Search Results (171)

This study presents an intercomparison of planetary boundary layer height (PBLH) estimates derived from three distinct approaches: the Morphological Image Processing Approach (MIPA) algorithm applied to ground-based lidar measurements, European Centre for Medium-Range Weather Forecasts (ECMWF) Reanalysis 5th Generation (ERA5) and Modern-Era Retrospective Analysis for Research and Applications Version 2 (MERRA-2) reanalysis model outputs, and radiosonde (RS) observations, this latter being taken as reference. The intercomparison was conducted during three measurement episodes, encompassing a total of 153 h (6 days), as part of the Boundary Layer Extensive Campaign with muLti-instrumentaL Analysis (BELLA), carried out in spring and early summer 2024 at the CNR-IMAA Atmospheric Observatory (CIAO) in southern Italy (40.60N, 15.72E). The study provides insights into the performance and reliability of these PBLH estimation approaches under diverse atmospheric scenarios. Visual and statistical analyses of selected case studies indicate that MIPA often tracked the aerosol layering structure and diurnal PBLH evolution more closely than ERA5 and MERRA-2, particularly during convective growth and evening transitions. On the other hand, it is found that ERA5 provides more accurate estimates of the nighttime PBLH, where MIPA shows poor nighttime estimation capabilities. Quantitative comparison against radiosonde data reveals that MIPA reaches a weighted root mean square error ($RMS{E}_w$) of $380\pm 41$ m with a coefficient of determination ($R^2$) of $0.68\pm 0.16$, while ERA5 shows an $RMS{E}_w$ of $292\pm 72$ m and an $R^2$ of $0.81\pm 0.11$; and MERRA-2 shows an $RMS{E}_w$ of $631\pm 124$ m and an $R^2$ of $0.34\pm 0.21$. By combining MIPA daytime and ERA5 nighttime PBLH, the overall results are improved, obtaining an $R^2=0.86\pm 0.08$ and an $RMS{E}_w$ of $213\pm 40$ m. This intercomparison highlights the strengths and limitations of each method and demonstrates the benefits of combining complementary PBLH retrieval techniques. The findings contribute to refining boundary layer monitoring methodologies and provide guidance for operational atmospheric observation networks. Full article

Simulated impact multipath (SIM) occurs when forward operators propagate Global Navigation Satellite System (GNSS) radio occultation (RO) signals through strongly nonspherical atmospheric structures, producing multivalued bending angles that cannot be assimilated directly. In this study, the relationships between SIM and planetary boundary layer (PBL) structures were quantified using COSMIC-2 RO observations and ERA5 reanalysis during two periods (January and July 2022). The results show that SIM affects ~36% of RO profiles, with more than 70% of cases occurring within 0.5 km above the diagnosed PBL top. By defining the simulated impact multipath height (SIMH) as the first detection level of SIM, we found that discarding data below the SIMH reduces bending angle biases by more than half and substantially decreases their scatter. These results provide direct physical evidence linking SIM to strong vertical gradients near PBL structures and establish a quantitative basis for simple, effective quality control, thereby improving weather prediction, particularly in the data-sparse tropical lower troposphere. Full article

Air pollution, particularly fine particulate matter (PM_2.5), poses significant public health and environmental risks. This study explores the effectiveness of spatiotemporal graph neural networks (ST-GNNs) in forecasting PM_2.5 concentrations by integrating remote-sensing hyperspectral indices with traditional meteorological and pollutant data. The model was evaluated using data from Switzerland and the Gauteng province in South Africa, with datasets spanning from January 2016 to December 2021. Key performance metrics, including root mean squared error (RMSE), mean absolute error (MAE), probability of detection (POD), critical success index (CSI), and false alarm rate (FAR), were employed to assess model accuracy. For Switzerland, the integration of spectral indices improved RMSE from 1.4660 to 1.4591, MAE from 1.1147 to 1.1053, CSI from 0.8345 to 0.8387, POD from 0.8961 to 0.8972, and reduced FAR from 0.0760 to 0.0719. In Gauteng, RMSE decreased from 6.3486 to 6.2319, MAE from 4.4891 to 4.4066, CSI from 0.9555 to 0.9560, and POD from 0.9699 to 0.9732, while FAR slightly increased from 0.0154 to 0.0181. Error analysis revealed that while the initial one-day ahead forecast without spectral indices had a marginally lower error, the dataset with spectral indices outperformed from the two-day ahead mark onwards. The error for Swiss monitoring stations stabilized over longer prediction lengths, indicating the robustness of the spectral indices for extended forecasts. The study faced limitations, including the exclusion of the Planetary Boundary Layer (PBL) height and K-index, lack of terrain data for South Africa, and significant missing data in remote sensing indices. Despite these challenges, the results demonstrate that ST-GNNs, enhanced with hyperspectral data, provide a more accurate and reliable tool for PM_2.5 forecasting. Future work will focus on expanding the dataset to include additional regions and further refining the model by incorporating additional environmental variables. This approach holds promise for improving air quality management and mitigating health risks associated with air pollution. Full article

