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Keywords = tunable laser

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11 pages, 1373 KB  
Communication
Research on Continuously Tunable Carbon Nanotube Mode-Locked Fiber Laser
by Zhengyu Yang, Fei Wang and Pingping Xiao
Micromachines 2026, 17(4), 455; https://doi.org/10.3390/mi17040455 - 7 Apr 2026
Viewed by 184
Abstract
This paper demonstrates a C-band continuously tunable mode-locked fiber laser based on a carbon nanotube saturable absorber (CNT-SA) and a commercial broadband tunable filter. The laser operates in the C-band with a continuous tuning range of 37.3 nm from 1532.6 nm to 1569.9 [...] Read more.
This paper demonstrates a C-band continuously tunable mode-locked fiber laser based on a carbon nanotube saturable absorber (CNT-SA) and a commercial broadband tunable filter. The laser operates in the C-band with a continuous tuning range of 37.3 nm from 1532.6 nm to 1569.9 nm. The erbium-doped fiber (EDF) has a wide gain range, enabling the laser to achieve ultrafast mode-locking. Meanwhile, the tunable filter offers a broad wavelength selection range. This continuously tunable mode-locked fiber laser features a simple structure and a broad operating wavelength range, making it highly suitable for applications in optical communication, sensing, and laser processing. Full article
(This article belongs to the Special Issue Optical and Laser Material Processing, 2nd Edition)
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17 pages, 2186 KB  
Article
An Estimate of Sulfur Isotope Fractionation Due to SO2 Self-Shielding in the Upper Atmosphere of Venus
by James R. Lyons
Atmosphere 2026, 17(4), 332; https://doi.org/10.3390/atmos17040332 - 24 Mar 2026
Viewed by 323
Abstract
Sulfur dioxide is a trace constituent of the upper atmosphere of Venus but plays a dominant role in the photochemistry above the cloud tops. Because SO2 undergoes indirect dissociation to a relatively long-lived excited state, it has a line-type absorption spectrum in [...] Read more.
Sulfur dioxide is a trace constituent of the upper atmosphere of Venus but plays a dominant role in the photochemistry above the cloud tops. Because SO2 undergoes indirect dissociation to a relatively long-lived excited state, it has a line-type absorption spectrum in the dissociation region (~190–220 nm). This leads to strong isotopic fractionation under optically thick conditions, a process referred to as self-shielding. Here, I use SO2 cross-sections, shielding functions, and a simple steady-state photochemical model to estimate sulfur isotope ratios in SO2. The results indicate that large isotope depletion relative to SO2 in the deep atmosphere is expected in SO2 below 70 km altitude, with δ34S ~ −100 to −200 permil. This is readily detectable by the VTLS tunable laser spectrometer planned for the NASA DAVINCI mission. Full article
(This article belongs to the Section Planetary Atmospheres)
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12 pages, 2042 KB  
Article
Performance Characterization and Optimization of a Miniaturized SERF Atomic Magnetometer via Tunable Laser Power
by Peng Shi, Chen Zuo, Qisong Li and Shulin Zhang
Sensors 2026, 26(6), 2000; https://doi.org/10.3390/s26062000 - 23 Mar 2026
Viewed by 306
Abstract
Spin-exchange relaxation-free (SERF) atomic magnetometers have emerged as highly promising candidates for ultra-weak magnetic field detection, particularly in biomagnetic imaging, owing to their exceptional sensitivity, amenability to miniaturization, and near-room-temperature operation. While current miniaturized magnetometers typically employ laser chips with fixed optical power, [...] Read more.
