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Keywords = nonlinear optics

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15 pages, 5236 KB  
Article
Continuous Domain Quasi-Bound State Enhances the Nonlinear Effects of Silicon Carbide
by Ning Wang, Dong Pan, Lijing Huang, Liping Liu, Yang Liu, Zijie Dai, Xiaoxian Song, Zhen Yue, Jiakang Shi, Zhaojian Zhang, Kejin Wei, Junbo Yang, Jingjing Zhang and Jianquan Yao
Photonics 2026, 13(4), 311; https://doi.org/10.3390/photonics13040311 - 24 Mar 2026
Abstract
We propose a silicon carbide (3C-SiC) periodic grating structure based on quasi-bound states in the continuum (q-BICs), which is used to significantly enhance the second-order optical nonlinear effect, including second-harmonic generation (SHG) and sum-frequency generation (SFG). By introducing a four-segment sub-wavelength grating on [...] Read more.
We propose a silicon carbide (3C-SiC) periodic grating structure based on quasi-bound states in the continuum (q-BICs), which is used to significantly enhance the second-order optical nonlinear effect, including second-harmonic generation (SHG) and sum-frequency generation (SFG). By introducing a four-segment sub-wavelength grating on the SiC thin film and tailor the dimension, the structure successfully excites two q-BIC modes with ultra-high Q factor (resonant wavelengths at 1713.2 nm and 1804.6 nm respectively), realizing enhanced localization and nonlinear interaction of the strong light field. The simulation results show that under oblique incidence, the structure significantly enhances SFG efficiency and exhibits strong robustness to variations in key structural parameters. In addition, the study also reveals the coexistence of forward and backward SHG, and resonant wavelength tuning can be achieved by adjusting the structure dimension. This work not only provides a new path to enhance the nonlinear conversion efficiency of SiC thin films and solve the problem of difficult phase matching, but also lays the theoretical and technical foundation for the development of compact, efficient and integrated SiC-based nonlinear photonic devices. Full article
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14 pages, 1136 KB  
Article
Achieving Maximum Chirality and Enhancing Third-Harmonic Generation via Quasi-Bound States in the Continuum in Nonlinear Metasurfaces
by Du Li, Yuchang Liu, Kun Liang and Li Yu
Nanomaterials 2026, 16(7), 388; https://doi.org/10.3390/nano16070388 - 24 Mar 2026
Abstract
Chiral bound states in the continuum (BIC) metasurfaces have emerged as a promising platform for enhancing light–matter interactions, which have potential applications in advanced photonic and quantum information devices. However, simultaneously achieving near-perfect circular dichroism and highly efficient nonlinear conversion with highly symmetric [...] Read more.
Chiral bound states in the continuum (BIC) metasurfaces have emerged as a promising platform for enhancing light–matter interactions, which have potential applications in advanced photonic and quantum information devices. However, simultaneously achieving near-perfect circular dichroism and highly efficient nonlinear conversion with highly symmetric structures in metasurfaces remains an open challenge. In this work, we design a C4-symmetric chiral metasurface composed of eight elliptical silicon nanorods on a SiO2 substrate, where monocrystalline silicon is used as the nonlinear optical material. By combining simulations and nonlinear time-domain coupled-mode theory (TCMT), we discovered that both the optimal chirality and the nonlinear conversion efficiency can be attained simultaneously due to the critical coupling between the metasurface mode and the quasi-BIC mode. Meanwhile, a near-perfect circular dichroism (CD = 0.99) and a high nonlinear conversion efficiency of 7×105 under a radiation intensity of 5kW/cm2 are numerically achieved due to the robustness of bound states in the continuum. This work offers a promising route toward high-performance chiral nonlinear photonic components, which is of great importance for the development of ultra-compact optical devices such as circular polarization detectors, chiral sensors, and nonlinear photonic chips for integrated optical and quantum information systems. Our research not only contributes to the fundamental understanding of chiral metasurfaces but also provides a practical approach for achieving high-efficiency nonlinear optical devices. Full article
(This article belongs to the Special Issue Nanophotonic: Structure, Devices and System)
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23 pages, 2873 KB  
Article
An Online Calibration Method for UAV Electro-Optical Pod Zoom Cameras Based on IMU-Vision Fusion
by Weiming Zhu, Zhangsong Shi, Huihui Xu, Qingping Hu, Wenjian Ying and Fan Gui
Drones 2026, 10(3), 224; https://doi.org/10.3390/drones10030224 - 22 Mar 2026
Viewed by 73
Abstract
To address the calibration challenge caused by the nonlinear variation in intrinsic parameters during continuous camera zooming in UAV electro-optical pods, this paper proposes an online calibration method based on IMU-visual fusion. Traditional offline calibration cannot adapt to dynamic scenarios, while existing self-calibration [...] Read more.