Low clouds significantly impact weather, climate, and multiple environmental and economic sectors such as agriculture, fire risk management, aviation, and renewable energy. Accurate knowledge of cloud base height (CBH) is critical for optimizing crop yields, improving fire danger forecasts, enhancing flight safety, and increasing solar energy efficiency. This study evaluates a shadow-based CBH retrieval method using Moderate Resolution Imaging Spectroradiometer (MODIS) satellite visible imagery and compares the results against collocated lidar measurements from the Micro-Pulse Lidar Network (MPLNET) ground stations. The shadow method leverages sun–sensor geometry to estimate CBH from the displacement of cloud shadows on the surface, offering a practical and high-resolution passive remote sensing technique, especially useful where active sensors are unavailable. The validation results show strong agreement, with a correlation coefficient (R) = 0.96 between shadow-based and lidar-derived CBH estimates, confirming the robustness of the approach for shallow, isolated cumulus clouds. The method’s advantages include direct physical height estimation without reliance on cloud top heights or stereo imaging, applicability across archived datasets, and suitability for diurnal studies. This work highlights the potential of shadow-based retrievals as a reliable, cost-effective tool for global low cloud monitoring, with important implications for atmospheric research and operational forecasting. Full article

The planetary boundary layer (PBL) exerts strong control on heat, moisture, and momentum exchange, yet its representation over the steep mountains and deep valleys of Liangshan remains poorly understood. This study evaluates six Weather Research and Forecasting (WRF) PBL schemes (ACM2, BL, MYJ, MYNN2.5, QNSE, and YSU) using multi-source observations from radiosondes, surface stations, and wind profiling radar during clear-sky dry-season cases in spring and winter. The schemes exhibit substantial differences in governing turbulent mixing and stratification. For the specific cases studied, QNSE best reproduces 2 m temperature in both seasons by realistically capturing nocturnal stability and large diurnal ranges, while non-local schemes overestimate nighttime temperatures due to excessive mixing. MYNN2.5 performs robustly for boundary layer growth in spring, and BL aligns most closely with radar-derived PBL height (PBLH). Vertical profile comparisons show that QNSE and MYJ better represent the lower–middle level thermodynamic structure, whereas all schemes underestimate extreme near-surface winds, reflecting unresolved terrain-induced variability. PBLH simulations reproduce diurnal cycles but differ in amplitude, with QNSE occasionally producing unrealistic spikes. Overall, no scheme performs optimally for all variables. However, QNSE and MYNN2.5 show the most balanced performance across seasons. These findings provide guidance for selecting PBL schemes for high-resolution modeling and fire–weather applications over complex terrain. Full article

Studies have established that extreme air pollution is more prevalent and is responsible for more deaths and disability-adjusted life years (DALY) in urban cities, especially in developing economies. However, the paucity of ground-based observation has greatly hindered extensive and long-term monitoring and, as such, a good understanding of the trend and characteristics of air quality where it matters most. Aerosol optical depth (AOD) from satellites retrievals provides good spatial and temporal resolutions of atmospheric aerosols and could be a good proxy for ground-level PM_2.5 concentration. This study used a Bayesian regression model to determine the parameters of a PM_2.5 model at four monitoring stations using AOD and selected atmospheric variables (PBLH and RH) as input. The dry-air reference value (K) and the integrated humidity coefficient (γ) were used to delineate the effects of the aerosol characteristics. The values of K and γ, $0.02<K<0.07$ (${\mathrm{m}}^2{\mathrm{g}}^{\mathrm{-1}}$) and $0.54<\gamma <3.14$, respectively, are site-specific even within the same country as is the case for Lekki and Benin (both in Nigeria). The PM_2.5 estimates from the developed observation-based model were in good agreement with the ground-based observations ($0.55<r<0.77$). RH and a combination of PBLH-RH were the best performers in the development of the model. Firstly, this study identifies the unique range of values for K and $\gamma$ for site-classes in the sub-Saharan tropical climate. Secondly, PBLH adds more explanatory power to the PM_2.5 estimates in Benin and Douala (both non-coastal cities) while RH improves the performance of the model significantly in Lekki and Owendo (both coastal cities). For West Africa and similar data-sparse regions, the methodology presented here offers a practical pathway to enhance air quality monitoring capabilities. Full article

