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27 pages, 1491 KiB  
Article
Spent Nuclear Fuel—Waste to Resource, Part 1: Effects of Post-Reactor Cooling Time and Novel Partitioning Strategies in Advanced Reprocessing on Highly Active Waste Volumes in Gen III(+) UOx Fuel Systems
by Alistair F. Holdsworth, Edmund Ireland and Harry Eccles
J. Nucl. Eng. 2025, 6(3), 29; https://doi.org/10.3390/jne6030029 - 5 Aug 2025
Abstract
Some of nuclear power’s primary detractors are the unique environmental challenges and impacts of radioactive wastes generated during fuel cycle operations. Key benefits of spent fuel reprocessing (SFR) are reductions in primary high active waste (HAW) masses, volumes, and lengths of radiotoxicity at [...] Read more.
Some of nuclear power’s primary detractors are the unique environmental challenges and impacts of radioactive wastes generated during fuel cycle operations. Key benefits of spent fuel reprocessing (SFR) are reductions in primary high active waste (HAW) masses, volumes, and lengths of radiotoxicity at the expense of secondary waste generation and high capital and operational costs. By employing advanced waste management and resource recovery concepts in SFR beyond the existing standard PUREX process, such as minor actinide and fission product partitioning, these challenges could be mitigated, alongside further reductions in HAW volumes, masses, and duration of radiotoxicity. This work assesses various current and proposed SFR and fuel cycle options as base cases, with further options for fission product partitioning of the high heat radionuclides (HHRs), rare earths, and platinum group metals investigated. A focus on primary waste outputs and the additional energy that could be generated by the reprocessing of high-burnup PWR fuel from Gen III(+) reactors using a simple fuel cycle model is used; the effects of 5- and 10-year spent fuel cooling times before reprocessing are explored. We demonstrate that longer cooling times are preferable in all cases except where short-lived isotope recovery may be desired, and that the partitioning of high-heat fission products (Cs and Sr) could allow for the reclassification of traditional raffinates to intermediate level waste. Highly active waste volume reductions approaching 50% vs. PUREX raffinate could be achieved in single-target partitioning of the inactive and low-activity rare earth elements, and the need for geological disposal could potentially be mitigated completely if HHRs are separated and utilised. Full article
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14 pages, 2310 KiB  
Article
A High-Fidelity Model of the Peach Bottom 2 Turbine-Trip Benchmark Using VERA
by Nicholas Herring, Robert Salko and Mehdi Asgari
J. Nucl. Eng. 2025, 6(3), 28; https://doi.org/10.3390/jne6030028 - 4 Aug 2025
Abstract
This work presents a high-fidelity simulation of the Peach Bottom turbine trip (PBTT) benchmark using the Virtual Environment for Reactor Applications (VERA), a multiphysics reactor modeling tool developed by the U.S. Department of Energy’s Consortium for Advanced Simulation of Light Water Reactors energy [...] Read more.
