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Open AccessArticle

Is Contact Nucleation Caused by Pressure Perturbation?

1
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY 11973, USA
2
Department of Physics, Michigan Technological University, Houghton, MI 49931, USA
*
Author to whom correspondence should be addressed.
Atmosphere 2020, 11(1), 1; https://doi.org/10.3390/atmos11010001
Received: 8 November 2019 / Revised: 8 December 2019 / Accepted: 13 December 2019 / Published: 18 December 2019
The reason why ice nucleation is more efficient by contact nucleation than by immersion nucleation has been elusive for over half a century. Six proposed mechanisms are summarized in this study. Among them, the pressure perturbation hypothesis, which arose from recent experiments, can qualitatively explain nearly all existing results relevant to contact nucleation. To explore the plausibility of this hypothesis in a more quantitative fashion and to guide future investigations, this study assessed the magnitude of pressure perturbation needed to cause contact nucleation and the associated spatial scales. The pressure perturbations needed were estimated using measured contact nucleation efficiencies for illite and kaolinite, obtained from previous experiments, and immersion freezing temperatures, obtained from well-established parameterizations. Pressure perturbations were obtained by assuming a constant pressure perturbation or a Gaussian distribution of the pressure perturbation. The magnitudes of the pressure perturbations needed were found to be physically reasonable, being achievable through possible mechanisms, including bubble formation and breakup, Laplace pressure arising from the distorted contact line, and shear. The pressure perturbation hypothesis provides a physically based and experimentally constrainable foundation for parameterizing contact nucleation that may be useful in future cloud-resolving models. View Full-Text
Keywords: ice nucleation; contact nucleation; pressure perturbation ice nucleation; contact nucleation; pressure perturbation
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Yang, F.; Cantrell, W.H.; Kostinski, A.B.; Shaw, R.A.; Vogelmann, A.M. Is Contact Nucleation Caused by Pressure Perturbation? Atmosphere 2020, 11, 1.

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