The PBLH affects the intensity of the surface turbulence and the state of pollutant dispersion. Current research on PBLH characteristics and their relationship with pollution in coastal megacities remains insufficient. Moreover, existing studies rarely evaluate the consistency of various boundary layer solution methods, making it difficult to identify deviations in single methods. So, we conducted enhanced observation experiments in Shenzhen, a megacity in China, between March and July 2023. The characteristics of the PBLH was analyzed by five months of observations from Micro-Pulse Lidar (MPL) and Microwave Radiometer (MWR). Five retrieval methods (Parcel, GRA, STD, WCT, and Theta) were applied for comparative assessment. The results shows that all methods captured similar diurnal patterns. During daytime, the PBLH ranged from 512 to 1345 m, with Theta yielding the highest and STD the lowest average values. At night, PBLH decreased overall, and method-dependent differences persisted. Under different pollution levels, this study also discussion the properties of PBLH using MPL and microwave radiometer. And aerosol optical depth (AOD) and PBLH showed a strong negative correlation, indicating aerosol-induced suppression of boundary layer growth. The study of boundary layer characteristics in coastal megacities can provide reference for atmospheric physics research in economically developed coastal areas. Full article

A notable decline in the frequency of sea fog inflows and an increase in low-cloud ceiling height were observed following the construction of the Saemangeum Seawall west of the Gunsan Airport, an area traditionally prone to frequent sea fog events. To the mechanisms underlying these changes, a numerical experiment was conducted using the Weather Research and Forecasting model. An 11-m-high seawall was used as a physical barrier, and an elevated sea surface temperature (SST) was established within the enclosed area to simulate realistic post-construction conditions. The model successfully reconstructed sea fog occurrences, and the cloud–water mixing ratio effectively captured the spatial distribution of sea fog. Deviations from the control experiment showed a consistent pattern of reduced cloud–water mixing ratios near the surface and enhanced concentrations at high levels. Decreased buoyancy frequency in the surface layer enhanced atmospheric instability, inducing upward motion and intensified condensation activity. Increases in the turbulence kinetic energy within the planetary boundary layer (TKE within the PBL), vertical wind shear, and temperature further corroborated the reduction in sea fog and enhanced stratus formation. These findings indicate that the increased SST and seawall significantly influence the modification of the sea fog structure and its inflow dynamics. Full article

The Planetary Boundary Layer (PBL) remains a popular research topic, given its fundamental role in the exchange of energy between the surface and the atmosphere. Understanding the PBL’s mechanisms can improve weather forecasting, climate and air quality modelling. This paper presents a PBL climatology based on 50 years of observations (1973–2023) from the Bucharest Băneasa radio sounding station in Romania (international identifier 15420). The Stull method was used to calculate the PBL height, which was extracted from the sounding at the Bucharest Băneasa observation point and considers virtual potential temperature (θ_v). This incorporates the effect of humidity on air density. The analysis of climatological seasons (DJF, MAM, JJA and SON) based on PBL height series determined at 00 and 12 UTC using RAOB software revealed that the mixed layer height, as calculated by the Stull method, mainly captures the nocturnal Stable Boundary Layer (SBL) at 00 UTC and highlights the mixed layer (ML) at 12 UTC. ERA5 reanalysis data were also used in parallel. Full article

This single high-impact case study investigates the impact of planetary boundary layer (PBL) representation on long-range transport of Amazon fire smoke that reached the Metropolitan Area of São Paulo (MASP) from 15 to 20 August 2019, using the WRF model to compare three PBL schemes (MYNN 2.5, YSU, and BouLac) and three source-tagged tracers. The simulations are evaluated against MODIS-derived aerosol optical depth (AOD), the Light Detection and Ranging (LiDAR) time–height curtain over MASP, and HYSPLIT forward trajectories. Transport is diagnosed along the source-to-MASP pathway using six-hourly cross-sections and two integrative metrics: the projected mean wind in the 700–600 hPa layer and the vertical moment of tracer mass above the boundary layer. Outflow and downwind impact are strongest when a persistent reservoir between 2 and 4 km coexists with projected winds for several hours. In this episode, MYNN maintains an elevated 2–5 km transport layer and matches the observed arrival time and altitude, YSU yields a denser but delayed column, and BouLac produces discontinuous pulses with reduced coherence over the city. A negatively tilted trough, jet coupling, and a nearly stationary front establish a northwest-to-southeast corridor consistent across model fields, trajectories, and satellite signal. Seasonal robustness should be assessed with multi-event, multi-model analyses. Full article

