1. Introduction
Heat transfer is an essential component in nearly all industrial processes [
1,
2,
3,
4,
5]. Consequences of improper heat transfer include nonreproducible processing conditions and lower product quality. Straight tube heat exchangers are the most common type of heat exchanger used in industrial processes due to ease of manufacturing and lower cost [
1]. There are several experimental works available in the literature that study forced convective heat transfer in nanofluids as it continues to be a subject of growing importance in many applications [
2,
3,
4,
5,
6,
7,
8,
9,
10,
11,
12,
13,
14,
15,
16,
17,
18,
19]. A straight tube heat exchanger with laminar flow condition has a lower heat transfer coefficient (HTC) as compared to turbulent flow conditions. Conventional heat transfer fluids such as water, ethylene glycol, and engine oil have relatively low thermal conductivity values, which thus limit the heat transfer rates. The heat transfer performance can be enhanced either by geometry perturbation or by the improvement of the fluid properties. The nanofluids are considered the next-generation heat transfer fluids because of the new possibilities (i.e., more heat transfer surface between particles and fluids, reduced pumping power to achieve equivalent heat transfer intensification, etc.) compared to pure liquids. The term nanofluids refers to a two-phase mixture composed of a continuous phase, usually a saturated liquid, and a dispersed phase constituted of extremely fine metallic particles of a size below 100 nm called nanoparticles.
It has been shown that the thermal properties of a nanofluid appear to be higher than those of the base fluid. Hence, nanofluids appear to be an interesting alternative for advanced thermal applications for microscale and nanoscale heat transfer. Alumina oxide nanoparticles (Al
2O
3) has been widely used for both experimental and numerical work [
20,
21,
22,
23,
24,
25,
26,
27,
28,
29,
30]. Wen and Ding [
20] developed a series of experiments using Al
2O
3-water nanofluids in a circular tube. They observed that the local HTC was enhanced by 47% using Al
2O
3 nanoparticles for
= 1.6%, in the laminar flow regime. Maïga et al. [
21] investigated Al
2O
3-water and Al
2O
3-ethylene glycol under constant heat flux boundary condition. The reported results show a 63% enhancement in HTC for
= 7.5%. Heris et al. [
22] studied the laminar convective heat transfer of CuO-water and Al
2O
3-water nanofluids flow in the straight tube and reported that the HTC increases with an increase in particle loading and a decrease in the particle size. The HTC was augmented by 40% for Al
2O
3-water at
= 2.5%. Anoop et al. [
23] conducted experiments using an aqueous solution of Al
2O
3-water in the developing region of a pipe flow to calculate the HTC considering the influence of particle size. The experimental results showed a 25% HTC enhancement for a 45-nm particle size and 11% for a 150-nm particle size. It was concluded that heat transfer enhancement was not only due to the intensification in thermal conductivity but also because of the effects of particle migration and thermal dispersion. Hwang et al. [
24] measured the pressure drop and convective heat transfer of water-based Al
2O
3 nanofluids flowing through a uniformly heated circular tube in the fully developed laminar flow regime. The experimental results showed that the HTC increases up to 8%, at
= 0.3% as compared to water.
Davarnejad et al. [
25] performed simulations to investigate the heat transfer characteristics of water-based Al
2O
3 nanofluid with
= 0.5%–2.5%, in a circular tube under constant heat flux and laminar flow conditions. It was reported that HTC enhanced marginally by 6% at
= 2.5%, as compared to the water. Kim et al. [
26] investigated the effect of nanofluids on convective heat transfer through a circular straight tube with constant heat flux condition under both the laminar and turbulent flow regimes. For Al
2O
3 nanofluids with
= 3%, the thermal conductivity and HTC increases by 8% and 20%, respectively. The enhancement of the convective HTC at the entrance region was due to the Brownian motion of the nanoparticles. Rea et al. [
27] investigated the laminar convective heat transfer and viscous pressure loss for Al
2O
3-water and ZrO
2-water nanofluids flow in a vertical heated tube. The HTC’s in the entrance and fully developed regions were found to be enhanced by 17% and 27%, respectively, for water-based Al
2O
3 nanofluid at
= 6%, as compared to the water. Purohit et al. [
28] studied the laminar forced convective heat transfer in a circular tube for three different nanofluids (Al
2O
3-water, ZrO
2-water and TiO
2-water). They reported that for the same Re comparison criteria, the HTC for nanofluids is found to be significantly higher (18%) as compared to the base fluid. Haghighi et al. [
29] investigated the heat transfer characteristics of a straight microtube for three different nanofluids (Al
2O
3-water, ZrO
2-water and TiO
2-water) under laminar condition (Re = 200–2200). For the nanofluids considered, the HTC was reported enhanced by 23% as compared to water. Salman et al. [
30] utilized a numerical method to investigate the convective heat transfer of nanofluids in microtube under constant heat flux with different types of nanoparticles (Al
2O
3, CuO, SiO
2 and ZnO) with different volume fractions ranged from 1% to 4% using ethylene glycol and water as a base fluid. The maximum heat transfer enhancement was 22%.