This work presents a high-fidelity simulation of the Peach Bottom turbine trip (PBTT) benchmark using the Virtual Environment for Reactor Applications (VERA), a multiphysics reactor modeling tool developed by the U.S. Department of Energy’s Consortium for Advanced Simulation of Light Water Reactors energy innovation hub. The PBTT benchmark, based on a 1977 transient event at the end of cycle 2 in a General Electric Type-4 boiling water reactor (BWR), is a critical test case for validating core physics models with thermal feedback during rapid reactivity events. VERA was employed to perform end-to-end, pin-resolved simulations from conditions at the beginning of cycle 1 through the turbine-trip transient, incorporating detailed neutron transport, fuel depletion, and subchannel thermal hydraulics. The simulation reproduced key benchmark observables with high accuracy: the peak power excursion occurred at 0.75 s, matching the scram time and closely aligning with the benchmark average of 0.742 s; the simulated maximum power spike was approximately 7600 MW, which is within 3% of the benchmark average of 7400 MW; and void-collapse dynamics were consistent with benchmark expectations. Reactivity predictions during cycles 1 and 2 remained within 1500 pcm and 400 pcm of criticality, respectively. These results confirm VERA’s ability to model complex coupled neutronic and thermal hydraulic behavior in a BWR turbine-trip transient, which will support its use in future studies of modeling dryout, fuel performance, and uncertainty quantification for transients of this type. Full article
(This article belongs to the Special Issue Validation of Code Packages for Light Water Reactor Physics Analysis)
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16 pages, 3999 KiB  
Article
Influence of TRISO Fuel Particle Arrangements on Pebble Neutronics and Isotopic Evolution
by Ben Impson, Mohamed Elhareef, Zeyun Wu and Braden Goddard
J. Nucl. Eng. 2025, 6(3), 27; https://doi.org/10.3390/jne6030027 - 14 Jul 2025
Viewed by 641
Abstract
Pebble Bed Reactors (PBRs) represent a new generation of nuclear reactors. However, modeling TRi-structural ISOtropic (TRISO) fuel particles employed in PBRs presents a unique challenge in comparison to most conventional reactor designs. Rapid generation of different possible fuel particle configurations for Monte-Carlo simulations [...] Read more.
Pebble Bed Reactors (PBRs) represent a new generation of nuclear reactors. However, modeling TRi-structural ISOtropic (TRISO) fuel particles employed in PBRs presents a unique challenge in comparison to most conventional reactor designs. Rapid generation of different possible fuel particle configurations for Monte-Carlo simulations provides improved insights into the effects of particle distribution irregularities on the neutron economy. Defective pebbles could cause changes in the neutron flux in a nuclear reactor due to increased or decreased moderating effects. Different configurations of particle fuel also impact isotope production within the nuclear reactor. This study simulates several TRISO configurations representing limited capabilities of randomization algorithms, manufacturing defects configurations and/or special pebble design. All predictions are compared to an equivalent homogenized model used as baseline. The results show that the TRISO configuration has a non-negligible impact on the parameters under consideration. To explain these results, the ratio of the thermal flux of each model to the thermal flux of the homogeneous model is calculated. A clear pattern is observed in the data: as irregularities in the moderator medium emerge due to the distribution of TRISO particles, the neutron spectrum softens, leading to higher values of k and better fuel utilization. This dependence of the spectrum on the TRISO configuration is used to explain the pattern observed in the depletion calculation. The results open the possibility of optimizing the TRISO configuration in manufactured pebbles for fuel utilization and safeguards. Future work should focus on full core simulations to determine the extent of these findings. Full article
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20 pages, 1338 KiB  
Article
Two-Dimensional Fuel Assembly Study for a Supercritical Water-Cooled Small Modular Reactor
by Valerio Giusti
J. Nucl. Eng. 2025, 6(3), 26; https://doi.org/10.3390/jne6030026 - 9 Jul 2025
Viewed by 195
Abstract
Burnable poisoning and fuel enrichment zoning are two techniques often combined in order to optimize the fuel assembly behavior during the burnup cycle. In the present work, these two techniques will be applied to the 2D optimization of the fuel assembly conceptual design [...] Read more.