To address the calibration challenge caused by the nonlinear variation in intrinsic parameters during continuous camera zooming in UAV electro-optical pods, this paper proposes an online calibration method based on IMU-visual fusion. Traditional offline calibration cannot adapt to dynamic scenarios, while existing self-calibration methods suffer from slow convergence and insufficient robustness. The proposed method aims to achieve real-time and accurate estimation of camera intrinsic parameters during zooming. Specifically, we first construct a unified state estimation framework that encodes the internal and external parameters of the camera and the 3D positions of scene feature points into a high-dimensional state vector, then establish a camera motion model based on IMU data, construct a visual observation model by combining the pinhole camera and second-order radial distortion model to establish a nonlinear mapping from 3D feature points to 2D pixel coordinates, and adopt an improved ORB algorithm for feature extraction and LK optical flow method to achieve high-precision cross-frame feature matching to enhance the stability of visual observation. Most importantly, we design a tight-coupling fusion strategy based on the Extended Kalman Filter (EKF) prediction-update iteration mechanism, which fuses IMU high-frequency motion constraints and visual geometric constraints in real time to suppress parameter drift induced by focal length changes. Finally, we recursively solve the state vector to complete the online dynamic estimation of intrinsic parameters. Monte Carlo simulation experiments and real UAV flight experiments confirm that the method has both high estimation accuracy and strong environmental adaptability, can meet the high-precision calibration needs of UAVs in dynamic scenarios, and provides reliable technical support for accurate target positioning. Full article
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21 pages, 32230 KB  
Article
Structure-Aware Feature Descriptor with Multi-Scale Side Window Filtering for Multi-Modal Image Matching
by Junhong Guo, Lixing Zhao, Quan Liang, Xinwang Du, Yixuan Xu and Xiaoyan Li
Appl. Sci. 2026, 16(6), 3018; https://doi.org/10.3390/app16063018 - 20 Mar 2026
Viewed by 31
Abstract
Traditional image feature matching methods often fail to achieve satisfactory performance on multimodal remote sensing images (MRSIs), mainly due to significant nonlinear radiometric distortion (NRD) and complex geometric deformation caused by different imaging mechanisms. The key to successful MRSI matching lies in preserving [...] Read more.