Spin-exchange relaxation-free (SERF) atomic magnetometers have emerged as highly promising candidates for ultra-weak magnetic field detection, particularly in biomagnetic imaging, owing to their exceptional sensitivity, amenability to miniaturization, and near-room-temperature operation. While current miniaturized magnetometers typically employ laser chips with fixed optical power, the quantitative impact of laser power on critical performance metrics remains to be fully elucidated. This study systematically investigates the influence of laser power on sensitivity, bandwidth, and dynamic range by incorporating considerations of power broadening, saturation absorption, and noise constraints. A miniaturized probe, integrated with an actively controlled vertical-cavity surface-emitting laser (VCSEL), was developed for experimental validation. Theoretical and experimental results consistently demonstrate that as optical power increases, sensitivity exhibits a non-monotonic dependence, whereas both bandwidth and dynamic range manifest a monotonic upward trend, aligning well with theoretical simulations. The optimized sensor achieved a peak sensitivity of 16 fT/√Hz at 300 μW, while the bandwidth and dynamic range reached 230 Hz and ±5.4 nT at 500 μW, respectively. This work establishes a robust theoretical and experimental framework for the comprehensive performance optimization of laser-integrated miniaturized atomic magnetometers. Full article
(This article belongs to the Section Optical Sensors)
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11 pages, 3141 KB  
Communication
ZrGeTe4 Nanoparticles as a Saturable Absorber for Mode-Locked Operations at 1 and 1.55 µm
by Xinxin Shang, Nannan Xu, Mengyu Zong, Weiyi Yu, Linguang Guo, Guanguang Gao, Ziqi Zhang, Huanian Zhang and Lianzheng Su
Photonics 2026, 13(3), 305; https://doi.org/10.3390/photonics13030305 - 20 Mar 2026
Cited by 1 | Viewed by 276
Abstract
In the current paper, the nonlinear absorption characteristics and laser modulation performance of the ternary anisotropic semiconductor material ZrGeTe4 were successfully explored. The recovery time of the ZrGeTe4-PVA thin film was measured to be 5.74 ps by the pump–probe technology. [...] Read more.
In the current paper, the nonlinear absorption characteristics and laser modulation performance of the ternary anisotropic semiconductor material ZrGeTe4 were successfully explored. The recovery time of the ZrGeTe4-PVA thin film was measured to be 5.74 ps by the pump–probe technology. By employing ZrGeTe4 as a saturable absorber, a passive mode-locked Yb-doped fiber laser was demonstrated for the first time. In the 1 µm mode-locked operation, the central wavelength was 1031.29 nm, the pulse repetition rate was 24.85 MHz, and the pulse width was 786.3 ps. In an Er-doped fiber laser operating at a wavelength of 1561.10 nm, the pulse width was as short as 1.26 ps with a repetition rate of 4.38 MHz. The results show that ZrGeTe4 has excellent broadband nonlinear optical characteristics. Full article
(This article belongs to the Special Issue Advancements in Ultrafast Laser Science and Technology)
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27 pages, 3211 KB  
Article
Performance Enhancement Study of WMS-TDLAS System for Online Measurement of High-Concentration CO2 in Flue Gas
by Xinhu Xu, Wanglong Shi and Liang Zhang
Appl. Sci. 2026, 16(6), 2865; https://doi.org/10.3390/app16062865 - 16 Mar 2026
Viewed by 335
Abstract
Accurate and stable measurement of carbon dioxide (CO2) concentrations in industrial flue gases is critical for emissions monitoring and carbon management. The present study developed a wavelength-modulated tunable diode laser absorption spectroscopy (WMS-TDLAS) system for measuring high-concentration carbon dioxide (CO2 [...] Read more.
