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Authors = Gérard Mourou

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13 pages, 8268 KB  
Article
Ultrafast Laser-Excited Optical Emission of Xe under Loose-Focusing Conditions
by Miloš Burger, Kyle S. Latty, Leandro Frigerio, Thiago Arnaud, Kyle C. Hartig and Igor Jovanovic
Sensors 2023, 23(23), 9374; https://doi.org/10.3390/s23239374 - 23 Nov 2023
Viewed by 2434
Abstract
The optical filament-based radioxenon sensing can potentially overcome the constraints of conventional detection techniques that are relevant for nuclear security applications. This study investigates the spectral signatures of pure xenon (Xe) when excited by ultrafast laser filaments at near-atmosphericpressure and in short and [...] Read more.
The optical filament-based radioxenon sensing can potentially overcome the constraints of conventional detection techniques that are relevant for nuclear security applications. This study investigates the spectral signatures of pure xenon (Xe) when excited by ultrafast laser filaments at near-atmosphericpressure and in short and loose-focusing conditions. The two focusing conditions lead to laser intensity differences of several orders of magnitude and different plasma transient behavior. The gaseous sample was excited at atmospheric pressure using ∼7 mJ pulses with a 35 fs pulse duration at 800 nm wavelength. The optical signatures were studied by time-resolved spectrometry and imaging in orthogonal light collection configurations in the ∼400 nm (VIS) and ∼800 nm (NIR) spectral regions. The most prominent spectral lines of atomic Xe are observable in both focusing conditions. An on-axis light collection from an atmospheric air–Xe plasma mixture demonstrates the potential of femtosecond filamentation for the remote sensing of noble gases. Full article
(This article belongs to the Special Issue Optical Spectroscopy for Sensing, Monitoring and Analysis)
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16 pages, 1658 KB  
Article
Impact of Glass Irradiation on Laser-Induced Breakdown Spectroscopy Data Analysis
by Londrea J. Garrett, Bryan W. Morgan, Miloš Burger, Yunu Lee, Hyeongbin Kim, Piyush Sabharwall, Sungyeol Choi and Igor Jovanovic
Sensors 2023, 23(2), 691; https://doi.org/10.3390/s23020691 - 7 Jan 2023
Cited by 8 | Viewed by 3471
Abstract
Increased absorption of optical materials arising from exposure to ionizing radiation must be accounted for to accurately analyze laser-induced breakdown spectroscopy (LIBS) data retrieved from high-radiation environments. We evaluate this effect on two examples that mimic the diagnostics placed within novel nuclear reactor [...] Read more.
Increased absorption of optical materials arising from exposure to ionizing radiation must be accounted for to accurately analyze laser-induced breakdown spectroscopy (LIBS) data retrieved from high-radiation environments. We evaluate this effect on two examples that mimic the diagnostics placed within novel nuclear reactor designs. The analysis is performed on LIBS data measured with 1% Xe gas in an ambient He environment and 1% Eu in a molten LiCl-KCl matrix, along with the measured optical absorption from the gamma- and neutron-irradiated low-OH fused silica and sapphire glasses. Significant changes in the number of laser shots required to reach a 3σ detection level are observed for the Eu data, increasing by two orders of magnitude after exposure to a 1.7 × 1017 n/cm2 neutron fluence. For all cases examined, the spectral dependence of absorption results in the introduction of systematic errors. Moreover, if lines from different spectral regions are used to create Boltzmann plots, this attenuation leads to statistically significant changes in the temperatures calculated from the Xe II lines and Eu II lines, lowering them from 8000 ± 610 K to 6900 ± 810 K and from 15,800 ± 400 K to 7200 ± 800 K, respectively, for exposure to the 1.7 × 1017 n/cm2 fluence. The temperature range required for a 95% confidence interval for the calculated temperature is also broadened. In the case of measuring the Xe spectrum, these effects may be mitigated using only the longer-wavelength spectral region, where radiation attenuation is relatively small, or through analysis using the iterative Saha–Boltzmann method. Full article
(This article belongs to the Special Issue Recent Trends and Advances in Laser Spectroscopy and Sensing)
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29 pages, 9649 KB  
Article
AnaBHEL (Analog Black Hole Evaporation via Lasers) Experiment: Concept, Design, and Status
by Pisin Chen, Gerard Mourou, Marc Besancon, Yuji Fukuda, Jean-Francois Glicenstein, Jiwoo Nam, Ching-En Lin, Kuan-Nan Lin, Shu-Xiao Liu, Yung-Kun Liu, Masaki Kando, Kotaro Kondo, Stathes Paganis, Alexander Pirozhkov, Hideaki Takabe, Boris Tuchming, Wei-Po Wang, Naoki Watamura, Jonathan Wheeler and Hsin-Yeh Wu
Photonics 2022, 9(12), 1003; https://doi.org/10.3390/photonics9121003 - 19 Dec 2022
Cited by 20 | Viewed by 7372
Abstract
Accelerating relativistic mirrors have long been recognized as viable settings where the physics mimic those of the black hole Hawking radiation. In 2017, Chen and Mourou proposed a novel method to realize such a system by traversing an ultra-intense laser through a plasma [...] Read more.