Traditional image feature matching methods often fail to achieve satisfactory performance on multimodal remote sensing images (MRSIs), mainly due to significant nonlinear radiometric distortion (NRD) and complex geometric deformation caused by different imaging mechanisms. The key to successful MRSI matching lies in preserving high-frequency edge structures that are robust to geometric deformation, while overcoming nonlinear intensity mappings induced by NRD. To address these challenges, this paper proposes a novel high-precision matching framework, termed structure-aware feature descriptor with multi-scale side window filtering (SA-SWF). The proposed framework consists of three stages: (1) an anisotropic morphological scale space is constructed based on multi-scale side window filtering to strictly preserve geometric edges, and feature points are extracted using a multi-scale adaptive structure tensor with sub-pixel refinement to ensure high localization precision; (2) a structure-aware feature descriptor is constructed by integrating gradient reversal invariance and entropy-weighted attention mechanisms, rendering the multi-modal description highly robust against contrast inversion and noise; and (3) a coarse-to-fine robust matching strategy is established to progressively refine correspondences from descriptor-space matching to strict sub-pixel geometric verification, thereby minimizing alignment errors. Experiments on 60 multimodal image pairs from six categories, including infrared-infrared, optical–optical, infrared–optical, depth–optical, map–optical, and SAR–optical datasets, demonstrate that SA-SWF consistently outperforms seven state-of-the-art competitors. Across all six dataset categories, SA-SWF achieves a 100% success rate, the highest average number of correct matches (356.8), and the lowest average root mean square error (1.57 pixels). These results confirm the superior robustness, stability, and geometric accuracy of SA-SWF under severe radiometric and geometric distortions. Full article
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11 pages, 3141 KB  
Communication
ZrGeTe4 Nanoparticles as a Saturable Absorber for Mode-Locked Operations at 1 and 1.55 µm
by Xinxin Shang, Nannan Xu, Mengyu Zong, Weiyi Yu, Linguang Guo, Guanguang Gao, Ziqi Zhang, Huanian Zhang and Lianzheng Su
Photonics 2026, 13(3), 305; https://doi.org/10.3390/photonics13030305 - 20 Mar 2026
Viewed by 34
Abstract
In the current paper, the nonlinear absorption characteristics and laser modulation performance of the ternary anisotropic semiconductor material ZrGeTe4 were successfully explored. The recovery time of the ZrGeTe4-PVA thin film was measured to be 5.74 ps by the pump–probe technology. [...] Read more.
In the current paper, the nonlinear absorption characteristics and laser modulation performance of the ternary anisotropic semiconductor material ZrGeTe4 were successfully explored. The recovery time of the ZrGeTe4-PVA thin film was measured to be 5.74 ps by the pump–probe technology. By employing ZrGeTe4 as a saturable absorber, a passive mode-locked Yb-doped fiber laser was demonstrated for the first time. In the 1 µm mode-locked operation, the central wavelength was 1031.29 nm, the pulse repetition rate was 24.85 MHz, and the pulse width was 786.3 ps. In an Er-doped fiber laser operating at a wavelength of 1561.10 nm, the pulse width was as short as 1.26 ps with a repetition rate of 4.38 MHz. The results show that ZrGeTe4 has excellent broadband nonlinear optical characteristics. Full article
(This article belongs to the Special Issue Advancements in Ultrafast Laser Science and Technology)
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16 pages, 7174 KB  
Article
Aberration-Conditioned Attention-Driven Centroid Localization: From Simulation Mechanism to Double-Spot Experiment
by Zhonghao Zhao, Jia Hou, Yuanting Liu, Anwei Liu and Zhiping He
Photonics 2026, 13(3), 304; https://doi.org/10.3390/photonics13030304 - 20 Mar 2026
Viewed by 13
Abstract
In size, weight, and power (SWaP)-constrained optical systems, such as spaceborne LiDAR, high-precision centroid localization often relies on focal-plane measurements without dedicated wavefront sensors. Under such conditions, the nonlinear coupling between optical aberrations and sensor noise introduces systematic bias that is difficult to [...] Read more.
