Search Results (10)

Aerosol research is important for the protection of the ecological environment, the improvement of air quality, and as a response to climate change. In this study, a random forest (RF) estimation model of aerosol optical depth (AOD) and extinction coefficient vertical profiles was, respectively, established using Orbiting Carbon Observatory-2 (OCO-2) oxygen-A band (O₂ A-band) data from China and its surrounding areas in 2016, combined with geographical information (longitude, latitude, and elevation) and viewing angle data. To address the high number of OCO-2 O₂ A-band channels, principal component analysis (PCA) was employed for dimensionality reduction. The model was then applied to estimate the aerosol extinction coefficients for the region in 2017, and its validity was verified by comparing the estimated values with the Cloud-Aerosol Lidar Infrared Pathfinder Satellite Observations (CALIPSO) Level 2 extinction coefficients. In the comprehensive analysis of overall performance, an AOD model was initially constructed using variables, achieving a correlation coefficient (R) of 0.676. Subsequently, predictions for aerosol extinction coefficients were generated, revealing a satisfactory agreement between the predicted and the actual values in the vertical direction, with an R of 0.535 and a root mean square error (RMSE) of 0.107 km⁻¹. Of the four seasons of the year, the model performs best in autumn (R = 0.557), while its performance was relatively lower in summer (R = 0.442). Height had a significant effect on the model, with both R and RMSE decreasing as height increased. Furthermore, the accuracy of aerosol profile inversion shows a dependence on AOD, with a better accuracy when AOD is less than 0.3 and RMSE can be less than 0.06 km⁻¹. Full article

The O₂ A-band night glow can be used to retrieve the temperature in the range of 80–120 km in the mesosphere and lower thermosphere (MLT). From the full spectrum of A-band night glow, the band used to retrieve temperature is selected based on the sensitivity of the emission line on temperature, taking into account the compromise relationship between the spectral band and resolution, inversion efficiency, and inversion accuracy. The non-linear iterative inversion method based on optimization theory is adopted for the retrieval of temperature. Meanwhile, considering the stability of inversion, Tikhonov regularization matrix is added as a constraint, and the optimal estimation inversion algorithm is optimized to suppress the influence of measurement noise on results. Through the recovering simulated noisy spectra from an interferometer, the temperature profile with vertical resolution better than 2 km and an average accuracy better than 2 K is obtained by the optimized inversion method in this paper. In addition, the influence of a priori constraints on the inversion accuracy is studied, and a priori accuracy limits the inversion accuracy. When a priori accuracy is controlled within ±5 K, the average temperature inversion accuracy can be optimized to 1.35 K, which is better than the accuracy of OSIRIS on Odin at 90–105 km. Full article

The Greenhouse gases Monitoring Instrument on GaoFen-5 satellite-II (GMI-II) uses spatial heterodyne spectroscopy (SHS) for quantitative monitoring of atmospheric greenhouse gases (GHG). Unlike the traditional SHS, the interferometer component of the GMI-II was designed with zero optical path difference offset, effectively improving spectral resolution while maintaining the same detector specifications. The secondary imaging system with non-isometric scaling of spatial and spectral dimensions was designed to decrease the integration time of a frame image or improve the spectral signal-to-noise ratio (SNR) under the same integration time. This paper introduces the design, manufacture, adjustment methods, and test results of the main performance indexes of the GMI-II that indicate that the spectral resolution of the O₂ A-band detection channel is better than 0.6 cm⁻¹ and other channels are better than 0.27 cm⁻¹. Under the typical radiance of other carbon monitors’ on-orbit statistics, the spectral SNR of the GMI-II is more than 300. These test results demonstrate that the GMI-II can be well adapted to quantitative remote sensing monitoring of atmospheric GHG. Full article

Aerosol vertical distribution is decisive and hard to be constrained. It is of great significance for the study of atmospheric climate and environment. Oxygen absorption A-bands (755–775 nm) provide a unique opportunity to acquire vertical aerosol profiles from satellites over a large spatial coverage. To investigate the ability of O₂ A-bands in retrieving aerosol vertical distribution, the dependence of retrieval on satellite observation geometry, spectral resolution, signal-to-noise ratio (SNR), size distribution, and a priori knowledge is quantified using information content theory. This work uses the radiative transfer model UNL to simulate four aerosol modes and the instrument noise model. The simulations show that a small scattering angle leads to an increase in the total amount of observed aerosol profile information, with the degrees freedom of signal (DFS) of a single band increasing from 0.4 to 0.85 at high spectral resolution (0.01 nm). The total DFS value of O₂ A-bands varies accordingly between 1.2–2.3 to 3.8–5.1 when the spectral resolution increases from 1 nm to 0.01 nm. The spectral resolution has a greater impact on DFS value than the impact from SNR (an improvement of roughly 41–53% resulted from the change in spectral resolution and the SNR led to 13–18%). The retrieval is more sensitive to aerosols with a coarse-dominated mode. The improvement in spectral resolution on information acquisition is demonstrated using the DFS and the posterior error at various previous errors and resolutions. Full article

