To determine the velocity of a particle during transportation by airlift pump, three variable parameters were considered: submergence ratio S
r, type of particle, and air flow rate Q
a. According to the results of two-phase flow (see
Figure 2), in this study, submergence ratios 0.7, 0.8, and 0.89 were considered to have more water velocity with the least amount of injecting air. Based on the data presented in
Figure 2, it is obvious that the airlift worked, as the Reynolds number (Re) varied from 6 × 10
3 to 1.4 × 10
5. Therefore, the vertical transport of the solid particle was in accordance with the turbulent flow conditions (laminar flow Re-Number is lower than 2300).
3.1. Flow Regimes
In terms of influent air flow rate (Q
a), different regimes of two-phase flow (gas-liquid) may be distinguished in the following order (
Figure 3): bubbly, slug, churn, annular, and dispersed flow regimes [
10]. The lack of same criterion for interpreting the flow behavior and the diversity of empirical results on different pumps led to a non-uniform agreement on the classification and illustration of upward two-phase flow boundaries and exposure to different two-phase upflow maps by researchers. Miller and Cain [
11] examined the influence of solid particles on vertical three-phase flow transitions. They concluded that solid particles accelerate the transitions of flow from bubble to slug flow and do not play an effective role in transitions of flow from the slug to churn flow. Therefore, the two-phase flow map presented by Taitel et al. [
12] is applicable for our experimental conditions.
Figure 4 shows the boundaries for different two-phase flow transitions together with our two-phase experimental results. Unlike other researchers whose results cover only certain dimensions of the pump, Taitel et al. [
12] presented a flow map based on the relationship between the pipe length and diameter (L/D). To find the transition zone from slug to churn, given the dimensions of the riser pipe in our test, this ratio is equal to 60, which stands between graph 50 and 100. It should be noted that in accordance with the environmental conditions of the experiments, the boundary of the transition flow from the churn to the annular is considered when the Kutateladze number is equal to 3.1 (V
air = 5.78 m/s). Therefore, from the observations in
Figure 4, it is also evident that our experiments are done in bubble, slug, and churn flow regime.
3.2. Particle Velocity
Since the focus of this work was on measuring the velocity of a particle pumped by an airlift, it was obtained by dividing the total length of the vertical tube through which the particle has travelled over time (V
p = (h
s + h
r)/t
i). For different measurement conditions, the arithmetic mean of velocity was calculated.
Figure 5 shows the correlation between the air velocity and solid lifting velocity for particles P
S, P
H, and P
C at a submergence ratio of 0.8. In
Figure 5, the starting point of each diagram corresponds to the amount of air required to reach the vertical velocity of the water, which is slightly higher than the settling velocity of the particle falling into the still water. Therefore, by injecting less compressed air than this amount, the particle cannot be sucked and pumped to a higher level. The vertical bold line in
Figure 5 corresponds to the transition zone from slug to churn flow. Beyond the type of flow regime, the velocity of a particle was increased by raising the velocity of the inlet air. This stepwise increment was more significant for coal, as it has a higher volume and lower density than the other glass particles.
Owing to the high speed of a transported particle and its severe impact on the separator tank wall, it was possible to destroy the particle and change its usual shape. Hence, the experiment could not be continued for annular flow regime.
Figure 5 also depicts that with increasing compressed air injection, the amplitude of velocity oscillations (vertical particle transporting time) enhance until it reaches the highest in the churn flow regime. In terms of the position of each phase inside the tube, the churn flow regime is very similar to the annular flow, where the main liquid phase is close to the wall of the pipe and large cores of gas are located in the middle. This condition raises the collision of the solid particle with the pipe wall, in which the irregular particles have a less chance of rolling on the wall and the friction caused by the collisions will definitely cause fluctuations in the particle transporting time. It can be concluded that the more irregular the shape of the particle, the greater the transporting velocity oscillation.
Due to the significant difference between the density of the gas and the liquid, the particles in the gas settle much faster than the liquid. Therefore, some researchers have argued that the water phase carries the solid particle and air has no contribution in vertical transportation [
5,
13,
14]. It should be noted that they monitored the state of small solid particles transportation in the range of bubble and slug flow. This point of view is in sharp contradiction with our empirical outcomes in the churn flow regime, which are displayed in
Figure 5. As seen in this figure, by increasing the velocity of inlet air by more than 2.4 m/s, the velocity of the liquid phase is almost constant and does not change much, but all types of particles still show an increase in velocity. Therefore, the above assumption in the already mentioned study does not hold true, and air also participates in carrying the particle upwards in the churn flow regime.