Burnable poisoning and fuel enrichment zoning are two techniques often combined in order to optimize the fuel assembly behavior during the burnup cycle. In the present work, these two techniques will be applied to the 2D optimization of the fuel assembly conceptual design for the supercritical water-cooled reactor developed in the framework of the Joint European Canadian Chinese development of Small Modular Reactor Technology project, funded within the Euratom Research and Training programme 2019–2020. The initial configuration of the fuel assembly does not include any burnable absorbers and uses a homogeneous fuel enrichment of 7.5% in 235U. The infinite multiplication factor, k, starts from approximately 1.32 and drops, almost linearly, to 1.0 after a burnup of 40.0 MWd·kg−1. The uniform enrichment is, however, responsible for a pin-power peaking factor that with fresh fuel starts from 1.32 and reduces to 1.08 at the end of the burnup cycle. A simplified analytical model is developed to assess the effect of different lumped burnable absorbers on the time dependence of the assembly k. It is shown that using an adequate number of B4C rods, positioned in the outer wall of the fuel assembly, together with a suitable distribution of six different 235U enrichments, it allows for obtaining an assembly k factor that starts from 1.11 at the beginning of the cycle and remains quite constant over a large fraction of the burnup cycle. Moreover, the pin-power peaking factor is reduced to 1.03 at the beginning of the cycle and remains almost unchanged until the end of the burnup cycle. Full article
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13 pages, 3753 KiB  
Article
Thermal Shock and Synergistic Plasma and Heat Load Testing of Powder Injection Molding Tungsten-Based Alloys
by Mauricio Gago, Steffen Antusch, Alexander Klein, Arkadi Kreter, Christian Linsmeier, Michael Rieth, Bernhard Unterberg and Marius Wirtz
J. Nucl. Eng. 2025, 6(3), 25; https://doi.org/10.3390/jne6030025 - 7 Jul 2025
Viewed by 310
Abstract
Powder injection molding (PIM) has been used to produce nearly net-shaped samples of tungsten-based alloys. These alloys have been previously shown to have favorable characteristics when compared with standard ITER-grade tungsten. Six different alloys were produced with this method: W-1TiC, W-2Y2O [...] Read more.
Powder injection molding (PIM) has been used to produce nearly net-shaped samples of tungsten-based alloys. These alloys have been previously shown to have favorable characteristics when compared with standard ITER-grade tungsten. Six different alloys were produced with this method: W-1TiC, W-2Y2O3, W-3Re-1TiC, W-3Re-2Y2O3, W-1HfC and W-1La2O3-1TiC. These were tested alongside ITER-grade tungsten in the PSI-2 linear plasma device under ITER-relevant plasma and heat loads to assess their suitability for use in a fusion reactor. All materials showed good behavior when exposed to the lower pulse number tests (≤1000 ELM-like pulses), although standard tungsten performed slightly better, with no observable difference in surface roughness. High-power shots, namely one laser pulse of 1.6 GWm−2, revealed that samples containing yttria are more prone to melting and droplet ejection. After high pulse number tests (10,000 and 100,000 pulses), with and without plasma, the reference tungsten showed the most cracking and highest surface roughness of all materials, while the PIM samples seemed to have a higher resistance to cracking. This can be attributed to the higher ductility of these alloys, particularly those containing rhenium. This means that tungsten-based alloys, whether produced via PIM or other methods, could potentially be used in certain areas of a fusion reactor. Full article
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52 pages, 476 KiB  
Article
The First- and Second-Order Features Adjoint Sensitivity Analysis Methodologies for Neural Integro-Differential Equations of Volterra Type: Mathematical Framework and Illustrative Application to a Nonlinear Heat Conduction Model
by Dan Gabriel Cacuci
J. Nucl. Eng. 2025, 6(3), 24; https://doi.org/10.3390/jne6030024 - 4 Jul 2025
Viewed by 218
Abstract
This work presents the mathematical frameworks of the “First-Order Features Adjoint Sensitivity Analysis Methodology for Neural Integro-Differential Equations of Volterra-Type” (1st-FASAM-NIDE-V) and the “Second-Order Features Adjoint Sensitivity Analysis Methodology for Neural Integro-Differential Equations of Volterra-Type” (2nd-FASAM-NIDE-V). It is shown that the 1st-FASAM-NIDE-V methodology [...] Read more.