China is developing the High-precision Greenhouse gases Monitoring Satellite (HGMS), carrying a high-spectral-resolution lidar (HSRL) for aerosol vertical profiles and imaging grating spectrometers for CO₂ measurements at the same time. By providing simultaneous evaluation of the aerosol scattering effect, HGMS would reduce the bias of the XCO₂ retrievals from the passive sensor. In this work, we propose a method to reduce aerosol-induced bias in XCO₂ retrievals for the future HGMS mission based on the correlation analysis among simulated radiance, XCO₂ bias, and aerosol optical depth (AOD) ratio. We exercise the method with the Orbiting Carbon Observatory-2 (OCO-2) XCO₂ retrievals and AOD ratio inferred from the OCO-2 O₂ A-band aerosol parameters at 755 nm and the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) AOD at 532 nm at several Total Carbon Column Observing Network (TCCON) sites in Europe. The results showed that 80% of measurements from OCO-2 were improved, and data from six TCCON sites show an average of 2.6 ppm reduction in mean bias and a 68% improvement in accuracy. We demonstrate the advantage of fused active–passive observation of the HGMS for more accurate global XCO₂ measurements in the future. Full article

The Chinese carbon dioxide measurement satellite (TanSat) has collected a large number of measurements in the solar calibration mode. To improve the accuracy of XCO2 retrieval, the Instrument Line Shape (ILS, also known as the slit function) must be accurately determined. In this study, we characterized the on-orbit ILS of TanSat by fitting measured solar irradiance from 2017 to 2018 with a well-calibrated high-spectral-resolution solar reference spectrum. We used various advanced analytical functions and the stretch/sharpen of the tabulated preflight ILS to represent the ILS for each wavelength window, footprint, and band. Using super Gaussian+P7 and the stretch/sharpen functions substantially reduced the fitting residual in O${}_2$ A-band and weak CO${}_2$ band compared with using the preflight ILS. We found that the difference between the derived ILS width and on-ground preflight ILS was up to −3.5% in the weak CO${}_2$ band, depending on footprint and wavelength. The large amplitude of the ILS wings, depending on the wavelength, footprint, and bands, indicated possible uncorrected stray light. Broadening ILS wings will cause additive offset (filling-in) on the deep absorption lines of the spectra, which we confirmed using offline bias correction of the solar-induced fluorescence retrieval. We estimated errors due to the imperfect ILS using simulated TanSat spectra. The results of the simulations showed that XCO2 retrieval is sensitive to errors in the ILS, and 4% uncertainty in the full width of half maximum (FWHM) or 20% uncertainty in the ILS wings can induce an error of up to 1 ppm in the XCO2 retrieval. Full article

Clouds act as a major reflector that changes the amount of sunlight reflected to space. Change in radiance intensity due to the presence of clouds interrupts the retrieval of trace gas or aerosol properties from satellite data. In this paper, we developed a fast and robust algorithm, named the fast cloud retrieval algorithm, using a triplet of wavelengths (469, 477, and 485 nm) of the O₂–O₂ absorption band around 477 nm (CLDTO4) to derive the cloud information such as cloud top pressure (CTP) and cloud fraction (CF) for the Geostationary Environment Monitoring Spectrometer (GEMS). The novel algorithm is based on the fact that the difference in the optical path through which light passes with regard to the altitude of clouds causes a change in radiance due to the absorption of O₂–O₂ at the three selected wavelengths. To reduce the time required for algorithm calculations, the look-up table (LUT) method was applied. The LUT was pre-constructed for various conditions of geometry using Vectorized Linearized Discrete Ordinate Radiative Transfer (VLIDORT) to consider the polarization of the scattered light. The GEMS was launched in February 2020, but the observed data of GEMS have not yet been widely released. To evaluate the performance of the algorithm, the retrieved CTP and CF using observational data from the Global Ozone Monitoring Experiment-2 (GOME-2), which cover the spectral range of GEMS, were compared with the results of the Fast Retrieval Scheme for Clouds from the Oxygen A band (FRESCO) algorithm, which is based on the O₂ A-band. There was good agreement between the results, despite small discrepancies for low clouds. Full article

