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Search Results (602)

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Keywords = uniform convergence

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23 pages, 4468 KB  
Article
Fixed-Time Target Tracking and Encirclement Control for Multi-UAVs with Bearing-Only Measurements
by Zican Zhou, Jiangping Hu, Xuesong Wu, Shangzhi Liao and Jiao Yuan
Drones 2026, 10(1), 63; https://doi.org/10.3390/drones10010063 - 15 Jan 2026
Abstract
This paper introduces a novel fixed-time control framework for simultaneous target tracking and circumnavigation in a multi-UAV system, using only bearing measurements. The proposed approach enables the UAV swarm to rapidly form and maintain a rigid circular formation around a moving target, with [...] Read more.
This paper introduces a novel fixed-time control framework for simultaneous target tracking and circumnavigation in a multi-UAV system, using only bearing measurements. The proposed approach enables the UAV swarm to rapidly form and maintain a rigid circular formation around a moving target, with continuous tracking and uniform angular spacing between agents. A key innovation is the development of a distributed fixed-time estimator, which allows each UAV to localize the target within a fixed time using only local bearing information and limited inter-agent communication. Building on this estimator, a hierarchical control strategy is designed, where a leader UAV guides the formation while followers achieve and maintain uniform distribution along the orbit. The fixed-time stability of the overall closed-loop system is rigorously established through Lyapunov analysis. Numerical simulations confirm the fixed-time convergence of the algorithm. Compared to an existing asymptotic-convergence benchmark, the proposed approach achieves significantly faster and deterministic convergence, with improved formation accuracy. Full article
(This article belongs to the Section Artificial Intelligence in Drones (AID))
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19 pages, 371 KB  
Article
Adjoint Bernoulli’s Kantorovich–Schurer-Type Operators: Univariate Approximations in Functional Spaces
by Harun Çiçek, Nadeem Rao, Mohammad Ayman-Mursaleen and Sunny Kumar
Mathematics 2026, 14(2), 276; https://doi.org/10.3390/math14020276 - 12 Jan 2026
Viewed by 145
Abstract
In this work, we first establish a new connection between adjoint Bernoulli’s polynomials and gamma function as a new sequence of linear positive operators denoted by Sr,ς,λ(.;.). Further, convergence results for these [...] Read more.
In this work, we first establish a new connection between adjoint Bernoulli’s polynomials and gamma function as a new sequence of linear positive operators denoted by Sr,ς,λ(.;.). Further, convergence results for these sequences of operators, i.e., Sr,ς,λ(.;.) are derived in various functional spaces with the aid of the Korovkin theorem, the Voronovskaja-type theorem, the first order of the modulus of continuity, the second order of the modulus of continuity, Peetre’s K-functional, the Lipschitz condition, etc. In the last section, we focus our research on the bivariate extension of these sequences of operators; their uniform rate of approximation and order of approximation are investigated in different functional spaces. Full article
(This article belongs to the Special Issue Numerical Analysis and Scientific Computing for Applied Mathematics)
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22 pages, 13102 KB  
Article
Enhancing Drafter Performance in Spunbonding of Polymeric Fibers via Airflow Simulation
by Behrang Mohajer, Mohamad Kheradmandkeysomi, Chul B. Park and Markus Bussmann
Polymers 2026, 18(2), 187; https://doi.org/10.3390/polym18020187 - 9 Jan 2026
Viewed by 148
Abstract
Spunbonding drafters play a decisive role in determining fiber attenuation, morphology, and final nonwoven quality; however, their internal airflow behavior remains poorly characterized due to limited physical accessibility and historically empirical design practices. This work employs high-fidelity computational fluid dynamics (CFD) to systematically [...] Read more.