In size, weight, and power (SWaP)-constrained optical systems, such as spaceborne LiDAR, high-precision centroid localization often relies on focal-plane measurements without dedicated wavefront sensors. Under such conditions, the nonlinear coupling between optical aberrations and sensor noise introduces systematic bias that is difficult to mitigate using conventional centroiding methods. To address this issue, we propose a physics-conditioned feature correction framework based on an aberration-conditioned attention mechanism. A hybrid CNN–Transformer architecture is employed to predict and compensate for systematic centroid bias. Specifically, convolutional layers encode the degraded spot morphology, while a multi-head attention mechanism leverages Seidel aberration coefficients to adaptively modulate spatial features for precise regression. Given the unavailability of absolute ground-truth coordinates in empirical scenarios, a physics-consistent simulation framework based on scalar diffraction theory is constructed to generate synthetic data for supervised learning. Simulation results indicate that the proposed method objectively reduces anisotropic systematic bias, achieving a localization root-mean-square error (RMSE) of 0.011 to 0.021 pixels, and maintains stable sub-pixel accuracy even under a 10% empirical prior perturbation. To evaluate generalization performance and engineering reliability, a wedge-based double-spot platform is developed to verify physical consistency via geometric invariance. Experimental results demonstrate a measured spacing standard deviation (SD) of 0.015 to 0.039 pixels. This validates the framework’s transferability from theoretical simulation to controlled physical measurements, providing an algorithmic foundation for precision optical metrology in hardware-constrained environments. Full article
(This article belongs to the Special Issue Advancements in Optics and Laser Measurement)
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17 pages, 4195 KB  
Article
Design and Implementation of a Low-Noise Analog Front-End Circuit for MEMS Capacitive Accelerometers
by Keru Gong, Jiacheng Li, Xiaoyi Wang, Huiliang Cao and Huikai Xie
Micromachines 2026, 17(3), 378; https://doi.org/10.3390/mi17030378 - 20 Mar 2026
Viewed by 77
Abstract
This paper presents a low-noise analog front-end (AFE) integrated circuit (IC) circuit for capacitive micro-electromechanical system (MEMS) accelerometers that can be used for optical image stabilization (OIS) in various optical imaging systems. The AFE circuit design features a fully differential chopper stabilization technique [...] Read more.
This paper presents a low-noise analog front-end (AFE) integrated circuit (IC) circuit for capacitive micro-electromechanical system (MEMS) accelerometers that can be used for optical image stabilization (OIS) in various optical imaging systems. The AFE circuit design features a fully differential chopper stabilization technique that efficiently minimizes low-frequency 1/f noise and parasitic coupling. The AFE circuit chip is fabricated in a 0.18 μm complementary metal-oxide-semiconductor (CMOS) technology and co-packaged with an x-axis capacitive MEMS accelerometer based on a silicon-on-glass (SOG) process. The SOG accelerometer has a footprint of 1000 μm × 950 μm. The packaged system demonstrates a sensitivity of 342 mV/g and a nonlinearity of 1.1% between −1 g and +1 g, a dynamic range of 88 dB, and an equivalent noise floor of 14 μg/Hz. Full article
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19 pages, 331 KB  
Article
Symmetry Transformations of a Nonlinear Model of Optical Wave Transmission
by Jean-Claude Ndogmo, Emmanuel Mayombo Mbala and Mensah Kekeli Folly-Gbetoula
Axioms 2026, 15(3), 231; https://doi.org/10.3390/axioms15030231 - 20 Mar 2026
Viewed by 8
Abstract
The full symmetry group is found for a system of nonlinear schrödinger equations describing the propagation of optical pulses in an isotropic media. It is shown, in particular, that the six-dimensional symmetry group found is composed of a scaling transformation and a rotation [...] Read more.
The full symmetry group is found for a system of nonlinear schrödinger equations describing the propagation of optical pulses in an isotropic media. It is shown, in particular, that the six-dimensional symmetry group found is composed of a scaling transformation and a rotation of the four-dimensional space, thereby proving that the symmetry group preserves the shape of solutions. A symmetry classification of one-dimensional subalgebras of the Lie algebra is performed and yields, in particular, the symmetry reduction to the most general system of equations satisfied by the solitary waves of the equation. Explicit soliton solutions of the equation are found by largely autonomous technics. The found solitons are used to recursively generate two new ones by means of two iterations using the symmetry group. Other properties of the system are also highlighted, as well as the possible connections between the theories of symmetry groups and Darboux transformations inspired by this study. Full article
(This article belongs to the Section Mathematical Analysis)
14 pages, 2274 KB  
Article
Ruthenium Materials: Synthesis, Characterization, Optical, Antioxidant, and Anticancer Applications
by Sampath Krishnan, Anusha Karunakaran, Nagoor Meeran Mohamed Ibrahim, Sampath Gayathri, Jong Hun Han and Paulraj Arunkumar
Processes 2026, 14(6), 947; https://doi.org/10.3390/pr14060947 - 16 Mar 2026
Viewed by 203
Abstract
The technological promise of nonlinear optical (NLO) compounds has stimulated intense interest in optoelectronic devices, data storage, photonics, and anticancer therapy. Thiosemicarbazone ruthenium materials are of growing interest because of their tunable ligand framework and coordination sphere, allowing fine control over geometry, electronics, [...] Read more.