In this paper, we present the Hefei EMI Cloud Retrieval Algorithm (HECORA), which uses information from the O₂-O₂ absorption band around 477 nm to retrieve effective cloud fraction and effective cloud pressure from satellite observations. The retrieved cloud information intends to improve the atmospheric trace gas products based on the Environment Monitoring Instrument (EMI) spectrometer. The HECORA method builds on OMCLDO2 and presents some evolutions. The Vector Linearized Discrete Ordinate Radiative Transfer (VLIDORT) model has been used to produce the Top of the Atmosphere (TOA) reflectance Look-up Tables (LUT) as a function of the cloud fraction and cloud pressure. Applying the Differential Optical Absorption Spectroscopy (DOAS) technique to the synthetic reflectance LUT, the reflectance spectra can be associated with O₂-O₂ geometrical vertical column densities (VCD_geo) and continuum reflectance. This is the core of the retrieval method, since there is a one-to-one relationship between O₂-O₂ VCD_geo and continuum reflectance, on the one hand, and effective cloud fraction and effective cloud pressure, on the other hand, for a given illumination and observing geometry and given surface height and surface albedo. We first used the VLIDORT synthetic spectra to verify the HECORA algorithm and obtained good results in both the Lambertian cloud model and the scattering cloud model. Secondly, HECORA is applied to OMI and TROPOMI and compared with OMCLDO2, FRESCO+, and OCRA/ROCINN cloud products. Later, the cloud pressure results from TROPOMI observations obtained using HECORA and FRESCO+ are compared with the CALIOP Cloud Layer product. HECORA is closer to the CALIOP results under low cloud conditions, while FRESCO+ is closer to high clouds due to the higher sensitivity of the O₂ A-band to cloud vertical information. Finally, HECORA is applied to the TROPOMI NO₂ retrieval. Validation of the tropospheric NO₂ VCD with ground-based MAX-DOAS measurements shows that choosing HECORA cloud products to correct for photon path variations on the TROPOMI tropospheric NO₂ VCD retrievals has better performance than using FRESCO+ under low cloud conditions. In conclusion, this paper shows that the HECORA cloud products are in good agreement with the well-established cloud products and that they are suitable for correcting the effect of cloud in trace gas retrievals. Therefore, HECORA has the potential to be applied to EMI. Full article

With three imaging grating spectrometers, the Orbiting Carbon Observatory-2 (OCO-2) measures high spectral resolution spectra ( $\lambda /\Delta \lambda \approx$ 19,000) of reflected solar radiation within the molecular oxygen (O ${}_2$ ) A-band at 0.765 $\mathsf{\mu }$ m and two carbon dioxide (CO ${}_2$ ) bands at 1.61 and 2.06 $\mathsf{\mu }$ m. OCO-2 uses onboard lamps with a reflective diffuser, solar observations through a transmissive diffuser, lunar measurements, and surface targets for radiometric calibration and validation. Separating calibrator aging from instrument degradation poses a challenge to OCO-2. Here we present a methodology for trending the OCO-2 Build 8R radiometric calibration using OCO-2 nadir observations over eight desert sites and nearly simultaneous observations from Moderate Resolution Imaging Spectroradiometer (MODIS) with sensor viewing zenith angles of 15 ± 0.5 ${}^{\circ }$ . For the O ${}_2$ A-band, this methodology is able to quantify a drift of −0.8 ± 0.1% per year and capture a small error in correcting the aging of the solar calibrator. For the other two OCO-2 bands, no measurable changes were seen, indicating less than 0.1% and less than 0.3% per year drift in the radiometric calibration of Band 2 and Band 3, respectively. Full article

Current atmospheric composition sensors provide a large amount of high spectral resolution data. The accurate processing of this data employs time-consuming line-by-line (LBL) radiative transfer models (RTMs). In this paper, we describe a method to accelerate hyperspectral radiative transfer models based on the clustering of the spectral radiances computed with a low-stream RTM and the regression analysis performed for the low-stream and multi-stream RTMs within each cluster. This approach, which we refer to as the Cluster Low-Streams Regression (CLSR) method, is applied for computing the radiance spectra in the O₂ A-band at 760 nm and the CO₂ band at 1610 nm for five atmospheric scenarios. The CLSR method is also compared with the principal component analysis (PCA)-based RTM, showing an improvement in terms of accuracy and computational performance over PCA-based RTMs. As low-stream models, the two-stream and the single-scattering RTMs are considered. We show that the error of this approach is modulated by the optical thickness of the atmosphere. Nevertheless, the CLSR method provides a performance enhancement of almost two orders of magnitude compared to the LBL model, while the error of the technique is below 0.1% for both bands. Full article