1. Introduction
The issue of Municipal Solid Waste (MSW) demands urgent global attention. As noted by World Data, the potential for repurposing materials beyond their original applications is significant. However, the sheer volume of waste produced, particularly plastic, poses a critical challenge. The United States, for instance, leads in per capita plastic waste production, generating an alarming 130.09 kg per person annually. This translates to over 42 million metric tons of plastic waste in 2016 alone, positioning the United States as the world’s largest plastic waste generator [
1]. Current waste generation rates are exceeding landfill capacity, highlighting the pressing need for sustainable recycling solutions. Both developed and developing nations are actively seeking alternatives to traditional methods like landfill disposal and incineration due to escalating costs, logistical complexities, and adverse environmental consequences.
Recycling and upcycling are acknowledged as refined alternatives to conventional waste management strategies. According to the European plastic strategy, it is essential to reuse and recycle waste materials as much as possible to minimize waste disposal or incineration [
2]. Recycling involves novel projects through techniques such as material extrusion printing and injection molding, specifically to generate items from plastic refuse [
3]. These recycling processes can be categorized as mechanical, chemical, or thermal. Conversely, upcycling prioritizes the metamorphosis of used materials into superior-quality new products. A case in point is the design of sustainable seating solutions from discarded automobile tires or the fabrication of roofing tiles from reclaimed plastic [
4].
Recent statistics from 2023 indicate that plastic packaging accounts for the majority (36%) of plastic production [
5]. Of even greater concern is the breakdown of plastic waste management: 46% ends up in landfills, 22% becomes litter, 17% is incinerated, and only 15% is collected for recycling, with less than 9% ultimately recycled after accounting for losses [
5]. MSW encompasses both organic waste, such as food waste, and inorganic waste, including wood, glass, metal, paper, and plastic. Plastic waste alone constitutes over 10% of global landfill content, lacking effective sorting mechanisms for recycling [
6]. This complex issue underscores the global challenge of managing MSW effectively and sustainably. As noted, “Thermoplastic composites can be reshaped and are easier to recycle. They have a long shelf life and exhibit a high level of resistance to harmful chemical environments. As a result, they can be used as geopolymers in concrete composites, serving as an alternative to natural aggregates” [
2].
While a heterogeneous array of plastic waste exists, a substantial proportion remains outside the ambit of significant recycling efforts. Each polymer exhibits discrete mechanical attributes that must be congruent with the intended utility of the reclaimed material. Moreover, the energetic cost inherent in the recycling process constitutes a salient consideration. To illustrate, polyethylene exists in two primary forms: low-density polyethylene (LDPE) and high-density polyethylene (HDPE). Each variant manifests unique mechanical characteristics that render it appropriate for specific applications. With a fusion point spanning from 120 to 160 °C, HDPE is particularly efficacious for concrete pavement applications in contrast to LDPE, which possesses a melting point within the range of 105 to 115 °C [
4,
7].
This research investigates the potential of utilizing a novel blend of recycled polyethylene terephthalate (PET) and recycled high-density polyethylene (HDPE) in concrete pavement applications. The specific blending ratios explored, in conjunction with established industry standards, offer a transferable methodology applicable to diverse plastic waste streams. This approach enables the assessment of requisite mechanical properties for various concrete applications within the construction sector. Furthermore, this research introduces a pioneering, adaptable framework capable of addressing a wide spectrum of plastic waste, thereby unlocking numerous avenues for effective waste migration. The originality of our material assessment lies in its integration of waste utilization within the construction industry, coupled with a systematic evaluation protocol based on the intrinsic attributes of each waste typology.
Plastics exhibit a wide range of properties, making them suitable for diverse applications. This article explores the experimental implementation of recycled polyethylene terephthalate (PET) and recycled high-density polyethylene (HDPE), emphasizing the latter, which is often sourced from flexible plastics like discarded containers. Recycled PET, commonly derived from used beverage bottles, is also examined [
1]. PET is favored in recycling streams due to its desirable characteristics and ubiquitous presence, contributing to its frequent repurposing [
1,
2,
3,
4,
5,
6,
7,
8].