In addition, simultaneous comparison of two glass particles (PS and PH) indicate that the drag coefficient in a low amount of incoming air in the churn flow regime is an effective parameter for faster particle transfer, while on increasing the amount of influent air, the effect of this case gradually minimizes and eventually the spherical and half-spherical particles are transported upwards at the same velocity. The cause of such an event still needs more research to better determine the orientation of the particles in high air flow and clarify the interaction between the three phases.
3.3. Effect of Submergence Ratio
The results of practical experiments for spherical particle (Ps) with three submergences ratios (S
r) along with water velocity are presented in
Figure 6. As can be seen from the three curves in
Figure 6, the relation between solid particle velocity and submergence ratios has a similar trend for round glass particles. At a constant air rate, the vertical velocity of the solid transportation rises with an increase in the submergence ratio. The starting point of vertical pumping of the particle is found to be different for each submergence ratio, and it moves to the right of the horizontal coordinate as the submergence ratio decreases from 0.89 to 0.7. Regardless of submergence level, the P
S particle always initiates movement whenever the velocity of water reaches around 1.4 m/s. It is quite clear that the maximum solid velocity does not belong to the time when we have the maximum velocity of displaced water.
At submergence ration equal to 0.7, in terms of particle velocity transfer, it can be inferred that in low incoming air velocity, 0.3–2.8 m/s, the most energy of compressed air is spent on vertical water pumping rather than on solid particles, which this role completely changes when the air velocity exceeds 2.8 m/s. Similar conditions are observed for the submergence ratios of 0.8 and 0.89 in
Figure 6. The only difference is that at higher submergence ratios, the solid reaches considerable velocity, even with just a lower amount of compressed air. By increasing the submergence ratio from 0.7 to 0.89, while the amount of injected air is the same, the particle transfer velocity can be increased up to three times. These results emphasize that the solid particle can move upwards faster if the amount of incoming air or the submergence ratio is increased. In general, under certain air velocity conditions, it is necessary to have a suitable water height to achieve the highest particle transfer velocity with the least amount of compressed air.
3.4. Theoretical Background
Unfortunately, there is no information in the accessible scientific and technical literature related to one solid particle movement in a vertical multiphase flow. To validate our results, we used the existing empirical correlations together with theoretical equations related to multiphase flow. In airlifts that use the radial air injection method (air-jacket), the process of transporting one solid particle should be divided into two parts: (1) moving the particle in a liquid (suction pipe) and (2) the area after the injection of compressed air, where the solid phase moves with a mixture of air and water. To better distinguish these sections, index ‘i’ was defined as follows: i = 1, if the solid particle is ambient in the water (suction pipe); i = 2 if the particle stands in the air–water mixture (riser pipe).
Assuming that the density of solid and fluid particles is not the same, due to the action of gravity, the velocity of the particles in the carrier fluid is less than the velocity of the fluid [
15]:
where V
S is the velocity of solid phase (m/s), V
f is the average velocity of fluid phase (m/s), and V
T is the terminal settling velocity of one solid particle falling in the center of the pipe with still water (m/s), determined by the following equation:
where v
P is the volume of solid particle (m
3), g is the free fall acceleration (m/s
2), ρ
S and ρ
f are the densities (kg/m
3) of solid and fluid phase, respectively. C
D is drag coefficient of solid particle (-) and A
C denotes the cross-section area of the particle in perpendicular to the direction of motion. In the literature, an ideal sphere is often assumed for calculating the volume and area of solid particles. Although the actual shapes of solids can be very different, there are several methods to estimate the geometry of non-spherical particles, such as equivalent volume diameter, angularity, and sphericity approaches; a detailed explanation of the procedure can be found in Reference [
16].
