Search Results (610)

In the context of an ultrafast laser interacting with solids, temperature plays a special role in the transformation processes. Some of these processes can be thermally activated, while others can be either solely driven or constrained by temperature—such as refractive index change (fictive temperature), nanopore erasure, micro-bubble formation, and phase transition-like crystallization. The objective of this paper is to use a recently developed analytic approximation to understand the limitations imposed by the spatial temperature distribution and its evolution over the writing time, based on the key laser parameter combinations, and subsequently determine the boundary conditions of these parameters. Full article

Ultrafast lasers operating at 740 nm and 820 nm have attracted widespread attention as two-photon light sources for the detection of biological metabolism. Here, we report on a solid-like quartz-encapsulated femtosecond laser with a repetition rate of 80 MHz, delivering 740 nm and 820 nm femtosecond laser pulses. This home-built laser system was realized by employing an erbium-doped 1560 nm fiber laser as the fundamental laser source. A quartz-encapsulated nonlinear frequency conversion stage, consisting of a second-harmonic generation (SHG) stage and self-phase modulation (SPM)-based nonlinear spectral broadening stage, was utilized to deliver 30 mW, 53.7 fs, 740 nm laser pulses and the 15 mW, 60.8 fs, 820 nm laser pulses. Further imaging capabilities of both wavelengths were validated using a custom-built inverted two-photon microscope. Clear imaging results were obtained from mouse kidney sections and pollen samples by collecting the corresponding fluorescence signals. The achieved results demonstrate the great potential of this laser source for advanced two-photon microscopy in metabolic detection. Full article

Whispering-gallery-mode (WGM) microresonators are amongst the most promising optical sensors for detecting bio-chemical targets. A number of laser interrogation methods have been proposed and demonstrated over the last decade, based on scattering and absorption losses or resonance splitting and shift, harnessing the high-quality factor and ultra-small volume of WGMs. Actually, regardless of the sensitivity enhancement, their practical sensing operation may be hampered by the complexity of coupling devices as well as the signalprocessing required to extract the WGM response. Here, we use a silica microsphere immersed in an aqueous environment and efficiently excite optical WGMs with a free-space visible laser, thus collecting the relevant information from the transmitted and back-scattered light without any optical coupler, fiber, or waveguide. We show that a 640-nm diode laser, actively frequency-locked on resonance, provides real-time, fast sensing of dielectric nanoparticles approaching the surface with direct analog readout. Thanks to our illumination scheme, the sensor can be kept in water and operate for days without degradation or loss of sensitivity. Diverse noise contributions are carefully considered and quantified in our system, showing a minimum detectable particle size below 1 nm essentially limited by the residual laser microcavity jitter. Further analysis reveals that the inherent laserfrequency instability in the short, -mid-term operation regime sets an ultimate bound of 0.3 nm. Based on this work, we envisage the possibility to extend our method in view of developing new viable approaches for detection of nanoplastics in natural water without resorting to complex chemical laboratory methods. Full article

Ultrafast laser welding of glass/metal heterostructures has found extensive applications in sensors, medical devices, and optical systems. However, achieving high-stability, high-quality welds under non-optical contact conditions remains challenging due to severe internal damage within glass materials. This study addresses thermal management through synergistic control of thermal accumulation effects and material ablation thresholds. Using the sapphire/Invar alloy system as a model for glass/metal welding, we investigated thermal accumulation effects during ultrafast laser ablation of Invar alloy through theoretical simulations. Under a repetition rate of 1 MHz, the femtosecond laser raised the lattice equilibrium temperature by 700 K within 10 microseconds, demonstrating that high repetition rate femtosecond lasers can induce effective heat accumulation in Invar alloy. Furthermore, ablation thresholds for both materials were determined across varying repetition rates via the D² method, with corresponding threshold curves systematically constructed. Finally, based on the simulation and ablation threshold calculation results, laser parameters were selected for ultrafast laser single point welding of sapphire and Invar alloy. The experimental results demonstrate effective thermal effect mitigation, achieving a maximum shear strength of 63.37 MPa. Comparative analysis against traditional scan welding further validates the superiority of our approach in thermal management. This work provides foundational theoretical and methodological guidance for ultrafast laser welding of glass/metal heterostructures. Full article

