Electrode/Electrolyte Interface in Lithium-Ion Batteries

Dear Colleagues,

The electrode–electrolyte interface has remained a critical concern since the birth of lithium(Li)-based batteries (Li or Li⁺-ion batteries) that operate via the use of liquid electrolytes, which have developed into solid-state electrolytes (polymer- or ceramic-electrolyte) in recent years. The interfacial components and properties have been demonstrated to have a significant effect on the electrochemical behavior of batteries. Understanding the relevant chemical/electrochemical reactions, structural/compositional characteristics, and thermodynamic/kinetic behaviors at the electrode–electrolyte interface is crucial to the development of strategies that enhance the overall performance of batteries. Although a large volume of research has been performed, both a fundamental understanding of the interfacial phenomena and the practical strategies required to enhance the interfacial properties remain limited and unverified. More relevant and meaningful work remains to be performed.

This Special Issue welcomes the submission of manuscripts that provide an in-depth exploration of the failure mechanisms of the electrode/electrolyte interface during cycling, as well as the design of strategies from the perspective of the near-surface modification of materials or electrolyte optimization. In addition, articles that present novel mechanisms for some generally established facts and critical reviews are welcome, as these can guide in the design of suitable interface modification strategies.

We are looking forward to the discovery of more meaningful and valuable ideas regarding electrode and electrolyte interfaces in order to promote the advancement of Li or Li⁺-ion batteries.

Dr. Xuerui Yang
Dr. Jianhui Li
Guest Editors

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• lithium/lithium-ion battery
• electrolyte
• interfaces and surface chemistry
• various cathodes and anodes