Accurate and stable measurement of carbon dioxide (CO2) concentrations in industrial flue gases is critical for emissions monitoring and carbon management. The present study developed a wavelength-modulated tunable diode laser absorption spectroscopy (WMS-TDLAS) system for measuring high-concentration carbon dioxide (CO2) in flue gases, covering a range of 3–20% (by volume). To mitigate optical intensity fluctuations caused by particle scattering and detector gain drift in harsh flue gas environments, a normalized second harmonic (2f/1f) detection scheme based on a single-harmonic peak was employed. A digital phase-locked amplification algorithm replaces the conventional hardware lock-in amplifier, enabling simultaneous demodulation of multiple harmonic components and enhancing system integration. A comparison of the digital locking method with a commercial lock-in amplifier reveals that the former demonstrates comparable or superior stability, with relative standard deviations of 0.04% for the 2f signal and 0.02% for the first-harmonic signal. In order to address the sensitivity degradation of WMS-TDLAS at elevated CO2 concentrations, a pressure control strategy was introduced. Maintaining the measurement cell pressure at 70 ± 0.005 kPa resulted in a 2.74-fold enhancement in system sensitivity at 13.01% CO2 and a more than one-order-of-magnitude increase at 20.01% CO2 compared to operation at atmospheric pressure. Concentration measurement error under reduced pressure also decreased from 1.101% to 0.075%. The system exhibited 0.6% repeatability in high-concentration CO2 measurements, signifying its aptitude for industrial flue gas monitoring applications. Full article
(This article belongs to the Section Optics and Lasers)
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19 pages, 2330 KB  
Article
Mercury: Accelerating 3D Parallel Training with an AWGR-WSS-Based All-Optical Reconfigurable Network
by Shi Feng, Jiawei Zhang, Huitao Zhou, Xingde Li and Yuefeng Ji
Photonics 2026, 13(3), 286; https://doi.org/10.3390/photonics13030286 - 16 Mar 2026
Viewed by 346
Abstract
The network traffic of 3D parallel training in large-scale deep learning, featuring burstiness, hot-spots, and periodic large-bandwidth patterns, severely challenges network efficiency, necessitating a high-performance and flexible optical network solution. To address this, this paper proposes Mercury, a hybrid optical network based on [...] Read more.
The network traffic of 3D parallel training in large-scale deep learning, featuring burstiness, hot-spots, and periodic large-bandwidth patterns, severely challenges network efficiency, necessitating a high-performance and flexible optical network solution. To address this, this paper proposes Mercury, a hybrid optical network based on physical optical components: its optical timeslot switching (OTS) subnet uses an arrayed waveguide grating router (AWGR) and tunable lasers for dynamic traffic, while the optical circuit switching (OCS) subnet relies on wavelength selective switches (WSSs) for low-latency high-bandwidth transmission, which is coordinated by selective valiant load balancing (S-VLB) and most efficient path configuration (MEPC) mechanisms. Validated via simulations and FPGA-based testbed experiments, Mercury outperforms the Sirius network by reducing epoch training time (e.g., 179s with five jobs) and relieving OTS congestion through offloading large flows to OCS. This work demonstrates that Mercury provides a flexible, high-performance physical optical solution for 3D parallel training of large-scale deep learning models. Full article
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26 pages, 10734 KB  
Article
A Residual Amplitude Modulation Noise Suppression Method Based on Multi-Harmonic Component Decoupling
by Qiwu Luo, Hang Su, Yibo Wang and Chunhua Yang
Sensors 2026, 26(6), 1841; https://doi.org/10.3390/s26061841 - 14 Mar 2026
Viewed by 304
Abstract
Wavelength modulation spectroscopy (WMS) is a representative implementation of tunable diode laser absorption spectroscopy (TDLAS), enabling reliable gas component analysis with concentration-related information derived from harmonic component extraction, while offering enhanced noise immunity for trace gas sensing in open environments. However, due to [...] Read more.