Polyethylene terephthalate (PET), a thermoplastic polymer in the polyester family, is renowned for its chemical, mechanical, and thermal resistance, as well as its dimensional stability [
9]. Despite its versatility and advantages like durability and strength [
1], PET is not biodegradable. Its widespread use stems from its favorable properties. High-density polyethylene (HDPE), another thermoplastic derived from petroleum, is considered a highly valuable plastic material. Characterized by its long chains of repeating monomer units (C
2H
4), HDPE exhibits a relatively low degree of branching compared to other polyethylene categories [
10]. This structural feature contributes to its high tensile strength and elevated melting point. HDPE enjoys extensive application across diverse products, including plastic bottles, piping, and cutting boards, and commands over 34% of the global market. Known as “Type 2 plastic”, HDPE is employed in the production of thicker, more robust containers compared to those made from PET. Typical examples include milk jugs, motor oil containers, detergent bottles, and bleach bottles [
8].
The benefits of incorporating recycled PET and HDPE in construction commence with the financial advantages of decreasing waste deposited in landfills. Employing recycled plastic can result in substantial cost savings in the production of new construction materials [
9]. The utilization of plastic waste curtails the quantity of construction materials needed for projects, as the plastic recycling procedure is approximately 10% less expensive than producing new materials without compromising the material’s properties. This has been thoroughly addressed in the ASTM Standard List (2023) [
8]. Furthermore, this utilization strategy enhances the material’s characteristics when recycled plastic is incorporated into construction. Research and testing have demonstrated that recycled PET and HDPE either maintain or improve the material’s properties [
10]. This occurs alongside a reduction in the construction industry’s energy requirements. A noteworthy global advantage is that development programs for plastic recycling in various countries allocate supplementary funding to promote the implementation of development plans [
10].
Figure 1 illustrates shredded PET and HDPE plastic [
11].
One compelling reason to prioritize plastic waste management is the correlation between high population density and substantial waste generation [
12]. Densely populated areas are likely to produce greater solid waste, particularly in the absence of effective waste management infrastructure. To advance sustainability goals, integrating a circular economy model through the utilization of recycled plastics is crucial. This approach has the potential to yield a 50% reduction in greenhouse gas emissions originating from the plastic sector [
10,
11,
12,
13]. As previously indicated from the standpoint of plastics, a circular economy can be realized through a multifaceted strategy encompassing product redesign, enhanced post-consumer collection systems, the increased adoption of reusable plastic products, and innovative business models, alongside expanded recycling capabilities [
13]. The traditional linear economic model, often referred to as “Cradle to Grave” [
14], is unsustainable, as it culminates in waste accumulation in landfills due to inadequate processing. In contrast, the circular economy fosters a continuous cycle of resource utilization, epitomized by the “Cradle to Cradle” framework [
14]. This approach aims to establish a perpetual product lifecycle, incorporating recycled materials to maintain a closed-loop system [
10]. The European Commission has emphasized in its European Plastics in a Circular Economy Strategy that by 2025, 50% of composite waste and all plastic waste must be reused or recycled, with the target increasing to 55% by 2030. This initiative underscores the urgent need to explore advanced recycling alternatives that can help reduce energy consumption and improve material efficiency [
15].
Synergistic collaboration between industries has the potential to yield significant progress in sustainability and energy conservation. Several nations have already adopted the use of recycled plastics in the production of pavement tiles, which can be processed into various sizes depending on the intended application [
16]. Furthermore, plastic can effectively substitute coarse aggregates in the concrete mixture [
17]. As noted, “The increasing preference for environmentally sound, cost-effective, and lightweight construction materials within the building sector has spurred a demand for research into methods that achieve these objectives while simultaneously benefiting the environment and adhering to material standards” [
18].
A significant drawback of plastic recycling lies in its temporal displacement of the landfill problem, burdening future generations with the accumulated waste. The environmental persistence of microplastics, resulting from weathering and abrasion, further intensifies this issue. However, it is important to acknowledge that plastic has been an environmental challenge since the material’s inception. By adhering to sustainability principles, we can proactively investigate and implement more effective environmental solutions [
19].
The significant contribution of plastics to climate change is another pressing concern. The vast majority of plastics are derived from fossil fuels, with only a negligible fraction originating from recycled sources.
Climate change is a multifaceted challenge impacted by numerous variables, including the methods employed in the production of construction materials and the disposal of solid waste [
17,
18,
19].