In recent years, the generation of circularly polarized attosecond pulses has garnered significant attention due to their potential applications in ultrafast spectroscopy and, notably, in chiral-sensitive molecular detection. The traditional methods for generating such pulses often involve complex laser configurations or specially engineered targets, limiting their experimental feasibility. In this study, we present a streamlined and effective approach to producing circularly polarized attosecond pulses by employing a linearly polarized laser field in conjunction with a stereosymmetric linear molecule, 1-butyne (C₄H₆). The generation of high-order harmonics by this molecular system reveals a distinct plateau in the perpendicular polarization component, which facilitates the generation of isolated attosecond pulses with circular polarization. Through a detailed analysis of the time-dependent charge density dynamics across atomic sites, we identify the atoms primarily responsible for the emission of circularly polarized harmonics in the plane orthogonal to the driving field. Moreover, we explore the role of multi-orbital contributions in shaping the polarization properties of the harmonic spectra. Our findings underscore the importance of molecular symmetry and the electronic structure in tailoring the harmonic polarization, and they demonstrate a viable pathway for using circularly polarized attosecond pulses to probe molecular chirality. This method offers a balance between simplicity and performance, opening new avenues for practical applications in chiral recognition and ultrafast stereochemical analysis. Full article

A spectral filter utilizing dispersive prisms and an optical fiber collimator is presented as an attractive alternative to diffraction grating-based spectral filters. A simplified analytical expression for this prism-based spectral filter is derived. A spectral filter constructed using SF11 flint glass prisms demonstrates Gaussian spectral filter profiles with bandwidths of 8 nm and 4 nm, closely matching with theoretical predictions. Using these filters, we demonstrate two types of mode-locking regimes: a dissipative soliton (DS) pulse and a self-similar (SS) pulse. The dissipative soliton pulses deliver 3.3 nJ with dechirped pulse durations of 206 fs, while the self-similar pulses deliver 2.1 nJ with durations of 120 fs. The results demonstrate that the prism-based filters are well-suited for ultrafast mode-locked fiber lasers. Full article

We report on the welding of optical borosilicate glass to an unpolished copper substrate (surface Ra of 0.27 µm and Rz of 1.89 µm) using bursts of femtosecond laser pulses. The present paper puts forth the hypothesis that glass–metal welding with a gap is contingent upon the ejection of molten jets of glass. We have ascertained the impact of pulse energy and focal position on weldability. This finding serves to substantiate our initial hypothesis and provides a framework for understanding the conditions under which this hypothesis is applicable. Under optimal conditions, but without the assistance of any clamping system, our welded samples maintained a breaking resistance of up to 10.9 MPa. Full article

Stress fields imparted with an ultrafast laser can correct low spatial frequency surface figure error of mirrors through ultrafast laser stress figuring (ULSF): the formation of nanograting structures within the bulk substrate generates localized stress, creating bending moments that equilibrize via wafer deformation. For ULSF to be used as an optical figuring process, the ultrafast laser generated stress must be effectively permanent or risk unwanted figure drift. Two isochronal annealing experiments were performed to measure ultrafast laser-generated stress stability in fused silica and Corning ultra-low expansion (ULE) wafers. The first experiment tracked changes to induced astigmatism up to 1000 °C on 25.4 mm-diameter wafers. Only small changes were measured after each thermal cycle up to 500 °C for both materials, but significant changes were observed at higher temperatures. The second experiment tracked stress changes in fused silica and ULE up to 500 °C but with 4 to 16× higher signal-to-noise ratio. Change in trefoil on 100 mm-diameter wafers was measured, and the induced stress in fused silica and ULE was found to be stable after thermal cycling up to 300 °C and 200 °C, respectively, with larger changes at higher temperatures. Full article

Glass enjoys a wide range of applications thanks to its superior optical properties and chemical stability. Conventional glass bonding techniques suffer from low efficiency, limited precision, and high cost. Moreover, for multilayer glass bonding, repeated alignment is often required, further complicating the process. These limitations have become major constraints on the advancement of microfluidic chip technologies. Laser bonding of microfluidic chips offers high precision and efficiency. This research first uses an ultrafast laser system to investigate how processing parameters affect weld morphology, identifying the optimal parameter range. Then, this paper proposes two methods for ultrafast-laser bonding of multilayer glass with different thicknesses and performs preliminary experiments to demonstrate their feasibility. The research in this paper could expand the fabrication method of microfluidic chips and lay a foundation for the wider application of microfluidic chips. Full article

In this paper, we develop a peridynamic computational framework to analyze thermomechanical interactions in fractured thin films subjected to ultrashort-pulsed laser excitation, employing nonlocal discrete material point discretization to eliminate mesh dependency artifacts. The generalized Cattaneo–Fourier thermal flux formulation uncovers contrasting dynamic responses: hyperbolic heat propagation ($F_T=0$) generates intensified temperature localization and elevates transient crack-tip stress concentrations relative to classical Fourier diffusion ($F_T=1$). A GSSSS (Generalized Single Step Single Solve) i-Integration temporal scheme achieves oscillation-free numerical solutions across picosecond-level laser–matter interactions, effectively resolving steep thermal fronts through adaptive stabilization. These findings underscore hyperbolic conduction’s essential influence on stress-mediated fracture evolution during ultrafast laser processing, providing critical guidelines for thermal management in micro-/nano-electromechanical systems. Full article