Spunbonding drafters play a decisive role in determining fiber attenuation, morphology, and final nonwoven quality; however, their internal airflow behavior remains poorly characterized due to limited physical accessibility and historically empirical design practices. This work employs high-fidelity computational fluid dynamics (CFD) to systematically resolve the airflow field inside a laboratory-scale drafter and to quantify the impact of geometry on fiber drawing conditions. The simulations reveal a previously unreported “braking effect,” where adverse flow structures reduce effective shear drag, limit drawability, and increase the likelihood of fiber breakage. Parametric virtual experimentation across seven geometric variables demonstrates that the drafter configuration strongly governs shear distribution, flow uniformity, and energy consumption. Using a performance-oriented optimization framework, three key processing objectives were targeted: (i) maximizing shear drag to promote stable fiber attenuation, (ii) improving axial drawing uniformity, and (iii) minimizing pressurized-air demand. CFD-guided design modifications—including controlled widening, tailored wall divergence and convergence, and an extensible lower section—were implemented and subsequently validated using a newly constructed prototype. Experimental measurements on polypropylene (PP) and high-density polyethylene (HDPE) fibers confirm substantial reductions in fiber breakage and improvements in drawing stability, thereby demonstrating the effectiveness of simulation-driven process optimization in spunbonding equipment design. Full article
(This article belongs to the Section Polymer Fibers)
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31 pages, 3452 KB  
Article
Improved Chimpanzee Optimization Algorithm Based on Multi-Strategy Fusion and Its Application in Multiphysics Parameter Optimization
by Bin Zhou, Chaoyun Shi, Ning Yan and Yangyang Chu
Symmetry 2026, 18(1), 108; https://doi.org/10.3390/sym18010108 - 7 Jan 2026
Viewed by 144
Abstract
To address the challenges of high computational costs, susceptibility to local optima, and heavy reliance on manual intervention in multi-physics parameter optimization for symmetric acoustic metamaterials, an enhanced Chimp Optimization Algorithm (DADCOA) is proposed in this paper. This algorithm integrates the double chaotic [...] Read more.
To address the challenges of high computational costs, susceptibility to local optima, and heavy reliance on manual intervention in multi-physics parameter optimization for symmetric acoustic metamaterials, an enhanced Chimp Optimization Algorithm (DADCOA) is proposed in this paper. This algorithm integrates the double chaotic initialization strategy (DCS), adaptive multimodal convergence mechanism (AMC), and dual-weight pinhole imaging update operator (DWPI). It employs a Logistic–Tent composite chaotic mapping strategy for population initialization, significantly enhancing distribution uniformity within high-dimensional parameter spaces. An AMC factor is then introduced to dynamically balance global exploration and local exploitation based on the real-time evolutionary state of the population. A dual-weight population update mechanism, incorporating distance and historical contributions, is integrated with a pinhole imaging opposition-based learning strategy to improve population diversity. Additionally, a composite single objective error feedback local differential mutation operation is introduced to improve optimization accuracy for coupled multi-physics objectives. Experimental validation based on the CEC 2022 test function suite and an acoustic metamaterial parameter optimization model demonstrates that compared to the standard COA algorithm and existing improved algorithms, the DADCOA algorithm reduces simulation time by 28.46% to 60.76% while maintaining high accuracy. This approach effectively addresses the challenges of high computational cost, stringent accuracy requirements, and composite single objective coupling in COMSOL physical parameter optimization, providing an effective solution for the design of acoustic metamaterials based on symmetric structures. Full article
(This article belongs to the Section Engineering and Materials)
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30 pages, 12874 KB  
Article
Multi-Objective Lightweight Optimization and Decision for CTB Battery Box Under Multi-Condition Performance
by Junming Huang, Shangyuan Ling, Shichao Zhang, Pinpin Qin, Juncheng Lu and Kaiyu Meng
World Electr. Veh. J. 2026, 17(1), 26; https://doi.org/10.3390/wevj17010026 - 6 Jan 2026
Viewed by 121
Abstract
To address the conflicts among objectives and the decision-making challenges in the multi-condition adaptive design of battery boxes for new energy vehicles, this study proposes a multi-objective collaborative optimization method based on an improved relaxation factor, aiming to achieve a comprehensive enhancement in [...] Read more.