Furthermore, sustainable design serves as a crucial strategy for attaining energy efficiency and fostering a healthier environment. This necessitates a delicate equilibrium between resource input and output. For example, mitigating the environmental impact and diminishing the carbon footprint of premium construction projects represent substantive progress toward achieving sustainability and the United Nations’ Sustainable Development Goals (SDGs) 2023 Agenda. The SDGs framework has been embraced globally, with the 17 goals outlining interconnected social, economic, and environmental sustainability indicators. Both developed and developing nations are called upon to engage in concerted action through this global partnership [
20].
Concrete manufacturing is a notably energy-intensive process. A typical concrete mix comprises cement, aggregates (both coarse and fine), and water. This process generates significant emissions, particularly carbon dioxide. As noted, “Over a 50-year life span, embodied energy constitutes 45% of the total energy demand. The recycling potential ranges between 35% and 40% of this embodied energy” [
21]. The embodied carbon in construction materials refers to the cumulative carbon dioxide emissions released during their production. This includes emissions throughout the entire construction lifecycle: from raw material extraction and transportation to the energy consumed by fixtures during a building’s operation and, finally, through demolition or ongoing maintenance.
Table 1 details the embodied carbon values for various building materials. Of those mentioned, steel demonstrates the most carbon-intensive, followed by glass, timber, brick, and concrete. For perspective, brick production averages 0.7 kg CO
2/kg, while concrete production averages 0.3 kg CO
2/kg [
22]. The primary carbon emission phases are the raw material sourcing and the concrete manufacturing processes [
23]. Raw material origins vary: Cement, the binding agent, is derived from limestone and clay; coarse aggregates are obtained from crushed natural stone; and fine aggregates from gravel.
A key factor in incentivizing the use of recycled materials, and thus, reducing embodied carbon, lies in the lower embodied carbon footprint associated with these materials [
23]; take, for example, the significant difference between virgin and recycled PET and HDPE plastics. Virgin PET carries an embodied carbon burden of 2.15 kg CO
2 equivalent per kilogram, while recycled PET demonstrates a substantially lower value of 0.45 kg CO
2 equivalent per kilogram. This translates to a 79% reduction in CO
2 emissions, as evidenced by a 2017 study conducted by a major PET producer in Austria, when utilizing recycled PET over virgin material [
22].
Beyond plastic, a wide array of waste materials can serve as viable substitutes for conventional coarse aggregates in concrete mixes [
23] by leveraging the embodied energy EE values provided by databases such as the Inventory of Carbon and Energy ICE [
22]. The overall embodied energy and, by extension, the embodied carbon of these modified concrete mixes can be accurately assessed based on the specific type of waste employed.
According to data from the Institute of Civil Engineers (ICE), each material possesses a unique embodied energy value, which is presented in
Table 1. It is evident that cement has the highest embodied energy per kilogram, exceeding that of both aggregate and water. In addition, the production of cement generates the most substantial carbon dioxide emissions when compared with aggregate production.
The nexus between elevated energy consumption, embodied carbon dioxide, carbon footprint metrics, reliance on fossil fuels, and plastic manufacturing is undeniable. The common thread linking these elements is the energy invested in production and the pursuit of sustainability [
22]. Each process demands a discrete energy expenditure to generate a refined, processed, or environmentally sustainable material. True sustainability is realized through adherence to established sustainability benchmarks, ultimately safeguarding our natural and nonrenewable energy reserves [
23].
This research employs laboratory experiments to rigorously evaluate and compare the mechanical properties of conventional and recycled plastic concrete, focusing on compressive and tensile strength, as well as fire resistance. A comparative analysis of these properties is conducted. Furthermore, a sensitivity analysis, derived from the experimental findings, serves as a model for the wider application of recycled materials in construction. The results of the sensitivity analysis for recycled pavement concrete demonstrate that the recycled plastic concrete exhibits comparable mechanical properties to conventional mixes. In certain instances, the compressive strength of the recycled plastic concrete even surpasses that of its conventional counterpart [
17,
18,
19,
20,
21,
22,
23,
24,
25]. While the incorporation of recycled plastic in concrete is prevalent in industrialized nations, awareness and adoption remain limited in other regions.