imaging and spectroscopic applications, including nuclear threat detection and non-proliferation, archaeological NDT, and Unmanned Aerial Vehicle radiological surveying. Cd(Zn)Te detectors hold significant promise in NDT&E due to their high-resolution imaging, superior spectroscopic capabilities, versatility, and portability. Full article
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11 pages, 50395 KB  
Article
Detection of Low-Density Foreign Objects in Infant Snacks Using a Continuous-Wave Sub-Terahertz Imaging System for Industrial Applications
by Byeong-Hyeon Na, Dae-Ho Lee, Jaein Choe, Young-Duk Kim and Mi-Kyung Park
Sensors 2024, 24(22), 7374; https://doi.org/10.3390/s24227374 - 19 Nov 2024
Viewed by 1808
Abstract
Low-density foreign objects (LDFOs) in foods pose significant safety risks to consumers. Existing detection methods, such as metal and X-ray detectors, have limitations in identifying low-density and nonmetallic contaminants. To address these challenges, our research group constructed and optimized a continuous-wave sub-terahertz (THz) [...] Read more.
Low-density foreign objects (LDFOs) in foods pose significant safety risks to consumers. Existing detection methods, such as metal and X-ray detectors, have limitations in identifying low-density and nonmetallic contaminants. To address these challenges, our research group constructed and optimized a continuous-wave sub-terahertz (THz) imaging system for the real-time, on-site detection of LDFOs in infant snacks. The system was optimized by adjusting the attenuation value from 0 to 9 dB and image processing parameters [White (W), Black (B), and Gamma (G)] from 0 to 100. Its detectability was evaluated across eight LDFOs underneath snacks with scanning at 30 cm/s. The optimal settings for puffed snacks and freeze-dried chips were found to be 3 dB attenuation with W, B, and G values of 100, 50, and 80, respectively, while others required 0 dB attenuation with W, B, and G set to 100, 0, and 100, respectively. Additionally, the moisture content of infant snacks was measured using a modified AOAC-based drying method at 105 °C, ensuring the removal of all free moisture. Using these optimized settings, the system successfully detected a housefly and a cockroach underneath puffed snacks and freeze-dried chips. It also detected LDFOs as small as 3 mm in size in a single layer of snacks, including polyurethane, polyvinyl chloride, ethylene–propylene–diene–monomer, and silicone, while in two layers of infant snacks, they were detected up to 7.5 mm. The constructed system can rapidly and effectively detect LDFOs in foods, offering a promising approach to enhance safety in the food industry. Full article
(This article belongs to the Section Sensing and Imaging)
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16 pages, 1918 KB  
Article
Convolutional Neural Network Processing of Radio Emission for Nuclear Composition Classification of Ultra-High-Energy Cosmic Rays
by Tudor Alexandru Calafeteanu, Paula Gina Isar and Emil Ioan Sluşanschi
Universe 2024, 10(8), 327; https://doi.org/10.3390/universe10080327 - 15 Aug 2024
Cited by 2 | Viewed by 1621
Abstract
Ultra-high-energy cosmic rays (UHECRs) are extremely rare energetic particles of ordinary matter in the Universe, traveling astronomical distances before reaching the Earth’s atmosphere. When primary cosmic rays interact with atmospheric nuclei, cascading extensive air showers (EASs) of secondary elementary particles are developed. Radio [...] Read more.