To address the conflicts among objectives and the decision-making challenges in the multi-condition adaptive design of battery boxes for new energy vehicles, this study proposes a multi-objective collaborative optimization method based on an improved relaxation factor, aiming to achieve a comprehensive enhancement in both structural lightweighting and mechanical performance. A finite element model of the CTB high-strength steel roll-formed battery box was established and validated through modal testing. According to the Chinese National Standard GB 38031-2025, the mechanical responses of the battery box under random vibration, extreme operating conditions, and impact loads were analyzed to identify performance weaknesses. Sensitivity analysis was conducted to screen the design variables, and an improved relaxation factor strategy based on weight distribution difference information was introduced to construct a multi-objective collaborative optimization model. Furthermore, the entropy-weighted TOPSIS method was employed to enable intelligent decision-making on the Pareto solution set. The results demonstrate that the proposed method outperforms conventional approaches in both convergence speed and solution distribution uniformity. After optimization, the mass of the battery box was reduced by 12.38%, while multiple mechanical performance indicators were simultaneously improved, providing valuable theoretical and engineering guidance for the structural design of power battery systems. Full article
(This article belongs to the Section Storage Systems)
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24 pages, 21815 KB  
Article
HGTA: A Hexagonal Grid-Based Task Allocation Method for Multi-Robot Coverage in Known 2D Environments
by Weixing Xia, Shihui Shen, Ping Wang and Jinjin Yan
Robotics 2026, 15(1), 15; https://doi.org/10.3390/robotics15010015 - 5 Jan 2026
Viewed by 191
Abstract
For multi-robot cooperative coverage, an effective spatial division strategy is essential to ensure balanced and spatially continuous task regions for each robot. Traditional grid-based partitioning approaches like DARP (Divide Areas based on Robots’ Positions) and TASR (Task Allocation based on Spatial Regions) often [...] Read more.
For multi-robot cooperative coverage, an effective spatial division strategy is essential to ensure balanced and spatially continuous task regions for each robot. Traditional grid-based partitioning approaches like DARP (Divide Areas based on Robots’ Positions) and TASR (Task Allocation based on Spatial Regions) often generate discontinuous sub-regions and imbalanced workloads, particularly in irregular or fragmented task spaces. To mitigate these issues, this paper introduces HGTA (Hexagonal Grid-based Task Allocation), a novel method that employs hexagonal tessellation for environmental representation. The hexagonal grid structure provides uniform neighbor connectivity and minimizes boundary fragmentation, yielding smoother partitions. HGTA integrates a multi-stage wavefront expansion algorithm with an iterative region-correction mechanism, jointly ensuring spatial contiguity and load equilibrium across robots. Extensive evaluations in 2D environments with varying obstacle densities and robot distributions show that HGTA enhances spatial continuity—achieving improvements of 18.2% in connectivity and 17.8% in boundary smoothness over DARP, and 7.5% and 9.5% over TASR, respectively—while also improving workload balance (variance reduction up to 18.5%) without compromising computational efficiency. The core contribution lies in the synergistic coupling of hexagonal tessellation, wavefront expansion, and dynamic correction, a design that fundamentally advances partition smoothness and convergence speed. HGTA thus offers a robust foundation for multi-robot cooperative coverage, area surveillance, and underwater search applications where connected and balanced partitions are critical. Full article
(This article belongs to the Section AI in Robotics)
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32 pages, 4374 KB  
Article
RFSCMOEA: A Dual-Population Cooperative Evolutionary Algorithm with Relaxed Feasibility Selection
by Yongchao Li, Heming Jia, Xinyan Lin, Yaqiao Li, Qian Shi and Shiwei Chen
Information 2026, 17(1), 36; https://doi.org/10.3390/info17010036 - 3 Jan 2026
Viewed by 163
Abstract
Achieving a dynamic equilibrium among feasibility, convergence, and diversity remains a fundamental challenge in Constrained Multi-objective Optimization Problems (CMOPs). To address the limitations of conventional methods in handling complex constraints and resource allocation, this paper proposes a Dual-Population Cooperative Evolutionary Algorithm based on [...] Read more.