This work presents the mathematical frameworks of the “First-Order Features Adjoint Sensitivity Analysis Methodology for Neural Integro-Differential Equations of Volterra-Type” (1st-FASAM-NIDE-V) and the “Second-Order Features Adjoint Sensitivity Analysis Methodology for Neural Integro-Differential Equations of Volterra-Type” (2nd-FASAM-NIDE-V). It is shown that the 1st-FASAM-NIDE-V methodology enables the efficient computation of exactly-determined first-order sensitivities of the decoder response with respect to the optimized NIDE-V parameters, requiring a single “large-scale” computation for solving the 1st-Level Adjoint Sensitivity System (1st-LASS), regardless of the number of weights/parameters underlying the NIE-net. The 2nd-FASAM-NIDE-V methodology enables the computation, with unparalleled efficiency, of the second-order sensitivities of decoder responses with respect to the optimized/trained weights involved in the NIDE-V’s decoder, hidden layers, and encoder, requiring only as many “large-scale” computations as there are non-zero first-order sensitivities with respect to the feature functions. These characteristics of the 1st-FASAM-NIDE-V and 2nd-FASAM-NIDE-V are illustrated by considering a nonlinear heat conduction model that admits analytical solutions, enabling the exact verification of the expressions obtained for the first- and second-order sensitivities of NIDE-V decoder responses with respect to the model’s functions of parameters (weights) that characterize the heat conduction model. Full article
18 pages, 2791 KiB  
Article
Deterministic Data Assimilation in Thermal-Hydraulic Analysis: Application to Natural Circulation Loops
by Lanxin Gong, Changhong Peng and Qingyu Huang
J. Nucl. Eng. 2025, 6(3), 23; https://doi.org/10.3390/jne6030023 - 3 Jul 2025
Viewed by 372
Abstract
Recent advances in high-fidelity modeling, numerical computing, and data science have spurred interest in model-data integration for nuclear reactor applications. While machine learning often prioritizes data-driven predictions, this study focuses on data assimilation (DA) to synergize physical models with measured data, aiming to [...] Read more.
Recent advances in high-fidelity modeling, numerical computing, and data science have spurred interest in model-data integration for nuclear reactor applications. While machine learning often prioritizes data-driven predictions, this study focuses on data assimilation (DA) to synergize physical models with measured data, aiming to enhance predictive accuracy and reduce uncertainties. We implemented deterministic DA methods—Kalman filter (KF) and three-dimensional variational (3D-VAR)—in a one-dimensional single-phase natural circulation loop and extended 3D-VAR to RELAP5, a system code for two-phase loop analysis. Unlike surrogate-based or model-reduction strategies, our approach leverages full-model propagation without relying on computationally intensive sampling. The results demonstrate that KF and 3D-VAR exhibit robustness against varied noise types, intensities, and distributions, achieving significant uncertainty reduction in state variables and parameter estimation. The framework’s adaptability is further validated under oceanic conditions, suggesting its potential to augment baseline models beyond conventional extrapolation boundaries. These findings highlight DA’s capacity to improve model calibration, safety margin quantification, and reactor field reconstruction. By integrating high-fidelity simulations with real-world data corrections, the study establishes a scalable pathway to enhance the reliability of nuclear system predictions, emphasizing DA’s role in bridging theoretical models and operational demands without compromising computational efficiency. Full article
(This article belongs to the Special Issue Advances in Thermal Hydraulics of Nuclear Power Plants)
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11 pages, 1699 KiB  
Article
Optimization of the LIBS Technique in Air, He, and Ar at Atmospheric Pressure for Hydrogen Isotope Detection on Tungsten Coatings
by Salvatore Almaviva, Lidia Baiamonte and Marco Pistilli
J. Nucl. Eng. 2025, 6(3), 22; https://doi.org/10.3390/jne6030022 - 1 Jul 2025
Viewed by 334
Abstract
In current and future fusion devices, detecting hydrogen isotopes, particularly tritium and deuterium, implanted or redeposited on the surface of Plasma-Facing Components (PFCs) will be increasingly important to ensure safe machine operations. The Laser-Induced Breakdown Spectroscopy (LIBS) technique has proven capable of performing [...] Read more.