The technological promise of nonlinear optical (NLO) compounds has stimulated intense interest in optoelectronic devices, data storage, photonics, and anticancer therapy. Thiosemicarbazone ruthenium materials are of growing interest because of their tunable ligand framework and coordination sphere, allowing fine control over geometry, electronics, and functional properties. Here, we report an N-substituted salicylaldehyde thiosemicarbazone ligand and a series of octahedral Ru(III) complexes bearing triphenylphosphine or triphenylarsine and halide (Cl, Br) co-ligands. The complexes were characterized by elemental analysis, FT-IR, UV–Vis, EPR, mass spectrometry, and magnetic susceptibility measurements, which together confirm NS-chelation to a low-spin Ru(III) center in a distorted octahedral environment. Their photophysical and NLO responses were assessed by UV–Vis spectroscopy and powder second-harmonic generation measurements (Kurtz–Perry method), revealing promising NLO behavior. In parallel, antioxidant activity and in vitro anticancer effects against HeLa cells were evaluated by 2,2-diphenyl-1-picrylhydrazyl (DPPH) radical-scavenging and 3-(4,5-dimethylthiazol-2-yl)-2,5-diphenyltetrazolium bromide (MTT) cytotoxicity assays. These results provide insight into ligand-controlled structure–activity relationships, in which the halide (Cl/Br) and ancillary triarylphosphine co-ligands regulate electronic interactions and lipophilicity and ultimately increase biological performance, underscoring the dual materials and medicinal potential of these Ru(III) complexes. Full article
(This article belongs to the Section Materials Processes)
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25 pages, 8047 KB  
Article
On the Numerical Reliability of Lyapunov-Based Chaos Analysis in Optically Injected Semiconductor Lasers: A Phasor-Quadrature Comparison
by Gerardo Antonio Castañón Ávila, Ana Maria Sarmiento-Moncada, Alejandro Aragón-Zavala and Ivan Aldaya Garde
Appl. Sci. 2026, 16(6), 2835; https://doi.org/10.3390/app16062835 - 16 Mar 2026
Viewed by 155
Abstract
Lyapunov-exponent-based diagnostics are widely used to quantify deterministic chaos in optically injected semiconductor lasers (OISLs). In most numerical implementations, the optical field is represented either in phasor coordinates (A,ψ,N) or in Cartesian quadrature coordinates [...] Read more.