Table 1 shows a summary of the different nanofluids and their process parameters (Re, Pr and
) for convection heat transfer under laminar flow condition. The parameters were selected based on the potential of the nanofluids for their practical applications as studied by previous authors and presented in
Table 1. The highest Prandtl number and volume fraction of nanoparticles were 753 and
= 10%, respectively.
The extensive studies, both experimental and theoretical have been conducted to calculate the convective HTC of the nanofluids flow in straight tube. It is conclusive from the literature review that the HTC not only enhanced by the thermal conductivity but also due to the disturbances of thermal boundary layer caused by the Brownian motion of the nanoparticles. It may also be noted that there are only few studies with a wider range of nanoparticles and particle concentrations. This is mainly because the experimental analysis can be complicated for the wider range of the design parameters.
A considerable amount of research has been done on nanofluids over the past decade, the conclusions on their behavior, characteristics, and performances remain somewhat controversial. There is still lack of consistency in experimental values found in the literature [
18,
19] and challenges that need to be addressed and overcome before this new field of study can be fully established. It is imperative to conduct more investigations to properly quantify the effects of nanoparticles in heat transfer enhancement.
Therefore, in this study, the single-phase model was used for a wide range of nanofluid properties including three different base fluids with Prandtl numbers ranging from 6–500 and five different nanoparticles viz. Al2O3, TiO2, CuO, SiO2, and ZnO. The wide range of fluid properties enables the evaluation of the performance of convective heat transfer in a larger number of engineering applications that can benefit from a better understanding of the thermal enhancement of nanofluids. Furthermore, it is important to understand that the usefulness of nanofluids for heat transfer applications depends not only on the thermal conductivity but also on other transport properties, such as viscosity, and on thermodynamic properties, such as specific heats. The wide range of nanofluid properties will allow us to produce relevant Nu correlations, and more importantly, enable control by proper selection of particles and base fluids.
3. Results & Discussion
An extensive number of numerical simulations were performed to determine the HTC enhancement of laminar nanofluids. For validation purpose, the present results of the Nu for straight tube were compared with the correlation (
) of Maïga et al. [
21] and the computational results of Singh et al. [
48] for constant heat flux condition.
Figure 1a shows a good agreement of the present results with the literature [
21,
48] for water-based Al
2O
3 nanofluid at
= 1%. The Nu results were also validated for constant wall temperature condition as shown in
Figure 1b. It may be noted that there is a good agreement between the present results and results predicted by Maïga et al. [
21] (
), for the Al
2O
3-water based nanofluid with
= 4%.
In this study, six different cases with different combinations of the geometry, nanoparticles concentration and base fluids were considered as shown in
Table 6. It may be noted from
Table 6 that three different base fluids and five different nanofluids with a wide range of particle volume fractions (
) are considered for the detailed investigation.
3.1. Case 1: Water-Based Nanofluid in Straight Tube with Constant Heat Flux Using SPH
In the first case, water-based nanofluids with the constant wall heat flux (
= 10,000 W/m
2) were considered.
Figure 2 shows the results for the fluid temperature in the radial direction and the wall temperature at the constant values of Re = 500 and T
o = 293.15 K. It may be noted from
Figure 2a, that the fluid temperature decreases with an increase of the nanoparticle concentration from 0 to 10%, especially near the tube wall, suggesting a higher heat transfer rate (above 10%) with nanoparticles.