In current and future fusion devices, detecting hydrogen isotopes, particularly tritium and deuterium, implanted or redeposited on the surface of Plasma-Facing Components (PFCs) will be increasingly important to ensure safe machine operations. The Laser-Induced Breakdown Spectroscopy (LIBS) technique has proven capable of performing this task directly in situ, without handling or removing PFCs, thus limiting analysis times and increasing the machine’s duty cycle. To increase sensitivity and the ability to discriminate between isotopes, LIBS analysis can be performed under different background gases at atmospheric pressure, such as air, He, and Ar. In this work, we present the results obtained on tungsten coatings enriched with deuterium and/or hydrogen as a deuterium–tritium nuclear fuel simulant, measured with the LIBS technique in air, He, and Ar at atmospheric pressure, and discuss the pros and cons of their use. The results obtained demonstrate that both He and Ar can improve the LIBS signal resolution of the hydrogen isotopes compared to air. However, using Ar has the additional advantage that the same procedure can also be used to detect He implanted in PFCs as a product of fusion reactions without any interference. Finally, the LIBS signal in an Ar atmosphere increases in terms of the signal-to-noise ratio (SNR), enabling the use of less energetic laser pulses to improve performance in depth profiling analyses. Full article
(This article belongs to the Special Issue Fusion Materials with a Focus on Industrial Scale-Up)
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18 pages, 2029 KiB  
Article
Development of Importance Measures Reflecting the Risk Triplet in Dynamic Probabilistic Risk Assessment: A Case Study Using MELCOR and RAPID
by Xiaoyu Zheng, Hitoshi Tamaki, Yasuteru Sibamoto, Yu Maruyama, Tsuyoshi Takada, Takafumi Narukawa and Takashi Takata
J. Nucl. Eng. 2025, 6(3), 21; https://doi.org/10.3390/jne6030021 - 28 Jun 2025
Viewed by 394
Abstract
While traditional risk importance measures in probabilistic risk assessment are effective for ranking safety-significant components, they often overlook critical aspects such as the timing of accident progression and consequences. Dynamic probabilistic risk assessment offers a framework to quantify such risk information, but standardized [...] Read more.
While traditional risk importance measures in probabilistic risk assessment are effective for ranking safety-significant components, they often overlook critical aspects such as the timing of accident progression and consequences. Dynamic probabilistic risk assessment offers a framework to quantify such risk information, but standardized approaches for estimating risk importance measures remain underdeveloped. This study addresses this gap by: (1) reviewing traditional risk importance measures and their regulatory applications, highlighting their limitations, and introducing newly proposed risk-triplet-based risk importance measures, consisting of timing-based worth, frequency-based worth, and consequence-based worth; (2) conducting a case study of Level 2 dynamic probabilistic risk assessment using the Japan Atomic Energy Agency’s RAPID tool coupled with the severe accident code of MELCOR 2.2 to simulate a station blackout scenario in a boiling water reactor, generating probabilistically sampled sequences with quantified timing, frequency, and consequence of source term release; (3) demonstrating that the new risk importance measures provide differentiated insights into risk significance, enabling multidimensional prioritization of systems and mitigation strategies; for example, the timing-based worth quantifies the delay effect of mitigation systems, and the consequence-based worth evaluates consequence-mitigating potential. This study underscores the potential of dynamic probabilistic risk assessment and risk-triplet-based risk importance measures to support risk-informed and performance-based regulatory decision-making, particularly in contexts where the timing and severity of accident consequences are critical. Full article
(This article belongs to the Special Issue Probabilistic Safety Assessment and Management of Nuclear Facilities)
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14 pages, 805 KiB  
Article
Ultra-Cold Neutrons in qBounce Experiments as Laboratory for Test of Chameleon Field Theories and Cosmic Acceleration
by Derar Altarawneh and Roman Höllwieser
J. Nucl. Eng. 2025, 6(3), 20; https://doi.org/10.3390/jne6030020 - 26 Jun 2025
Viewed by 369
Abstract
The study of scalar field theories like the chameleon field model is of increasing interest due to the Universe’s accelerated expansion, which is believed to be caused in part by dark energy. These fields can elude experimental bounds set on them in high-density [...] Read more.