Lyapunov-exponent-based diagnostics are widely used to quantify deterministic chaos in optically injected semiconductor lasers (OISLs). In most numerical implementations, the optical field is represented either in phasor coordinates (A,ψ,N) or in Cartesian quadrature coordinates (X,Y,N). Although these representations are mathematically related through a smooth coordinate transformation away from vanishing field amplitude, their numerical realizations can exhibit markedly different robustness in variational calculations, directly impacting the reliability of Lyapunov exponent estimation and chaoticity maps. In this work, we present a systematic assessment of the numerical reliability of Lyapunov-based chaos analysis in master-slave optically injected semiconductor lasers using both phasor and quadrature formulations. The full Lyapunov spectrum was computed via a noise-free variational method that integrates the nonlinear dynamics together with the corresponding Jacobian equations using a fourth-order Runge-Kutta scheme combined with periodic QR orthonormalization. High-resolution Lyapunov maps were constructed in the injection strength-frequency detuning parameter space, and the consistency between both formulations was quantitatively evaluated. While both approaches reproduce the overall structure of chaotic and non-chaotic regions, the phasor formulation may generate spurious positive Lyapunov exponents in regimes where the optical field amplitude approaches low values. These discrepancies originate from singular terms proportional to 1/A and 1/A2 in the variational Jacobian of the phasor model, which can lead to numerical amplification and artificial chaotic signatures. The quadrature formulation avoids these singularities and provides numerically stable and physically consistent Lyapunov spectra across the explored parameter space. The results establish practical guidelines for robust chaos quantification in optically injected semiconductor lasers and highlight the importance of representation choice in variational Lyapunov analysis of nonlinear photonic systems. Full article
(This article belongs to the Special Issue Advances in Optical Communication and Photonic Integrated Devices)
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17 pages, 2515 KB  
Article
Temperature Evolution of Crystal Structure, Ferroelectricity and Ionic Conductivity of Ca9La(VO4)7
by Oksana V. Baryshnikova, Bogdan I. Lazoryak, Vladimir A. Morozov, Sergey Yu. Stefanovich, Alexander V. Mosunov, Eldar M. Gallyamov, Sergey M. Aksenov and Dina V. Deyneko
Molecules 2026, 31(6), 984; https://doi.org/10.3390/molecules31060984 - 15 Mar 2026
Viewed by 216
Abstract
The properties of a Ca9La(VO4)7 single crystal were studied using dielectric spectroscopy and second-harmonic generation. The crystal structure of Ca9La(VO4)7 grown using the Czochralski technique was refined using single-crystal data. The distribution of [...] Read more.
The properties of a Ca9La(VO4)7 single crystal were studied using dielectric spectroscopy and second-harmonic generation. The crystal structure of Ca9La(VO4)7 grown using the Czochralski technique was refined using single-crystal data. The distribution of Ca2+ and La3+ cations over structural positions was determined. The crystal structure refinement results were compared with those obtained previously from powder X-ray diffraction data. It was shown that the refinement carried out using two different data sets leads to approximately the same results for the distances in the polyhedra, but their distortion is significantly less in the case of using single-crystal data for calculation. Dielectric properties and conductivity measurements were performed on polished single-crystal wafers cut parallel and perpendicular to the c axis. Second-harmonic generation and dielectric temperature measurements revealed the presence of a reversible ferroelectric first-order phase transition at about 1224 K from the ferroelectric β-phase (space group R3c) to the paraelectric β′-phase. The ferroelectric–paraelectric phase transition is accompanied by a complex structural rearrangement, including a 60° rotation of the V1O4 tetrahedron, as well as slight displacements of the Ca2+ and La3+ cations. It has been shown that the conductivity differs only slightly along the polar axis and perpendicular to it. Above the phase transition temperature, the activation energy of the conductivity is the same for all directions, Ea~1.2 eV. The influence of composition on the phase transition temperature and the formation of ferroelectric and nonlinear optical properties is discussed. Full article
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16 pages, 4714 KB  
Article
Metasurface-Enabled Dual-Channel Optical Image Authentication Based on Polarization Multiplexing
by Yanfeng Su, Biao Zhu, Wenming Chen, Ruijie Xue, Zijing Li, Zhijian Cai, Qibin Feng and Guoqiang Lv
Photonics 2026, 13(3), 280; https://doi.org/10.3390/photonics13030280 - 15 Mar 2026
Viewed by 153
Abstract
In this paper, a metasurface-enabled dual-channel optical image authentication based on polarization multiplexing is proposed. During encryption, authentication phases corresponding to dual-channel plaintext images are firstly calculated by using a sparse-constraint-driven authentication-holography (SCDAH) algorithm. Then, target transmission phase and geometric phase of metasurface [...] Read more.