Figure 2b demonstrates the diminution of the wall temperature at different nanoparticle concentrations. The wall temperature decreases by 40 K for the Al
2O
3-water nanofluid with nanoparticle concentrations from 0 to 10%. The diminution in temperature reflects a better heat transfer rate at the tube wall. These effects may be explained by the fact that with the presence of the nanoparticles, the thermal properties of the resulting mixture have become more important as the product of
and the thermal conductivity have increase with respect to pure water.
Figure 3 shows the effect of nanoparticle concentration on the fluid mean temperature and wall temperature in axial direction. It may be noted from
Figure 3a that the fluid mean temperature decreases with an increase in the value of
. The decrease in the fluid mean temperature is caused mainly due to the higher thermal conductivity (up to 32%) of the Al
2O
3-water nanofluid. The radial, wall and fluid mean temperatures demonstrate that Al
2O
3-water nanofluid offers a higher thermal capacity as compared to the water. It may also be observed that at the higher thermal conductivity, the wall-to-fluid heat transfer is more important as it augments the heat transfer rate. Three nanoparticles (Al
2O
3, TiO
2 and CuO) with two different concentrations (
= 1% and
= 10%) were considered to investigate the thermal efficiency of the nanofluids with increase in the particle concentrations as shown in
Figure 3b.
For the higher nanoparticle concentration (
= 10%), the wall temperature for Al
2O
3-water nanofluid is lower than the TiO
2-water and CuO-water nanofluids. This lower temperature can be explained with the higher values of thermal conductivity which is 4% higher as compared to TiO
2-water and 1% higher as compared to CuO-water. The results revealed that Al
2O
3-water nanofluids will have a higher transfer coefficient (at least 1%) than the other two nanofluids considered. The nanoparticles concentration has effect on heat transfer performance. A larger number of nanoparticles in the base-fluid increases the thermal conductivity of the nanofluid but it is accompanied with higher values of the wall shear stress. Although, the use of nanofluids has heat transfer enhancement capabilities due to their increase viscosity, they will also increase friction/pressure losses. For example, Maïga et al. [
21] found that there is a 2.5-fold increase in the wall shear stress with a
= 5% for an Al
2O
3-water nanofluid. Because of the friction/pressure losses, the benefits of the higher transfer rates versus the corresponding and drastic increases in viscosity must be considered.
In this study, two different nanoparticle concentrations (
= 1% and
= 4%) of the water-based Al
2O
3 nanofluid were used to determine the effect of the nanoparticle concentration.
Figure 4 shows that the Nu increases with an increase in nanoparticle concentration for any given value of Re. This is mainly because the nanoparticles increase the thermal conductivity of the base fluid and, hence, augments the convective heat transfer. At low Re (below 100) the Nu is 2.2 times higher for
= 4% as compared to
= 1%. For high Re (above 1000) Nu increases less than 10%. Considering this reduction of Nu and the increases of the wall shear stresses using more than
= 5%, a higher nanoparticle concentration would have to be determined by the specific application.
Figure 5 shows a comparison of Nu for the different nanoparticles considered. Among the nanoparticles studied Al
2O
3, TiO
2, CuO, SiO
2, ZnO there is evidence that the Al
2O
3 nanofluid has a marginally higher value (by 4%) of Nu for the Al
2O
3-water based nanofluid as compared to the ZnO-water nanofluid. This enhancement in the Nu is relatively lower as the Pr of all the selected nanofluids are in the range of 6.7 to 7.3 at
= 4%. The Nu of SiO
2-water nanofluid was the second highest since SiO
2 nanofluid has the highest average velocity among the fluids because of the lowest value of density (ρ = 1046 kg/m
3). The result indicate that the fluid velocity plays a role on the heat transfer.
3.2. Case 2: Ethylene Glycol-Based Nanofluid in Straight Tube with Constant Heat Flux Using SPH
This case considers ethylene-glycol (EG)-based nanofluids with equal parameters as previous case for comparison purposes.
Figure 6 shows the axial development of the wall temperatures at lower (
= 1%) and higher (
= 10%) values of nanoparticle concentration. For the lower nanoparticle concentration (
= 1%), the T
w with Al
2O
3-EG nanofluid is approximately the same to TiO
2-EG and CuO-EG because of the marginal difference in the values of the thermal conductivities (0.3% higher as compared to TiO
2-EG nanofluid and 0.2% as compared to CuO-EG nanofluid). For the higher nanoparticle concentration (
= 10%), the T
w decreases by 15 K for the Al
2O
3-EG nanofluid due to the movement of the nanoparticles at a higher Re, which results in a higher thermal efficiency.