Chemically strengthened glass is widely used for its remarkable fracture strength, mechanical performance, and scratch resistance. Assessing its hardness is crucial to evaluating improvements from chemical tempering. However, conventional methods like Vickers hardness tests are destructive, altering the sample surface. This study presents a novel, rapid, and nondestructive testing (NDT) approach by correlating the nonlinear refractive index (n₂) with surface hardness. Using ultrafast laser pulses, we measured the n₂ cross-section via the nonlinear ellipse rotation (NER) signal in Gorilla^®-type glass subjected to ion exchange (Na⁺ by K⁺). A microscope objective lens provided a penetration resolution of ≈5.5 μm, enabling a localized NER signal analysis. We demonstrate a correlation between the NER signal and hardness, offering a promising pathway for advanced, noninvasive characterization. This approach provides a reliable alternative to traditional destructive techniques, with potential applications in industrial quality control and material science research. Full article

Optically pumped semiconductor disk lasers—known as vertical-external-cavity surface-emitting lasers (VECSELs)—are promising devices for ultrashort pulse formation. For it, a “SESAM-free” approach labeled “self-mode-locking” received considerable attention in the past decade, relying solely on a chip-related nonlinear optical property which can establish adequate pulsing conditions—thereby suggesting a reduced reliance on a semiconductor saturable-absorber mirror (the SESAM) in the cavity. Self-mode-locked (SML) VECSELs with sub-ps pulse durations were reported repeatedly. This motivated investigations on a Kerr-lensing type effect acting as an artificial saturable absorber. So-called Z-scan and ultrafast beam-deflection experiments were conducted to emphasize the role of nonlinear lensing in the chip for pulse formation. Recently, in addition to allowing stable ultrashort pulsed operation, self-starting mode-locked operation gave rise to another emission regime related to frequency comb formation. While amplitude-modulated combs relate to signal peaks in time, providing a so-called pulse train, a frequency-modulated comb is understood to cause quasi continuous-wave output with its sweep of instantaneous frequency over the range of phase-locked modes. With gain-bandwidth-enhanced chips, as well as with an improved understanding of the impacts of dispersion and nonlinear lensing properties and cavity configurations on the device output, an enhanced employment of SML VECSELs is to be expected. Full article

We demonstrate a novel bidirectional mode-locked ultrafast fiber laser based on an asymmetric dual-cavity architecture that enables freely tunable repetition rate differentials at the kilohertz level, while maintaining inherent common-mode noise suppression through precision thermomechanical stabilization. Through cascaded amplification and nonlinear temporal compression, we obtained bidirectional pulse durations of 33.2 fs (clockwise) and 61.6 fs (counterclockwise), respectively. The developed source demonstrates exceptional capability for asynchronous optical sampling applications, particularly in enabling the compact implementation of real-time measurement systems such as terahertz time-domain spectroscopy (THz-TDS) systems. Full article

Laser-induced periodic surface structures (LIPSSs) produced via ultrafast laser-induced oxidation offer a promising route for high-quality nanostructuring, with reduced thermal damage compared to conventional ablation-based methods. However, the influence of laser repetition frequency on the formation and morphology of oxidized LIPSSs remains insufficiently explored. In this study, we systematically investigate the effects of varying the femtosecond laser repetition frequency from 1 kHz to 100 kHz while keeping the total pulse number constant on the oxidation-induced LIPSSs formed on amorphous silicon films. Scanning electron microscopy and Fourier analysis reveal a transition between two morphological regimes with increasing repetition frequency: at low frequencies, the long inter-pulse intervals result in irregular, disordered oxidation patterns; at high frequencies, closely spaced pulses promote the formation of highly ordered, periodic surface structures. Statistical measurements show that the laser-modified area decreases with frequency, while the LIPSS period remains relatively stable and the ridge width exhibits a peak at 10 kHz. Finite-difference time-domain (FDTD) and finite-element simulations suggest that the observed patterns result from a dynamic balance between light-field modulation and oxidation kinetics, rather than thermal accumulation. These findings advance the understanding of oxidation-driven LIPSS formation dynamics and provide guidance for optimizing femtosecond laser parameters for precise surface nanopatterning. Full article

In recent years, ultrafast bursts with high power have been applied in many significant fields. However, the peak power of the pulse train generated by fiber lasers is limited by fiber characteristics from nonlinear effects, which can only be at the level of milliwatt. In this research, the pulse frequency is reduced by an AOM pulse picker-integrated modulator. With M2 and pulse width guaranteed, the frequency of the reduced pulse train is amplified by a solid-state three-stage Nd:YVO₄ amplifier system. Finally, the peak power of the pulse train is increased. The final output pulse repetition rate of the experiment is 1 MHz with a pulse width of 8.09 picoseconds and a peak power of up to 3.7 MW. Full article