In this paper, a metasurface-enabled dual-channel optical image authentication based on polarization multiplexing is proposed. During encryption, authentication phases corresponding to dual-channel plaintext images are firstly calculated by using a sparse-constraint-driven authentication-holography (SCDAH) algorithm. Then, target transmission phase and geometric phase of metasurface to be designed are obtained accordingly by the composite phase modulation (CPM) principle. Next, the nanopillar-type metasurface unit is performed with parameter scanning to establish the transmission and geometric phase databases. Finally, the structural parameters of each nanopillar are determined on a pixel-by-pixel basis to complete the construction of polarization-multiplexing authentication metasurface (PMAM). During authentication, the PMAM are respectively illuminated by the left-handed circularly polarized (LCP) and right-handed circularly polarized (RCP) light to obtain pseudo-random images produced by far-field diffraction, and then the nonlinear correlation distribution between diffraction image and corresponding channel plaintext image is calculated, and the final authentication result of each channel is determined based on whether the signal-to-noise ratio of the nonlinear correlation distribution meets the standard. In fact, a new physical-characteristic-driven dual-channel optical image authentication technology is formed, where double identities of the user holding this PMAM can be simultaneously verified, breaking through the rigid constraint of conventional single metasurface-to-single image, meanwhile improving the capacity and efficiency for authentication metasurface from the perspective of physical mechanism. Numerical simulations are performed to demonstrate the feasibility of the proposed method, and the simulation results prove that the proposed method exhibits high feasibility and security as well as strong robustness against cropping attack, showing a promising application potential in the field of identity recognition and authentication. Full article
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6 pages, 1246 KB  
Short Note
Synthesis, Structural Characterization, and SHG Behavior of a Lanthanum/β-d-Fructose-Based Metal–Organic Framework
by Domenica Marabello and Paola Benzi
Molbank 2026, 2026(2), M2151; https://doi.org/10.3390/M2151 - 13 Mar 2026
Viewed by 147
Abstract
Interest in non-centrosymmetric crystalline materials exhibiting second harmonic generation (SHG) has increased due to their potential applications in optical sensing and biosensing. Saccharide-based metal complexes are particularly attractive systems, as chiral sugars can promote non-centrosymmetric crystal packing. In this work, a new lanthanum–β- [...] Read more.
Interest in non-centrosymmetric crystalline materials exhibiting second harmonic generation (SHG) has increased due to their potential applications in optical sensing and biosensing. Saccharide-based metal complexes are particularly attractive systems, as chiral sugars can promote non-centrosymmetric crystal packing. In this work, a new lanthanum–β-d-fructose compound, [La(C6H12O6)(H2O)5]Cl3 (LaFRUCl), was synthesized using a simple and low-cost method and characterized by single-crystal X-ray diffraction. The compound crystallizes in the orthorhombic space group P212121 and consists of infinite (La3+–fructose)n chains extending along the [001] direction, forming a one-dimensional Metal–Organic Framework. The nonlinear optical response was evaluated using the Kurtz–Perry powder technique with a Nd:YAG laser (1064 nm) and compared to a sucrose reference. The measured SHG efficiency is comparable to that of previously reported alkaline earth metal–sugar analogs. While the compound’s SHG emission is significant, evaluation of its structural stability under aqueous or physiological conditions is be required before considering biological applications. Full article
(This article belongs to the Section Structure Determination)
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11 pages, 8363 KB  
Article
Ultrafast Optical Analysis and Control of Spectral Flatness in Cavity-Less Electro-Optic Combs
by Xin Chen, Hongyu Zhang, Meicheng Fu, Huan Chen, Yi Zhang, Yao Xu, Mengjun Zhu, Wenjun Yi, Qi Yu, Junli Qi, Qi Huang, Yubo Luo and Xiujian Li
Micromachines 2026, 17(3), 350; https://doi.org/10.3390/mi17030350 - 12 Mar 2026
Viewed by 216
Abstract
The cavity-less electro-optic combs (EOCs), recognized for exceptional tunability, stability and high power, are a crucial enabler for the fields such as optical communications, precision measurement and metrology, and microwave photonics. This work systematically investigates the fundamental physical factors that govern the spectral [...] Read more.