Carbonaceous aerosols represent a significant component of atmospheric aerosol, with implications for climate and human health. The recent EU Directive 2024/2881 highlights the need to monitor emerging pollutants like black carbon more effectively. This study presents an brief field campaign at an urban background site aimed at characterizing carbonaceous aerosols. Daily samples of PM₁₀ and PM_2.5 were analyzed using a Sunset thermal-optical analyzer to determine organic and elemental carbon (OC, EC), while real-time equivalent black carbon (eBC) was measured with three independent instruments: MAAP, AE33, and Giano BC1. Total carbon (TC) was monitored using an online TCA08 thermo-catalytic analyzer. The average concentration of PM₁₀ was 17.1 µg/m³ and 10.4 µg/m³ for PM_2.5. On average, OC and EC represented 16.5% and 3.6% of PM₁₀ mass, and 22.6% and 5.5% of PM_2.5. SOC accounted for 36% of OC. The in situ Mass Absorption Cross-section (MAC), recalculated for the ECO site, was between 8.0 and 12.2 m²/g. eBC concentrations were modulated by the daily evolution of the planetary boundary-layer height and combustion sources. The apportionment of eBC was 65% from fossil fuel and 35% from biomass burning. Biomass-burning emissions were further confirmed by optical measurements, with BrC contributing 35% of absorption at 370 nm. Full article

Atmospheric pollution constitutes one of the key environmental challenges hindering Atmospheric pollution is a key environmental challenge constraining the sustainable development of Gansu Province’s land-based Belt and Road corridor and its regional ecological barrier function. The spatiotemporal heterogeneity of aerosol optical depth (AOD) profoundly impacts regional environmental quality. Based on MODIS AOD, NCEP reanalysis, and emission data, this study employed trend analysis (Mann–Kendall test) and attribution analysis (multiple linear regression combined with LMG and Spearman correlation) to investigate the spatiotemporal evolution of AOD over Gansu Province during 2009–2019 and its meteorological and emission drivers. Key findings include the following: (1) AOD exhibited significant spatial heterogeneity, with high values concentrated in the Hexi Corridor and central regions; monthly variation showed a unimodal pattern (peak value of 0.293 in April); and AOD generally declined slowly province-wide during 2009–2019 (52.8% of the area showed significant decreases). (2) Following the implementation of the Air Pollution Prevention and Control Action Plan in 2013 (2014–2019), AOD trends stabilized or declined in 99.8% of the area, indicating significant improvement. (3) Meteorological influences displayed distinct regional-seasonal specificity—the Hexi Corridor (arid zone) was characterized by strong negative correlations with relative humidity (RH2) and wind speed (WS) year-round, and positive correlations with temperature (T2) in spring but negative in summer in the north; the Hedong region (industrial zone) featured strong positive correlations with planetary boundary layer height (PBLH) in summer (r > 0.6) and with T2 in spring/summer; and the Gannan Plateau (alpine zone) showed positive WS correlations in spring and weak positive RH2 correlations in spring/autumn, highlighting the decisive regulatory role of underlying surface properties. (4) Emission factors (PM_2.5, ${\mathrm{SO}}_4^{2-}$, ${\mathrm{NO}}_3^{-}$, ${\mathrm{NH}}_4^{+}$, OM, and BC) dominated (>50% relative contribution) in 80% of seasonal scenarios, prevailing in most regions (Hexi: 71–95% year-round; Hedong: 68–80% year-round; and Gannan: 69–72% in spring/summer). Key components included BC (contributing > 30% in 11 seasons, e.g., 52.5% in Hedong summer), ${\mathrm{NO}}_3^{-}$ + ${\mathrm{NH}}_4^{+}$ (>57% in Hexi summer/autumn), and OM (20.3% in Gannan summer, 19.0% province-wide spring). Meteorological factors were the primary driver exclusively in Gannan winter (82%, T2-dominated) and province-wide summer (67%, RH2 + WS-dominated). In conclusion, Gansu’s AOD evolution is co-driven by emission factors (dominant province-wide) and meteorological factors (regionally and seasonally specific). Post-2013 environmental policies effectively promoted regional air quality improvement, providing a scientific basis for differentiated aerosol pollution control in arid, industrial, and alpine zones. Full article

