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Open AccessFeature PaperArticle

Comparing Graphene Oxide and Reduced Graphene Oxide as Blending Materials for Polysulfone and Polyvinylidene Difluoride Membranes

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Department of Environmental Engineering, Yonsei University, 1, Yonseidae-gil, Wonju-si 26493, Gangwon-do, Korea
2
Electronic Material and Device Research Center, Korea Electronics Technology Institute, 25, Saenari-ro, Bundang-gu, Seongnam-si 13509, Gyeonggi-do, Korea
3
School of Civil and Environmental Engineering, Addis Ababa institute of Technology, Addis Ababa University, King George VI Street, P.O. Box 385 Addis Ababa, Ethiopia
*
Author to whom correspondence should be addressed.
Appl. Sci. 2020, 10(6), 2015; https://doi.org/10.3390/app10062015
Received: 17 February 2020 / Revised: 10 March 2020 / Accepted: 10 March 2020 / Published: 16 March 2020
(This article belongs to the Special Issue Innovative Water Treatment Technology for Sustainability)
Graphene is a single atomic plane of graphite, and it exhibits unique electronic, thermal, and mechanical properties. Exfoliated graphene oxide (GO) contains various hydrophilic functional groups, such as hydroxyl, epoxide, and carboxyl groups, that can modify the hydrophobic characteristics of a membrane surface. Though reduced graphene oxide (rGO) has fewer functional groups than GO, its associated sp2 structures and physical properties can be recovered. A considerable amount of research has focused on the use of GO to obtain a pristine graphene material via reduction processes. In this study, polysulfone (PSf) and polyvinylidene fluoride (PVDF) membranes that were blended with GO and rGO, respectively, were fabricated by using the immersion phase inversion method and an n-methylpyrrolidone (NMP) solvent. Results showed that the graphene nanomaterials, GO and rGO, can change the pore morphology (size and structure) of both PSf and PVDF membranes. The optimum content of both was then investigated, and the highest flux enhancement was observed with the 0.10 wt% GO-blended PSf membrane. The presence of functional groups in GO within prepared PSf and PVDF membranes alters the membrane characteristics to hydrophilic. An antifouling test and rejection efficiency evaluation also showed that the 0.10 wt% membrane provided the best performance. View Full-Text
Keywords: graphene oxide; reduced graphene oxide; membrane; polysulfone; polyvinylidene fluoride; water treatment graphene oxide; reduced graphene oxide; membrane; polysulfone; polyvinylidene fluoride; water treatment
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Yoon, Y.; Kye, H.; Yang, W.S.; Kang, J.-W. Comparing Graphene Oxide and Reduced Graphene Oxide as Blending Materials for Polysulfone and Polyvinylidene Difluoride Membranes. Appl. Sci. 2020, 10, 2015.

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