Achieving a dynamic equilibrium among feasibility, convergence, and diversity remains a fundamental challenge in Constrained Multi-objective Optimization Problems (CMOPs). To address the limitations of conventional methods in handling complex constraints and resource allocation, this paper proposes a Dual-Population Cooperative Evolutionary Algorithm based on Relaxed Feasibility Selection and Shrinking Contribution Resource Allocation (RFSCMOEA). First, a relaxed feasibility selection strategy is designed with a dynamically shrinking threshold, allowing near-feasible solutions to survive in early stages to enhance boundary exploration. Second, a dual-criterion environmental selection mechanism integrates non-dominated sorting with k-nearest neighbor density estimation to prevent premature convergence and ensure solution uniformity. Furthermore, a dynamic resource allocation model optimizes computational configuration by adjusting offspring generation ratios based on the real-time evolutionary contribution of each population. Extensive experiments on 47 benchmark functions and 12 real-world engineering problems demonstrate that RFSCMOEA significantly outperforms eight state-of-the-art algorithms in Feasibility Rate, Inverted Generational Distance, and Hypervolume. Full article
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19 pages, 4790 KB  
Article
Hierarchical Fuzzy Adaptive Observer-Based Fault-Tolerant Consensus Tracking for High-Order Nonlinear Multi-Agent Systems Under Actuator and Sensor Faults
by Lei Zhao and Shiming Chen
Sensors 2026, 26(1), 252; https://doi.org/10.3390/s26010252 - 31 Dec 2025
Viewed by 352
Abstract
This paper investigates the consensus tracking problem for a class of high-order nonlinear multi-agent systems subject to actuator faults, sensor faults, unknown disturbances, and model uncertainties. To effectively address this problem, a hierarchical fault-tolerant control framework with fuzzy adaptive mechanisms is proposed. First, [...] Read more.
This paper investigates the consensus tracking problem for a class of high-order nonlinear multi-agent systems subject to actuator faults, sensor faults, unknown disturbances, and model uncertainties. To effectively address this problem, a hierarchical fault-tolerant control framework with fuzzy adaptive mechanisms is proposed. First, a distributed output predictor based on a finite-time differentiator is constructed for each follower to estimate the leader’s output trajectory and to prevent fault propagation across the network. Second, a novel state and actuator-fault observer is designed to reconstruct unmeasured states and detect actuator faults in real time. Third, a sensor-fault compensation strategy is integrated into a backstepping procedure, resulting in a fuzzy adaptive consensus-tracking controller. This controller guarantees the uniform boundedness of all closed-loop signals and ensures that the tracking error converges to a small neighborhood of the origin. Finally, numerical simulations validate the effectiveness and robustness of the proposed method in the presence of multiple simultaneous faults and disturbances. Full article
(This article belongs to the Special Issue Sensor-Based Fault Diagnosis and Prognosis)
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14 pages, 4855 KB  
Article
Generalized Synchronization of a Novel Hyperchaotic System and Application in Secure Communication
by Mohamed M. El-Dessoky, Nehad Almohammadi and Mansoor Alsulami
Mathematics 2026, 14(1), 111; https://doi.org/10.3390/math14010111 - 28 Dec 2025
Viewed by 178
Abstract
In this paper, a generalized synchronization (GS) framework for identical hyperchaotic systems is presented. The main objective is to achieve generalized synchronization with guaranteed global stability and effective convergence, which remains a key challenge in synchronization-based secure communication systems. The proposed controller is [...] Read more.