The vertical distribution of volatile organic compounds (VOCs) within the planetary boundary layer (PBL) is critical for understanding ozone (O₃) formation, yet knowledge remains limited in complex urban environments. In this study, vertical measurements of 117 VOC species were conducted using an unmanned aerial vehicle (UAV) equipped with a VOC multi-channel sampling system, up to a height of 500 m in Shenzhen, China. Results showed that total VOC (TVOC) concentrations decreased with altitude in the morning, reflecting the influence of surface-level local emissions, but increased with height at midday, likely driven by regional transport and potentially stronger photochemical processes. Source apportionment revealed substantial industrial emissions across all altitudes, vehicular emissions concentrated near the surface, and biomass burning primarily impacting higher layers. Clear evidence of enhanced secondary formation of oxygenated VOCs (OVOCs) was observed along the vertical gradient, particularly at midday, indicating intensified photochemical processes at higher altitudes. These findings underscore the importance of considering vertical heterogeneity in VOC distributions when modeling O₃ formation or developing measures to reduce emissions at different altitudes, and also demonstrate the potential of UAV platforms to provide high-resolution atmospheric chemical data in complex urban environments. Full article

This study investigates the use of a Random Forest (RF), an artificial intelligence (AI) model, to estimate the planetary boundary layer height (PBLH) over Central Amazonia from climatic elements data collected during the GoAmazon experiment, held in 2014 and 2015, as it is a key metric for air quality, weather forecasting, and climate modeling. The novelty of this study lies in estimating PBLH using only surface-based meteorological observations. This approach is validated against remote sensing measurements (e.g., LIDAR, ceilometer, and wind profilers), which are seldom available in the Amazon region. The dataset includes various meteorological features, though substantial missing data for the latent heat flux (LE) and net radiation (Rn) measurements posed challenges. We addressed these gaps through different data-cleaning strategies, such as feature exclusion, row removal, and imputation techniques, assessing their impact on model performance using the Root Mean Square Error (RMSE), Mean Absolute Error (MAE), and $r^2$ metrics. The best-performing strategy achieved an RMSE of 375.9 m. In addition to the RF model, we benchmarked its performance against Linear Regression, Support Vector Regression, LightGBM, XGBoost, and a Deep Neural Network. While all models showed moderate correlation with observed PBLH, the RF model outperformed all others with statistically significant differences confirmed by paired t-tests. SHAP (SHapley Additive exPlanations) values were used to enhance model interpretability, revealing hour of the day, air temperature, and relative humidity as the most influential predictors for PBLH, underscoring their critical role in atmospheric dynamics in Central Amazonia. Despite these optimizations, the model underestimates the PBLH values—by an average of 197 m, particularly in the spring and early summer austral seasons when atmospheric conditions are more variable. These findings emphasize the importance of robust data preprocessing and higtextight the potential of ML models for improving PBLH estimation in data-scarce tropical environments. Full article

Marine atmospheric boundary-layer height (MABLH) is crucial for ocean heat, momentum, and substance transfer, affecting ocean circulation, climate, and ecosystems. Due to the unique geographical location of the South China Sea (SCS), coupled with its complex atmospheric environment and sparse ground-based observation stations, accurately determining the MABLH remains challenging. Coherent Doppler wind lidar (CDWL), as a laser-based active remote sensing technology, provides high-resolution wind profiling by transmitting pulsed laser beams and analyzing backscattered signals from atmospheric aerosols. In this study, we developed a stacking optimal ensemble model (SOEM) to estimate MABLH in the vicinity of the site by integrating CDWL measurements from a representative SCS site with ERA5 (fifth-generation reanalysis dataset from the European Centre for Medium-Range Weather Forecasts) data from December 2019 to May 2021. Based on the categorization of the total cloud cover data into weather conditions such as clear/slightly cloudy, cloudy/transitional, and overcast/rainy, the SOEM demonstrates enhanced performance with an average mean absolute percentage error of 3.7%, significantly lower than the planetary boundary-layer-height products of ERA5. The SOEM outperformed random forest, extreme gradient boosting, and histogram-based gradient boosting models, achieving a robustness coefficient ($R^2$) of 0.95 and the lowest mean absolute error of 32 m under the clear/slightly cloudy condition. The validation conducted in the coastal city of Qingdao further confirmed the superiority of the SOEM in resolving meteorological heterogeneity. The predictions of the SOEM aligned well with CDWL observations during Typhoon Sinlaku (2020), capturing dynamic disturbances in MABLH. Overall, the SOEM provides a precise approach for estimating convective boundary-layer height, supporting marine meteorology, onshore wind power, and coastal protection applications. Full article