3.3. Case 3: Turbine Oil-Based Nanofluid in Straight Tube with Constant Heat Flux Using SPH
Case 3 considers turbine oil-based nanofluids with the same parameters used in previous two cases. The effect of base fluid was investigated using three different base fluids viz. water, ethylene glycol and turbine oil with the same nanoparticle (Al
2O
3,
= 4%) as shown in
Figure 7.
All the nanofluids (Al2O3-water, Al2O3-EG and Al2O3-turbine oil) significantly enhance the value of Nu as compared to the any base fluid alone. It may be noted that the Nu enhanced by 16% for Al2O3-water nanofluid as compared to the water, 12% for the Al2O3-EG nanofluid as compared to ethylene glycol and 8% for the Al2O3-turbine oil when compared to turbine oil. The Nu enhancement is due to similar reasons as previous two cases.
The heat transfer enhancement using nanofluids may be affected by several factors such as Brownian motion, Brownian diffusion, dispersion and friction force between the fluid and nanoparticles. Because of this several factors, the heat characteristics of nanofluids are dependent on the properties of the base liquid, the dispersed phases and particle concentration. Therefore, the general form of the Nu yields:
In the present study a new correlation for Nu (Equation (13)) has been developed covering a wide range of the nanoparticle concentration (0% ≤ ≤ 10%) and Prandtl number (6.0–500) under the constant heat flow and laminar flow conditions (25 < Re < 1500).
Figure 8 shows the comparison between the present computed Nu results, the experimental results and the computed data from the literature with the present proposed correlation (Equation (13)). It may be observed from
Figure 8 that the present results of Nu are in good agreement with the experimental results developed by Wen & Ding [
20], Anoop et al. [
23], Heris et al. [
46], Heris et al. [
49] and with the computational results from Maïga et al. [
21].
3.4. Case 4: Water-Based Nanofluid in Straight Tube with Constant Wall Temperature Using SPH
In this case water-based nanofluids are used at a constant wall temperature (T
w = 313.15 K) condition with an inlet fluid temperature of T
o = 293.15 K, at Re = 500.
Figure 9 demonstrates the effect of the nanoparticle concentration on the T
m for constant wall temperature condition.
It can be observed that the T
m decreases with increase in the concentration of nanoparticles due to the improved heat capacity (up to 23%). The T
m for a highest nanoparticle concentration (
= 10%) was lower by 10 K as compared to the water. The diminution of temperature reflects the improvement in the thermal properties of the resulting mixture caused by the Brownian motion. The effect of the different water based nanofluids was investigated using different nanoparticles viz Al
2O
3, TiO
2, CuO, SiO
2 and ZnO, as shown in
Figure 10a. It may be noted that the Al
2O
3-water nanofluid has a higher heat transfer rate than all other nanofluids. The enhancement in Nu for the Al
2O
3-water is 14% higher as compared to ZnO-water nanofluid.
Figure 10b shows the overall effect of the different base fluids on Nu for constant temperature boundary condition. The Nu at Re = 950 enhanced by 16% for Al
2O
3-water nanofluid as compared to water, 10% for Al
2O
3-EG nanofluid as compared to ethylene glycol and 8% for Al
2O
3-turbine oil nanofluid as compared to turbine oil. The enhancement in the Nu is mainly due to the thermophysical properties of the nanoparticles.
For the average Nu in a straight tube with constant wall temperature a new correlation (Equation (14)) is proposed by fitting the data obtained from the numerical simulations. The correlation covers a wide range of the nanoparticle concentration (0% ≤
≤ 10%) and Prandtl number (6.0–500) under the laminar flow condition (25 < Re < 1500).
Figure 11 shows the comparison between the present computed Nu results, with the experimental results from Heris et al. [
22], Ting et al. [
50] and the computed data from Maïga et al. [
21] with the present proposed correlation (Equation (14)). A good agreement was attained between the computed and previous experimental work with the predicted values of the Nu with a variation of ±5%.
3.5. Case 5: Water-Based Nanofluid in Straight Microtube with Constant Heat Flux Using SPH
In case 5, all the different nanofluids Al
2O
3-water, TiO
2-water, CuO-water, SiO
2-water and ZnO-water are used to investigate the Nu in a straight microtube with a length of 0.3 m and an inner diameter (d
t) of 0.5 mm. Results from the numerical simulation were compared with Shah’s [
51] correlation (Equation (15)) for validation purpose. A good agreement can be seen in between the present computed results of Nu with the predicted values from Shah’s correlation, as shown in
Figure 12.