In this paper, a generalized synchronization (GS) framework for identical hyperchaotic systems is presented. The main objective is to achieve generalized synchronization with guaranteed global stability and effective convergence, which remains a key challenge in synchronization-based secure communication systems. The proposed controller is systematically derived to ensure global asymptotic convergence of the synchronization errors for arbitrary initial conditions and distinct scaling factors. This formulation unifies complete, anti-, and generalized synchronization within a single control structure. To demonstrate the applicability of the proposed method, it is integrated into an image encryption algorithm, where the hyperchaotic trajectories of the drive system generate highly random permutation and diffusion sequences. Simulation results verify that the designed controller achieves effective generalized synchronization and that the encrypted images exhibit uniform histograms and low pixel correlation, indicating strong security and resistance to statistical attacks. Full article
(This article belongs to the Special Issue Chaotic Systems and Their Applications, 2nd Edition)
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36 pages, 35595 KB  
Article
Robust ISAR Autofocus for Maneuvering Ships Using Centerline-Driven Adaptive Partitioning and Resampling
by Wenao Ruan, Chang Liu and Dahu Wang
Remote Sens. 2026, 18(1), 105; https://doi.org/10.3390/rs18010105 - 27 Dec 2025
Viewed by 278
Abstract
Synthetic aperture radar (SAR) is a critical enabling technology for maritime surveillance. However, maneuvering ships often appear defocused in SAR images, posing significant challenges for subsequent ship detection and recognition. To address this problem, this study proposes an improved iteration phase gradient resampling [...] Read more.
Synthetic aperture radar (SAR) is a critical enabling technology for maritime surveillance. However, maneuvering ships often appear defocused in SAR images, posing significant challenges for subsequent ship detection and recognition. To address this problem, this study proposes an improved iteration phase gradient resampling autofocus (IIPGRA) method. First, we extract the defocused ships from SAR images, followed by azimuth decompression and translational motion compensation. Subsequently, a centerline-driven adaptive azimuth partitioning strategy is proposed: the geometric centerline of the vessel is extracted from coarsely focused images using an enhanced RANSAC algorithm, and the target is partitioned into upper and lower sub-blocks along the azimuth direction to maximize the separation of rotational centers between sub-blocks, establishing a foundation for the accurate estimation of spatially variant phase errors. Next, phase gradient autofocus (PGA) is employed to estimate the phase errors of each sub-block and compute their differential. Then, resampling the original echoes based on this differential phase error linearizes non-uniform rotational motion. Furthermore, this study introduces the Rotational Uniformity Coefficient (β) as the convergence criterion. This coefficient can stably and reliably quantify the linearity of the rotational phase, thereby ensuring robust termination of the iterative process. Simulation and real airborne SAR data validate the effectiveness of the proposed algorithm. Full article
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24 pages, 2190 KB  
Article
Improving Coating Stability Using Slip Conditions: An Analytical Approach to Curtain Coating
by Laraib Mehboob, Khadija Maqbool, Abdul Majeed Siddiqui and Zaheer Abbas
Lubricants 2026, 14(1), 11; https://doi.org/10.3390/lubricants14010011 - 27 Dec 2025
Viewed by 263
Abstract
Curtain deflector coating is a widely employed technique for producing thin, uniform films in numerous industrial applications. The flow dynamics in curtain coating become complex near the corner region due to the interaction of the moving substrate and the falling liquid curtain. In [...] Read more.