Wavelength modulation spectroscopy (WMS) is a representative implementation of tunable diode laser absorption spectroscopy (TDLAS), enabling reliable gas component analysis with concentration-related information derived from harmonic component extraction, while offering enhanced noise immunity for trace gas sensing in open environments. However, due to the strong coupling between laser wavelength and intensity, wavelength modulation inevitably introduces residual amplitude modulation (RAM), which significantly degrades measurement accuracy. To address this issue, this study introduces a RAM suppression algorithm based on multiple harmonic component decoupling (MHCD), using the second-harmonic lateral peak inclination angle (LPIA) as a characteristic indicator. Unit harmonic operators for the first, second, and third harmonics are designed, and an original harmonic reconstruction model is established via linear superposition of harmonic components. The optimal harmonic component ratio is determined at the composite operator with the maximum cross-correlation coefficient, and RAM noise is eliminated through a multi-harmonic decoupling matrix. Repetitive measurements on 22 mm pharmaceutical vials with 4% oxygen concentration demonstrate that MHCD reduces the second-harmonic LPIA from 18.07° to 8.56°. Concentration discrimination experiments conducted on seven groups of 22 mm vials with 2% concentration steps (0–12%) show that MHCD increases the true positive rate by 6–11% and decreases the false positive rate by 4–9%, confirming its effectiveness for pharmaceutical online inspection applications. Full article
(This article belongs to the Special Issue Advanced Sensing Technologies in Industrial Defect Detection)
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32 pages, 6543 KB  
Review
MOCVD Growth of Next-Generation III–V Semiconductor Devices: In Review
by Zoya Noor, Muhammad Usman, Shazma Ali, Anis Naveed, Amina Hafeez and Ahmed Ali
Photonics 2026, 13(3), 273; https://doi.org/10.3390/photonics13030273 - 12 Mar 2026
Viewed by 1171
Abstract
Metal–organic chemical vapor deposition (MOCVD) is a crystal growth technique used to achieve high-purity thin films, especially III–V materials, for fabricating semiconductor devices. It allows for thickness tunability, controlled doping, and composition of epilayers. This review focuses on the principle of MOCVD, its [...] Read more.
Metal–organic chemical vapor deposition (MOCVD) is a crystal growth technique used to achieve high-purity thin films, especially III–V materials, for fabricating semiconductor devices. It allows for thickness tunability, controlled doping, and composition of epilayers. This review focuses on the principle of MOCVD, its historical background, and its applications in III–V semiconductor devices such as solar cells, high electron mobility transistors (HEMTs), light-emitting diodes (LEDs), laser diodes (LDs), and photonic integrated circuits (PICs). This review highlights the recent developments in MOCVD aimed at improving its efficiency, performance, and sustainability. Finally, we emphasize emerging trends and challenges in MOCVD process innovation, reactor design, and material integration that are poised to drive the development of next-generation optoelectronic, photonic, and quantum technologies. Together, these findings underscore MOCVD’s pivotal role in enabling high-performance devices and sustaining leadership in post-Moore semiconductor technologies. Full article
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14 pages, 3808 KB  
Article
A Multichannel Vortex Beam Generator via Spatially Structured Bidirectional Two-Color-Pump Four-Wave Mixing in a Single 133Cs Vapor Cell
by Dan Wang, Meng-Yu Bian, Zi-Yi Gao, Liang-Hui Huang, Hai-Tao Zhou and Jun-Xiang Zhang
Photonics 2026, 13(3), 247; https://doi.org/10.3390/photonics13030247 - 3 Mar 2026
Viewed by 356
Abstract
Multichannel vortex beams serve as an essential physical source for enabling multi-spot laser processing and high-dimensional spatial multiplexing communications. We demonstrate a compact, flexibly tunable multichannel vortex beam generator using spatially structured bidirectional two-color pump vortex four-wave mixing in a single 133Cs [...] Read more.