The cavity-less electro-optic combs (EOCs), recognized for exceptional tunability, stability and high power, are a crucial enabler for the fields such as optical communications, precision measurement and metrology, and microwave photonics. This work systematically investigates the fundamental physical factors that govern the spectral flatness via ultrafast measurements and modeling simulations. The ultrafast analysis results demonstrate that, the finite effective modulation extinction ratio of the electro-optic intensity modulators will result in generation of coherent spectral components with identical frequencies but varying phases and amplitudes in ultrashort temporal scale, finally lead to remarkable spectral interference and further intensity fluctuations across the combs spectrum. Furthermore, the established mathematical relationship between the spectral flatness and the modulation extinction ratio of the intensity modulators exhibits a nonlinear dependence up to the third order. Cascading intensity modulators has been exploited to mitigate the spectral interference and improve the modulation extinction ratio, which has been verified by using home-made high sensitive autocorrelator and frequency-resolved optical gating (FROG), and finely spectral flatness of 0.54 dB among 11 lines has been achieved, which recognized for the first time that modulation extinction ratio related spectral interference phenomenon play a subtle role in EOCs generation. Furthermore, photonic analog-to-digital converters (PADCs) have been investigated and an obvious enhancement in signal-to-noise-and-distortion (SINAD) is achieved, These findings will provide crucial theoretical and experimental support for optimizing EOCs performance, and advance the development and application. Full article
(This article belongs to the Special Issue Advanced Optoelectronic Materials/Devices and Their Applications)
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23 pages, 1246 KB  
Article
Accuracy of Fiber Propagation Evaluation Using Phenomenological Attenuation and Raman Scattering Models in Multiband Optical Networks
by Giuseppina Maria Rizzi and Vittorio Curri
Network 2026, 6(1), 16; https://doi.org/10.3390/network6010016 - 12 Mar 2026
Viewed by 152
Abstract
The constant growth of IP data traffic, driven by sustained annual increases surpassing 26%, is pushing current optical transport infrastructures towards their capacity limits. Since the deployment of new fiber cables is economically demanding, ultra-wideband transmission is emerging as a promising cost-effective solution, [...] Read more.
The constant growth of IP data traffic, driven by sustained annual increases surpassing 26%, is pushing current optical transport infrastructures towards their capacity limits. Since the deployment of new fiber cables is economically demanding, ultra-wideband transmission is emerging as a promising cost-effective solution, enabled by multi-band amplifiers and transceivers spanning the entire low-loss window of standard single-mode fibers. In this scenario, an accurate modeling of the frequency-dependent fiber parameters is essential to reliably model optical signal propagation. In particular, the combined impact of attenuation variations with frequency and inter-channel stimulated Raman scattering (SRS) fundamentally shapes the power evolution of wide wavelength division multiplexing (WDM) combs and directly affects nonlinear interference (NLI) generation, as well as the amount of ASE noise. In this work, we review a set of analytical approximations, based on phenomenological approaches, for frequency-dependent attenuation and Raman scattering gain, and analyze their impact on achieving an effective balance between computational efficiency and physical fidelity. Through extensive analyses performed with the open-source software GNPy (version 2.12, Telecom Infra Project) on an optical line system exploring multi-band scenarios spanning C+L+S, C+L+E, and U-to-E transmission, we demonstrate that the proposed approximations reproduce the reference SRS power evolution and NLI profiles with root mean square errors (RMSEs) consistently below 0.03 dB, and down to the 10−3–10−2 dB range for the most accurate configurations. Although the current implementation does not yet provide a direct reduction in computational time, the proposed framework lays the groundwork for future developments toward closed-form or semi-analytical solutions, enabling more efficient modeling and optimization of ultra-wideband optical transmission. Full article
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