Curtain deflector coating is a widely employed technique for producing thin, uniform films in numerous industrial applications. The flow dynamics in curtain coating become complex near the corner region due to the interaction of the moving substrate and the falling liquid curtain. In this study, an analytical investigation is conducted for the steady, in-compressible, and creeping flow of a Maxwell fluid, under the Navier slip condition at the substrate. The mathematical model is derived from the conservation of mass and momentum representing the nonlinear system which is solved using the Langlois recursive technique in combination with the inverse method. The inclusion of the Navier slip boundary condition in this research makes it novel and remove the singularity which produce the unstable stresses at a sharp corner due to no slip, but the Navier slip gives a stable solution for the stresses at a sharp corner. The analysis demonstrates that substrate slip significantly reduces tangential stresses and enhances the stability of the coating flow. Residual error analysis is also performed to verify the accuracy and convergence of the analytical solutions. The results provide a deeper understanding of how slip effects can be utilized to improve coating uniformity and optimize the operational performance of curtain deflector coating systems. Full article
(This article belongs to the Special Issue Wear-Resistant Coatings and Film Materials, 2nd Edition)
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35 pages, 5561 KB  
Article
A Hybrid Optimization Algorithm with Multi-Strategy Integration and Multi-Subpopulation Cooperation for Engineering Problem Solving
by Liang Kang and Weini Xia
Mathematics 2026, 14(1), 95; https://doi.org/10.3390/math14010095 - 26 Dec 2025
Viewed by 209
Abstract
To solve the limitations of single optimization algorithms, such as premature convergence, insufficient global exploration, and high susceptibility to local optima, a Hybrid Optimization Algorithm (HOA) based on multi-subpopulation collaboration and multi-strategy fusion is proposed. The HOA uses Logistic chaotic mapping for population [...] Read more.
To solve the limitations of single optimization algorithms, such as premature convergence, insufficient global exploration, and high susceptibility to local optima, a Hybrid Optimization Algorithm (HOA) based on multi-subpopulation collaboration and multi-strategy fusion is proposed. The HOA uses Logistic chaotic mapping for population initialization to enhance uniformity and diversity. The population is then divided into four subpopulations; each is optimized independently using different strategies, including the genetic algorithm (GA), Gray Wolf Optimizer (GWO), self-attention mechanism, and k-nearest neighbor graph (kNN). This design leverages the strengths of individual algorithms while mitigating their respective limitations. An elite information exchange mechanism facilitates knowledge transfer by randomly reassigning elite individuals across subpopulations at fixed iteration intervals. Additionally, global optimization strategies including differential evolution (DE), Simulated Annealing (SA), Local Search (LS), and time of arrival (TOA) position adjustment are integrated to balance exploration and exploitation, thereby enhancing convergence accuracy and the ability to escape local optima. Evaluated on the CEC2017 benchmark suite and real-world engineering problems, the HOA demonstrates superior performance in convergence speed, accuracy, and robustness compared to single-algorithm approaches—notably, HOA ranks 1st in 30-dimensional CEC2017 functions. By effectively integrating multiple optimization strategies, the HOA provides an effective and reliable solution to complex optimization challenges. Full article
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22 pages, 338 KB  
Article
Optimal Quantization on Spherical Surfaces: Continuous and Discrete Models—A Beginner-Friendly Expository Study
by Mrinal Kanti Roychowdhury
Mathematics 2026, 14(1), 63; https://doi.org/10.3390/math14010063 - 24 Dec 2025
Cited by 1 | Viewed by 174
Abstract
This expository paper provides a unified and pedagogical introduction to optimal quantization for probability measures supported on spherical curves and discrete subsets of the sphere, emphasizing both continuous and discrete settings. We first present a detailed geometric and analytical foundation for intrinsic quantization [...] Read more.
