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State-of-the-Art Conductive Hydrogels

A special issue of Polymers (ISSN 2073-4360). This special issue belongs to the section "Polymer Networks and Gels".

Deadline for manuscript submissions: 30 September 2025 | Viewed by 537

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School of Materials Science and Engineering, Hainan University, Haikou 570228, China
Interests: DNA biosensor; nucleic acid; polymer gel electrolyte; wearable/implantable flexible devices
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Dear Colleagues,

Conductive hydrogels, a unique class of materials merging the properties of hydrogels and electrical conductivity, have emerged as a focal point of intense scientific and technological exploration. These hydrogels, characterized by their three-dimensional network structure capable of retaining large amounts of water, have the remarkable ability to conduct electrical signals, which sets them apart from traditional hydrogels.

In recent years, significant progress has been made in the development of conductive hydrogels. Novel synthesis routes have been devised, enabling the precise control of their microstructure and composition. This has led to the creation of hydrogels with enhanced conductivity, mechanical strength, and biocompatibility. For example, the incorporation of conductive nanomaterials such as carbon nanotubes, graphene, and conductive polymers into the hydrogel matrix has been a prevalent strategy to boost their electrical performance.

The application potential of conductive hydrogels spans across multiple disciplines. In the biomedical field, they are being explored for use in biosensors, where they can detect various biological analytes with high sensitivity and selectivity. They also hold great promise for tissue engineering, as they can mimic the extracellular matrix environment and provide electrical stimulation to promote cell growth and tissue regeneration. In addition, in the realm of soft robotics, conductive hydrogels can act as actuators, responding to electrical signals with mechanical deformations, enabling the development of more flexible and adaptable robotic systems.

The continuous pursuit of better performing conductive hydrogels is driven by the need to overcome the limitations of existing materials and technologies. Conventional materials often struggle to combine the desired mechanical flexibility, high water content, and efficient electrical conductivity. There is a pressing demand for practical, reliable, and multifunctional conductive hydrogels that can meet the requirements of diverse applications.

For this Special Issue, we invite you to contribute original research or comprehensive review articles. We encourage submissions that offer novel insights into the design, synthesis, and characterization of conductive hydrogels. Articles demonstrating their innovative applications in emerging fields such as wearable electronics, environmental sensing, and energy storage are also highly welcome.

We aim to showcase a rich tapestry of research efforts from around the world. By presenting a wide range of strategies and findings, we hope to provide readers with a profound understanding of the cutting-edge developments in the field of conductive hydrogels. This will not only highlight the remarkable achievements but also help in identifying the remaining challenges and limitations that need to be addressed.

We eagerly anticipate your valuable contributions, which will undoubtedly enrich this Special Issue and further inspire advancements in the exciting domain of conductive hydrogels.

Prof. Dr. Jie Du
Guest Editor

Manuscript Submission Information

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Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2700 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • conductive hydrogels
  • synthesis routes
  • microstructure control
  • conductive nanomaterials
  • biomedical applications
  • biosensors
  • tissue engineering
  • soft robotics
  • wearable electronics
  • environmental sensing

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Published Papers (1 paper)

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Review

33 pages, 4921 KiB  
Review
Recent Progress in Cellulose-Based Conductive Hydrogels
by Zhenrui Du, Na Wang and Jie Du
Polymers 2025, 17(8), 1089; https://doi.org/10.3390/polym17081089 - 17 Apr 2025
Viewed by 429
Abstract
Cellulose, a widely abundant natural polymer, is well recognized for its remarkable properties, such as biocompatibility, degradability, and mechanical strength. Conductive hydrogels, with their unique ability to conduct electricity, have attracted significant attention in various fields. The combination of cellulose and conductive hydrogels [...] Read more.
Cellulose, a widely abundant natural polymer, is well recognized for its remarkable properties, such as biocompatibility, degradability, and mechanical strength. Conductive hydrogels, with their unique ability to conduct electricity, have attracted significant attention in various fields. The combination of cellulose and conductive hydrogels has led to the emergence of cellulose-based conductive hydrogels, which show great potential in flexible electronics, biomedicine, and energy storage. This review article comprehensively presents the latest progress in cellulose-based conductive hydrogels. Firstly, it provides an in-depth overview of cellulose, covering aspects like its structure, diverse sources, and classification. This emphasizes cellulose’s role as a renewable and versatile material. The development and applications of different forms of cellulose, including delignified wood, bacterial cellulose, nanocellulose, and modified cellulose, are elaborated. Subsequently, cellulose-based hydrogels are introduced, with a focus on their network structures, such as single-network, interpenetrating network, and semi-interpenetrating network. The construction of cellulose-based conductive hydrogels is then discussed in detail. This includes their conductive forms, which are classified into electronic and ionic conductive hydrogels, and key performance requirements, such as cost-effectiveness, mechanical property regulation, sensitive response to environmental stimuli, self-healing ability, stable conductivity, and multifunctionality. The applications of cellulose-based conductive hydrogels in multiple areas are also presented. In wearable sensors, they can effectively monitor human physiological signals in real time. In intelligent biomedicine, they contribute to wound healing, tissue engineering, and nerve regeneration. In flexible supercapacitors, they offer potential for green and sustainable energy storage. In gel electrolytes for conventional batteries, they help address critical issues like lithium dendrite growth. Despite the significant progress, there are still challenges to overcome. These include enhancing the multifunctionality and intelligence of cellulose-based conductive hydrogels, strengthening their connection with artificial intelligence, and achieving simple, green, and intelligent large-scale industrial production. Future research directions should center around exploring new synthesis methods, optimizing material properties, and expanding applications in emerging fields, aiming to promote the widespread commercialization of these materials. Full article
(This article belongs to the Special Issue State-of-the-Art Conductive Hydrogels)
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