Multichannel vortex beams serve as an essential physical source for enabling multi-spot laser processing and high-dimensional spatial multiplexing communications. We demonstrate a compact, flexibly tunable multichannel vortex beam generator using spatially structured bidirectional two-color pump vortex four-wave mixing in a single 133Cs vapor cell. To enhance spatial multiplexing, both sides of the cell are utilized. By engineering the propagation directions and frequencies of five input beams, we establish a nonlinear interaction region that supports 16 concurrent phase-matching conditions, thereby enabling the parallel generation of up to eight vortex channels. The orbital angular momentum of the output beams follows deterministic algebraic rules, allowing for programmable control via tailored input orbital angular momentum combinations. Moreover, the channel count can be linearly tuned by selectively deactivating pumps—each switched-off pump reduces the number of output channels by two. This flexible control over orbital angular momentum states, together with channel count and spatial arrangement, establishes a highly integrated platform for on-demand vortex generation. This work highlights the potential of spatially bidirectional structured pumping in atomic vapor to expand optical dimensionality and enhance multiplexing capacity, paving the way toward multidimensional communications, quantum networks, and integrated photonics. Full article
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19 pages, 3546 KB  
Article
Algorithm for the Simultaneous Measurement of Multiple Parameters Based on Wavelength Modulation Spectroscopy
by Xiangyu Zhong, Qing Shi, Buqiang Zhang, Huiwen Niu, Gui Meng, Jianfa Zhou and Yongqing Peng
Sensors 2026, 26(5), 1585; https://doi.org/10.3390/s26051585 - 3 Mar 2026
Viewed by 350
Abstract
To ensure personnel safety and prevent serious accidents, it is crucial to monitor parameters such as temperature, pressure, and gas composition concentrations in confined spaces. This study proposes a multi-parameter simultaneous inversion algorithm based on tunable diode laser absorption spectroscopy (TDLAS). The algorithm [...] Read more.
To ensure personnel safety and prevent serious accidents, it is crucial to monitor parameters such as temperature, pressure, and gas composition concentrations in confined spaces. This study proposes a multi-parameter simultaneous inversion algorithm based on tunable diode laser absorption spectroscopy (TDLAS). The algorithm integrates the Levenberg–Marquardt (L-M) fitting method, single-line thermometry and manometry methods, spectral separation, and alternating iteration techniques, with an adaptive feedback mechanism adding to enhance convergence stability. Through this approach, simultaneous inversion of H2O, CO2, CO, and O2 concentrations, temperature, and pressure was successfully achieved. Simulation results demonstrated that the measurement accuracy meets practical requirements. This study provides an effective monitoring method for multi-parameter detection in confined spaces within conventional environments and lays a foundation for expanding the application scope of TDLAS technology. Full article
(This article belongs to the Special Issue Spectroscopy Gas Sensing and Applications)
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20 pages, 2787 KB  
Article
Vibrational Characteristics of High-Quality MBE Grown GaAs1−x−ySbyNx/GaAs (001) Epilayers
by Devki N. Talwar and Hao-Hsiung Lin
Materials 2026, 19(5), 923; https://doi.org/10.3390/ma19050923 - 28 Feb 2026
Viewed by 381
Abstract
The significant disparity between the size and electronegativity of N and group-V (P, As, Sb) atoms in dilute III–V-Ns remains a cornerstone for developing the next-generation electronics. Variations in the structural, optical, and phonon properties of the quaternary GaAs1−x−ySbyN [...] Read more.
The significant disparity between the size and electronegativity of N and group-V (P, As, Sb) atoms in dilute III–V-Ns remains a cornerstone for developing the next-generation electronics. Variations in the structural, optical, and phonon properties of the quaternary GaAs1−x−ySbyNx alloys are being used for improving the high-performance photovoltaic energy and optoelectronic technologies. Bandgap Eg tunability has assisted efficient light emission/detection to cover the crucial optical fiber wavelengths for the low-cost integrated chips in data communications and sensing devices. The lattice dynamical properties of these materials are critical for assessing the reliability to evaluate the performance of long-wavelength lasers, photodetectors, and multi-junction solar cells. Our systematic Raman measurements on high-quality MBE grown GaAs0.946Sb0.032N0.022/GaAs samples have detected ωTO(Γ)GaAs and ωTO(Γ)GaAs phonons along with a high frequency NAs local mode near ~476 cm−1. Weak phonon structures on both sides of the broad 476 cm−1 band are interpreted forming a complex NAs–Ga–SbAs defect center. Using a realistic rigid-ion model in the Green’s function framework, the simulations of impurity modes for isolated and complex defects have provided corroboration to the experimental data. Full article
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28 pages, 6545 KB  
Article
Tailored Nitrogen-Doped Laser-Induced Graphene on Novel Synthesized Cross-Linked Aromatic Polyimides for Targeted Applications
by Katarina Tošić, Marija V. Pergal, Igor Pašti, Marko Bošković, Danica Bajuk Bogdanović and Marko Spasenović
Polymers 2026, 18(5), 588; https://doi.org/10.3390/polym18050588 - 27 Feb 2026
Viewed by 442
Abstract
Laser-induced graphene (LIG) is most often produced from commercial Kapton; the properties of LIG are inherently linked to those of the polymer substrate, which results in a limited field of applications for LIG on Kapton. This study demonstrates that tailored properties of LIG, [...] Read more.