Ultra-high-energy cosmic rays (UHECRs) are extremely rare energetic particles of ordinary matter in the Universe, traveling astronomical distances before reaching the Earth’s atmosphere. When primary cosmic rays interact with atmospheric nuclei, cascading extensive air showers (EASs) of secondary elementary particles are developed. Radio detectors have proven to be a reliable method for reconstructing the properties of EASs, such as the shower’s axis, its energy, and its maximum (Xmax). This aids in understanding fundamental astrophysical phenomena, like active galactic nuclei and gamma-ray bursts. Concurrently, data science has become indispensable in UHECR research. By applying statistical, computational, and deep learning methods to both real-world and simulated radio data, researchers can extract insights and make predictions. We introduce a convolutional neural network (CNN) architecture designed to classify simulated air shower events as either being generated by protons or by iron nuclei. The classification achieved a stable test error of 10%, with Accuracy and F1 scores of 0.9 and an MCC of 0.8. These metrics indicate strong prediction capability for UHECR’s nuclear composition, based on data that can be gathered by detectors at the world’s largest cosmic rays experiment on Earth, the Pierre Auger Observatory, which includes radio antennas, water Cherenkov detectors, and fluorescence telescopes. Full article
(This article belongs to the Special Issue Advanced Studies in Ultra-High-Energy Cosmic Rays)
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13 pages, 1478 KB  
Article
Enhancing Gamma-Ray Burst Detection: Evaluation of Neural Network Background Estimator and Explainable AI Insights
by Riccardo Crupi, Giuseppe Dilillo, Giovanni Della Casa, Fabrizio Fiore and Andrea Vacchi
Galaxies 2024, 12(2), 12; https://doi.org/10.3390/galaxies12020012 - 14 Mar 2024
Cited by 3 | Viewed by 2332
Abstract
The detection of Gamma-Ray Bursts (GRBs) using spaceborne X/gamma-ray photon detectors depends on a reliable background count rate estimate. This study focuses on evaluating a data-driven background estimator based on a neural network designed to adapt to various X/gamma-ray space telescopes. Three trials [...] Read more.
The detection of Gamma-Ray Bursts (GRBs) using spaceborne X/gamma-ray photon detectors depends on a reliable background count rate estimate. This study focuses on evaluating a data-driven background estimator based on a neural network designed to adapt to various X/gamma-ray space telescopes. Three trials were conducted to assess the effectiveness and limitations of the proposed estimator. Firstly, quantile regression was employed to obtain an estimation with a confidence range prediction. Secondly, we assessed the performance of the neural network, emphasizing that a dataset of four months is sufficient for training. We tested its adaptability across various temporal contexts, identified its limitations and recommended re-training for each specific period. Thirdly, utilizing Explainable Artificial Intelligence (XAI) techniques, we delved into the neural network output, determining distinctions between a network trained during solar maxima and one trained during solar minima. This entails conducting a thorough analysis of the neural network behavior under varying solar conditions. Full article
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20 pages, 8814 KB  
Article
Bridgman-Grown (Cd,Mn)Te and (Cd,Mn)(Te,Se): A Comparison of Suitability for X and Gamma Detectors
by Aneta Masłowska, Dominika M. Kochanowska, Adrian Sulich, Jaroslaw Z. Domagala, Marcin Dopierała, Michał Kochański, Michał Szot, Witold Chromiński and Andrzej Mycielski
Sensors 2024, 24(2), 345; https://doi.org/10.3390/s24020345 - 6 Jan 2024
Cited by 2 | Viewed by 1924
Abstract
This study explores the suitability of (Cd,Mn)Te and (Cd,Mn)(Te,Se) as room-temperature X-ray and gamma-ray detector materials, grown using the Bridgman method. The investigation compares their crystal structure, mechanical and optical properties, and radiation detection capabilities. Both crystals can yield large-area single crystal samples [...] Read more.
This study explores the suitability of (Cd,Mn)Te and (Cd,Mn)(Te,Se) as room-temperature X-ray and gamma-ray detector materials, grown using the Bridgman method. The investigation compares their crystal structure, mechanical and optical properties, and radiation detection capabilities. Both crystals can yield large-area single crystal samples measuring approximately 30 × 30 mm2. In low-temperature photoluminescence analysis, both materials showed defect states, and annealing in cadmium vapors effectively eliminated donor–acceptor pair luminescence in (Cd,Mn)Te but not in (Cd,Mn)(Te,Se). Moreover, harder (Cd,Mn)(Te,Se) exhibited a higher etch pit density compared to softer (Cd,Mn)Te. X-ray diffraction examination revealed uniform lattice constant distribution in both compounds, with variations at a part per million level. (Cd,Mn)Te crystals demonstrated excellent single crystal properties with narrower omega scan widths, while (Cd,Mn)(Te,Se) exhibited a high contribution of block-like structures with significantly larger misorientation angles. Spectroscopic evaluations revealed better performance of a pixelated (Cd,Mn)Te detector, in comparison to (Cd,Mn)(Te,Se), achieving a mean full width at half maximum of 14% for the 122 keV gamma peak of Co-57. The reduced performance of the (Cd,Mn)(Te,Se) detector may be attributed to deep trap-related luminescence or block-like structures with larger misorientation angles. In conclusion, Bridgman-grown (Cd,Mn)Te emerges as a more promising material for X-ray and gamma-ray detectors when compared to (Cd,Mn)(Te,Se). Full article
(This article belongs to the Section Sensor Materials)
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14 pages, 6974 KB  
Article
Crystal Growth of the R2SiO5 Compounds (R = Dy, Ho, and Er) by the Floating Zone Method Using a Laser-Diode-Heated Furnace
by Vasile Cristian Ciomaga Hatnean, Aurel Pui, Arkadiy Simonov and Monica Ciomaga Hatnean
Crystals 2023, 13(12), 1687; https://doi.org/10.3390/cryst13121687 - 14 Dec 2023
Cited by 3 | Viewed by 2364
Abstract
In recent years, rare earth silicate compounds have attracted the extensive attention of researchers owing to their potential for applications in scintillation crystals in gamma ray or X-ray detectors, as well as in thermal or environmental barrier coatings. Large high quality crystals of [...] Read more.
