Atmospheric Nucleation Processes: New Particle Formation and Representation in Models

A special issue of Atmosphere (ISSN 2073-4433). This special issue belongs to the section "Aerosols".

Deadline for manuscript submissions: closed (31 October 2019) | Viewed by 3485

Special Issue Editors


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Guest Editor
Brookhaven National Laboratory, Environmental and Climate Sciences Department, Upton, USA
Interests: nucleation processes; thermodynamics; atmospheric aerosols; aerosol dynamics; quadrature method of moments; drizzle formation

E-Mail Website
Guest Editor
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY, USA
Interests: new particle formation; heterogeneous nucleation; cluster growth dynamics; single molecule condensational detection; inversion techniques; vertically-resolved cluster measurement

Special Issue Information

Dear Colleagues,

Nucleation in the atmosphere is responsible for the formation of new particles that can subsequently grow to exert a significant impact on the global climate either directly, through the scattering and absorption of solar radiation, or indirectly, by serving as sites for cloud droplet condensation. There is evidence that both homogeneous and heterogeneous nucleation (including ion induced nucleation) pathways contribute to this process. Nevertheless, significant knowledge gaps remain: new experimental, modeling, and theoretical efforts are needed to better understand and quantify the chemistry of gas-phase particle precursors, the spatial and vertical extent of new particle formation events, and the role of meteorological conditions. Overall, the significance of these effects and their impacts on atmospheric aerosol processes and aerosol–cloud interactions remain largely unconstrained and not well understood.

This Special Issue focuses on this timely topic. We invite contributions from laboratory and field measurements and from theoretical and modeling studies relevant to the effects above, including: atmospheric precursor chemistry, multicomponent homogeneous and heterogeneous nucleation mechanisms, ion-induced nucleation, and growth processes leading to the formation of cloud condensation nuclei. The submission of studies that clarify condensed-phase homogeneous and heterogeneous nucleation mechanisms relating to ice nucleation is also encouraged. Parameterization studies that help bridge the gap between nucleation-related processes and their couplings and impacts on clouds and climate are welcomed, as are theoretical studies geared towards process-level understanding of nucleation mechanisms and their representation in models at different scales.

Dr. Robert L. McGraw
Dr. Chongai Kuang
Guest Editors

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Keywords

  • atmospheric nucleation
  • nucleation theory and measurement
  • new particle formation
  • vapor condensation on nanoparticles
  • ion-induced nucleation
  • ice nucleation mechanisms and rates
  • chemical precursors to nucleation
  • cloud condensation nuclei
  • aerosol lifecycle
  • impacts on clouds and climate

Published Papers (1 paper)

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Research

16 pages, 796 KiB  
Article
Is Contact Nucleation Caused by Pressure Perturbation?
by Fan Yang, Will H. Cantrell, Alexander B. Kostinski, Raymond A. Shaw and Andrew M. Vogelmann
Atmosphere 2020, 11(1), 1; https://doi.org/10.3390/atmos11010001 - 18 Dec 2019
Cited by 12 | Viewed by 3109
Abstract
The reason why ice nucleation is more efficient by contact nucleation than by immersion nucleation has been elusive for over half a century. Six proposed mechanisms are summarized in this study. Among them, the pressure perturbation hypothesis, which arose from recent experiments, can [...] Read more.
The reason why ice nucleation is more efficient by contact nucleation than by immersion nucleation has been elusive for over half a century. Six proposed mechanisms are summarized in this study. Among them, the pressure perturbation hypothesis, which arose from recent experiments, can qualitatively explain nearly all existing results relevant to contact nucleation. To explore the plausibility of this hypothesis in a more quantitative fashion and to guide future investigations, this study assessed the magnitude of pressure perturbation needed to cause contact nucleation and the associated spatial scales. The pressure perturbations needed were estimated using measured contact nucleation efficiencies for illite and kaolinite, obtained from previous experiments, and immersion freezing temperatures, obtained from well-established parameterizations. Pressure perturbations were obtained by assuming a constant pressure perturbation or a Gaussian distribution of the pressure perturbation. The magnitudes of the pressure perturbations needed were found to be physically reasonable, being achievable through possible mechanisms, including bubble formation and breakup, Laplace pressure arising from the distorted contact line, and shear. The pressure perturbation hypothesis provides a physically based and experimentally constrainable foundation for parameterizing contact nucleation that may be useful in future cloud-resolving models. Full article
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