The study of scalar field theories like the chameleon field model is of increasing interest due to the Universe’s accelerated expansion, which is believed to be caused in part by dark energy. These fields can elude experimental bounds set on them in high-density environments since they interact with matter in a density-dependent way. This paper analyzes the effect of chameleon fields on the quantum gravitational states of ultra-cold neutrons (UCNs) in qBounce experiments with mirrors. We discuss the deformation of the neutron wave function due to chameleon interactions and quantum systems in potential wells from gravitational forces and chameleon fields. Unlike other works that aim to put bounds on the chameleon field parameters, this work focuses on the quantum mechanics of the chameleonic neutron. The results deepen our understanding of the interplay between quantum states and modified gravity, as well as fundamental physics experiments carried out in the laboratory. Full article
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23 pages, 4820 KiB  
Review
Review: Pipeline Layout Effect on the Wall Thinning of Mihama Nuclear Power Plants
by Nobuyuki Fujisawa
J. Nucl. Eng. 2025, 6(2), 19; https://doi.org/10.3390/jne6020019 - 18 Jun 2025
Viewed by 502
Abstract
The subject of the effect of pipeline layout on wall thinning in Mihama nuclear power plants was reviewed in relation to flow-accelerated corrosion (FAC). The pipeline consists of a complex layout with a straight pipe, elbow, curved pipe, orifice, and T-junction. To understand [...] Read more.
The subject of the effect of pipeline layout on wall thinning in Mihama nuclear power plants was reviewed in relation to flow-accelerated corrosion (FAC). The pipeline consists of a complex layout with a straight pipe, elbow, curved pipe, orifice, and T-junction. To understand the mechanism of wall thinning in the pipeline, the basics of FAC, experimental and numerical approaches, and flow and mass transfer studies of the pipeline were reviewed and compared with actual Mihama pipeline data. The results indicate that the wall thinning in the Mihama pipeline was caused by the asymmetric mass transfer phenomenon arising from the pipeline layout effect induced by the swirl flow, resulting in the generation of a spiral flow downstream of the elbow and an increased mass transfer coefficient downstream of the orifice. Swirl flow can be generated by the coupled T-junction and elbow in the upstream pipeline. Furthermore, related topics in flow and mass transfer studies on short elbows and dual and triple elbows were reviewed in relation to wall thinning, which could depend on the elbow curvature, Reynolds number, and surface roughness. The low-frequency flow oscillation in a short elbow, the swirl flow generation in dual and triple elbows, and the influence of wall roughness could be other sources of the increased mass transfer coefficient in the pipeline. Full article
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14 pages, 2534 KiB  
Article
Dynamic Probabilistic Risk Assessment of Passive Safety Systems for LOCA Analysis Using EMRALD
by Saikat Basak and Lixuan Lu
J. Nucl. Eng. 2025, 6(2), 18; https://doi.org/10.3390/jne6020018 - 13 Jun 2025
Viewed by 513
Abstract
This research explores Dynamic Probabilistic Risk Assessment (DPRA) using EMRALD to evaluate the reliability and safety of passive safety systems in nuclear reactors, with a focus on mitigating Loss of Coolant Accidents (LOCAs). The BWRX-300 Small Modular Reactor (SMR) is used as an [...] Read more.
