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Structure–Property Relationships of Multi-Functional Polymer Composites

A special issue of Polymers (ISSN 2073-4360). This special issue belongs to the section "Polymer Composites and Nanocomposites".

Deadline for manuscript submissions: 20 September 2025 | Viewed by 513

Special Issue Editors


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Guest Editor
School of System Design and Intelligent Manufacturing, Southern University of Science and Technology, Shenzhen, China
Interests: polymer composite; composite structure; sandwich structure; multi-functional polymers; electromagnetic wave absorption; additive manufacturing; bio-inspired design
School of Civil Engineering, Central South University, Changsha 410083, China
Interests: mechanical properties of cellular materials; multifunctional polymer composites and structures; additive manufacturing; design and characterization of mechanical metamaterials; bioinspired materials; impact dynamics
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Special Issue Information

Dear Colleagues,

Polymer (nano)composites are revolutionizing material science by bridging the gap between functional versatility and structural precision. These advanced materials, which integrate nanoscale fillers into polymer matrices, enable an unprecedented range of mechanical, thermal, electrical, and dynamic properties. This Special Issue explores the intricate interplay between material structure and functionality, showcasing innovations that advance both theoretical understanding and practical applications. Key highlights include breakthroughs in nanofiller design and functionalization—such as hybrid graphene composites and bio-based nanoparticles—alongside cutting-edge fabrication techniques like additive manufacturing and in situ polymerization, paving the way for sustainable, high-performance materials.

A theme of this Special Issue is the dynamic and stimuli-responsive nature of polymer nanocomposites, which are unlocking transformative applications in fields such as soft robotics, biomedical engineering, and wearable technology. Researchers have demonstrated remarkable advances in self-healing mechanisms, where materials autonomously repair damages, and in shape-memory behavior, enabling structures to respond adaptively to external stimuli. These breakthroughs not only enhance functionality but also extend the lifespan and reliability of these materials, creating new possibilities in advanced engineering systems.

Material structure–property relationships form the foundation of polymer composite design, enabling the creation of materials with tailored functionalities. By manipulating the structural arrangement of polymer matrices and nanofillers, researchers can achieve specific combinations of properties, such as high strength-to-weight ratios, thermal stability, or electrical conductivity. These relationships are essential for bridging the gap between theoretical modeling and real-world applications, guiding innovations in composite performance for diverse fields ranging from aerospace to biomedical devices. Understanding these interactions not only allows for the optimization of individual properties but also supports the development of multi-functional composites that address complex engineering challenges.

This Special Issue emphasizes the critical role of advanced characterization techniques in deciphering material structure–property relationships. Tools such as atomic force microscopy, X-ray diffraction, and dynamic mechanical analysis are shedding light on nanoscale interactions between fillers and polymer matrices, offering a deeper understanding of how these interactions influence macroscopic properties. Additionally, in situ characterization methods, such as additive manufacturing, allow researchers to observe real-time changes during processing or operation, ensuring a comprehensive evaluation of material performance.

Sustainability is another prominent focus, with efforts directed toward eco-friendly nanofillers, bio-based polymers, and energy-efficient fabrication techniques. These advancements align with global priorities to reduce environmental impact while maintaining high-performance standards. Researchers are also exploring circular economy principles, such as recyclability and lifecycle optimization, to create composites that meet both technical and ecological requirements. Such innovations are vital for scaling up these materials to industrial applications while addressing environmental challenges.

This Special Issue exemplifies the interdisciplinary collaboration that drives the field of polymer (nano)composites, merging insights from chemistry, materials science, and engineering. By advancing the understanding of material structure–property relationships, it opens new pathways for designing multi-functional and sustainable materials. The featured research not only highlights current achievements but also sets the stage for future exploration, inspiring solutions to the complex challenges of modern technology and environmental sustainability.

Dr. Quanjin Ma
Dr. Yong Tao
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Polymers is an international peer-reviewed open access semimonthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2700 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • polymer composite
  • nanofillers
  • material structure–property
  • nanocomposites
  • multi-functional polymers
  • multi-scale mechanics
  • thermal properties
  • dielectric properties
  • mechanical properties
  • additive manufacturing

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Published Papers (1 paper)

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Research

16 pages, 13437 KiB  
Article
Theoretical Prediction Method for Tensile Properties of High-Strength Steel/Carbon Fiber-Reinforced Polymer Laminates
by Haichao Hu, Qiang Wei, Tianao Wang, Quanjin Ma, Shupeng Pan, Fengqi Li, Chuancai Wang and Jie Ding
Polymers 2025, 17(7), 846; https://doi.org/10.3390/polym17070846 - 21 Mar 2025
Viewed by 342
Abstract
This study introduces a method for predicting the tensile properties of high-strength steel/carbon fiber-reinforced polymer (CFRP) composite laminates using Metal Volume Fraction (MVF) theory. DP590 and DP980 high-strength steels (thickness ~0.8 mm) were selected as substrates, and composite laminates were fabricated by compression [...] Read more.
This study introduces a method for predicting the tensile properties of high-strength steel/carbon fiber-reinforced polymer (CFRP) composite laminates using Metal Volume Fraction (MVF) theory. DP590 and DP980 high-strength steels (thickness ~0.8 mm) were selected as substrates, and composite laminates were fabricated by compression molding with CFRP prepreg. Tensile tests were performed on an MTS universal testing machine, and fracture morphology was analyzed using scanning electron microscopy (SEM). The results demonstrated a typical mixed failure mode: necking and fracture in the metal layer, and neat fiber fracture in the CFRP layer. Comparisons of experimental tensile strength with theoretical predictions revealed that the model based on the metal strength at fracture significantly outperformed the model using tensile strength for predictions, with narrower error ranges. For example, the error for DP590/CFRP laminates ranged from 2.31% to 12.89%, whereas for DP980/CFRP laminates, it was –6.12%. Additionally, the study showed that using metals with higher plasticity in fiber metal laminates could underutilize the metal layer’s potential at peak stress, leading to significant deviations when predictions rely on tensile strength. Therefore, it is recommended to use the metal strength corresponding to peak stress for more accurate MVF-based tensile property predictions. This method provides a robust theoretical foundation for predicting the tensile performance of high-strength steel/CFRP laminates, aiding in optimizing structural designs for automotive and aerospace applications. Future research could explore the effects of different metal and fiber combinations, as well as more complex stacking designs. Full article
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