It is worth noting that the density of the air–water mixture (ρ
2) is strongly dependent on the ratio of each of the phases, which is known as the void fraction (α). It is highly unlikely that one correlation can estimate void fraction for the entire range of vertical flow regimes. For this aim, among the studies published in the literature, the equations proposed by Nicklin et al. [
17] for range of slug flow [Equation (3)] and Hasan [
18] for Churn flow [Equation (4)] are considered for vertical two-phase flow:
where, j
g and j
w are the superficial velocity of gas and water, respectively. D is the pipe diameter, ρ
G and ρ
w are the densities of gas and water, respectively. The density of the gas-phase at the level of gas-injection can be determined using the following relation as:
By ignoring the volume of one solid particle compared to the volume of air and water, the density of fluid in the raiser pipe can be determined according to the equation proposed by Fujimoto et al. [
19] as:
in which α
w denotes the volumetric fraction of water in the riser pipe. Assuming the motion of a particle and a fluid are in the same direction, the velocity of the solid for the individual phases, (i = 1, 2), derives from Equation (1):
where V
S1 and V
S2 (m/s) are the velocities of solid particle in water and air–water flow, respectively. Note that if the velocity of the particle falling into the fluid is greater than the velocity upward of the fluid, the result of the calculation will be a negative value. In this case, the solid velocity is considered zero. The average velocity of a solid particle in transporting an airlift pipe with a total length of h (see
Figure 1) can be determined as:
where h
s and h
r (m) are the length of the suction and riser pipe, respectively. t
1 denotes the time spent for transporting the particle from the entrance of the suction pipe to the height h
s, t
2 is the time needed for the particle to pass the riser pipe with a length of h
r. Assuming the particle does not collide with the pipe wall, the following relationship is easily derived:
By combining Equations (10) and (11), we can write:
By substituting Equations (2) and (7–9) in Equation (12), the final form can be written as follows:
3.5. Validity of Meagerd Data
Experimental data are now evaluating with the Equation (13). So far, different empirical equations have been proposed to estimate the drag coefficients of spherical and non-spherical isometric particles, and the final answer varies. A drag coefficient of the sphere particle was calculated from the equation provided by Ferguson and Church [
20]. The obtained value was equal to 0.44. The drag coefficient, especially for non-spherical particles, can affect the accuracy of velocity evaluation. The lack of a comprehensive correlation and the variability of the experimental results led to inconsistent agreement among the researchers when calculating the drag coefficient for irregular-shaped particles. Based on the temperature and pressure of the test medium, the drag coefficients for particles P
H and P
C were determined experimentally. The settling time of the particles in the still water was measured 50 times in a tube with a diameter of 40 cm, and average drag coefficients are equal to 1.01 and 0.426, respectively.
The values predicted by Equation (13), together with the experimental points for S
r equal to 0.8, are plotted in
Figure 7a–c. The vertical bold line in
Figure 7a–c indicate the point that the flow regime is transient from slug to churn flow. Many researchers have tried to offer the best and optimum working condition for an airlift that can be used for solid transportation. Deendarliantoa et al. [
8] in a study on the transport of sand and coal with a maximum size of 0.8 mm concluded that the appropriate flow regime for pumping these particles is slug flow. The results of our study confirmed that when the slug flow is maintained in the airlift, the velocity of the water in the suction pipe is insufficient to suck even a particle in centimetres, let alone carry it to the end of the riser pipe. According to research by Pougatch and Salcudean [
21], the transition in the type of flow can be delayed by breaking up large bubbles after they collide with solid particles. Therefore, the optimal flow regime is highly dependent on the operating conditions of this type of pump.
Based on the data presented in
Figure 7a, the computation result with Equation (13) had the same slope as the experimental data and was not too far off from the values for spherical particle (P
S); hence, agreement between the experimental data and theoretical calculation is good, except in the early stage of churn flow, where trends in the calculating suggest a transporting velocity lower than is examined.
A lower velocity estimation was also observed for particles P
H and P
C. As is clear from the theory part, the density of the air–water mixture along with its velocity play an important role in estimating the vertical velocity of a particle. They can be well estimated when the ratio of air volume to water volume in the riser tube is correctly determined. The reason for small deviation between the predicted and average measured velocity for particles may be related to the accuracy of the equation, as developed by Hasan [
18] to apprise the void fraction in the churn flow regime.
For particles P
H and P
C, the values calculated by the formula in the high air flow range often correspond to the maximum velocity obtained in practical experiments, which can be attributed to several factors. In vertical pumping, one particle moves in the center of the suction pipe, because this area has the highest vertical velocity compared to the surrounding, but in the lift tube, the velocity distribution does not always follow a same pattern so that with the onset of churn flow, the liquid phase is distributed axisymmetric around the perimeter of the tube, where the center of the pipe is occupied by a large gas core. We assumed that solid-free flow occurred without any collision with the pipe wall, but with the further development of churn flow due to increased air injection, this assumption is sometimes unrealistic, especially for large and irregular particles, which cause a deceleration. Moreover, the water flow in churn flow is not always upwards and sometimes moves in the opposite direction of main air flow [
22]. Therefore, this may lead to irregular particle rotation and impair the estimation of the largest particle area during upward motion. Therefore, for irregularly shaped particles, it is highly recommended to use the average drag coefficient in the formula, which is obtained from the main faces of the particle.
The difference between theoretical and practical results can also be attributed to the indirect motion of the particle. In a study by Yoshinaga et al. [
23], the zigzag motion of a particle was noted while it was moving upward in a mixture of air and water. Hence, the particle trajectories in the vertical plane may enhance the transportation time, which in turn diminishes the velocity of practical measurement.