This research explores Dynamic Probabilistic Risk Assessment (DPRA) using EMRALD to evaluate the reliability and safety of passive safety systems in nuclear reactors, with a focus on mitigating Loss of Coolant Accidents (LOCAs). The BWRX-300 Small Modular Reactor (SMR) is used as an example to illustrate the proposed DPRA methodology, which is broadly applicable for enhancing traditional Probabilistic Safety Assessment (PSA). Unlike static PSA, DPRA incorporates time-dependent interactions and system dynamics, allowing for a more realistic assessment of accident progression. EMRALD enables the modelling of system failures and interactions in real time using dynamic event trees and Monte Carlo simulations. This study identifies critical vulnerabilities in passive safety systems and quantifies the Core Damage Frequency (CDF) under LOCA scenarios. The findings demonstrate the advantages of DPRA over traditional PSA in capturing complex failure mechanisms and providing a more comprehensive and accurate risk assessment. The insights gained from this research contribute to improving passive safety system designs and enhancing nuclear reactor safety strategies for next-generation reactors. Full article
(This article belongs to the Special Issue Probabilistic Safety Assessment and Management of Nuclear Facilities)
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17 pages, 1481 KiB  
Article
Radiolysis of Sub- and Supercritical Water Induced by 10B(n,α)7Li Recoil Nuclei at 300–500 °C and 25 MPa
by Md Shakhawat Hossen Bhuiyan, Jintana Meesungnoen and Jean-Paul Jay-Gerin
J. Nucl. Eng. 2025, 6(2), 17; https://doi.org/10.3390/jne6020017 - 9 Jun 2025
Viewed by 492
Abstract
(1) Background: Generation IV supercritical water-cooled reactors (SCWRs), including small modular reactor (SCW-SMR) variants, are pivotal in nuclear technology. Operating at 300–500 °C and 25 MPa, these reactors require detailed understanding of radiation chemistry and transient species to optimize water chemistry, reduce corrosion, [...] Read more.
(1) Background: Generation IV supercritical water-cooled reactors (SCWRs), including small modular reactor (SCW-SMR) variants, are pivotal in nuclear technology. Operating at 300–500 °C and 25 MPa, these reactors require detailed understanding of radiation chemistry and transient species to optimize water chemistry, reduce corrosion, and enhance safety. Boron, widely used as a neutron absorber, plays a significant role in reactor performance and safety. This study focuses on the yields of radiolytic species in subcritical and supercritical water exposed to 4He and 7Li recoil ions from the 10B(n,α)7Li fission reaction in SCWR/SCW-SMR environments. (2) Methods: We use Monte Carlo track chemistry simulations to calculate yields (G values) of primary radicals (eaq, H, and OH) and molecular species (H2 and H2O2) from water radiolysis by α-particles and Li3⁺ recoils across 1 picosecond to 0.1 millisecond timescales. (3) Results: Simulations show substantially lower radical yields, notably eaq and OH, alongside higher molecular product yields compared to low linear energy transfer (LET) radiation, underscoring the high-LET nature of 10B(n,α)7Li recoil nuclei. Key changes include elevated G(OH) and G(H2), and a decrease in G(H), primarily driven during the homogeneous chemical stage of radiolysis by the reaction H + H2O → OH + H2. This reaction significantly contributes to H2 production, potentially reducing the need for added hydrogen in coolant water to mitigate oxidizing species. In supercritical conditions, low G(H₂O₂) suggests that H2O2 is unlikely to be a major contributor to material oxidation. (4) Conclusions: The 10B(n,α)7Li reaction’s yield estimates could significantly impact coolant chemistry strategies in SCWRs and SCW-SMRs. Understanding radiolytic behavior in these conditions aids in refining reactor models and coolant chemistry to minimize corrosion and radiolytic damage. Future experiments are needed to validate these predictions. Full article
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12 pages, 2302 KiB  
Article
Radiological Assessment of Building Materials Containing Processed Bauxite
by Uku Andreas Reigo, Cansu Özcan Kılcan and Alan H. Tkaczyk
J. Nucl. Eng. 2025, 6(2), 16; https://doi.org/10.3390/jne6020016 - 17 May 2025
Viewed by 493
Abstract
Supplementary cementitious materials (SCMs) may be prepared using industrial byproduct streams, aiding in the development of a more environmentally sustainable circular economy. However, these byproducts may carry a risk of exhibiting elevated levels of radioactivity because of the preceding processing that may have [...] Read more.