In recent years, rare earth silicate compounds have attracted the extensive attention of researchers owing to their potential for applications in scintillation crystals in gamma ray or X-ray detectors, as well as in thermal or environmental barrier coatings. Large high quality crystals of three members of the rare earth monosilicates family of compounds, R2SiO5 (with R = Dy, Ho, and Er), have been grown by the floating zone method, using a laser-diode-heated floating zone furnace. Crystal growths attempts were carried out using different parameters in order to determine the optimum conditions for the growth of these materials. The phase purity and the crystalline quality of the crystal boules were analysed using powder and Laue X-ray diffraction. Single crystal X-ray diffraction experiments were carried out to determine the crystal structures of the boules. The optimum conditions used for the crystal growth of R2SiO5 materials are reported. The phase purity and high crystalline quality of the crystals produced makes them ideal for detailed investigations of the intrinsic physical and chemical properties of these materials. Full article
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13 pages, 2051 KB  
Article
Improving the Time Resolution of Large-Area LaBr3:Ce Detectors with SiPM Array Readout
by Maurizio Bonesini, Roberto Bertoni, Andrea Abba, Francesco Caponio, Marco Prata and Massimo Rossella
Condens. Matter 2023, 8(4), 99; https://doi.org/10.3390/condmat8040099 - 17 Nov 2023
Cited by 6 | Viewed by 2566
Abstract
LaBr3:Ce crystals have good scintillation properties for X-ray spectroscopy. Initially, they were introduced for radiation imaging in medical physics with either a photomultiplier or SiPM readout, and they found extensive applications in homeland security and gamma-ray astronomy. We used 1 [...] Read more.
LaBr3:Ce crystals have good scintillation properties for X-ray spectroscopy. Initially, they were introduced for radiation imaging in medical physics with either a photomultiplier or SiPM readout, and they found extensive applications in homeland security and gamma-ray astronomy. We used 1 round LaBr3:Ce crystals to realize compact detectors with the SiPM array readout. The aim was a good energy resolution and a fast time response to detect low-energy X-rays around 100 keV. A natural application was found inside the FAMU experiment, at RIKEN RAL. Its aim is a precise measurement of the proton Zemach radius with impinging muons, to contribute to the solution to the so-called “proton radius puzzle”. Signals to be detected are characteristic X-rays around 130 KeV. A limit for this type of detector, as compared to the ones with a photomultiplier readout, is its poorer timing characteristics due to the large capacity of the SiPM arrays used. In particular, long signal falltimes are a problem in experiments such as FAMU, where a “prompt” background component must be separated from a “delayed” one (after 600 ns) in the signal X-rays to be detected. Dedicated studies were pursued to improve the timing characteristics of the used detectors, starting from hybrid ganging of SiPM cells; then developing a suitable zero pole circuit with a parallel ganging, where an increased overvoltage for the SiPM array was used to compensate for the signal decrease; and finally designing ad hoc electronics to split the 1 detector’s SiPM array into four quadrants, thus reducing the involved capacitances. The aim was to improve the detectors’ timing characteristics, especially falltime, while keeping a good FWHM energy resolution for low-energy X-ray detection. Full article
(This article belongs to the Special Issue High Precision X-ray Measurements 2023)
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14 pages, 5715 KB  
Article
Combined Spectroscopy System Utilizing Gas Electron Multiplier and Timepix3 Technology for Laser Plasma Experiments
by Veronica De Leo, Gerardo Claps, Francesco Cordella, Gabriele Cristoforetti, Leonida Antonio Gizzi, Petra Koester, Danilo Pacella and Antonella Tamburrino
Condens. Matter 2023, 8(4), 98; https://doi.org/10.3390/condmat8040098 - 17 Nov 2023
Cited by 1 | Viewed by 2109
Abstract
We present an innovative X-ray spectroscopy system to address the complex study of the X-ray emissions arising from laser–target interactions, where the emissions occur within extremely brief intervals from femtoseconds to nanoseconds. Our system combines a Gas Electron Multiplier (GEM) detector with a [...] Read more.