Laser-induced graphene (LIG) is most often produced from commercial Kapton; the properties of LIG are inherently linked to those of the polymer substrate, which results in a limited field of applications for LIG on Kapton. This study demonstrates that tailored properties of LIG, including nitrogen doping, which is favorable for electronic applications, can be achieved by using synthesized cross-linked polyimides (PIs) as substrates for graphene induction. Three amorphous polyimides containing 4-[(4-aminophenyl)sulfonyl]aniline (PI-APSA), 1,2-diaminoethane (PI-EDA), and urea (PI-Urea), as crosslinkers, were prepared from different diamines and maleic anhydride, and subsequently used as substrates to produce in situ nitrogen-doped LIG. The resulting materials were comprehensively characterized and compared with LIG on Kapton. Raman spectroscopy confirmed lower defect densities and higher crystallinity than in LIG on Kapton, while sheet resistance was up to three times smaller. The LIG with PI-EDA showed the highest nitrogen content and a specific areal capacitance of 3.1 mF/cm2, which is more than an order of magnitude higher than that of LIG/on Kapton, highlighting its strong potential for energy storage devices. PI-APSA-based LIG exhibited the best adhesion and lowest sheet resistance, making it suitable for wearable electrodes, whereas PI-urea-based LIG maintained hydrophilicity. Thus, chemically tailored polyimides enable the formation of nitrogen-doped LIG with tunable interfacial properties, higher structural order, and improved electrical and electrochemical performance compared to commercial Kapton. Full article
(This article belongs to the Section Polymer Composites and Nanocomposites)
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13 pages, 12795 KB  
Article
Validation of a Compact and Tunable Continuous Gas-Flow Laser-Plasma Target for Electron Beam Production Above 150 MeV
by Pierre Drobniak, Jana Serhal, Maria Pia Anania, Elsa Baynard, Arnaud Beck, Christelle Bruni, Antoine Cauchois, Gemma Costa, Lucio Crincoli, Denis Douillet, Julien Gautier, Jean-Philippe Goddet, Coline Guyot, Gregory Iaquaniello, Gueladio Kane, Sophie Kazamias, Olena Kononenko, Viacheslav Kubytskyi, Bruno Lucas, Ali Mahjoub, Antoine Maitrallain, Olivier Neveu, Yann Peinaud, Moana Pittman, Pascal Rousseau, Johan Sebastián Ramírez Amado, Arnd Specka, Cédric Thaury and Kevin Cassouadd Show full author list remove Hide full author list
Appl. Sci. 2026, 16(5), 2312; https://doi.org/10.3390/app16052312 - 27 Feb 2026
Viewed by 316
Abstract
The present article reports on the generation of stable 50 pC low-divergence electron beams above 150 MeV from laser-driven wakefield acceleration using a continuous-flow gas target prototype tested at the 60 TW Salle Jaune facility at LOA. The gas target design is meant [...] Read more.