Supplementary cementitious materials (SCMs) may be prepared using industrial byproduct streams, aiding in the development of a more environmentally sustainable circular economy. However, these byproducts may carry a risk of exhibiting elevated levels of radioactivity because of the preceding processing that may have concentrated the radionuclides naturally occurring in the raw material. This processing causes the byproducts to be considered technologically enhanced naturally occurring radioactive material (NORM). Thus, the safe use of such SCMs requires robust data on the activity concentrations of three main radionuclides (226Ra, 232Th, 40K) represented by the activity concentration index (ACI) used as a radiological suitability indicator. In this work, candidate SCMs derived from the alumina industry byproduct processed bauxite (PB), also referred to as bauxite residue, were assessed by measuring the activity of all available samples, including input raw materials and intermediate substances, through gamma spectrometry. PB was found to significantly impact the final ACI value of the building material. As a key analysis outcome applicable to the substances assessed in this work, no additional dose assessment is required, given the low ACI value of the building materials. This result indicates that, from a radiological perspective, the PB samples studied are suitable precursors for SCMs. In addition, a generalized approach was found to provide good estimations of the ACI value of building materials, which is useful to screen materials for regulatory compliance, without needing to prepare samples of the materials in question. Full article
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13 pages, 4280 KiB  
Article
Performance Characteristics of the Battery-Operated Silicon PIN Diode Detector with an Integrated Preamplifier and Data Acquisition Module for Fusion Particle Detection
by Allan Xi Chen, Benjamin F. Sigal, John Martinis, Alfred YiuFai Wong, Alexander Gunn, Matthew Salazar, Nawar Abdalla and Kai-Jian Xiao
J. Nucl. Eng. 2025, 6(2), 15; https://doi.org/10.3390/jne6020015 - 15 May 2025
Viewed by 687
Abstract
We present the performance and application of a commercial off-the-shelf Si PIN diode (Hamamatsu S14605) as a charged particle detector in a compact ion beam system (IBS) capable of generating D–D and p–B fusion charged particles. This detector is inexpensive, widely available, and [...] Read more.
We present the performance and application of a commercial off-the-shelf Si PIN diode (Hamamatsu S14605) as a charged particle detector in a compact ion beam system (IBS) capable of generating D–D and p–B fusion charged particles. This detector is inexpensive, widely available, and operates in photoconductive mode under a reverse bias voltage of 12 V, supplied by an A23 battery. A charge-sensitive preamplifier (CSP) is mounted on the backside of the detector’s four-layer PCB and powered by two ±3 V lithium batteries (A123). Both the detector and CSP are housed together on the vacuum side of the IBS, facing the fusion target. The system employs a CF-2.75-flanged DB-9 connector feedthrough to supply the signal, bias voltage, and rail voltages. To mitigate the high sensitivity of the detector to optical light, a thin aluminum foil assembly is used to block optical emissions from the ion beam and target. Charged particles generate step responses at the preamplifier output, with pulse rise times in the order of 0.2 to 0.3 µs. These signals are recorded using a custom-built data acquisition unit, which features an optical fiber data link to ensure the electrical isolation of the detector electronics. Subsequent digital signal processing is employed to optimally shape the pulses using a CR-RCn filter to produce Gaussian-shaped signals, enabling the accurate extraction of energy information. Performance results indicate that the detector’s baseline RMS ripple noise can be as low as 0.24 mV. Under actual laboratory conditions, the estimated signal-to-noise ratios (S/N) for charged particles from D–D fusion—protons, tritons, and helions—are approximately 225, 75, and 41, respectively. Full article
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