We present an innovative X-ray spectroscopy system to address the complex study of the X-ray emissions arising from laser–target interactions, where the emissions occur within extremely brief intervals from femtoseconds to nanoseconds. Our system combines a Gas Electron Multiplier (GEM) detector with a silicon-based Timepix3 (TPX3) detector. These detectors work in tandem, allowing for a spectroscopic radiation analysis along the same line of sight. With an active area of 10 × 10 cm2, the GEM detector allows for 1D measurements for X-ray energies (2–50 keV) by utilizing the full 10 cm gas depth. The high-energy part of the radiation beam exits through a downstream side window of the GEM without being absorbed in the gas volume. Positioned side-on at the GEM detector’s exit, the TPX3 detector, equipped with a pixelated sensor (55 µm × 55 µm; active area 14 mm × 14 mm), uses its full 14 mm silicon sensor to detect hard X-rays (50–500 keV) and gamma rays (0.5–10 MeV). We demonstrate the correct operation of the entire detection system and provide a detailed description of the Timepix3 detector’s calibration procedure, highlighting the suitability of the combined system to work in laser plasma facilities. Full article
(This article belongs to the Special Issue High Precision X-ray Measurements 2023)
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17 pages, 18899 KB  
Article
Impact of Bulk and Nano Bismuth Oxide on the Attenuation Parameters of Bentonite Barite Composites
by Mahmoud I. Abbas, Mona M. Gouda, Sarah N. EL-Shimy, Mirvat F. Dib, Hala M. Abdellatif, Raqwana Baharoon, Mohamed Elsafi and Ahmed M. El-Khatib
Coatings 2023, 13(10), 1670; https://doi.org/10.3390/coatings13101670 - 24 Sep 2023
Cited by 3 | Viewed by 1756
Abstract
Since bentonite can absorb neutrons and gamma rays without sacrificing structural integrity, it is frequently used as the main shielding material in many nuclear installations. Recently, there has been a trend toward enhancing the shielding qualities of bentonite by adding various chemicals. However, [...] Read more.