Accelerating relativistic mirrors have long been recognized as viable settings where the physics mimic those of the black hole Hawking radiation. In 2017, Chen and Mourou proposed a novel method to realize such a system by traversing an ultra-intense laser through a plasma target with a decreasing density. An international AnaBHEL (Analog Black Hole Evaporation via Lasers) collaboration was formed with the objectives of observing the analog Hawking radiation, shedding light on the information loss paradox. To reach these goals, we plan to first verify the dynamics of the flying plasma mirror and characterize the correspondence between the plasma density gradient and the trajectory of the accelerating plasma mirror. We will then attempt to detect the analog Hawking radiation photons and measure the entanglement between the Hawking photons and their “partner particles”. In this paper, we describe our vision and strategy of AnaBHEL using the Apollon laser as a reference, and we report on the progress of our R&D concerning the key components in this experiment, including the supersonic gas jet with a graded density profile, and the superconducting nanowire single-photon Hawking detector. In parallel to these hardware efforts, we performed computer simulations to estimate the potential backgrounds, and derived analytic expressions for modifications to the blackbody spectrum of the Hawking radiation for a perfectly reflecting point mirror, due to the semi-transparency and finite-size effects specific to flying plasma mirrors. Based on this more realistic radiation spectrum, we estimate the Hawking photon yield to guide the design of the AnaBHEL experiment, which appears to be achievable. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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14 pages, 3376 KB  
Article
Laser Wakefield Photoneutron Generation with Few-Cycle High-Repetition-Rate Laser Systems
by Daniel Papp, Ales Necas, Nasr Hafz, Toshiki Tajima, Sydney Gales, Gerard Mourou, Gabor Szabo and Christos Kamperidis
Photonics 2022, 9(11), 826; https://doi.org/10.3390/photonics9110826 - 3 Nov 2022
Cited by 11 | Viewed by 4994
Abstract
Simulations of photoneutron generation are presented for the anticipated experimental campaign at ELI-ALPS using the under-commissioning e-SYLOS beamline. Photoneutron generation is a three-step process starting with the creation of a relativistic electron beam which is converted to gamma radiation, which in turn generates [...] Read more.