The present article reports on the generation of stable 50 pC low-divergence electron beams above 150 MeV from laser-driven wakefield acceleration using a continuous-flow gas target prototype tested at the 60 TW Salle Jaune facility at LOA. The gas target design is meant to be easily transported and integrated as an element of the beamline with a differential pumping system offering some 10−4 mbar pressure in the rest of the line. A dedicated gas injection system allows for the control of the gas mixture concentration and gas pressure in two different regions of the target within the frame of controlled ionisation injection schemes. The measured electron beam parameters show the importance of gas density profiles and longitudinal gas mixture confinement. Full article
(This article belongs to the Special Issue Trends and Prospects in Laser–Plasma Accelerator)
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11 pages, 2745 KB  
Article
Monolithic Integration of an FP-SA Optical Spiking Neuron and SOA Synapse by Photonic Crystals
by Haodong Xuan, Guangliang Sun, Yang Chen, Ningning Chen, Zeyu Wang, Hailing Wang and Wanhua Zheng
Photonics 2026, 13(3), 220; https://doi.org/10.3390/photonics13030220 - 26 Feb 2026
Viewed by 340
Abstract
We demonstrate a monolithically integrated photonic chip that combines an optical spiking neuron with a tunable synaptic element. The spiking neuron is realized using a quantum-well Fabry–Perot laser integrated with a saturable absorber (FP-SA), while a semiconductor optical amplifier (SOA) functions as a [...] Read more.
We demonstrate a monolithically integrated photonic chip that combines an optical spiking neuron with a tunable synaptic element. The spiking neuron is realized using a quantum-well Fabry–Perot laser integrated with a saturable absorber (FP-SA), while a semiconductor optical amplifier (SOA) functions as a photonic synapse. Two photonic-crystal (PC) mirrors define the laser cavity and enable effective modulation of the synaptic weight. Experimental results further confirm the capability of the SOA for continuous and controllable synaptic weight tuning. This work represents an important step toward scalable on-chip photonic spiking neural networks. Full article
(This article belongs to the Section Lasers, Light Sources and Sensors)
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12 pages, 3134 KB  
Article
CO2 Sensing Using Symmetrical Three-Wavelength Precompensated Current-Modulated Tunable Diode Laser Absorption Spectroscopy
by Giacomo Zanetti, Peter John Rodrigo and Christian Pedersen
Sensors 2026, 26(5), 1420; https://doi.org/10.3390/s26051420 - 24 Feb 2026
Viewed by 296
Abstract
In this paper, a novel symmetrical three-wavelength toggling archetype for measuring the concentration of gases using a tunable diode laser absorption spectroscopy (TDLAS) system is introduced and demonstrated. The system was operated at 1.5714 µm with a 2 kHz update rate, targeting an [...] Read more.
In this paper, a novel symmetrical three-wavelength toggling archetype for measuring the concentration of gases using a tunable diode laser absorption spectroscopy (TDLAS) system is introduced and demonstrated. The system was operated at 1.5714 µm with a 2 kHz update rate, targeting an absorption line of gaseous CO2. Precompensated diode–current pulses are introduced to offset the inherent thermal time constants of the diode laser by orders of magnitude. Here, repetition rates matching that of contemporary methods can be achieved, while simultaneously providing a noteworthy wavelength stability of 0.6 pm for the three targeted wavelengths that are approximately 70 pm apart (142 pm maximum wavelength excursion). A 10 Hz current loop locks one of the wavelengths to a CO2 absorption peak, thus providing an absolute and stable wavelength reference. The flexibility in choosing the shape and repetition frequency of the current pulses makes this approach easily adaptable to other gases and/or absorption lines, since wavelength filters are avoided. The new method is benchmarked against a two-wavelength precompensated continuous-wave TDLAS technique, revealing a fourfold improvement in reproducibility with system restart over the span of 24 days, while outperforming other widespread spectroscopic techniques applied to comparable transmittance levels. The effect of the analytical model was further studied by thermally inducing baseline changes, showing a 7.9 ± 0.2 times weaker correlation between concentration and temperature with respect to the one observed using the two-wavelength TDLAS archetype. These results demonstrate the system’s suitability for sensitive applications. Full article
(This article belongs to the Special Issue Advanced Sensors for Gas Monitoring: 2nd Edition)
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