Since bentonite can absorb neutrons and gamma rays without sacrificing structural integrity, it is frequently used as the main shielding material in many nuclear installations. Recently, there has been a trend toward enhancing the shielding qualities of bentonite by adding various chemicals. However, the majority of the added materials either require particular handling procedures or pose health risks. The availability of environmentally friendly additives would be wonderful. The addition of barite to bentonite composites greatly raises the density of the specimens. Additionally, the performance of bentonite–barite composites as radiation shielding materials is improved by adding various amounts of bulk and nano Bi2O3 as a filler (6%, 13%, and 20%). Energy dispersive X-ray analysis (EDX) was used to determine the chemical makeup of the produced specimens. The scanning electron microscopy (SEM) pictures showed the samples’ cross-sections’ porosity and homogeneity. 241Am, 133Ba, 137Cs, and 60Co are radioactive sources that emit energies of 59.53, 80.99, 356.01, 661.66, 1173.23, and 1332.5 keV, respectively, and the NaI (Tl) scintillation detector was used in this investigation. The area under the peak of the observed energy spectra was measured using the Genie 2000 program in both the specimen’s absence and presence. The coefficients for linear and mass attenuation were calculated. To determine the theoretical mass attenuation coefficients, the XCOM program was utilized and then compared to the corresponding experimental values. Various radiation shielding parameters dependent on the linear attenuation coefficient were computed for each studied composite. These parameters include the mean free path (MFP), half value layer (HVL), and tenth value layer (TVL). Also, the Zeff and the EABF were determined for each specimen. According to the findings, bismuth oxide was added to bentonite–barite composites to reduce the transmitted flux through the specimens, which increased the LAC of the bentonite–barite composites. Furthermore, adding nanosized bismuth oxide particles increased the sample’s density and improved the material’s shielding properties. At a photon energy of 0.356 keV, the relative deviation (∆%) between the experimental nano- and micro values for Bi2O3 (20 wt%) was 12.1974, confirming that the nanoparticles increase attenuation efficiency. Full article
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18 pages, 6027 KB  
Article
Potentialities of CdZnTe Quasi-Hemispherical Detectors for Hard X-ray Spectroscopy of Kaonic Atoms at the DAΦNE Collider
by Leonardo Abbene, Antonino Buttacavoli, Fabio Principato, Gaetano Gerardi, Manuele Bettelli, Andrea Zappettini, Massimiliano Bazzi, Mario Bragadireanu, Michael Cargnelli, Marco Carminati, Alberto Clozza, Griseld Deda, Raffaele Del Grande, Luca De Paolis, Laura Fabbietti, Carlo Fiorini, Carlo Guaraldo, Mihail Iliescu, Misahiko Iwasaki, Aleksander Khreptak, Simone Manti, Johann Marton, Marco Miliucci, Pawel Moskal, Fabrizio Napolitano, Szymon Niedźwiecki, Hiroaky Ohnishi, Kristian Piscicchia, Yuta Sada, Francesco Sgaramella, Hexi Shi, Michalł Silarski, Diana Laura Sirghi, Florin Sirghi, Magdalena Skurzok, Antonio Spallone, Kairo Toho, Marlene Tüchler, Oton Vazquez Doce, Chihiro Yoshida, Johannes Zmeskal, Alessandro Scordo and Catalina Curceanuadd Show full author list remove Hide full author list
Sensors 2023, 23(17), 7328; https://doi.org/10.3390/s23177328 - 22 Aug 2023
Cited by 6 | Viewed by 1810
Abstract
Kaonic atom X-ray spectroscopy is a consolidated technique for investigations on the physics of strong kaon–nucleus/nucleon interaction. Several experiments have been conducted regarding the measurement of soft X-ray emission (<20 keV) from light kaonic atoms (hydrogen, deuterium, and helium). Currently, there have been [...] Read more.
Kaonic atom X-ray spectroscopy is a consolidated technique for investigations on the physics of strong kaon–nucleus/nucleon interaction. Several experiments have been conducted regarding the measurement of soft X-ray emission (<20 keV) from light kaonic atoms (hydrogen, deuterium, and helium). Currently, there have been new research activities within the framework of the SIDDHARTA-2 experiment and EXCALIBUR proposal focusing on performing precise and accurate measurements of hard X-rays (>20 keV) from intermediate kaonic atoms (carbon, aluminum, and sulfur). In this context, we investigated cadmium–zinc–telluride (CdZnTe or CZT) detectors, which have recently demonstrated high-resolution capabilities for hard X-ray and gamma-ray detection. A demonstrator prototype based on a new cadmium–zinc–telluride quasi-hemispherical detector and custom digital pulse processing electronics was developed. The detector covered a detection area of 1 cm2 with a single readout channel and interesting room-temperature performance with energy resolution of 4.4% (2.6 keV), 3% (3.7 keV), and 1.4% (9.3 keV) FWHM at 59.5, 122.1, and 662 keV, respectively. The results from X-ray measurements at the DAΦNE collider at the INFN National Laboratories of Frascati (Italy) are also presented with particular attention to the effects and rejection of electromagnetic and hadronic background. Full article
(This article belongs to the Special Issue Particle Detector R&D: Design, Characterization and Applications)
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15 pages, 5941 KB  
Article
Effect of Waste Iron Filings (IF) on Radiation Shielding Feature of Polyepoxide Composites
by Mohammed T. Alresheedi and Mohamed Elsafi
Crystals 2023, 13(8), 1168; https://doi.org/10.3390/cryst13081168 - 27 Jul 2023
Cited by 5 | Viewed by 1565
Abstract
In the present work, photon and neutron attenuation properties of polyepoxide composites produced by doping waste iron filings (IF) at different percentages (0%, 20%, 40%, and 60% iron filing percentage) were obtained using theoretical and experimental techniques. The experimental technique was performed using [...] Read more.