Simulations of photoneutron generation are presented for the anticipated experimental campaign at ELI-ALPS using the under-commissioning e-SYLOS beamline. Photoneutron generation is a three-step process starting with the creation of a relativistic electron beam which is converted to gamma radiation, which in turn generates neutrons via the γ,n interaction in high-Z material. Electrons are accelerated to relativistic energies using the laser wakefield acceleration (LWFA) mechanism. The LWFA process is simulated with a three-dimensional particle in cell code to generate an electron bunch of 100s pC charge from a 100 mJ, 9 fs laser interaction with a helium gas jet target. The resultant electron spectrum is transported through a lead sphere with the Monte Carlo N-Particle (MCNP) code to convert electrons to gammas and gammas to neutrons in a single simulation. A neutron yield of 3×107 per shot over 4π is achieved, with a corresponding neutron yield per kW of 6×1011 n/s/kW. The paper concludes with a discussion on the attractiveness of LWFA-driven photoneutron generation on high impact, and societal applications. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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12 pages, 4014 KB  
Article
Compressing High Energy Lasers through Optical Polymer Films
by Jonathan Wheeler, Gabriel Petrişor Bleotu, Andrei Naziru, Riccardo Fabbri, Masruri Masruri, Radu Secareanu, Deano M. Farinella, Gabriel Cojocaru, Razvan Ungureanu, Elsa Baynard, Julien Demailly, Moana Pittman, Razvan Dabu, Ioan Dancus, Daniel Ursescu, David Ros, Toshiki Tajima and Gerard Mourou
Photonics 2022, 9(10), 715; https://doi.org/10.3390/photonics9100715 - 30 Sep 2022
Cited by 10 | Viewed by 4062
Abstract
The thin-film post-compression technique has the ability to reduce the pulse duration in PW-class lasers, increasing the peak power. Here, the nonlinear response of an increasingly available optical thermoplastic demonstrates enhanced spectral broadening, with corresponding shorter pulse duration compared to fused silica glass. [...] Read more.
The thin-film post-compression technique has the ability to reduce the pulse duration in PW-class lasers, increasing the peak power. Here, the nonlinear response of an increasingly available optical thermoplastic demonstrates enhanced spectral broadening, with corresponding shorter pulse duration compared to fused silica glass. The thermoplastic can be used close to its damage threshold when refreshed using a roller mechanism, and the total amount of material can be varied by folding the film. As a proof-of-principle demonstration scalable to 10-PW, a roller mechanism capable of up to 6 passes through a sub-millimeter thermoplastic film is used in vacuum to produce two-fold post-compression of the pulse. The compact design makes it an ideal method to further boost ultrahigh laser pulse intensities with benefits to many areas, including driving high energy acceleration. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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12 pages, 4235 KB  
Article
Laser Ion Acceleration in a Near Critical Density Trap
by Ales Necas, Toshiki Tajima, Gerard Mourou and Karoly Osvay
Photonics 2022, 9(7), 453; https://doi.org/10.3390/photonics9070453 - 28 Jun 2022
Cited by 3 | Viewed by 3707
Abstract
In order to accelerate ions by a laser, we go back to the original and the fundamental idea of how longitudinal field structure generation can be carried out in an ionized media and how particles may be trapped by the created wakefield. The [...] Read more.
In order to accelerate ions by a laser, we go back to the original and the fundamental idea of how longitudinal field structure generation can be carried out in an ionized media and how particles may be trapped by the created wakefield. The latter condition is characterized by the phase velocity of the longitudinal structure vph be equal to the particle trapping width vtr. Since the trapping width is inversely proportional to the square-root of the mass of the accelerated particles, this width is much shorter for ions than for electrons. Thus, our dictum for laser ion acceleration is to impose a near critical density trap to decelerate laser group velocity, vg and subsequently to generate longitudinal wakefield to be able to trap ions under the condition of vtr = vph. We demonstrate this concept by PIC simulation and find that this method is effective, and the efficiency of laser ion acceleration is enhanced by a couple of orders of magnitude toward unity. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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14 pages, 1924 KB  
Review
Ultrafast Fiber Technologies for Compact Laser Wake Field in Medical Application
by Weijian Sha, Jean-Christophe Chanteloup and Gérard Mourou
Photonics 2022, 9(6), 423; https://doi.org/10.3390/photonics9060423 - 16 Jun 2022
Cited by 14 | Viewed by 5485
Abstract
Technologies, performances and maturity of ultrafast fiber lasers and fiber delivery of ultrafast pulses are discussed for the medical deployment of laser-wake-field acceleration (LWFA). The compact ultrafast fiber lasers produce intense laser pulses with flexible hollow-core fiber delivery to facilitate electron acceleration in [...] Read more.