It may be noted from
Figure 13a,b that similar to the straight tube results, the wall temperature as well as fluid mean temperature in the straight microtube also decreases with increase in the nanoparticle concentration. The decrease in the temperatures of the wall and the fluid will result in a better heat transfer.
Figure 14a shows the effect of the different type of nanoparticles for a water-based nanofluid. The Al
2O
3-water nanofluid has a better heat transfer enhancement as compared to that of all the other nanoparticles due to the higher thermal conductivity.
Figure 14b shows the Nu for different fluids at the same Re = 950. The turbine oil-based nanofluid has the higher Nu, however it is not the nanofluid with the higher enhancement.
The Nu enhancement was 6% for Al2O3-water compared to water, 12% for Al2O3-EG compared to ethylene glycol and 5% for Al2O3-turbine oil compared to turbine oil. Based on these results, it may be concluded that ethylene glycol-based nanofluids are the best choice for heat transfer enhancement at the same Re and .
For the average Nu in a microtube with constant heat flux a new correlation (Equation (16)) is proposed by fitting the data obtained from the numerical simulations. The correlation covers a wide range of the process parameters (25 < Re < 1500, 0 < < 10, 6 < Pr < 500) under the laminar flow condition.
Figure 15 shows the comparison between the present Nu results along with the experiments from Haghighi et al. [
52] and the computed data from Salman et al. [
53] with the present proposed correlation (Equation [
16]). The predicted values of Nu are in good agreement (variation of ±5%) with the computed values and the previous experimental results.
3.6. Case 6: Water-Based Nanofluid in Straight Tube with Constant Heat Flux Using SPD
Case 6 purpose is to simulate the nanofluid flow for a constant heat flux condition in a straight tube using the SPD.
Figure 16 shows a comparison of the computed Nu results using SPD and SPH. It may be noted that the Nu increases with the increase of the Re. The SPD shows a higher Nu due to a higher thermal conductivity and viscosity of the nanofluid. Results of the SPD model show agreement with Liu et al. [
31], where the Nu of the nanofluid is better predicted in the SPD than in the SPH. The SPD model is recommended as the appropriate model for predicting the heat transfer characteristics of nanofluid flow in a straight tube.
4. Conclusions
In the present study, heat transfer of different nanofluid types were investigated using two configurations: straight tube and straight microtube. Both geometries presented an enhancement in the Nu using nanofluids. In case of the straight tube with = 4%, the Nu increases 16% for Al2O3-water as compared to water, 12% for Al2O3-EG as compared to EG and 8% for Al2O3-turbine oil as compared to turbine oil. For the straight microtube with = 4% the Nu increases 6% for Al2O3-water as compared to water, 12% for Al2O3-EG as compared to ethylene glycol and 5% for Al2O3-turbine oil as compared to turbine oil.
Despite the better heat transfer enhancement in Al2O3-EG and Al2O3-turbine oil it is imperative to consider the associated higher values of the wall shear stress (e.g., quadruple of the corresponding based fluid for an Al2O3-EG nanofluid with high nanoparticle concentration = 10%). It is important to notice that having nanofluids with high nanoparticle concentrations ( > 4%) is not recommended as the nanoparticle loadings increases the viscosity.
The comparison between the different nanoparticles viz. Al2O3, TiO2, CuO, SiO2 and ZnO revealed that the Al2O3 nanoparticle with the three based fluids (water, ethylene glycol, and turbine oil) has a higher Nu due to the higher thermal capacity. The present results clearly showed that the addition of nanoparticles increases the Nu up to 16% as compared to the base fluid. For all the cases, the Nu enhancement becomes more pronounced due to nanoparticles. Two different boundary conditions were considered (constant heat flux and constant temperature), and thus two new convective heat transfer correlations were proposed for the straight tube covering a wide range of the process parameters (25 < Re < 1500, 0 < < 10, 6 < Pr < 500) under laminar flow condition. Also, a new Nu correlation for the straight microtube was proposed for the same range of process parameters to that of straight tube. The new correlations can be applicable to a wide range of applications that will allow this new field of study to move a step forward.