In the present work, photon and neutron attenuation properties of polyepoxide composites produced by doping waste iron filings (IF) at different percentages (0%, 20%, 40%, and 60% iron filing percentage) were obtained using theoretical and experimental techniques. The experimental technique was performed using an HPGe detector with four different gamma lines (0.0595, 0.6617, 1.173, and 1.333 MeV) emitted from three gamma-ray sources (241Am, 137Cs, and 60Co). The theoretical techniques for shielding parameters calculation are estimated with Phy-X software and the XCOM program as well. The experimental and theoretical values of the mass/linear attenuation coefficient (M/LAC), half/tenth value layer (H/TVL), mean free path (MFP), lead equivalent thickness (LEth), and radiation shielding efficiency (RSE) have been determined and compared. A good agreement was achieved during the comparison. The shielding performance of the prepared composites increased with increasing the iron filing rate, where we can arrange the performance of shielding according to EP–IF60 > EP–IF40 > EP–IF20 > EP–IF0 at all different experimental and theoretical energies. The effective and equivalent (Zeff, Zeq) atomic numbers as well as the exposure buildup factor (EBF) at different depletion distances or mean free paths (MFPs) have been calculated for all EP–IF composites. The lowest EBF was for EP–IF60 while the highest EBF was for EP–IF0 through the discussed energy from 0.015 to 15 MeV. Finally, the fast neutron removal cross-section (FRNC) has been calculated for the prepared composites and the results showed improvement in FNRC with increasing the iron filing rate. Full article
(This article belongs to the Topic Recent Advances in Ionizing Radiation Shielding Materials)
(This article belongs to the Section Hybrid and Composite Crystalline Materials)
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18 pages, 2949 KB  
Article
Study of Prepared Lead-Free Polymer Nanocomposites for X- and Gamma-ray Shielding in Healthcare Applications
by Abdulrhman Hasan Alsaab and Sadek Zeghib
Polymers 2023, 15(9), 2142; https://doi.org/10.3390/polym15092142 - 29 Apr 2023
Cited by 19 | Viewed by 3636
Abstract
Polymer composites were synthesized via melt mixing for radiation shielding in the healthcare sector. A polymethyl-methacrylate (PMMA) matrix was filled with Bi2O3 nanoparticles at 10%, 20%, 30%, and 40% weight percentages. The characterization of nanocomposites included their morphological, structural, and [...] Read more.
Polymer composites were synthesized via melt mixing for radiation shielding in the healthcare sector. A polymethyl-methacrylate (PMMA) matrix was filled with Bi2O3 nanoparticles at 10%, 20%, 30%, and 40% weight percentages. The characterization of nanocomposites included their morphological, structural, and thermal properties, achieved using SEM, XRD, and TGA, respectively. The shielding properties for all synthesized samples including pristine PMMA were measured with gamma spectrometry using a NaI (Tl) scintillator detector spanning a wide range of energies and using different radioisotopes, namely Am-241 (59.6 keV), Co-57 (122.2 keV), Ra-226 (242.0), Ba-133 (80.99 and 356.02 keV), Cs-137 (661.6 keV), and Co-60 (1173.2 and 1332.5 keV). A substantial increase in the mass attenuation coefficients was obtained at low and medium energies as the filler weight percentage increased, with minor variations at higher gamma energies (1173 and 1332 keV). The mass attenuation coefficient decreased with increasing energy except under 122 keV gamma rays due to the K-absorption edge of bismuth (90.5 keV). At 40% loading of Bi2O3, the mass attenuation coefficient for the cesium 137Cs gamma line at 662 keV reached the corresponding value for the toxic heavy element lead. The synthesized PMMA-Bi2O3 nanocomposites proved to be highly effective, lead-free, safe, and lightweight shielding materials for X- and gamma rays within a wide energy range (<59 keV to 1332 keV), making them of interest for healthcare applications. Full article
(This article belongs to the Section Polymer Composites and Nanocomposites)
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11 pages, 3519 KB  
Article
Ellipsometry Characterisation for the Cd1-xZnxTe1-ySey Semiconductor Used in X-ray and Gamma Radiation Detectors
by Lidia Martínez Herraiz, Jose Luis Plaza Canga-argüelles and Alejandro Francisco Braña de Cal
Crystals 2023, 13(4), 693; https://doi.org/10.3390/cryst13040693 - 18 Apr 2023
Cited by 1 | Viewed by 1812
Abstract
The study of the optical properties of the Cd1-xZnxTe1-ySey (CZTS) crystal provides a clear idea about its response to incident X-ray or gamma radiation. This is important for selecting a proper composition of CZTS to achieve [...] Read more.