Technologies, performances and maturity of ultrafast fiber lasers and fiber delivery of ultrafast pulses are discussed for the medical deployment of laser-wake-field acceleration (LWFA). The compact ultrafast fiber lasers produce intense laser pulses with flexible hollow-core fiber delivery to facilitate electron acceleration in the laser-stimulated wake field near treatment site, empowering endoscopic LWFA brachytherapy. With coherent beam combination of multiple fiber amplifiers, the advantages of ultrafast fiber lasers are further extended to bring in more capabilities in compact LWFA applications. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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10 pages, 1446 KB  
Perspective
Fiber-Optic Based Laser Wakefield Accelerated Electron Beams and Potential Applications in Radiotherapy Cancer Treatments
by Dante Roa, Jeffrey Kuo, Harry Moyses, Peter Taborek, Toshiki Tajima, Gerard Mourou and Fuyuhiko Tamanoi
Photonics 2022, 9(6), 403; https://doi.org/10.3390/photonics9060403 - 8 Jun 2022
Cited by 12 | Viewed by 5761
Abstract
Ultra-compact electron beam technology based on laser wakefield acceleration (LWFA) could have a significant impact on radiotherapy treatments. Recent developments in LWFA high-density regime (HD-LWFA) and low-intensity fiber optically transmitted laser beams could allow for cancer treatments with electron beams from a miniature [...] Read more.
Ultra-compact electron beam technology based on laser wakefield acceleration (LWFA) could have a significant impact on radiotherapy treatments. Recent developments in LWFA high-density regime (HD-LWFA) and low-intensity fiber optically transmitted laser beams could allow for cancer treatments with electron beams from a miniature electronic source. Moreover, an electron beam emitted from a tip of a fiber optic channel could lead to new endoscopy-based radiotherapy, which is not currently available. Low-energy (10 keV–1 MeV) LWFA electron beams can be produced by irradiating high-density nano-materials with a low-intensity laser in the range of ~1014 W/cm2. This energy range could be useful in radiotherapy and, specifically, brachytherapy for treating superficial, interstitial, intravascular, and intracavitary tumors. Furthermore, it could unveil the next generation of high-dose-rate brachytherapy systems that are not dependent on radioactive sources, do not require specially designed radiation-shielded rooms for treatment, could be portable, could provide a selection of treatment energies, and would significantly reduce operating costs to a radiation oncology clinic. Full article
(This article belongs to the Special Issue Progress in Laser Accelerator and Future Prospects)
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12 pages, 3348 KB  
Letter
Remote Detection of Uranium Using Self-Focusing Intense Femtosecond Laser Pulses
by Miloš Burger, Patrick J. Skrodzki, Lauren A. Finney, John Nees and Igor Jovanovic
Remote Sens. 2020, 12(8), 1281; https://doi.org/10.3390/rs12081281 - 18 Apr 2020
Cited by 20 | Viewed by 5182
Abstract
Optical measurement techniques can address certain important challenges associated with nuclear safety and security. Detection of uranium over long distances presents one such challenge that is difficult to realize with traditional ionizing radiation detection, but may benefit from the use of techniques based [...] Read more.
Optical measurement techniques can address certain important challenges associated with nuclear safety and security. Detection of uranium over long distances presents one such challenge that is difficult to realize with traditional ionizing radiation detection, but may benefit from the use of techniques based on intense femtosecond laser pulses. When a high-power laser pulse propagates in air, it experiences collapse and confinement into filaments over an extended distance even without external focusing. In our experiments, we varied the initial pulse chirp to optimize the emission signal from the laser-produced uranium plasma at an extended distance. While the ablation efficiency of filaments formed by self-focusing is known to be significantly lower when compared to filaments produced by external focusing, we show that filaments formed by self-focusing can still generate luminous spectroscopic signatures of uranium detectable within seconds over a 10-m range. The intensity of uranium emission varies periodically with laser chirp, which is attributed to the interplay among self-focusing, defocusing, and multi-filament fragmentation along the beam propagation axis. Grouping of multi-filaments incident on target is found to be correlated with the uranium emission intensity. The results show promise towards long-range detection, advancing the diagnostics and analytical capabilities in ultrafast laser-based spectroscopy of high-Z elements. Full article
(This article belongs to the Section Remote Sensing Perspective)
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