This expository paper provides a unified and pedagogical introduction to optimal quantization for probability measures supported on spherical curves and discrete subsets of the sphere, emphasizing both continuous and discrete settings. We first present a detailed geometric and analytical foundation for intrinsic quantization on the unit sphere, including definitions of great and small circles, spherical triangles, geodesic distance, Slerp interpolation, the Fréchet mean, spherical Voronoi regions, centroid conditions, and quantization dimensions. Building upon this framework, we develop explicit continuous and discrete quantization models on spherical curves, namely great circles, small circles, and great circular arcs—supported by rigorous derivations and pedagogical exposition. For uniform continuous distributions, we compute optimal sets of n-means and the associated quantization errors on these curves; for discrete distributions, we analyze antipodal, equatorial, tetrahedral, and finite uniform configurations, illustrating convergence to the continuous model. The central conclusion is that for a uniform probability distribution supported on a one-dimensional geodesic subset of total length L, the optimal n-means form a uniform partition and the quantization error satisfies Vn=L2/(12n2).The exposition emphasizes geometric intuition, detailed derivations, and clear step-by-step reasoning, making it accessible to beginning graduate students and researchers entering the study of quantization on manifolds. This article is intended as an expository and tutorial contribution, with the main emphasis on geometric reformulation and pedagogical clarity of intrinsic quantization on spherical curves, rather than on the development of new asymptotic quantization theory. Full article
13 pages, 318 KB  
Article
Weighted Approximation by Szász–Mirakyan–Durrmeyer Operators Reproducing Exponential Functions
by Gülsüm Ulusoy Ada and Ali Aral
Mathematics 2026, 14(1), 59; https://doi.org/10.3390/math14010059 - 24 Dec 2025
Viewed by 237
Abstract
We examine a Szász–Mirakyan–Durrmeyer type operator that reproduces the functions 1 and e2ax for a fixed parameter a>0. While its exponential reproduction property has been described in the classical literature, the effect of exponential weights on its [...] Read more.
We examine a Szász–Mirakyan–Durrmeyer type operator that reproduces the functions 1 and e2ax for a fixed parameter a>0. While its exponential reproduction property has been described in the classical literature, the effect of exponential weights on its approximation behavior has not been studied. In this work, we provide a detailed analysis of the operator in weighted spaces and show that combining exponential reproduction with weighted norms improves the approximation behavior for exponentially growing functions. We also prove that the corresponding sequence of operator norms remains uniformly bounded for a family of exponential weights, ensuring the stability of the operators in the weighted framework. Moreover, we establish new Korovkin-type approximation theorems involving weighted convergence and obtain sharp uniform error estimates in the presence of exponential weights. These results extend the classical theory to weighted exponential settings and highlight several quantitative features that do not arise in the classical case. Full article
(This article belongs to the Special Issue Advances in Operator Theory and Nonlinear Evolution Equations)
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17 pages, 3231 KB  
Article
Spectroscopic Real-Time Monitoring of Plasmonic Gold Nanoparticle Formation in ZnO Thin Films via Pulsed Laser Annealing
by Edgar B. Sousa, N. F. Cunha, Joel Borges and Michael Belsley
Micro 2026, 6(1), 1; https://doi.org/10.3390/micro6010001 - 24 Dec 2025
Viewed by 188
Abstract
We demonstrate that pulsed laser annealing induces plasmonic gold nanoparticles in ZnO thin films, monitored in real-time via pulse-by-pulse spectroscopy. Initially embedded gold nanoparticles (smaller than 5 nm) in sputtered ZnO films were annealed using 532 nm pulses from a Q-switched Nd:YAG laser [...] Read more.
We demonstrate that pulsed laser annealing induces plasmonic gold nanoparticles in ZnO thin films, monitored in real-time via pulse-by-pulse spectroscopy. Initially embedded gold nanoparticles (smaller than 5 nm) in sputtered ZnO films were annealed using 532 nm pulses from a Q-switched Nd:YAG laser while monitoring transmission spectra in situ. A plasmonic resonance dip emerged after ~100 pulses in the 530–550 nm region, progressively deepening with continued exposure. Remarkably, different incident energies converged to a thermodynamically stable optical state centered near 555 nm, indicating robust nanoparticle configurations. After several hundred laser shots, the process stabilized, producing larger nanoparticles (40–200 nm diameter) with significant surface protrusion. SEM analysis confirmed substantial gold nanoparticle growth. Theoretical modeling supports these observations, correlating spectral evolution with particle size and embedding depth. The protruding gold nanoparticles can be functionalized to detect specific biomolecules, offering significant advantages for biosensing applications. This approach offers superior spatial selectivity and real-time process monitoring compared to conventional thermal annealing, with potential for optimizing uniform nanoparticle distributions with pronounced plasmonic resonances for biosensing applications. Full article
(This article belongs to the Section Microscale Physics)
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