The study of the optical properties of the Cd1-xZnxTe1-ySey (CZTS) crystal provides a clear idea about its response to incident X-ray or gamma radiation. This is important for selecting a proper composition of CZTS to achieve superior quality and high-resolution X-ray and gamma radiation detectors at room temperature and reduce their production cost. This article’s novelty is in lowering the cost of the optical and compositional characterisation of CZTS using the ellipsometry technique. The most significant successes achieved are the composition ellipsometry model determination of CZTS based on the Effective Medium Approximation (EMA) substrate of the binary compound CdTe and ZnSe with an oxide layer of CdTe and the experimental verification that the bandgap moves to lower energies with the addition of Se. Full article
(This article belongs to the Topic Advanced Structural Crystals)
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16 pages, 14577 KB  
Article
Investigation of Gamma-Ray Shielding Properties of Bismuth Oxide Nanoparticles with a Bentonite–Gypsum Matrix
by Mahmoud I. Abbas, Ahmed M. El-Khatib, Mohamed Elsafi, Sarah N. El-Shimy, Mirvat F. Dib, Hala M. Abdellatif, Raqwana Baharoon and Mona M. Gouda
Materials 2023, 16(5), 2056; https://doi.org/10.3390/ma16052056 - 2 Mar 2023
Cited by 17 | Viewed by 3984
Abstract
Due to the present industrial world, the risk of radioactivity is notably increasing. Thus, an appropriate shielding material needs to be designed to protect humans and the environment against radiation. In view of this, the present study aims to design new composites of [...] Read more.
Due to the present industrial world, the risk of radioactivity is notably increasing. Thus, an appropriate shielding material needs to be designed to protect humans and the environment against radiation. In view of this, the present study aims to design new composites of the main matrix of bentonite–gypsum with a low-cost, abundant, and natural matrix. This main matrix was intercalated in various amounts with micro- and nanosized particles of bismuth oxide (Bi2O3) as the filler. Energy dispersive X-ray analysis (EDX) recognized the chemical composition of the prepared specimen. The morphology of the bentonite–gypsum specimen was tested using scanning electron microscopy (SEM). The SEM images showed the uniformity and porosity of a cross-section of samples. The NaI (Tl) scintillation detector was used with four radioactive sources (241Am, 137Cs, 133Ba, and 60Co) of various photon energies. Genie 2000 software was used to determine the area under the peak of the energy spectrum observed in the presence and absence of each specimen. Then, the linear and mass attenuation coefficients were obtained. After comparing the experimental results of the mass attenuation coefficient with the theoretical values from XCOM software, it was found that the experimental results were valid. The radiation shielding parameters were computed, including the mass attenuation coefficients (MAC), half-value layer (HVL), tenth-value layer (TVL), and mean free path (MFP), which are dependent on the linear attenuation coefficient. In addition, the effective atomic number and buildup factors were calculated. The results of all of these parameters provided the same conclusion, which confirms the improvement of the properties of γ-ray shielding materials using a mixture of bentonite and gypsum as the main matrix, which is much better than using bentonite alone. Moreover, bentonite mixed with gypsum is a more economical means of production. Therefore, the investigated bentonite–gypsum materials have potential uses in applications such as gamma-ray shielding materials. Full article
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